JEFF-3.0 file header. Release April 2002 9.424000+4 2.379920+2 1 1 2 09440 1451 1 0.000000+0 1.000000+0 0 0 0 69440 1451 2 1.000000+0 2.000000+7 0 0 10 309440 1451 3 0.000000+0 0.000000+0 0 0 453 1529440 1451 4 94-PU-240 CEA - NEA EVAL-APRIL2002 O.Bouland,H.Derrien,S.Masetti9440 1451 5 DIST-APR02 9440 1451 6 ----JEFF-30 MATERIAL 9440 9440 1451 7 -----INCIDENT NEUTRON DATA 9440 1451 8 ------ENDF-6 FORMAT 9440 1451 9 ***************************** JEFF-3.0 ***********************9440 1451 10 9440 1451 11 DATA TAKEN FROM :- JENDL-3.2 (DIST-SEP89) 9440 1451 12 MODIFICATIONS 9440 1451 13 by H.Derrien, O.Bouland in the Resolved Range (see below) 9440 1451 14 by O.Bouland in the Unresolved Range (see below) 9440 1451 15 by S.Masetti, A.Ventura, A.Trkov 9440 1451 16 by A. Nouri 9440 1451 17 Fission energies from ENDF/B-VI.7 9440 1451 18 Number of Prompt Neutrons (MF=1 MT=456): use the same 9440 1451 19 representation as for Total Nuetron emission in Fission 9440 1451 20 (MT=452). Convert LNU=1 (polynomial (linear) representation) 9440 1451 21 in MT=456 to (LNU=2) tabular representation. 9440 1451 22 9440 1451 23 ******************************************************************9440 1451 24 9440 1451 25 SUMMARY OF REVISED PARTS 9440 1451 26 9440 1451 27 ******************************************************************9440 1451 28 9440 1451 29 MF=2 9440 1451 30 MT=151 RESOLVED RESONANCE PARAMETERS UP TO 5.7 KeV 9440 1451 31 H.Derrien and O.Bouland (January,1996) 9440 1451 32 NSE 127,105-129(1997) 9440 1451 33 ---------------------------- 9440 1451 34 Work supported by EDF(France),CEA(France) and OECD 9440 1451 35 ---------------------------- 9440 1451 36 9440 1451 37 The JEF-2 validation has been recently performed on a 9440 1451 38 large integral data base including thermal and fast critical 9440 1451 39 data /1/. It was found that the capture and the fission cross 9440 1451 40 sections of 240Pu could be significantly too large particularly 9440 1451 41 in the resolved resonance region. The resonance parameters 9440 1451 42 proposed in the present file were obtained by a sequential 9440 1451 43 SAMMY analysis of existing experimental data. The input 9440 1451 44 parameters of the analysis where those found in the ENDF/B-VI 9440 1451 45 file in the energy range from thermal to 5700 eV. The reaction 9440 1451 46 formalism used in SAMMY is the Reich-Moore formalism. The 240Pu 9440 1451 47 cross sections could be represented by the multilevel Breit- 9440 1451 48 Wigner formalism in the energy ranges between the class II 9440 1451 49 states; but the Reich-Moore representation is very useful in 9440 1451 50 the resonances near the class II states where the fission 9440 1451 51 widths could be very large. In the next section the main 9440 1451 52 results of the new evaluation are given. More details can 9440 1451 53 be found in reference/2/. 