4.61100+ 4 1.08961+ 2 1 0 0 14649 1451 1 0.0 + 0 0.0 + 0 0 0 0 04649 1451 2 0.0 + 0 0.0 + 0 0 0 210 474649 1451 3 46-PD-110 JNDC EVAL-MAR90 JNDC FP NUCLEAR DATA W.G. 4649 1451 4 DIST-NOV90 4649 1451 5 HISTORY 4649 1451 6 84-10 EVALUATION FOR JENDL-2 WAS MADE BY JNDC FPND W.G./1/ 4649 1451 7 90-03 MODIFICATION FOR JENDL-3 WAS MADE/2/. 4649 1451 8 4649 1451 9 MF = 1 GENERAL INFORMATION 4649 1451 10 MT=451 COMMENTS AND DICTIONARY 4649 1451 11 4649 1451 12 MF = 2 RESONANCE PARAMETERS 4649 1451 13 MT=151 RESOLVED AND UNRESOLVED RESONANCE PARAMETERS 4649 1451 14 RESOLVED RESONANCE REGION (MLBW FORMULA) : BELOW 8 KEV 4649 1451 15 RESONANCE PARAMETERS ARE THE SAME AS JENDL-2 WHICH WERE MAINLY4649 1451 16 TAKEN FROM THE RECOMMENDATION BY MUGHABGHAB ET AL./3/ AVERAGE 4649 1451 17 RADIATION WIDTH OF 0.06 EV/3/ WAS ASSUMED. A NEGATIVE 4649 1451 18 RESONANCE WAS ADDED AT -20 EV SO AS TO REPRODUCE THE THERMAL 4649 1451 19 CAPTURE CROSS SECTIONS GIVEN BY MUGHABGHAB ET AL. 4649 1451 20 4649 1451 21 UNRESOLVED RESONANCE REGION : 8 KEV - 100 KEV 4649 1451 22 THE NEUTRON STRENGTH FUNCTION S1 WAS BASED ON THE COMPILATION 4649 1451 23 OF MUGHABGHAB ET AL./3/, AND S0 AND S2 WERE CALCULATED WITH 4649 1451 24 OPTICAL MODEL CODE CASTHY/4/. THE OBSERVED LEVEL SPACING WAS 4649 1451 25 DETERMINED TO REPRODUCE THE CAPTURE CROSS SECTION CALCULATED 4649 1451 26 WITH CASTHY. THE EFFECTIVE SCATTERING RADIUS WAS OBTAINED 4649 1451 27 FROM FITTING TO THE CALCULATED TOTAL CROSS SECTION AT 100 KEV.4649 1451 28 THE RADIATION WIDTH GG WAS BASED ON THE COMPILATION OF 4649 1451 29 MUGHABGHAB ET AL. 4649 1451 30 4649 1451 31 TYPICAL VALUES OF THE PARAMETERS AT 70 KEV: 4649 1451 32 S0 = 0.810E-4, S1 = 6.000E-4, S2 = 0.950E-4, SG = 2.64E-4, 4649 1451 33 GG = 0.060 EV, R = 4.124 FM. 4649 1451 34 4649 1451 35 CALCULATED 2200-M/S CROSS SECTIONS AND RES. INTEGRALS (BARNS) 4649 1451 36 2200 M/S RES. INTEG. 4649 1451 37 TOTAL 5.222 - 4649 1451 38 ELASTIC 4.995 - 4649 1451 39 CAPTURE 0.2270 2.82 4649 1451 40 4649 1451 41 MF = 3 NEUTRON CROSS SECTIONS 4649 1451 42 BELOW 100 KEV, RESONANCE PARAMETERS WERE GIVEN. 4649 1451 43 ABOVE 100 KEV, THE SPHERICAL OPTICAL AND STATISTICAL MODEL 4649 1451 44 CALCULATION WAS PERFORMED WITH CASTHY/4/, BY TAKING ACCOUNT OF 4649 1451 45 COMPETING REACTIONS, OF WHICH CROSS SECTIONS WERE CALCULATED 4649 1451 46 WITH PEGASUS/5/ STANDING ON A PREEQUILIBRIUM AND MULTI-STEP 4649 1451 47 EVAPORATION MODEL. THE OMP'S FOR NEUTRON GIVEN IN TABLE 1 WERE 4649 1451 48 DETERMINED TO REPRODUCE THE