4.61040+ 4 1.03011+ 2 1 0 0 14631 1451 1 0.0 + 0 0.0 + 0 0 0 0 04631 1451 2 0.0 + 0 0.0 + 0 0 0 204 494631 1451 3 46-PD-104 JNDC EVAL-MAR90 JNDC FP NUCLEAR DATA W.G. 4631 1451 4 DIST-NOV90 4631 1451 5 HISTORY 4631 1451 6 84-10 EVALUATION FOR JENDL-2 WAS MADE BY JNDC FPND W.G./1/ 4631 1451 7 90-03 MODIFICATION FOR JENDL-3 WAS MADE/2/. 4631 1451 8 4631 1451 9 MF = 1 GENERAL INFORMATION 4631 1451 10 MT=451 COMMENTS AND DICTIONARY 4631 1451 11 4631 1451 12 MF = 2 RESONANCE PARAMETERS 4631 1451 13 MT=151 RESOLVED AND UNRESOLVED RESONANCE PARAMETERS 4631 1451 14 RESOLVED RESONANCE REGION (SLBW FORMULA) : BELOW 279 EV 4631 1451 15 RESONANCE PARAMETERS WERE TAKEN FROM JENDL-2; 4631 1451 16 PARAMETERS OF 182.3-EV RESONANCE WERE TAKEN FROM THE DATA 4631 1451 17 MEASURED BY POPOV ET AL./3/ 4631 1451 18 4631 1451 19 UNRESOLVED RESONANCE REGION : 279 EV - 100 KEV 4631 1451 20 THE NEUTRON STRENGTH FUNCTION S1 WAS BASED ON THE COMPILATION 4631 1451 21 OF MUGHABGHAB ET AL./4/, AND S0 AND S2 WERE CALCULATED WITH 4631 1451 22 OPTICAL MODEL CODE CASTHY/5/. THE OBSERVED LEVEL SPACING WAS 4631 1451 23 DETERMINED TO REPRODUCE THE CAPTURE CROSS SECTION CALCULATED 4631 1451 24 WITH CASTHY. THE EFFECTIVE SCATTERING RADIUS WAS OBTAINED 4631 1451 25 FROM FITTING TO THE CALCULATED TOTAL CROSS SECTION AT 100 KEV.4631 1451 26 THE RADIATION WIDTH GG WAS BASED ON THE SYSTEMATICS OF 4631 1451 27 MEASURED VALUES FOR NEIGHBORING NUCLIDES. 4631 1451 28 4631 1451 29 TYPICAL VALUES OF THE PARAMETERS AT 70 KEV: 4631 1451 30 S0 = 0.810E-4, S1 = 5.300E-4, S2 = 1.000E-4, SG = 6.18E-4, 4631 1451 31 GG = 0.160 EV, R = 4.725 FM. 4631 1451 32 4631 1451 33 CALCULATED 2200-M/S CROSS SECTIONS AND RES. INTEGRALS (BARNS) 4631 1451 34 2200 M/S RES. INTEG. 4631 1451 35 TOTAL 5.440 - 4631 1451 36 ELASTIC 4.917 - 4631 1451 37 CAPTURE 0.5231 21.9 4631 1451 38 4631 1451 39 MF = 3 NEUTRON CROSS SECTIONS 4631 1451 40 BELOW 100 KEV, RESONANCE PARAMETERS WERE GIVEN. 4631 1451 41 ABOVE 100 KEV, THE SPHERICAL OPTICAL AND STATISTICAL MODEL 4631 1451 42 CALCULATION WAS PERFORMED WITH CASTHY, BY TAKING ACCOUNT OF 4631 1451 43 COMPETING REACTIONS, OF WHICH CROSS SECTIONS WERE CALCULATED 4631 1451 44 WITH PEGASUS/6/ STANDING ON A PREEQUILIBRIUM AND MULTI-STEP 4631 1451 45 EVAPORATION MODEL. THE OMP'S FOR NEUTRON GIVEN IN TABLE 1 WERE 4631 1451 46 DETERMINED TO REPRODUCE THE CD-NATURAL TOTAL CROSS SECTIONS 4631 1451 47 MEASURED BY FOSTER AND GLASGOW/7/, POENITZ AND WHALEN/8/ AND 4631 1451 48 SO ON, AND APPLIED TO PD ISOTOPES TOO. THE OMP'S FOR CHARGED 4631 1451 49 PARTICLES ARE AS FOLLOWS: 4631 1451 50 PROTON = PEREY/9/ 4631 1451 51 ALPHA = HUIZENGA AND IGO/10/ 4631 1451 52 DEUTERON = LOHR AND HAEBERLI/11/ 4631 1451 53 HELIUM-3 AND TRITON = BECCHETTI AND GREENLEES/12/ 4631 1451 54 PARAMETERS FOR THE COMPOSITE LEVEL DENSITY FORMULA OF GILBERT 4631 1451 55 AND CAMERON/13/ WERE EVALUATED BY IIJIMA ET AL./14/ MORE 4631 1451 56 EXTENSIVE DETERMINATION AND MODIFICATION WERE MADE IN THE 4631 1451 57 PRESENT WORK. TABLE 2 SHOWS THE LEVEL DENSITY PARAMETERS USED 4631 1451 58 IN THE PRESENT CALCULATION. ENERGY DEPENDENCE OF SPIN CUT-OFF 4631 1451 59 PARAMETER IN THE ENERGY RANGE BELOW E-JOINT IS DUE TO GRUPPELAAR4631 1451 60 /15/. 4631 1451 61 4631 1451 62 MT = 1 TOTAL 4631 1451 63 SPHERICAL OPTICAL MODEL CALCULATION WAS ADOPTED. 4631 1451 64 4631 1451 65 MT = 2 ELASTIC SCATTERING 4631 1451 66 CALCULATED AS (TOTAL - SUM OF PARTIAL CROSS SECTIONS). 4631 1451 67 4631 1451 68 MT = 4, 51 - 91 INELASTIC SCATTERING 4631 1451 69 SPHERICAL OPTICAL AND STATISTICAL MODEL CALCULATION WAS 4631 1451 70 ADOPTED. THE LEVEL SCHEME WAS TAKEN FROM REF./16/. 4631 1451 71 4631 1451 72 NO. ENERGY(MEV) SPIN-PARITY DWBA-CAL 4631 1451 73 GR. 0.0 0 + 4631 1451 74 1 0.5558 2 + * 4631 1451 75 2 1.3236 4 + 4631 1451 76 3 1.3336 0 + 4631 1451 77 4 1.3417 2 + 4631 1451 78 5 1.7929 0 + 4631 1451 79 6 1.7938 2 + 4631 1451 80 7 1.8207 3 + 4631 1451 81 8 1.9416 5 + 4631 1451 82 9 2.0824 4 + 4631 1451 83 LEVELS ABOVE 2.2 MEV WERE ASSUMED TO BE OVERLAPPING. 4631 1451 84 4631 1451 85 FOR THE LEVELS WITH AN ASTERISK, THE CONTRIBUTION OF DIRECT 4631 1451 86 INELASTIC SCATTERING CROSS SECTIONS WAS CALCULATED BY THE 4631 1451 87 DWUCK-4 CODE/17/. DEFORMATION PARAMETER (BETA2 = 0.209) WAS 4631 1451 88 BASED ON THE DATA COMPILED BY RAMAN ET AL./18/ 4631 1451 89 4631 1451 90 MT = 102 CAPTURE 4631 1451 91 SPHERICAL OPTICAL AND STATISTICAL MODEL CALCULATION WITH 4631 1451 92 CASTHY/5/ WAS ADOPTED. DIRECT AND SEMI-DIRECT CAPTURE CROSS 4631 1451 93 SECTIONS WERE ESTIMATED ACCORDING TO THE PROCEDURE OF BENZI 4631 1451 94 AND REFFO/19/ AND NORMALIZED TO 1 MILLI-BARN AT 14 MEV. 4631 1451 95 4631 1451 96 THE GAMMA-RAY STRENGTH FUNCTION (6.50E-4) WAS ADJUSTED TO 4631 1451 97 REPRODUCE THE CAPTURE CROSS SECTION OF 220 MILLI-BARNS AT 50 4631 1451 98 KEV MEASURED BY CORNELIS ET AL./20/ 4631 1451 99 4631 1451 100 MT = 16 (N,2N) CROSS SECTION 