9440 1451 54 A consistent SAMMY fit of Block/3/ total cross section, 9440 1451 55 Harvey transmission/4/ and Leonard fission data/5/ was performed 9440 1451 56 in the energy range from 0.02 eV to 1.5 eV in order to obtain 9440 1451 57 the values of the cross sections at 0.0253 eV and the parameters 9440 1451 58 of the resonance at 1.056 eV which contributes to more than 90% 9440 1451 59 to the capture resonance integral. The parameters obtained for 9440 1451 60 this resonance are very close to those obtained by Spencer/6/ and9440 1451 61 used in JEF-2 and ENDF/B-VI. The values of the cross sections at 9440 1451 62 0.0253 eV are the following: 9440 1451 63 Total 288.66 b 9440 1451 64 Scattering 2.67 b 9440 1451 65 Capture 285.93 b 9440 1451 66 Fission 0.059 b 9440 1451 67 9440 1451 68 In the energy range from 10 eV to 5700 eV, the SAMMY fits 9440 1451 69 were performed on the experimental transmissions of Kolar/7/ 9440 1451 70 two thicknesses in the energy range 20 eV to 700 eV and one 9440 1451 71 thickness in the energy range 20 eV to 5700 eV and on the 9440 1451 72 experimental fission cross sections of Weston/8/. Some 9440 1451 73 preliminary fits were performed on the transmissions of Kolar 9440 1451 74 in order to check the normalization and background correction 9440 1451 75 parameters and the experimental resolution parameters. Compared 9440 1451 76 to the current evaluated data files, much more resonances were 9440 1451 77 used in the present evaluation, particularly above the energy 9440 1451 78 of 1500 eV. These added resonances are resonances with small 9440 1451 79 neutron widths which could be identified above the small 9440 1451 80 background in the experimental fission data or in the 9440 1451 81 experimental statistical fluctuations of the transmission 9440 1451 82 data. This attempt to identify the small resonances in the 9440 1451 83 high energy region of the data leads to a more realistic 9440 1451 84 average value of the resonance spacing over the entire energy 9440 1451 85 range of the analysis and allows to avoid the use of a smooth 9440 1451 86 background cross section in the high energy range. The 9440 1451 87 comparison between ENDF/B-VI and the present evaluation is given 9440 1451 88 in the following Table, for the strength function and the number 9440 1451 89 of resonances: 9440 1451 90 Energy Strength Number of 9440 1451 91 Range eV Function Resonances 9440 1451 92 Present ENDF/B-VI Present ENDF/B-VI9440 1451 93 0- 500 1.089 1.102 42 36 9440 1451 94 500-1000 1.049 1.027 42 33 9440 1451 95 1000-1500 1.021 1.008 45 32 9440 1451 96 1500-2000 1.221 1.167 39 26 9440 1451 97 2000-2500 0.993 0.911 40 25 9440 1451 98 2500-3000 1.041 0.948 36 21 9440 1451 99 3000-3500 0.731 0.628 37 17 9440 1451 100 3500-4000 0.661 0.539 34 16 9440 1451 101 4000-4500 1.215 0.952 35 18 9440 1451 102 4500-5000 1.032 0.896 31 18 9440 1451 103 5000-5700 1.206 1.047 44 25 9440 1451 104 9440 1451 105 The low values of the strength function between 3 keV and 9440 1451 106 4 keV, whicy not consistent with the values in other energy 9440 1451 107 ranges (sampling error of about 22%), are not due to the 9440 1451 108 missing resonances in the corresponding energy ranges. The 9440 1451 109 same kind of fluctuations of the local values of the strength 9440 1451 110 function are also observed in 238U data/10/ and others nuclei. 