CD-NATURAL TOTAL CROSS SECTIONS 4649 1451 49 MEASURED BY FOSTER AND GLASGOW/6/, POENITZ AND WHALEN/7/ AND 4649 1451 50 SO ON, AND APPLIED TO PD ISOTOPES. THE OMP'S FOR CHARGED 4649 1451 51 PARTICLES ARE AS FOLLOWS: 4649 1451 52 PROTON = PEREY/8/ 4649 1451 53 ALPHA = HUIZENGA AND IGO/9/ 4649 1451 54 DEUTERON = LOHR AND HAEBERLI/10/ 4649 1451 55 HELIUM-3 AND TRITON = BECCHETTI AND GREENLEES/11/ 4649 1451 56 PARAMETERS FOR THE COMPOSITE LEVEL DENSITY FORMULA OF GILBERT 4649 1451 57 AND CAMERON/12/ WERE EVALUATED BY IIJIMA ET AL./13/ MORE 4649 1451 58 EXTENSIVE DETERMINATION AND MODIFICATION WERE MADE IN THE 4649 1451 59 PRESENT WORK. TABLE 2 SHOWS THE LEVEL DENSITY PARAMETERS USED 4649 1451 60 IN THE PRESENT CALCULATION. ENERGY DEPENDENCE OF SPIN CUT-OFF 4649 1451 61 PARAMETER IN THE ENERGY RANGE BELOW E-JOINT IS DUE TO GRUPPELAAR4649 1451 62 /14/. 4649 1451 63 4649 1451 64 MT = 1 TOTAL 4649 1451 65 SPHERICAL OPTICAL MODEL CALCULATION WAS ADOPTED. 4649 1451 66 4649 1451 67 MT = 2 ELASTIC SCATTERING 4649 1451 68 CALCULATED AS (TOTAL - SUM OF PARTIAL CROSS SECTIONS). 4649 1451 69 4649 1451 70 MT = 4, 51 - 91 INELASTIC SCATTERING 4649 1451 71 SPHERICAL OPTICAL AND STATISTICAL MODEL CALCULATION WAS 4649 1451 72 ADOPTED. THE LEVEL SCHEME WAS TAKEN FROM REF./15/. 4649 1451 73 4649 1451 74 NO. ENERGY(MEV) SPIN-PARITY DWBA CAL. 4649 1451 75 GR. 0.0 0 + 4649 1451 76 1 0.3738 2 + * 4649 1451 77 2 0.8138 2 + 4649 1451 78 3 0.9205 4 + 4649 1451 79 4 0.9463 0 + 4649 1451 80 5 1.1710 0 + 4649 1451 81 6 1.2124 3 + 4649 1451 82 7 1.2145 2 + 4649 1451 83 8 1.3980 4 + 4649 1451 84 9 1.4701 1 + 4649 1451 85 10 1.5739 6 + 4649 1451 86 LEVELS ABOVE 1.67 MEV WERE ASSUMED TO BE OVERLAPPING. 4649 1451 87 4649 1451 88 FOR THE LEVELS WITH AN ASTERISK, THE CONTRIBUTION OF DIRECT 4649 1451 89 INELASTIC SCATTERING CROSS SECTIONS WAS CALCULATED BY THE 4649 1451 90 DWUCK-4 CODE/16/. DEFORMATION PARAMETER (BETA2 = 257) WAS 4649 1451 91 BASED ON THE DATA COMPILED BY RAMAN ET AL./17/ 4649 1451 92 4649 1451 93 MT = 102 CAPTURE 4649 1451 94 SPHERICAL OPTICAL AND STATISTICAL MODEL CALCULATION WITH 4649 1451 95 CASTHY/4/ WAS ADOPTED. DIRECT AND SEMI-DIRECT CAPTURE CROSS 4649 1451 96 SECTIONS WERE ESTIMATED ACCORDING TO THE PROCEDURE OF BENZI 4649 1451 97 AND REFFO/18/ AND NORMALIZED TO 1 MILLI-BARN AT 14 MEV. 4649 1451 98 4649 1451 99 THE GAMMA-RAY STRENGTH FUNCTION (2.65E-4) WAS ADJUSTED TO 4649 1451 100 REPRODUCE THE CAPTURE CROSS SECTION OF 80.0 MILLI-BARNS AT 1004649 1451 101 KEV MEASURED BY MACKLIN