4631 1451 101 MT = 17 (N,3N) CROSS SECTION 4631 1451 102 MT = 22 (N,N'A) CROSS SECTION 4631 1451 103 MT = 28 (N,N'P) CROSS SECTION 4631 1451 104 MT = 32 (N,N'D) CROSS SECTION 4631 1451 105 MT =103 (N,P) CROSS SECTION 4631 1451 106 MT =104 (N,D) CROSS SECTION 4631 1451 107 MT =105 (N,T) CROSS SECTION 4631 1451 108 MT =106 (N,HE3) CROSS SECTION 4631 1451 109 MT =107 (N,ALPHA) CROSS SECTION 4631 1451 110 THESE REACTION CROSS SECTIONS WERE CALCULATED WITH THE 4631 1451 111 PREEQUILIBRIUM AND MULTI-STEP EVAPORATION MODEL CODE PEGASUS. 4631 1451 112 4631 1451 113 THE KALBACH'S CONSTANT K (= 89.7) WAS ESTIMATED BY THE 4631 1451 114 FORMULA DERIVED FROM KIKUCHI-KAWAI'S FORMALISM/21/ AND LEVEL 4631 1451 115 DENSITY PARAMETERS. 4631 1451 116 4631 1451 117 FINALLY, THE (N,P) AND (N,ALPHA) CROSS SECTIONS WERE 4631 1451 118 NORMALIZED TO THE FOLLOWING VALUES AT 14.5 MEV: 4631 1451 119 (N,P) 58.00 MB (RECOMMENDED BY FORREST/22/) 4631 1451 120 (N,ALPHA) 10.40 MB (SYSTEMATICS OF FORREST/22/) 4631 1451 121 4631 1451 122 MT = 251 MU-BAR 4631 1451 123 CALCULATED WITH CASTHY. 4631 1451 124 4631 1451 125 MF = 4 ANGULAR DISTRIBUTIONS OF SECONDARY NEUTRONS 4631 1451 126 LEGENDRE POLYNOMIAL COEFFICIENTS FOR ANGULAR DISTRIBUTIONS ARE 4631 1451 127 GIVEN IN THE CENTER-OF-MASS SYSTEM FOR MT=2 AND DISCRETE INELAS-4631 1451 128 TIC LEVELS, AND IN THE LABORATORY SYSTEM FOR MT=91. THEY WERE 4631 1451 129 CALCULATED WITH CASTHY. CONTRIBUTION OF DIRECT INELASTIC 4631 1451 130 SCATTERING WAS CALCULATED WITH DWUCK-4. FOR OTHER REACTIONS, 4631 1451 131 ISOTROPIC DISTRIBUTIONS IN THE LABORATORY SYSTEM WERE ASSUMED. 4631 1451 132 4631 1451 133 MF = 5 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS 4631 1451 134 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS WERE CALCULATED WITH 4631 1451 135 PEGASUS FOR INELASTIC SCATTERING FROM OVERLAPPING LEVELS AND FOR4631 1451 136 OTHER NEUTRON EMITTING REACTIONS. 4631 1451 137 4631 1451 138 TABLE 1 NEUTRON OPTICAL POTENTIAL PARAMETERS 4631 1451 139 4631 1451 140 DEPTH (MEV) RADIUS(FM) DIFFUSENESS(FM) 4631 1451 141 ---------------------- ------------ --------------- 4631 1451 142 V = 50.01-0.5528E R0 = 5.972 A0 = 0.56 4631 1451 143 WS = 8.165 RS = 6.594 AS = 0.44 4631 1451 144 VSO= 5.261 RSO= 5.97 ASO= 0.267 4631 1451 145 THE FORM OF SURFACE ABSORPTION PART IS DER. WOODS-SAXON TYPE. 4631 1451 146 4631 1451 147 TABLE 2 LEVEL DENSITY PARAMETERS 4631 1451 148 4631 1451 149 NUCLIDE SYST