9440 1451 111 The average values of the capture cross section are given 9440 1451 112 in the following Table: 9440 1451 113 Energy Range Weston/10/ Present B-VI JEF-2 JENDL-39440 1451 114 eV b b b b b 9440 1451 115 9440 1451 116 0.02- 1.5 5922 5930 5897 5652 9440 1451 117 1.5- 50 56.85 56.83 55.34 57.33 9440 1451 118 50- 100 49.96 48.40 48.57 48.71 9440 1451 119 100- 200 23.30 24.64 25.57 25.64 9440 1451 120 200- 300 8.71+/-0.61 7.27 7.41 9.07 9.08 9440 1451 121 300- 400 10.27+/-0.72 7.93 7.89 9.92 9.94 9440 1451 122 400- 500 6.60+/-0.46 6.01 5.97 7.02 7.03 9440 1451 123 500- 600 7.14+/-0.50 6.22 5.91 7.15 7.16 9440 1451 124 600- 700 5.09+/-0.36 4.44 4.64 4.65 4.65 9440 1451 125 700- 800 2.63+/-0.18 2.04 1.64 3.31 3.31 9440 1451 126 800- 900 6.63+/-0.46 5.70 5.25 5.31 5.31 9440 1451 127 900-1000 5.53+/-0.39 5.75 5.47 6.15 6.15 9440 1451 128 1000-1500 3.50+/-0.25 3.13 2.89 3.46 3.46 9440 1451 129 1500-2000 3.03+/-0.21 2.52 2.24 3.05 3.05 9440 1451 130 2000-3000 2.42+/-0.17 1.90 1.54 2.40 2.40 9440 1451 131 3000-4000 1.89+/-0.13 1.20 1.29 1.89 1.90 9440 1451 132 4000-5000 1.67+/-0.12 1.13 1.55 1.76 1.75 9440 1451 133 5000-5700 0.95 1.54 1.60 1.60 9440 1451 134 9440 1451 135 0.02- 200 81.76 82.09 81.99 80.73 9440 1451 136 200-5000 3.02 2.42 2.37 3.03 3.03 9440 1451 137 9440 1451 138 These average cross sections were calculated by NJOY-94.0 9440 1451 139 at the NEA Data Bank. 9440 1451 140 In the energy range 200 eV to 5000 eV, the values of 9440 1451 141 JEF-2 and JENDL-3 were normalized to the experimental values 9440 1451 142 of Weston. The values of the present evaluation and of ENDF/B-VI 9440 1451 143 are 25% and 27% lower respectively. One should note that Weston 9440 1451 144 in his evaluation for ENDF/B-VI/11/ did not take into account 9440 1451 145 his own experimental data. 9440 1451 146 The average values of the fission cross section are given 9440 1451 147 in the following Table: 9440 1451 148 Energy Range Present B-VI JEF-2 JENDL-39440 1451 149 eV mb mb mb mb 9440 1451 150 9440 1451 151 0.02- 1.5 1649 1170 1140 1048 9440 1451 152 1.5- 50 91 94 381 94 9440 1451 153 50- 100 74 76 346 76 9440 1451 154 100- 200 46 50 337 50 9440 1451 155 200- 300 52 53 222 53 9440 1451 156 300- 400 15 18 228 18 9440 1451 157 400- 500 47 49 188 49 9440 1451 158 500- 600 20 23 185 21 9440 1451 159 600- 700 54 54 208 66 9440 1451 160 700- 800 879 905 1020 938 9440 1451 161 800- 900 698 615 693 613 9440 1451 162 900-1000 86 80 155 75 9440 1451 163 1000-1500 206 199 257 147 9440 1451 164 1500-2000 316 297 422 312 9440 1451 165 2000-3000 210 181 332 242 9440 1451 166 3000-4000 75 74 116 6 9440 1451 167 4000-5000 60 50 88 67 9440 1451 168 5000-5700 150 145 91 124 9440 1451 169 9440 1451 170 1.5 -5700 159.5 149 228 158 9440 1451 171 9440 1451 172 These average cross sections