4.61020+ 4 1.01031+ 2 1 0 0 14625 1451 1 0.0 + 0 0.0 + 0 0 0 0 04625 1451 2 0.0 + 0 0.0 + 0 0 0 200 684625 1451 3 46-PD-102 JNDC EVAL-MAR90 JNDC FP NUCLEAR DATA W.G. 4625 1451 4 DIST-NOV90 4625 1451 5 HISTORY 4625 1451 6 90-03 NEW EVALUATION FOR JENDL-3 WAS COMPLETED BY JNDC FPND 4625 1451 7 W.G./1/ 4625 1451 8 4625 1451 9 MF = 1 GENERAL INFORMATION 4625 1451 10 MT=451 COMMENTS AND DICTIONARY 4625 1451 11 4625 1451 12 MF = 2 RESONANCE PARAMETERS 4625 1451 13 MT=151 RESOLVED AND UNRESOLVED RESONANCE PARAMETERS 4625 1451 14 RESOLVED RESONANCE REGION (MLBW FORMULA) : BELOW 0.25 KEV 4625 1451 15 RESONANCE PARAMETERS WERE BASED ON MUGHABGHAB ET AL./2/ 4625 1451 16 4625 1451 17 UNRESOLVED RESONANCE REGION : 0.25 KEV - 100 KEV 4625 1451 18 THE NEUTRON STRENGTH FUNCTION S1 WAS BASED ON THE SYSTEMATICS 4625 1451 19 OF MUGHABGHAB ET AL., AND S0 AND S2 WERE CALCULATED WITH 4625 1451 20 OPTICAL MODEL CODE CASTHY/3/. THE OBSERVED LEVEL SPACING WAS 4625 1451 21 DETERMINED TO REPRODUCE THE CAPTURE CROSS SECTION CALCULATED 4625 1451 22 WITH CASTHY. THE EFFECTIVE SCATTERING RADIUS WAS OBTAINED 4625 1451 23 FROM FITTING TO THE CALCULATED TOTAL CROSS SECTION AT 100 KEV.4625 1451 24 THE RADIATION WIDTH GG WAS BASED ON THE SYSTEMATICS OF 4625 1451 25 MEASURED VALUES FOR NEIGHBORING NUCLIDES. 4625 1451 26 4625 1451 27 TYPICAL VALUES OF THE PARAMETERS AT 70 KEV: 4625 1451 28 S0 = 0.800E-4, S1 = 5.000E-4, S2 = 1.000E-4, SG = 9.09E-4, 4625 1451 29 GG = 0.150 EV, R = 4.951 FM. 4625 1451 30 4625 1451 31 CALCULATED 2200-M/S CROSS SECTIONS AND RES. INTEGRALS (BARNS) 4625 1451 32 2200 M/S RES. INTEG. 4625 1451 33 TOTAL 8.387 - 4625 1451 34 ELASTIC 5.024 - 4625 1451 35 CAPTURE 3.363 19.5 4625 1451 36 4625 1451 37 MF = 3 NEUTRON CROSS SECTIONS 4625 1451 38 BELOW 100 KEV, RESONANCE PARAMETERS WERE GIVEN. 4625 1451 39 ABOVE 100 KEV, THE SPHERICAL OPTICAL AND STATISTICAL MODEL 4625 1451 40 CALCULATION WAS PERFORMED WITH CASTHY, BY TAKING ACCOUNT OF 4625 1451 41 COMPETING REACTIONS, OF WHICH CROSS SECTIONS WERE CALCULATED 4625 1451 42 WITH PEGASUS/4/ STANDING ON A PREEQUILIBRIUM AND MULTI-STEP 4625 1451 43 EVAPORATION MODEL. THE OMP'S FOR NEUTRON GIVEN IN TABLE 1 WERE 4625 1451 44 DETERMINED TO REPRODUCE THE CD-NATURAL TOTAL CROSS SECTIONS 4625 1451 45 MEASURED BY FOSTER AND GLASGOW/5/, POENITZ AND WHALEN/6/ AND 4625 1451 46 SO ON, AND APPLIED TO PD ISOTOPES ALSO. THE OMP'S FOR CHARGED 4625 1451 47 PARTICLES ARE AS FOLLOWS: 4625 1451 48 PROTON = PEREY/7/ 4625 1451 49 ALPHA = HUIZENGA AND IGO/8/ 4625 1451 50 