ET AL./19,20/ AND CORNELIS ET AL. 4649 1451 102 /21/ 4649 1451 103 4649 1451 104 MT = 16 (N,2N) CROSS SECTION 4649 1451 105 MT = 17 (N,3N) CROSS SECTION 4649 1451 106 MT = 22 (N,N'A) CROSS SECTION 4649 1451 107 MT = 28 (N,N'P) CROSS SECTION 4649 1451 108 MT =103 (N,P) CROSS SECTION 4649 1451 109 MT =104 (N,D) CROSS SECTION 4649 1451 110 MT =105 (N,T) CROSS SECTION 4649 1451 111 MT =107 (N,ALPHA) CROSS SECTION 4649 1451 112 THESE REACTION CROSS SECTIONS WERE CALCULATED WITH THE 4649 1451 113 PREEQUILIBRIUM AND MULTI-STEP EVAPORATION MODEL CODE PEGASUS. 4649 1451 114 4649 1451 115 THE KALBACH'S CONSTANT K (= 61.9) WAS ESTIMATED BY THE 4649 1451 116 FORMULA DERIVED FROM KIKUCHI-KAWAI'S FORMALISM/22/ AND LEVEL 4649 1451 117 DENSITY PARAMETERS. 4649 1451 118 4649 1451 119 FINALLY, THE (N,P) AND (N,ALPHA) CROSS SECTIONS WERE 4649 1451 120 NORMALIZED TO THE FOLLOWING VALUES AT 14.5 MEV: 4649 1451 121 (N,P) 5.57 MB (SYSTEMATICS OF FORREST/23/) 4649 1451 122 (N,ALPHA) 1.17 MB (SYSTEMATICS OF FORREST) 4649 1451 123 4649 1451 124 MT = 251 MU-BAR 4649 1451 125 CALCULATED WITH CASTHY. 4649 1451 126 4649 1451 127 MF = 4 ANGULAR DISTRIBUTIONS OF SECONDARY NEUTRONS 4649 1451 128 LEGENDRE POLYNOMIAL COEFFICIENTS FOR ANGULAR DISTRIBUTIONS ARE 4649 1451 129 GIVEN IN THE CENTER-OF-MASS SYSTEM FOR MT=2 AND DISCRETE INELAS-4649 1451 130 TIC LEVELS, AND IN THE LABORATORY SYSTEM FOR MT=91. THEY WERE 4649 1451 131 CALCULATED WITH CASTHY. CONTRIBUTION OF DIRECT INELASTIC 4649 1451 132 SCATTERING WAS CALCULATED WITH DWUCK-4. FOR OTHER REACTIONS, 4649 1451 133 ISOTROPIC DISTRIBUTIONS IN THE LABORATORY SYSTEM WERE ASSUMED. 4649 1451 134 4649 1451 135 MF = 5 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS 4649 1451 136 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS WERE CALCULATED WITH 4649 1451 137 PEGASUS FOR INELASTIC SCATTERING FROM OVERLAPPING LEVELS AND FOR4649 1451 138 OTHER NEUTRON EMITTING REACTIONS. 4649 1451 139 4649 1451 140 TABLE 1 NEUTRON OPTICAL POTENTIAL PARAMETERS 4649 1451 141 4649 1451 142 DEPTH (MEV) RADIUS(FM) DIFFUSENESS(FM) 4649 1451 143 ---------------------- ------------ --------------- 4649 1451 144 V = 50.01-0.5528E R0 = 5.972 A0 = 0.56 4649 1451 145 WS = 8.165 RS = 6.594 AS = 0.44 4649 1451 146 VSO= 5.261 RSO= 5.97 ASO= 0.267 4649 1451 147 THE FORM OF SURFACE ABSORPTION PART IS DER. WOODS-SAXON TYPE. 4649 1451 148 4649 1451 149 TABLE 2 LEVEL DENSITY PARAMETERS 4649 1451 150 4649 1451 151 NUCLIDE SYST A(1/MEV) T(MEV) C(1/MEV) EX(MEV) PAIRING 4649 1451 152 --------------------------------------------------------------- 4649 1451 153 44-RU-106 1.870E+01 6.300E-01 1.097E+00 7.896E+00 2.530E+00 4649 1451 154 44-RU-107 2.030E+01 6.000E-01 1.043E+01 6.637E+00 1.280E+00 4649 1451 155 44-RU-108 * 1.826E+01 6.306E-01 1.050E+00 7.617E+00 2.420E+00 4649 1451 156 44-RU-109 * 1.807E+01 6.282E-01 5.592E+00 6.353E+00 1.280E+00 4649 1451 157 4649 1451 158 45-RH-107 1.963E+01 5.480E-01 3.151E+00 5.336E+00 1.250E+00 4649 1451 159 45-RH-108 * 1.861E+01 6.306E-01 5.818E+01 5.341E+00 0.0 4649 1451 160 45-RH-109 1.608E+01 6.270E-01 2.572E+00 5.371E+00 1.140E+00 4649 1451 161 45-RH-110 * 1.824E+01 6.258E-01 4.505E+01 5.092E+00 0.0 4649 1451 162 4649 1451 163 46-PD-108 1.790E+01 6.460E-01 8.844E-01 7.957E+00 2.600E+00 4649 1451 164 46-PD-109 2.071E+01 6.030E-01 1.194E+01 6.925E+00 1.350E+00 4649 1451 165 46-PD-110 1.880E+01 6.300E-01 1.215E+00 7.897E+00 2.490E+00 4649 1451 166 46-PD-111 2.143E+01 5.610E-01 7.376E+00 6.267E+00 1.350E+00 4649 1451 167 --------------------------------------------------------------- 4649 1451 168 SYST: * = LDP'S WERE DETERMINED FROM SYSTEMATICS. 4649 1451 169 4649 1451 170 SPIN CUTOFF PARAMETERS WERE CALCULATED AS 0.146*SQRT(A)*A**(2/3).4649 1451 171 IN THE CASTHY CALCULATION, SPIN CUTOFF FACTORS AT 0 MEV WERE 4649 1451 172 ASSUMED TO BE 5.824 FOR PD-110 AND 5.0 FOR PD-111. 4649 1451 173 4649 1451 174 REFERENCES 4649 1451 175 1) AOKI, T. ET AL.: PROC. INT. CONF. ON NUCLEAR DATA FOR BASIC 4649 1451 176 AND APPLIED SCIENCE, SANTA FE., VOL. 2, P.1627 (1985). 4649 1451 177 2) KAWAI, M. ET AL.: PROC. INT. CONF. ON NUCLEAR DATA FOR SCIENCE4649 1451 178 AND TECHNOLOGY, MITO, P. 569 (1988). 4649 1451 179 3) MUGHABGHAB, S.F. ET AL.: "NEUTRON CROSS SECTIONS, VOL. I, 4649 1451 180 PART A", ACADEMIC PRESS (1981). 4649 1451 181 4) IGARASI, S.: J. NUCL. SCI. TECHNOL., 12, 67 (1975). 4649 1451 182 5) IIJIMA, S. ET AL.: JAERI-M 87-025, P. 337 (1987). 4649 1451 183 6) FOSTER, D.G. JR. AND GLASGOW, D. W.: PHYS. REV., C3, 576 4649 1451 184 (1971). 4649 1451 185 7) POENITZ, W.P. AND WHALEN, J.F.: ANL-NDM-80 (1983). 4649 1451 186 8) PEREY, F.G: PHYS. REV. 131, 745 (1963). 4649 1451 187 9) HUIZENGA, J.R. AND IGO, G.: NUCL. PHYS. 29, 462 (1962). 4649 1451 188 10) LOHR, J.M. AND HAEBERLI, W.: NUCL. PHYS. A232, 381 (1974). 4649 1451 189 11) BECCHETTI, F.D., JR. AND GREENLEES, G.W.: POLARIZATION 4649 1451 190 PHENOMENA IN NUCLEAR REACTIONS ((EDS) H.H. BARSHALL AND 4649 1451 191 W. HAEBERLI), P. 682, THE UNIVERSITY OF WISCONSIN PRESS. 