were calculated by NJOY-94.0 9440 1451 173 at the NEA Data Bank. 9440 1451 174 In the energy range 1.5 eV to 700 eV, the average fis- 9440 1451 175 sions of J are much larger than the other values. The present 9440 1451 176 results are in general consistent with B-VI and JENDL-3. Note 9440 1451 177 an inconsistent value in JENDL-3 in the energy range 3000 eV to 9440 1451 178 4000 eV. 9440 1451 179 9440 1451 180 The capture and fission resonance integrals are given 9440 1451 181 in the following Table: 9440 1451 182 9440 1451 183 Present B-VI JEF-2 JENDL-3 9440 1451 184 b b b b 9440 1451 185 9440 1451 186 Capture 8481 8494 8445 8102 9440 1451 187 Fission 3.16 2.46 3.52 2.29 9440 1451 188 9440 1451 189 For the capture, the difference between JENDL-3 and the 9440 1451 190 others is mainly due to a smaller value of the neutron width of 9440 1451 191 the resonance at 1.056 eV. 9440 1451 192 9440 1451 193 The comparison of the present results with JEF-2 shows 9440 1451 194 a significant decrease of the capture cross section and of the 9440 1451 195 fission cross section in the resolved energy range,in agreement 9440 1451 196 with the tendancy observed in the validation of the JEF-2 general 9440 1451 197 purpose file/1/. 9440 1451 198 9440 1451 199 9440 1451 200 9440 1451 201 MF=2 9440 1451 202 MT=151 Unresolved Resonance energy Range between 5.7-40 KeV 9440 1451 203 O.Bouland (April,2002) 9440 1451 204 (see JEF/document JEFF/EFF meeting April 2002) 9440 1451 205 ---------------------------- 9440 1451 206 Work supported by EDF(France),CEA(France) 9440 1451 207 ---------------------------- 9440 1451 208 9440 1451 209 In the unresolved region, the point cross-sections given in mf=3 9440 1451 210 are considered as correct. The unresolved parameters given in 9440 1451 211 mf=2 mt=151 are only to be used for self-shielding calculations. 9440 1451 212 The use of the parameters with ENDF processing does not lead to 9440 1451 213 cross sections consistent with mf=3 as the codes use a more pri- 9440 1451 214 mitive version of the formalism. 9440 1451 215 9440 1451 216 REFERENCES: 9440 1451 217 1) E.Fort et al., Gatlinburg Conference,Tennessee,May 9-16,1994 9440 1451 218 2) 0.Bouland et al.,NSE 127, 2, 105-129 (Oct 1997) 9440 1451 219 3) R.C.Block et al.,NSE 8,112(1960) 9440 1451 220 4) J.H.Harvey,Private communication at ORNL (1995) 9440 1451 221 5) B.R.Leonard et al.,Hanford Report Series 67219,4 (1960) 9440 1451 222 6) R.Spencer et al.,NSE 96,318(1987) 9440 1451 223 7) W.Kolar et al., J.Nucl.Energy 22,299(1968) 9440 1451 224 8) L.W.Weston et al.,NSE 88,567(1984) 9440 1451 225 9) D.K.Olsen et al.,NSE 94,102(1986) 9440 1451 226 10) L.W.Weston et al.,NSE 63,143(1977) 9440 1451 227 11) L.W.Weston et al.,ORNL-TM-10386(1988) 9440 1451 228 9440 1451 229 ******************************************************************9440 1451 230 HISTORY 9440 1451 231 *** Comments below are from the original JENDL-3.2 evaluation 9440 1451 232 9.42400+ 4 2.37992+ 2 1 1 0 39440 1451 233 0.00000+ 0 1.00000+ 