DEUTERON = LOHR AND HAEBERLI/9/ 4625 1451 51 HELIUM-3 AND TRITON = BECCHETTI AND GREENLEES/10/ 4625 1451 52 PARAMETERS FOR THE COMPOSITE LEVEL DENSITY FORMULA OF GILBERT 4625 1451 53 AND CAMERON/11/ WERE EVALUATED BY IIJIMA ET AL./12/ MORE 4625 1451 54 EXTENSIVE DETERMINATION AND MODIFICATION WERE MADE IN THE 4625 1451 55 PRESENT WORK. TABLE 2 SHOWS THE LEVEL DENSITY PARAMETERS USED 4625 1451 56 IN THE PRESENT CALCULATION. ENERGY DEPENDENCE OF SPIN CUT-OFF 4625 1451 57 PARAMETER IN THE ENERGY RANGE BELOW E-JOINT IS DUE TO GRUPPELAAR4625 1451 58 /13/. 4625 1451 59 4625 1451 60 MT = 1 TOTAL 4625 1451 61 SPHERICAL OPTICAL MODEL CALCULATION WAS ADOPTED. 4625 1451 62 4625 1451 63 MT = 2 ELASTIC SCATTERING 4625 1451 64 CALCULATED AS (TOTAL - SUM OF PARTIAL CROSS SECTIONS). 4625 1451 65 4625 1451 66 MT = 4, 51 - 91 INELASTIC SCATTERING 4625 1451 67 SPHERICAL OPTICAL AND STATISTICAL MODEL CALCULATION WAS 4625 1451 68 ADOPTED. THE LEVEL SCHEME WAS BASED ON EVALUATED NUCLEAR 4625 1451 69 STRUCTURE DATA FILE (1987 VERSION)/14/ AND NUCLEAR DATA 4625 1451 70 SHEETS/15/. 4625 1451 71 4625 1451 72 NO. ENERGY(MEV) SPIN-PARITY 4625 1451 73 GR. 0.0 0 + 4625 1451 74 1 0.5565 2 + 4625 1451 75 2 1.2760 4 + 4625 1451 76 3 1.5346 2 + 4625 1451 77 4 1.5930 0 + 4625 1451 78 5 1.6582 0 + 4625 1451 79 6 1.7150 6 + 4625 1451 80 7 1.9190 3 + 4625 1451 81 8 1.9444 2 + 4625 1451 82 9 2.1115 6 + 4625 1451 83 10 2.1118 3 + 4625 1451 84 11 2.1381 4 + 4625 1451 85 12 2.2487 2 + 4625 1451 86 13 2.2947 4 - 4625 1451 87 14 2.3014 4 + 4625 1451 88 15 2.3430 3 + 4625 1451 89 16 2.3912 1 + 4625 1451 90 17 2.4316 3 + 4625 1451 91 18 2.4745 5 - 4625 1451 92 LEVELS ABOVE 2.48 MEV WERE ASSUMED TO BE OVERLAPPING. 4625 1451 93 4625 1451 94 MT = 102 CAPTURE 4625 1451 95 SPHERICAL OPTICAL AND STATISTICAL MODEL CALCULATION WITH 4625 1451 96 CASTHY WAS ADOPTED. DIRECT AND SEMI-DIRECT CAPTURE CROSS 4625 1451 97 SECTIONS WERE ESTIMATED ACCORDING TO THE PROCEDURE OF BENZI 4625 1451 98 AND REFFO/16/ AND NORMALIZED TO 1 MILLI-BARN AT 14 MEV. 4625 1451 99 4625 1451 100 THE GAMMA-RAY STRENGTH FUNCTION (9.55E-04) WAS DETERMINED FROM4625 1451 101 THE SYSTEMATICS. 4625 1451 102 4625 1451 103 MT = 16 (N,2N) CROSS SECTION 4625 1451 104 MT = 17 (N,3N) CROSS SECTION 4625 1451 105 MT = 22 (N,N'A) CROSS SECTION 4625 1451 106 MT = 28 (N,N'P) CROSS SECTION 4625 1451 107 MT = 32 (N,N'D) CROSS SECTION 4625 1451 108 MT =103 (N,P) CROSS SECTION 4625 1451 109 MT =104 (N,D) CROSS SECTION 4625 1451 110 MT =105 (N,T) CROSS SECTION 4625 1451 111 MT =106 (N,HE3) CROSS SECTION 4625 1451 112 MT =107 (N,ALPHA) CROSS SECTION 4625 1451 113 MT =111 (N,2P) CROSS SECTION 4625 1451 114 THESE REACTION CROSS SECTIONS WERE CALCULATED WITH THE 4625 1451 115 PREEQUILIBRIUM AND MULTI-STEP EVAPORATION MODEL CODE PEGASUS. 