A(1/MEV) T(MEV) C(1/MEV) EX(MEV) PAIRING 4631 1451 150 --------------------------------------------------------------- 4631 1451 151 44-RU-100 1.520E+01 7.200E-01 7.835E-01 8.078E+00 2.570E+00 4631 1451 152 44-RU-101 1.726E+01 6.700E-01 7.228E+00 6.836E+00 1.280E+00 4631 1451 153 44-RU-102 1.643E+01 6.550E-01 8.872E-01 7.106E+00 2.220E+00 4631 1451 154 44-RU-103 1.890E+01 6.480E-01 1.210E+01 7.110E+00 1.280E+00 4631 1451 155 4631 1451 156 45-RH-101 * 1.596E+01 6.476E-01 2.608E+00 5.832E+00 1.290E+00 4631 1451 157 45-RH-102 * 1.703E+01 6.452E-01 3.197E+01 4.966E+00 0.0 4631 1451 158 45-RH-103 1.570E+01 6.550E-01 4.298E+00 5.499E+00 9.400E-01 4631 1451 159 45-RH-104 1.714E+01 5.910E-01 1.771E+01 4.018E+00 0.0 4631 1451 160 4631 1451 161 46-PD-102 1.831E+01 6.210E-01 6.406E-01 7.665E+00 2.640E+00 4631 1451 162 46-PD-103 1.733E+01 6.550E-01 5.327E+00 6.637E+00 1.350E+00 4631 1451 163 46-PD-104 1.630E+01 6.650E-01 8.743E-01 7.305E+00 2.290E+00 4631 1451 164 46-PD-105 1.791E+01 6.700E-01 9.137E+00 7.207E+00 1.350E+00 4631 1451 165 --------------------------------------------------------------- 4631 1451 166 SYST: * = LDP'S WERE DETERMINED FROM SYSTEMATICS. 4631 1451 167 4631 1451 168 SPIN CUTOFF PARAMETERS WERE CALCULATED AS 0.146*SQRT(A)*A**(2/3).4631 1451 169 IN THE CASTHY CALCULATION, SPIN CUTOFF FACTORS AT 0 MEV WERE 4631 1451 170 ASSUMED TO BE 5.680 FOR PD-104 AND 6.279 FOR PD-105. 4631 1451 171 4631 1451 172 REFERENCES 4631 1451 173 1) AOKI, T. ET AL.: PROC. INT. CONF. ON NUCLEAR DATA FOR BASIC 4631 1451 174 AND APPLIED SCIENCE, SANTA FE., VOL. 2, P.1627 (1985). 4631 1451 175 2) KAWAI, M. ET AL.: PROC. INT. CONF. ON NUCLEAR DATA FOR SCIENCE4631 1451 176 AND TECHNOLOGY, MITO, P. 569 (1988). 4631 1451 177 3) POPOV, JU. P., ET AL.: JINR-P3-11013 (1977). 4631 1451 178 4) MUGHABGHAB, S.F. ET AL.: "NEUTRON CROSS SECTIONS, VOL. I, 4631 1451 179 PART A", ACADEMIC PRESS (1981). 4631 1451 180 5) IGARASI, S.: J. NUCL. SCI. TECHNOL., 12, 67 (1975). 4631 1451 181 6) IIJIMA, S. ET AL.: JAERI-M 87-025, P. 337 (1987). 4631 1451 182 7) FOSTER, D.G. JR. AND GLASGOW, D. W.: PHYS. REV., C3, 576 4631 1451 183 (1971). 4631 1451 184 8) POENITZ, W.P. AND WHALEN, J.F.: ANL-NDM-80 (1983). 4631 1451 185 9) PEREY, F.G: PHYS. REV. 131, 745 (1963). 4631 1451 186 10) HUIZENGA, J.R. AND IGO, G.: NUCL. PHYS. 29, 462 (1962). 4631 1451 187 11) LOHR, J.M. AND HAEBERLI, W.: NUCL. PHYS. A232, 381 (1974). 