0 0 0 0 69440 1451 234 1.00000+ 0 0.00000+ 0 0 0 10 39440 1451 235 0.00000+ 0 0.00000+ 0 0 0 221 839440 1451 236 94-PU-240 NAIG+ EVAL-MAY87 T.MURATA, A.ZUKERAN 9440 1451 237 DIST-SEP89 REV2-AUG93 9440 1451 238 ----JENDL-3.2 MATERIAL 9440 9440 1451 239 -----INCIDENT NEUTRON DATA 9440 1451 240 ------ENDF-6 FORMAT 9440 1451 241 HISTORY 9440 1451 242 87-05 EVALUATION WAS MADE BY 9440 1451 243 T.MURATA (NAIG) : CROSS SECTIONS ABOVE RESONANCE REGION 9440 1451 244 AND OTHER QUANTITIES, 9440 1451 245 A.ZUKERAN(HITACHI): RESONANCE PARAMETERS. 9440 1451 246 88-06 MT'S=16, 17, 37 AND 102 WERE MODIFIED. 9440 1451 247 89-02 FP YIELDS WERE TAKEN FROM JNDC FP DECAY FILE VERSION-2. 9440 1451 248 COMPILATION WAS MADE BY T. NAKAGAWA (JAERI). 9440 1451 249 90-07 FP YIELD DATA WERE MODIFIED. 9440 1451 250 90-10 MF=5, MT=16, 17, 91: MODIFIED AT THRESHOLD ENERGIES. 9440 1451 251 93-08 JENDL-3.2. 9440 1451 252 COMPILED BY T.NAKAGAWA (NDC/JAERI) 9440 1451 253 9440 1451 254 ***** MODIFIED PARTS FOR JENDL-3.2 ******************** 9440 1451 255 (1,452), (1,455) 9440 1451 256 *********************************************************** 9440 1451 257 9440 1451 258 9440 1451 259 MF=1 GENERAL INFORMATION 9440 1451 260 MT=451 COMMENTS AND DICTIONARY 9440 1451 261 MT=452 NUMBER OF NEUTRONS PER FISSION 9440 1451 262 SUM OF MT=455(DELAYED NEUTRONS) AND MT=456(PROMPT NEUTRONS).9440 1451 263 MT=455 DELAYED NEUTRON DATA 9440 1451 264 BELOW 5 MEV, NU-D OF 0.00911 MEASURED BY BENEDETTI ET AL. 9440 1451 265 /1/ WAS ADOPTED. ABOVE 6 MEV, 0.0067 WAS GIVEN ON THE BASIS9440 1451 266 OF TUTTLE'S SYSTEMATICS /2/. DECAY CONSTANTS WERE TAKEN 9440 1451 267 FROM EVALUATION BY BARDY AND ENGLAND /3/. 9440 1451 268 MT=456 NUMBER OF PROMPT NEUTRONS 9440 1451 269 LINEAR LEAST-SQUARES FITTING TO THE EXPERIMENTAL DATA OF 9440 1451 270 FREHAUT ET AL. /4/ RENORMALIZED TO CF-252 NU-P=3.756. 9440 1451 271 9440 1451 272 MF=2 RESONANCE PARAMETERS 9440 1451 273 MT=151 RESOLVED AND UNRESOLVED RESONANCE PARAMETERS 9440 1451 274 1) RESOLVED RESONANCES FOR MLBW FORMULA (1.0E-5 TO 4 KEV) 9440 1451 275 PARAMETERS OF A NEGATIVE AND THE 1.057-EV RESONANCES WERE 9440 1451 276 REVISED ON THE BASIS OF RECOMMENDATION BY MUGHABGHAB /5/. 9440 1451 277 NEUTRON AND CAPTURE WIDTHS OF OTHER LEVELS WERE BASED ON THE9440 1451 278 EXPERIMENTAL DATA BY HOCKENBURY ET AL. /6/ IN THE ENERGY 9440 1451 279 RANGE FROM 20 TO 500 EV, AND KOLAR AND BOECKHOFF /7/ FROM 9440 1451 280 500 EV TO 4 KEV. THE AVERAGE CAPTURE WIDTH OF 29.5 MILLI-EV9440 1451 281 WAS ASSUMED FOR THE RESONANCES WHOSE CAPTURE WIDTHS WERE 9440 1451 282 UNKNOWN. BELOW 610 EV, THE SUB-THRESHOLD FISSION WIDTHS 9440 1451 283 WERE CALCULATED FROM THE AREA DATA BY WESTON AND TODD /8/. 9440 1451 284 ABOVE 610 EV, THEY WERE TAKEN FROM THE DATA BY AUCHAMPAUGH 9440 1451 285 AND WESTON /9/. 9440 1451 286 2) UNRESOLVED RESONANCES (4 TO 40 KEV) 9440 1451 287 ENERGY DEPENDENT PARAMETERS WERE DETERMINED TO REPRODUCE THE9440 1451 288 EVALUATED CROSS SECTIONS IN THIS ENERGY REGION. FISSION 9440 1451 289 WIDTHS WERE ADJUSTED TO AVERAGE CROSS SECTIONS MEASURED BY 9440 1451 290 WESTON AND TODD /8/. 