4625 1451 116 4625 1451 117 THE KALBACH'S CONSTANT K (= 93.4) WAS ESTIMATED BY THE 4625 1451 118 FORMULA DERIVED FROM KIKUCHI-KAWAI'S FORMALISM/17/ AND LEVEL 4625 1451 119 DENSITY PARAMETERS. 4625 1451 120 4625 1451 121 FINALLY, THE (N,P) AND (N,ALPHA) CROSS SECTIONS WERE 4625 1451 122 NORMALIZED TO THE FOLLOWING VALUES AT 14.5 MEV: 4625 1451 123 (N,P) 93.60 MB (RECOMMENDED BY FORREST/18/) 4625 1451 124 (N,ALPHA) 19.60 MB (SYSTEMATICS OF FORREST/18/) 4625 1451 125 4625 1451 126 MT = 251 MU-BAR 4625 1451 127 CALCULATED WITH CASTHY. 4625 1451 128 4625 1451 129 MF = 4 ANGULAR DISTRIBUTIONS OF SECONDARY NEUTRONS 4625 1451 130 LEGENDRE POLYNOMIAL COEFFICIENTS FOR ANGULAR DISTRIBUTIONS ARE 4625 1451 131 GIVEN IN THE CENTER-OF-MASS SYSTEM FOR MT=2 AND DISCRETE INELAS-4625 1451 132 TIC LEVELS, AND IN THE LABORATORY SYSTEM FOR MT=91. THEY WERE 4625 1451 133 CALCULATED WITH CASTHY. FOR OTHER REACTIONS, ISOTROPIC DISTRI- 4625 1451 134 BUTIONS IN THE LABORATORY SYSTEM WERE ASSUMED. 4625 1451 135 4625 1451 136 MF = 5 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS 4625 1451 137 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS WERE CALCULATED WITH 4625 1451 138 PEGASUS FOR INELASTIC SCATTERING FROM OVERLAPPING LEVELS AND FOR4625 1451 139 OTHER NEUTRON EMITTING REACTIONS. 4625 1451 140 4625 1451 141 TABLE 1 NEUTRON OPTICAL POTENTIAL PARAMETERS 4625 1451 142 4625 1451 143 DEPTH (MEV) RADIUS(FM) DIFFUSENESS(FM) 4625 1451 144 ---------------------- ------------ --------------- 4625 1451 145 V = 50.01-0.5528E R0 = 5.972 A0 = 0.56 4625 1451 146 WS = 8.165 RS = 6.594 AS = 0.44 4625 1451 147 VSO= 5.261 RSO= 5.97 ASO= 0.267 4625 1451 148 THE FORM OF SURFACE ABSORPTION PART IS DER. WOODS-SAXON TYPE. 4625 1451 149 4625 1451 150 TABLE 2 LEVEL DENSITY PARAMETERS 4625 1451 151 4625 1451 152 NUCLIDE SYST A(1/MEV) T(MEV) C(1/MEV) EX(MEV) PAIRING 4625 1451 153 --------------------------------------------------------------- 4625 1451 154 44-RU- 98 1.382E+01 7.400E-01 6.070E-01 7.507E+00 2.400E+00 4625 1451 155 44-RU- 99 1.650E+01 6.570E-01 4.016E+00 6.235E+00 1.280E+00 4625 1451 156 44-RU-100 1.520E+01 7.200E-01 7.835E-01 8.078E+00 2.570E+00 4625 1451 157 44-RU-101 1.726E+01 6.700E-01 7.228E+00 6.836E+00 1.280E+00 4625 1451 158 4625 