4631 1451 188 12) BECCHETTI, F.D., JR. AND GREENLEES, G.W.: POLARIZATION 4631 1451 189 PHENOMENA IN NUCLEAR REACTIONS ((EDS) H.H. BARSHALL AND 4631 1451 190 W. HAEBERLI), P. 682, THE UNIVERSITY OF WISCONSIN PRESS. 4631 1451 191 (1971). 4631 1451 192 13) GILBERT, A. AND CAMERON, A.G.W.: CAN. J. PHYS., 43, 1446 4631 1451 193 (1965). 4631 1451 194 14) IIJIMA, S., ET AL.: J. NUCL. SCI. TECHNOL. 21, 10 (1984). 4631 1451 195 15) GRUPPELAAR, H.: ECN-13 (1977). 4631 1451 196 16) MATSUMOTO, J., ET AL.: JAERI-M 7734 (1978). 4631 1451 197 17) KUNZ, P.D.: PRIVATE COMMUNICATION. 4631 1451 198 18) RAMAN, S., ET AL.: ATOM. DATA AND NUCL. DATA TABLES 36, 1 4631 1451 199 (1987) 4631 1451 200 19) BENZI, V. AND REFFO, G.: CCDN-NW/10 (1969). 4631 1451 201 20) CORNELIS, E., ET AL.: PROC. INT. CONF. NUCLEAR DATA FOR 4631 1451 202 SCIENCE AND TECHNOLOGY, ANTWERP 1982, P.222 (1982). 4631 1451 203 21) KIKUCHI, K. AND KAWAI, M.: "NUCLEAR MATTER AND NUCLEAR 4631 1451 204 REACTIONS", NORTH HOLLAND (1968). 4631 1451 205 22) FORREST, R.A.: AERE-R 12419 (1986). 4631 1451 206 4631 1451 207 1 451 256 14631 1451 208 2 151 146 14631 1451 209 3 1 25 14631 1451 210 3 2 25 14631 1451 211 3 4 14 14631 1451 212 3 16 8 14631 1451 213 3 17 5 14631 1451 214 3 22 13 14631 1451 215 3 28 10 14631 1451 216 3 32 6 14631 1451 217 3 51 14 14631 1451 218 3 52 12 14631 1451 219 3 53 12 14631 1451 220 3 54 11 14631 1451 221 3 55 10 14631 1451 222 3 56 10 14631 1451 223 3 57 10 14631 1451 224 3 58 9 14631 1451 225 3 59 9 14631 1451 226 3 91 8 14631 1451 227 3 102 20 14631 1451 228 3 103 14 14631 1451 229 3 104 11 14631 1451 230 3 105 9 14631 1451 231 3 106 11 14631 1451 232 3 107 15 14631 1451 233 3 251 22 14631 1451 234 4 2 244 14631 1451 235 4 16 10 14631 1451 236 4 17 10 14631 1451 237 4 22 10 14631 1451 238 4 28 10 14631 1451 239 4 32 10 14631 1451 240 4 51 100 14631 1451 241 4 52 23 14631 1451 242 4 53 23 14631 1451 243 4 54 23 14631 1451 244 4 55 23 14631 1451 245 4 56 23 14631 1451 246 4 57 23 14631 1451 247 4 58 23 14631 1451 248 4 59 23 14631 1451 249 4 91 23 14631 1451 250 5 16 56 14631 1451 251 5 17 20 14631 1451 252 5 22 208 14631 1451 253 5 28 91 14631 1451 254 5 32 32 14631 1451 255 5 91 123 14631 1451 256 4631 1 0 257 4631 0 0 258 4.61040+ 4 1.03011+ 2 0 0 1 04631 2151 259 4.61040+ 4 1.00000+ 0 0 0 2 04631 2151 260 1.00000- 5 2.79000+ 2 1 1 0 04631 2151 261 0.0 + 0 6.50000- 1 0 0 1 04631 2151 262 1.03011+ 2 0.0 + 0 0 0 6 14631 2151 263 1.86000+ 2 5.00000- 1 4.89000- 1 2.70000- 1 2.19000- 1 0.0 + 04631 2151 264 2.79000+ 2 1.00000+ 5 2 2 0 04631 2151 265 0.0 + 0 4.72530- 1 0 0 3 04631 2151 266 1.03010+ 2 0.0 + 0 0 0 1 04631 2151 267 5.00000- 1 0.0 + 0 5 0 156 254631 2151 268 0.0 + 0 0.0 + 0 0.0 + 0 1.00000+ 0 0.0 + 0 0.0 + 04631 2151 269 2.79000+ 2 2.53725+ 2 0.0 + 0 2.05514- 2 1.60000- 1 0.0 + 04631 2151 270 3.00000+ 2 2.54510+ 2 0.0 + 0 2.06150- 2 1.60000- 1 0.0 + 04631 2151 271 4.00000+ 2 2.57100+ 2 0.0 + 0 2.08250- 2 1.60000- 1 0.0 + 04631 2151 272 5.00000+ 2 2.61020+ 2 0.0 + 0 2.11430- 2 1.60000- 1 0.0 + 04631 2151 273 6.00000+ 2 2.65100+ 2 0.0 + 0 2.14730- 2 1.60000- 1 0.0 + 04631 2151 274 8.00000+ 2 2.73510+ 2 0.0 + 0 2.21550- 2 1.60000- 1 0.0 + 04631 2151 275 1.00000+ 3 2.81980+ 2 0.0 + 0 2.28410- 2 1.60000- 1 0.0 + 04631 2151 276 1.50000+ 3 3.02460+ 2 0.0 + 0 2.44990- 2 1.60000- 1 0.0 + 04631 2151 277 2.00000+ 3 3.19590+ 2 0.0 + 0 2.58870- 2 1.60000- 1 0.0 + 04631 2151 278 3.00000+ 3 3.41200+ 2 0.0 + 0 2.76370- 2 1.60000- 1 0.0 + 04631 2151 279 4.00000+ 3 3.51280+ 2 0.0 + 0 2.84530- 2 1.60000- 1 0.0 + 04631 2151 280 5.00000+ 3 3.52520+ 2 0.0 + 0 2.85540- 2 1.60000- 1 0.0 + 04631 2151 281 6.00000+ 3 3.50330+ 2 0.0 + 0 2.83770- 2 1.60000- 1 0.0 + 04631 2151 282 7.00000+ 3 3.46180+ 2 0.0 + 0 2.80410- 2 1.60000- 1 0.0 + 04631 2151 283 8.00000+ 3 3.40500+ 2 0.0 + 0 2.75810- 2 1.60000- 1 0.0 + 04631 2151 284 1.00000+ 4 3.32040+ 2 0.0 + 0 2.68950- 2 1.60000- 1 0.0 + 04631 2151 285 1.50000+ 4 3.14980+ 2 0.0 + 0 2.55130- 2 1.60000- 1 0.0 + 04631 2151 286 2.50000+ 4 2.94430+ 2 0.0 + 0 2.38490- 2 1.60000- 1 0.0 + 04631 2151 287 3.00000+ 4 2.87750+ 2 0.0 + 0 2.33080- 2 1.60000- 1 0.0 + 04631 2151 288 4.00000+ 4 2.78830+ 2 0.0 + 0 2.25850- 2 1.60000- 1 0.0 + 04631 2151 289 5.00000+ 4 2.70000+ 2 0.0 + 0 2.18700- 2 1.60000- 1 0.0 + 04631 2151 290 6.00000+ 4 2.63800+ 2 0.0 + 0 2.13680- 2 1.60000- 1 0.0 + 04631 2151 291 7.00000+ 4 2.58990+ 2 0.0 + 0 2.09780- 2 1.60000- 1 0.0 + 04631 2151 292 8.00000+ 4 2.53740+ 2 0.0 + 0 2.05530- 2 1.60000- 1 0.0 + 04631 2151 293 1.00000+ 5 2.44020+ 2 0.0 + 0 1.97660- 2 1.60000- 1 0.0 + 04631 2151 294 1.03010+ 2 0.0 + 0 1 0 2 04631 2151 295 5.00000- 1 0.0 + 0 5 0 156 254631 2151 296 0.0 + 0 0.0 + 0 0.0 + 0 1.00000+ 0 0.0 + 0 0.0 + 04631 2151 297 2.79000+ 2 2.53725+ 2 0.0 + 0 1.34474- 1 1.60000- 1 0.0 + 04631 2151 298 3.00000+ 2 2.54510+ 2 0.0 + 0 1.34890- 1 1.60000- 1 0.0 + 04631 2151 299 4.00000+ 2 2.57100+ 2 0.0 + 0 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