9440 1451 291 9440 1451 292 CALCULATED 2200-M/SEC CROSS SECTIONS AND RES. INTEGERALS. 9440 1451 293 2200-M/SEC RES. INTEG. 9440 1451 294 TOTAL 291.13 B 9440 1451 295 ELASTIC 1.644 B - 9440 1451 296 FISSION 0.0588 B 8.94 B 9440 1451 297 CAPTURE 289.4 B 8110. B 9440 1451 298 9440 1451 299 MF=3 NEUTRON CROSS SECTIONS 9440 1451 300 BELOW 4 KEV: BACKGROUND CROSS SECTIONS ARE GIVEN TO THE CAPTURE 9440 1451 301 CROSS SECTION. 9440 1451 302 ABOVE 4 KEV: EVALUATED AS FOLLOWS. IN THE ENERGY RANGE FROM 4 9440 1451 303 TO 40 KEV, THE CROSS SECTIONS ARE REPRESENTED WITH 9440 1451 304 THE UNRESOLVED RESONANCE PARAMETERS, AND THE BACK- 9440 1451 305 GROUND CROSS SECTIONS ARE GIVEN IN MF=3. 9440 1451 306 MT=1 TOTAL 9440 1451 307 EVALUATED WITH SPLINE FITTING TO THE EXPERIMENTAL DATA OF 9440 1451 308 SMITH ET AL./10/, KAEPPELER ET AL./11/ AND POENITZ ET 9440 1451 309 AL./12/ 9440 1451 310 9440 1451 311 MT=2 ELASTIC SCATTERING 9440 1451 312 OBTAINED BY SUBTRACTING THE OTHER CROSS SECTIONS FROM TOTAL 9440 1451 313 CROSS SECTION. 9440 1451 314 9440 1451 315 MT=4 TOTAL INELASTIC SCATTERING 9440 1451 316 SUM OF PARTIAL INELASTIC SCATTERING CROSS SECTIONS (MT=51 9440 1451 317 TO MT=91). 9440 1451 318 9440 1451 319 MT=51-78, 91 PARTIAL INELASTIC SCATTERING 9440 1451 320 BELOW 3 MEV, THE RESULTS OF STATISTICAL AND COUPLED-CHANNEL 9440 1451 321 CALCULATION MADE BY LAGRANGE ET AL. /13/ WERE ADOPTED. FOR 9440 1451 322 SOME LEVELS, FOR WHICH SMITH'S EXPERIMENTAL DATA /14/ WERE 9440 1451 323 AVAILABLE, THE CALCULATED RESULTS WERE NORMALIZED (FOR 1ST, 9440 1451 324 2ND, 3RD, 5TH AND 9 TO 11TH LEVELS). 9440 1451 325 9440 1451 326 LEVEL SCHEME 9440 1451 327 NO. ENERGY(MEV) SPIN-PARITY 9440 1451 328 G.S. 0.0 0 + 9440 1451 329 1 0.04285 2 + 9440 1451 330 2 0.14169 4 + 9440 1451 331 3 0.29431 6 + 9440 1451 332 4 0.4976 8 + 9440 1451 333 5 0.59736 1 - 9440 1451 334 6 0.64889 3 - 9440 1451 335 7 0.74232 5 - 9440 1451 336 8 0.8607 0 + 9440 1451 337 9 0.90032 2 + 9440 1451 338 10 0.93807 1 - 9440 1451 339 11 0.95887 2 - 9440 1451 340 12 0.9924 4 + 9440 1451 341 13 1.0018 3 - 9440 1451 342 14 1.0306 3 + 9440 1451 343 15 1.0375 4 - 9440 1451 344 16 1.0764 4 + 9440 1451 345 17 1.0895 0 + 9440 1451 346 18 1.1155 5 - 9440 1451 347 19 1.1370 2 + 9440 1451 348 20 1.1615 6 - 9440 1451 349 21 1.1778 3 + 9440 1451 350 22 1.2230 2 + 9440 1451 351 23 1.2325 4 + 9440 1451 352 24 1.2408 2 - 9440 1451 353 25 1.2621 3 + 9440 1451 354 26 1.2820 3 - 9440 1451 355 27 1.30873 5 - 9440 1451 356 28 1.41079 0 + 9440 1451 357 LEVELS ABOVE 1.4108 MEV WERE ASSUMED TO BE CONTINUUM. 9440 1451 358 9440 1451 359 MT=16,17,37 (N,2N),(N,3N) AND (N,4N) 9440 1451 360 CALCULATED FROM NEUTRON EMISSION CROSS SECTION AND BRANCHING9440 1451 361 RATIO TO EACH REACTION CHANNEL. NEUTRON EMISSION CROSS 9440 1451 362 SECTION WAS OBTAINED BY SUBTRACTING THE FISSION AND CAPTURE 9440 1451 363 CROSS SECTIONS FROM COMPOUND NUCLEUS FORMATION CROSS SECTION9440 1451 364 CALCULATED WITH SPHERICAL OPTICAL MODEL. BRANCHING RATIO 9440 1451 365 WAS OBTAINED FROM FORMALISM GIVEN BY SEGEV ET AL. /15/ 9440 1451 366 9440 1451 367 MT=18 FISSION 9440 1451 368 BELOW 100 KEV: AVERAGE VALUES OF FISSION CROSS SECTION 9440 1451 369 MEASURED BY WESTON AND TODD /8/ WERE NORMALIZED TO THE 9440 1451 370 VALUE AT 100 KEV OF THE SIMULTANEOUS EVALUATION. 