1451 159 45-RH- 99 * 1.386E+01 6.566E-01 1.354E+00 4.866E+00 1.120E+00 4625 1451 160 45-RH-100 * 1.490E+01 6.500E-01 1.162E+01 4.114E+00 0.0 4625 1451 161 45-RH-101 * 1.596E+01 6.476E-01 2.608E+00 5.832E+00 1.290E+00 4625 1451 162 45-RH-102 * 1.703E+01 6.452E-01 3.197E+01 4.966E+00 0.0 4625 1451 163 4625 1451 164 46-PD-100 * 1.400E+01 6.500E-01 1.679E-01 6.179E+00 2.470E+00 4625 1451 165 46-PD-101 1.689E+01 6.410E-01 3.454E+00 6.175E+00 1.350E+00 4625 1451 166 46-PD-102 1.831E+01 6.210E-01 6.406E-01 7.665E+00 2.640E+00 4625 1451 167 46-PD-103 1.733E+01 6.550E-01 5.327E+00 6.637E+00 1.350E+00 4625 1451 168 --------------------------------------------------------------- 4625 1451 169 SYST: * = LDP'S WERE DETERMINED FROM SYSTEMATICS. 4625 1451 170 4625 1451 171 SPIN CUTOFF PARAMETERS WERE CALCULATED AS 0.146*SQRT(A)*A**(2/3).4625 1451 172 IN THE CASTHY CALCULATION, SPIN CUTOFF FACTORS AT 0 MEV WERE 4625 1451 173 ASSUMED TO BE 7.569 FOR PD-102 AND 5.0 FOR PD-103. 4625 1451 174 4625 1451 175 REFERENCES 4625 1451 176 1) KAWAI, M. ET AL.: PROC. INT. CONF. ON NUCLEAR DATA FOR SCIENCE4625 1451 177 AND TECHNOLOGY, MITO, P. 569 (1988). 4625 1451 178 2) MUGHABGHAB, S.F. ET AL.: "NEUTRON CROSS SECTIONS, VOL. I, 4625 1451 179 PART A", ACADEMIC PRESS (1981). 4625 1451 180 3) IGARASI, S.: J. NUCL. SCI. TECHNOL., 12, 67 (1975). 4625 1451 181 4) IIJIMA, S. ET AL.: JAERI-M 87-025, P. 337 (1987). 4625 1451 182 5) FOSTER, D.G. JR. AND GLASGOW, D. W.: PHYS. REV., C3, 576 4625 1451 183 (1971). 4625 1451 184 6) POENITZ, W.P. AND WHALEN, J.F.: ANL-NDM-80 (1983). 4625 1451 185 7) PEREY, F.G: PHYS. REV. 131, 745 (1963). 4625 1451 186 8) HUIZENGA, J.R. AND IGO, G.: NUCL. PHYS. 29, 462 (1962). 4625 1451 187 9) LOHR, J.M. AND HAEBERLI, W.: NUCL. PHYS. A232, 381 (1974). 4625 1451 188 10) BECCHETTI, F.D., JR. AND GREENLEES, G.W.: POLARIZATION 4625 1451 189 PHENOMENA IN NUCLEAR REACTIONS ((EDS) H.H. BARSHALL AND 4625 1451 190 W. HAEBERLI), P. 682, THE UNIVERSITY OF WISCONSIN PRESS. 4625 1451 191 (1971). 4625 1451 192 11) GILBERT, A. AND CAMERON, A.G.W.: CAN. J. PHYS., 43, 1446 4625 1451 193 (1965). 4625 1451 194 12) IIJIMA, S., ET AL.: J. NUCL. SCI. TECHNOL. 21, 10 (1984). 4625 1451 195 13) GRUPPELAAR, H.: ECN-13 (1977). 4625 1451 196 14) ENSDF: EVALUATED NUCLEAR STRUCTURE DATA FILE (JUNE 1987). 4625 1451 197 15) NUCLEAR DATA SHEET, 35, 443 (1982). 4625 1451 198 16) BENZI, V. AND REFFO, G.: CCDN-NW/10 (1969). 4625 1451 199 17) KIKUCHI, K. AND KAWAI, M.: "NUCLEAR MATTER AND NUCLEAR 4625 1451 200 REACTIONS", NORTH HOLLAND (1968). 