4649 1451 192 (1971). 4649 1451 193 12) GILBERT, A. AND CAMERON, A.G.W.: CAN. J. PHYS., 43, 1446 4649 1451 194 (1965). 4649 1451 195 13) IIJIMA, S., ET AL.: J. NUCL. SCI. TECHNOL. 21, 10 (1984). 4649 1451 196 14) GRUPPELAAR, H.: ECN-13 (1977). 4649 1451 197 15) MATSUMOTO, J., ET AL.: JAERI-M 7734 (1978). 4649 1451 198 16) KUNZ, P.D.: PRIVATE COMMUNICATION. 4649 1451 199 17) RAMAN, S., ET AL.: ATOM. DATA AND NUCL. DATA TABLES 36, 1 4649 1451 200 (1987) 4649 1451 201 18) BENZI, V. AND REFFO, G.: CCDN-NW/10 (1969). 4649 1451 202 19) MACKLIN, R.L., ET AL.: PROC. SPECIALISTS' MEETING ON NEUTRON 4649 1451 203 CROSS SECTIONS OF FISSION PRODUCTS, BOLOGNA 1979, NEANDC(E) 4649 1451 204 209L, 103. 4649 1451 205 20) MACKLIN, R.L. AND WINTERS, R.R.: NUCL. SCI. ENG., 78, 110 4649 1451 206 110(1981). 4649 1451 207 21) CORNELIS, E., ET AL.: PROC. INT. CONF. NUCLEAR DATA FOR 4649 1451 208 SCIENCE AND TECHNOLOGY, ANTWERP 1982, P.222 (1982). 4649 1451 209 22) KIKUCHI, K. AND KAWAI, M.: "NUCLEAR MATTER AND NUCLEAR 4649 1451 210 REACTIONS", NORTH HOLLAND (1968). 4649 1451 211 23) FORREST, R.A.: AERE-R 12419 (1986). 4649 1451 212 4649 1451 213 1 451 260 14649 1451 214 2 151 182 14649 1451 215 3 1 26 14649 1451 216 3 2 26 14649 1451 217 3 4 15 14649 1451 218 3 16 10 14649 1451 219 3 17 6 14649 1451 220 3 22 13 14649 1451 221 3 28 9 14649 1451 222 3 51 15 14649 1451 223 3 52 13 14649 1451 224 3 53 13 14649 1451 225 3 54 12 14649 1451 226 3 55 12 14649 1451 227 3 56 11 14649 1451 228 3 57 11 14649 1451 229 3 58 10 14649 1451 230 3 59 10 14649 1451 231 3 60 9 14649 1451 232 3 91 9 14649 1451 233 3 102 21 14649 1451 234 3 103 12 14649 1451 235 3 104 11 14649 1451 236 3 105 9 14649 1451 237 3 107 15 14649 1451 238 3 251 23 14649 1451 239 4 2 247 14649 1451 240 4 16 10 14649 1451 241 4 17 10 14649 1451 242 4 22 10 14649 1451 243 4 28 10 14649 1451 244 4 51 104 14649 1451 245 4 52 26 14649 1451 246 4 53 26 14649 1451 247 4 54 26 14649 1451 248 4 55 23 14649 1451 249 4 56 23 14649 1451 250 4 57 23 14649 1451 251 4 58 23 14649 1451 252 4 59 23 14649 1451 253 4 60 23 14649 1451 254 4 91 23 14649 1451 255 5 16 60 14649 1451 256 5 17 35 14649 1451 257 5 22 164 14649 1451 258 5 28 75 14649 1451 259 5 91 130 14649 1451 260 4649 1 0 261 4649 0 0 262 4.61100+ 4 1.08961+ 2 0 0 1 04649 2151 263 4.61100+ 4 1.00000+ 0 0 0 2 04649 2151 264 1.00000- 5 8.00000+ 3 1 2 0 04649 2151 265 0.0 + 0 6.50000- 1 0 0 1 04649 2151 266 1.08961+ 2 0.0 + 0 0 0 642 1074649 2151 267 -2.00000+ 1 5.00000- 1 7.19000- 2 1.30000- 