9440 1451 371 ABOVE 100 KEV: SIMULTANEOUS EVALUATION WAS MADE BY TAKING 9440 1451 372 ACCOUNT OF EXPERIMENTAL DATA OF FISSION RATIO AND ABSOLUTE 9440 1451 373 CROSS SECTIONS OF U-235, U-238, PU-239, PU-240 AND PU-241, 9440 1451 374 AND CAPTURE CROSS SECTION OF AU-197 /16/. 9440 1451 375 9440 1451 376 MT=102 CAPTURE 9440 1451 377 BELOW 350 KEV: BASED ON THE EXPERIMENTAL DATA OF HOCKENBURY ET9440 1451 378 AL. /6/, WESTON AND TODD /17/ AND THE RATIO DATA OF WISSHAK 9440 1451 379 AND KAEPPELER /18/ WITH THE CAPTURE CROSS SECTION OF AU-197 9440 1451 380 /16/. AS A GUIDE LINE, STATISTICAL MODEL CALCULATION WAS 9440 1451 381 MADE WITH CASTHY CODE /19/. 9440 1451 382 ABOVE 350 KEV: THE STATISTICAL MODEL CALCULATION WAS 9440 1451 383 NORMALIZED TO THE VALUE AT 350 KEV. DIRECT AND COLLECTIVE 9440 1451 384 CAPTURE WAS INCLUDED IN HIGH ENERGY REGION ADOPTING THE 9440 1451 385 VALUE FOR U-238 GIVEN BY KITAZAWA ET AL. /20/. 9440 1451 386 9440 1451 387 THE SPHERICAL OPTICAL POTENTIAL PARAMETERS 9440 1451 388 V = 40.6 - 0.05*EN, WS = 6.5 + 0.15*EN (MEV) 9440 1451 389 VSO= 7.0 (MEV) 9440 1451 390 R = RSO =1.32 , RS = 1.38 (FM) 9440 1451 391 A = AS = ASO =0.47 (FM) 9440 1451 392 LEVEL DENSITY PARAMETERS WERE DETERMINED TO REPRODUCE THE 9440 1451 393 RESONANCE LEVEL SPACINGS AND STAIRCASES OF DISCRETE LEVELS. 9440 1451 394 9440 1451 395 MT=251 MU-BAR 9440 1451 396 THE SAME AS JENDL-1 /21/ EXCEPT FOR 20 MEV. 9440 1451 397 9440 1451 398 MF=4 ANGULAR DISTRIBUTIONS OF SECONDARY NEUTRONS 9440 1451 399 MT=2 9440 1451 400 TAKEN FROM JENDL-1 /21/. 9440 1451 401 MT=16,17,18,37,91 9440 1451 402 ASSUMED TO BE ISOTROPIC IN THE LABORATORY SYSTEM. 9440 1451 403 MT=51-78 9440 1451 404 FOR THE 1ST AND 2ND LEVELS, RESULTS OF LAGRANGE ET AL. /13/ 9440 1451 405 WERE ADOPTED. FOR OTHERS, STATISTICAL AND DWBA CALCULATIONS9440 1451 406 WERE MADE. 9440 1451 407 9440 1451 408 MF=5 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS 9440 1451 409 MT=16,17,91 9440 1451 410 CALCULATED WITH PRE-COMPOUND AND MULTI-STEP EVAPORATION 9440 1451 411 THEORY CODE PEGASUS /22/. 9440 1451 412 MT=37 9440 1451 413 EVAPORATION SPECTRUM WAS GIVEN. 9440 1451 414 MT=18 FISSION SPECTRA 9440 1451 415 CALCULATED FROM MADLAND-NIX FORMULA /23/. 9440 1451 416 AVERAGE ENERGY RELEASE = 199.179 MEV 9440 1451 417 TOTAL AVERAGE FF KINETIC ENERGY = 177.53 MEV 9440 1451 418 AVERAGE MASS NUMBER OF LIGHT FF = 101 9440 1451 419 AVERAGE MASS NUMBER OF HEAVY FF = 140 9440 1451 420 LEVEL DENSITY PARAMETER = A/10.0 9440 1451 421 MT=455 DELAYED NEUTRON SPECTRA 9440 1451 422 ASSUMED TO BE THE SAME AS PU-239 WHICH WERE TAKEN FROM THE 9440 1451 423 EVALUATION BY SAPHIER ET AL. /24/. 