4625 1451 201 18) FORREST, R.A.: AERE-R 12419 (1986). 4625 1451 202 4625 1451 203 1 451 271 14625 1451 204 2 151 147 14625 1451 205 3 1 31 14625 1451 206 3 2 31 14625 1451 207 3 4 17 14625 1451 208 3 16 8 14625 1451 209 3 17 4 14625 1451 210 3 22 13 14625 1451 211 3 28 10 14625 1451 212 3 32 6 14625 1451 213 3 51 17 14625 1451 214 3 52 15 14625 1451 215 3 53 14 14625 1451 216 3 54 14 14625 1451 217 3 55 14 14625 1451 218 3 56 13 14625 1451 219 3 57 13 14625 1451 220 3 58 12 14625 1451 221 3 59 12 14625 1451 222 3 60 11 14625 1451 223 3 61 11 14625 1451 224 3 62 11 14625 1451 225 3 63 10 14625 1451 226 3 64 10 14625 1451 227 3 65 10 14625 1451 228 3 66 9 14625 1451 229 3 67 9 14625 1451 230 3 68 9 14625 1451 231 3 91 8 14625 1451 232 3 102 23 14625 1451 233 3 103 14 14625 1451 234 3 104 12 14625 1451 235 3 105 9 14625 1451 236 3 106 11 14625 1451 237 3 107 15 14625 1451 238 3 111 11 14625 1451 239 3 251 25 14625 1451 240 4 2 271 14625 1451 241 4 16 10 14625 1451 242 4 17 10 14625 1451 243 4 22 10 14625 1451 244 4 28 10 14625 1451 245 4 32 10 14625 1451 246 4 51 26 14625 1451 247 4 52 23 14625 1451 248 4 53 23 14625 1451 249 4 54 23 14625 1451 250 4 55 23 14625 1451 251 4 56 23 14625 1451 252 4 57 23 14625 1451 253 4 58 23 14625 1451 254 4 59 23 14625 1451 255 4 60 23 14625 1451 256 4 61 23 14625 1451 257 4 62 23 14625 1451 258 4 63 22 14625 1451 259 4 64 23 14625 1451 260 4 65 23 14625 1451 261 4 66 23 14625 1451 262 4 67 23 14625 1451 263 4 68 22 14625 1451 264 4 91 23 14625 1451 265 5 16 57 14625 1451 266 5 17 16 14625 1451 267 5 22 212 14625 1451 268 5 28 98 14625 1451 269 5 32 36 14625 1451 270 5 91 113 14625 1451 271 4625 1 0 272 4625 0 0 273 4.61020+ 4 1.01030+ 2 0 0 1 04625 2151 274 4.61020+ 4 1.00000+ 0 0 0 2 04625 2151 275 1.00000- 5 2.50000+ 2 1 2 0 04625 2151 276 0.0 + 0 6.40000- 1 0 0 1 04625 2151 277 1.01030+ 2 0.0 + 0 0 0 12 24625 2151 278 -1.00000+ 1 5.00000- 1 1.11179- 1 2.17881- 3 1.09000- 1 0.0 + 04625 2151 279 1.90730+ 2 5.00000- 1 3.78000- 1 2.69000- 1 1.09000- 1 0.0 + 04625 2151 280 2.50000+ 2 1.00000+ 5 2 2 0 04625 2151 281 0.0 + 0 4.95110- 1 0 0 3 04625 2151 282 1.01031+ 2 0.0 + 0 0 0 1 04625 2151 283 5.00000- 1 0.0 + 0 5 0 156 254625 2151 284 0.0 + 0 0.0 + 0 0.0 + 0 1.00000+ 0 0.0 + 0 0.0 + 04625 2151 285 2.50000+ 2 1.57830+ 2 0.0 + 0 1.26270- 2 1.50000- 1 0.0 + 04625 2151 286 3.00000+ 2 1.58710+ 2 0.0 + 0 1.26970- 2 1.50000- 1 0.0 + 04625 2151 287 4.00000+ 2 1.60530+ 2 0.0 + 0 1.28420- 2 1.50000- 1 0.0 + 04625 2151 288 5.00000+ 