3 7.06000- 2 0.0 + 04649 2151 268 8.63300+ 1 5.00000- 1 6.04800- 2 4.80000- 4 6.00000- 2 0.0 + 04649 2151 269 1.76900+ 2 5.00000- 1 6.02400- 2 2.40000- 4 6.00000- 2 0.0 + 04649 2151 270 2.63200+ 2 5.00000- 1 6.55000- 2 5.50000- 3 6.00000- 2 0.0 + 04649 2151 271 5.53700+ 2 5.00000- 1 6.47000- 2 4.70000- 3 6.00000- 2 0.0 + 04649 2151 272 5.78800+ 2 5.00000- 1 6.09100- 2 9.10000- 4 6.00000- 2 0.0 + 04649 2151 273 6.36500+ 2 5.00000- 1 6.07100- 2 7.10000- 4 6.00000- 2 0.0 + 04649 2151 274 7.35100+ 2 5.00000- 1 6.12700- 2 1.27000- 3 6.00000- 2 0.0 + 04649 2151 275 8.57900+ 2 5.00000- 1 8.88000- 2 2.88000- 2 6.00000- 2 0.0 + 04649 2151 276 8.99900+ 2 5.00000- 1 1.69000- 1 1.22000- 1 4.70000- 2 0.0 + 04649 2151 277 9.54000+ 2 5.00000- 1 6.68000- 2 6.80000- 3 6.00000- 2 0.0 + 04649 2151 278 9.58000+ 2 5.00000- 1 7.75000- 2 1.75000- 2 6.00000- 2 0.0 + 04649 2151 279 1.00400+ 3 5.00000- 1 1.20000- 1 6.00000- 2 6.00000- 2 0.0 + 04649 2151 280 1.17400+ 3 5.00000- 1 8.46000- 2 2.46000- 2 6.00000- 2 0.0 + 04649 2151 281 1.32100+ 3 5.00000- 1 7.94000- 2 1.94000- 2 6.00000- 2 0.0 + 04649 2151 282 1.42900+ 3 5.00000- 1 6.54000- 2 5.40000- 3 6.00000- 2 0.0 + 04649 2151 283 1.60600+ 3 5.00000- 1 7.54000- 2 1.54000- 2 6.00000- 2 0.0 + 04649 2151 284 1.66500+ 3 5.00000- 1 1.01700+ 0 9.60000- 1 5.70000- 2 0.0 + 04649 2151 285 1.69400+ 3 5.00000- 1 8.32000- 2 2.32000- 2 6.00000- 2 0.0 + 04649 2151 286 1.78900+ 3 5.00000- 1 6.30000- 2 3.00000- 3 6.00000- 2 0.0 + 04649 2151 287 1.85500+ 3 5.00000- 1 7.23000- 2 1.23000- 2 6.00000- 2 0.0 + 04649 2151 288 2.00600+ 3 5.00000- 1 7.58000- 2 1.58000- 2 6.00000- 2 0.0 + 04649 2151 289 2.07400+ 3 5.00000- 1 1.21000- 1 6.10000- 2 6.00000- 2 0.0 + 04649 2151 290 2.23900+ 3 5.00000- 1 6.28000- 2 2.80000- 3 6.00000- 2 0.0 + 04649 2151 291 2.31300+ 3 5.00000- 1 7.57000- 2 1.57000- 2 6.00000- 2 0.0 + 04649 2151 292 2.51800+ 3 5.00000- 1 2.20000- 1 1.60000- 1 6.00000- 2 0.0 + 04649 2151 293 2.61300+ 3 5.00000- 1 6.25000- 1 5.50000- 1 7.50000- 2 0.0 + 04649 2151 294 2.68700+ 3 5.00000- 1 5.46000- 1 4.80000- 1 6.60000- 2 0.0 + 04649 2151 295 2.80300+ 3 5.00000- 1 2.69700- 1 1.47000- 2 2.55000- 1 0.0 + 04649 2151 296 2.97200+ 3 5.00000- 1 6.83000- 2 8.30000- 3 6.00000- 2 0.0 + 04649 2151 297 3.03800+ 3 5.00000- 1 7.00000- 2 1.00000- 2 6.00000- 2 0.0 + 04649 2151 298 3.06900+ 3 5.00000- 1 6.23000- 2 2.30000- 3 6.00000- 2 0.0 + 04649 2151 299 3.10400+ 3 5.00000- 1 6.56000- 2 5.60000- 3 6.00000- 2 0.0 + 04649 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