9440 1451 424 9440 1451 425 REFERENCES 9440 1451 426 1) BENEDETTI G., ET AL.: NUCL. SCI. ENG., 80, 379 (1982). 9440 1451 427 2) TUTTLE R.J.: INDC(NDS)-107/G-SPECIAL, P.29 (1979). 9440 1451 428 3) BRADY M.C. AND ENGLAND T.R.: NUCL. SCI. ENG., 103, 129(1989). 9440 1451 429 4) FREHAUT J., ET AL.: CEA(R) 4626 (1974). 9440 1451 430 5) MUGHABGHAB S.F.: "NEUTRON CROSS SECTIONS, VOL. 1, PART B", 9440 1451 431 ACADEMIC PRESS (1984). 9440 1451 432 6) HOCKENBURY R.W. ET AL.: NUCL. SCI. ENG., 49, 153 (1972). 9440 1451 433 7) KOLAR W. AND BOECKHOFF K.H.: J. NUCL. ENERGY, 22, 299 (1968). 9440 1451 434 8) WESTON L.W. AND TODD J.H.: NUCL. SCI. ENG., 88, 567 (1984). 9440 1451 435 9) AUCHAMPAUGH G.F. AND WESTON L.E.: PHYS. REV., C12, 1850 9440 1451 436 (1975). 9440 1451 437 10) SMITH A.B. ET AL.: NUCL. SCI. ENG., 47, 19 (1972). 9440 1451 438 11) KAEPPLER F., ET AL.: PROC. OF MEETING ON NUCLEAR DATA OF 9440 1451 439 HIGHER PU AND AM ISOTOPES FOR REACTOR APPLICATION, HELD AT 9440 1451 440 BNL, P.49 (1978) 9440 1451 441 12) POENITZ W.P., ET AL.; NUCL. SCI. ENG., 78, 333 (1981), AND 9440 1451 442 ANL/NDM-80 (1983). 9440 1451 443 13) LAGRANGE CH. AND JARY J.: NEANDC(E) 198"L" (1978). 9440 1451 444 14) SMITH A.B., ET AL.: IAEA-153, P.447 (1973). 9440 1451 445 15) SEGEV M., ET AL.: ANNALS OF NUCL. ENERGY, 5, 239 (1978). 9440 1451 446 16) KANDA Y. ET AL.: 1985 SANTA FE, 2, 1567 (1986). 9440 1451 447 17) WESTON L.W. AND TODD J.H.: NUCL. SCI. ENG.,63, 143 (1977). 9440 1451 448 18) WISSHAK K. AND KAEPPELER F.: NUCL. SCI. ENG., 66, 363 (1978) 9440 1451 449 AND NUCL. SCI. ENG., 69, 39 (1979). 9440 1451 450 19) IGARASI S. AND FUKAHORI T.: JAERI 1321 (1991). 9440 1451 451 20) KITAZAWA H., ET AL.: NUCL. PHYS., A307, 1 (1978). 9440 1451 452 21) IGARASI S., ET AL.: JAERI 1261 (1979). 9440 1451 453 22) IIJIMA S., ET AL.: JAERI-M 87-025, P.337 (1987). 9440 1451 454 23) MADLAND D.G. AND NIX J.R.: NUCL. SCI. ENG., 81, 213 (1982). 9440 1451 455 24) SAPHIER D., ET AL.: NUCL. SCI. ENG., 62, 660 (1977). 9440 1451 456 9440 1451 457 1 451 609 09440 1451 458 1 452 6 09440 1451 459 1 455 7 09440 1451 460 1 456 6 09440 1451 461 1 458 5 09440 1451 462 2 151 554 09440 1451 463 3 1 303 09440 1451 464 3 2 302 09440 1451 465 3 4 32 09440 1451 466 3 16 18 09440 1451 467 3 17 9 09440 1451 468 3 18 237 09440 1451 469 3 37 4 09440 1451 470 3 51 23 09440 1451 471 3 52 21 09440 1451 472 3 53 20 09440 1451 473 3 54 19 09440 1451 474 3 55 19 09440 1451 475 3 56 18 09440 1451 476 3 57 18 09440 1451 477 3 58 17 09440 1451 478 3 59 17 09440 1451 479 3 60 16 09440 1451 480 3 61 16 09440 1451 481 3 62 16 09440 1451 482 3 63 15 09440 1451 483 3 64 15 09440 1451 484 3 65 14 09440 1451 485 3 66 14 09440 1451 486 3 67 14 09440 1451 487 3 68 13 09440 1451 488 3 69 13 09440 1451 489 3 70 13 09440 1451 490 3 71 12 09440 1451 491 3 72 12 09440 1451 492 3 73 12 09440 1451 493 3 74 11 09440 1451 494 3 75 11 09440 1451 495 3 76 11 09440 1451 496 3 77 10 09440 1451 497 3 78 10 09440 1451 498 3 91 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