2 1.62350+ 2 0.0 + 0 1.29880- 2 1.50000- 1 0.0 + 04625 2151 289 6.00000+ 2 1.64710+ 2 0.0 + 0 1.31770- 2 1.50000- 1 0.0 + 04625 2151 290 8.00000+ 2 1.68630+ 2 0.0 + 0 1.34900- 2 1.50000- 1 0.0 + 04625 2151 291 1.00000+ 3 1.72660+ 2 0.0 + 0 1.38130- 2 1.50000- 1 0.0 + 04625 2151 292 1.50000+ 3 1.81540+ 2 0.0 + 0 1.45240- 2 1.50000- 1 0.0 + 04625 2151 293 2.00000+ 3 1.91280+ 2 0.0 + 0 1.53030- 2 1.50000- 1 0.0 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1.23388-21 1.21250+ 7 7.12839-22 1.22500+ 7 3.10819-224625 5 22 1929 1.23750+ 7 1.73113-22 1.25000+ 7 7.14516-23 1.26250+ 7 3.72495-234625 5 22 1930 1.27500+ 7 1.38329-23 1.28750+ 7 6.21209-24 1.30000+ 7 1.73367-244625 5 22 1931 1.31250+ 7 3.93973-25 1.32500+ 7 5.40402-29 1.35000+ 7 5.94599-304625 5 22 1932 1.36250+ 7 0.0 + 0 4625 5 22 1933 0.0 + 0 1.80000+ 7 0 0 3 814625 5 22 1934 2 2 80 4 81 24625 5 22 1935 0.0 + 0 0.0 + 0 1.25000+ 5 3.52460- 7 2.50000+ 5 4.96411- 74625 5 22 1936 3.75000+ 5 5.43167- 7 5.00000+ 5 5.46380- 7 7.50000+ 5 5.00087- 74625 5 22 1937 1.12500+ 6 4.04460- 7 1.62500+ 6 2.82593- 7 2.50000+ 6 1.35651- 74625 5 22 1938 3.62500+ 6 4.94482- 8 6.00000+ 6 5.24698- 9 6.62500+ 6 3.02453- 94625 5 22 1939 6.75000+ 6 2.65891- 9 6.87500+ 6 2.39921- 9 7.12500+ 6 1.83301- 94625 5 22 1940 7.37500+ 6 1.21870- 9 7.50000+ 6 9.53550-10 7.62500+ 6 7.66454-104625 5 22 1941 7.75000+ 6 5.85110-10 7.87500+ 6 4.62894-10 8.00000+ 6 3.46036-104625 5 22 1942 8.12500+ 6 2.70009-10 8.25000+ 6 1.97165-10 8.37500+ 6 1.51264-104625 5 22 1943 8.50000+ 6 1.07862-10 8.62500+ 6 8.12277-11 8.75000+ 6 5.61227-114625 5 22 1944 8.87500+ 6 4.13805-11 9.00000+ 6 2.77542-11 9.12500+ 6 2.00131-114625 5 22 1945 9.25000+ 6 1.28984-11 9.37500+ 6 9.05703-12 9.50000+ 6 5.62354-124625 5 22 1946 9.62500+ 6 3.84608-12 9.75000+ 6 2.27051-12 9.87500+ 6 1.50102-124625 5 22 1947 1.00000+ 7 8.45169-13 1.01250+ 7 5.42800-13 1.02500+ 7 2.87076-134625 5 22 1948 1.03750+ 7 1.75943-13 1.05000+ 7 8.72100-14 1.06250+ 7 5.13857-144625 5 22 1949 1.07500+ 7 2.33905-14 1.08750+ 7 1.29107-14 1.10000+ 7 5.40596-154625 5 22 1950 1.11250+ 7 2.86600-15 1.12500+ 7 1.09167-15 1.13750+ 7 5.38582-164625 5 22 1951 1.15000+ 7 1.97873-16 1.16250+ 7 1.05720-16 1.17500+ 7 4.72709-174625 5 22 1952 1.18750+ 7 2.88282-17 1.20000+ 7 1.44679-17 1.21250+ 7 8.78895-184625 5 22 1953 1.22500+ 7 4.38985-18 1.23750+ 7 2.65593-18 1.25000+ 7 1.31979-184625 5 22 1954 1.26250+ 7 7.94713-19 1.27500+ 7 3.92532-19 1.28750+ 7 2.35026-194625 5 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