JENDL-4.0 Tc- 99 0 0 0 0 4.309900+4 9.805660+1 1 0 6 14331 1451 1 0.000000+0 1.000000+0 0 0 0 64331 1451 2 1.000000+0 2.000000+7 0 0 10 44331 1451 3 0.000000+0 0.000000+0 0 0 259 654331 1451 4 43-Tc- 99 JNDC EVAL-Mar90 JNDC FP ND W.G., T.Nakagawa 4331 1451 5 DIST-MAY10 20090901 4331 1451 6 ----JENDL-4.0 MATERIAL 4331 4331 1451 7 -----INCIDENT NEUTRON DATA 4331 1451 8 ------ENDF-6 FORMAT 4331 1451 9 4331 1451 10 HISTORY 4331 1451 11 84-10 Evaluation for JENDL-2 was made by JNDC FPND W.G./1/. 4331 1451 12 90-03 Modification for JENDL-3 was made/2/. 4331 1451 13 93-11 JENDL-3.2 was made by JNDC FPND W.G./3/. 4331 1451 14 ***** Modified parts for JENDL-3.2 ******************** 4331 1451 15 (2,151) Resolved resonance parameters 4331 1451 16 *********************************************************** 4331 1451 17 4331 1451 18 02-02 Modification was made by T.Nakagawa 4331 1451 19 4331 1451 20 ***** Modified parts ************************************** 4331 1451 21 (2,151) RRP and URP 4331 1451 22 (3,1),(3,2),(3,4),(3,22),(3,51-91),(3,102) 4331 1451 23 All of MF04 and MF05 4331 1451 24 *********************************************************** 4331 1451 25 4331 1451 26 06-01 The neutron width of the negative energy resonance was 4331 1451 27 revised by K.Furutaka (jaea). 4331 1451 28 09-08 The total cross section was re-calculated from partial cross4331 1451 29 sections. 4331 1451 30 Compiled by K.Shibata (jaea) for JENDL-4.0. 4331 1451 31 4331 1451 32 MF = 1 General information 4331 1451 33 MT=451 Comments and dictionary 4331 1451 34 4331 1451 35 MF = 2 Resonance parameters 4331 1451 36 MT=151 Resolved and unresolved resonance parameters 4331 1451 37 Resolved resonance region (MLBW formula) : below 6.0 keV 4331 1451 38 All the resolved resonance parameters were brought 4331 1451 39 unmodified from JENDL-3.3 except for the negative-energy one4331 1451 40 : in JENDL-3.3/4/, resonance parameters obtained by 4331 1451 41 Gunsing et al./5/ were adopted. They analyzed their 4331 1451 42 transmission data with REFIT code, and obtaind the 4331 1451 43 parameters up to 10 keV. The upper boundary of the resolved4331 1451 44 resonance region was set to 6 keV in this file as in 4331 1451 45 JENDL-3.3, because the capture cross section calculated from4331 1451 46 their parameters were smaller than experimental data above 4331 1451 47 the energy. Neutron width of the negative-energy resonance 4331 1451 48 was slightly adjusted so as to reproduce the value of 4331 1451 49 capture cross section for thermal neutrons adopted in this 4331 1451 50 file. The adopted value is 23.6 b, which is the weighted 4331 1451 51 average of the cross sections reported by Molnar et al.6/ 4331 1451 52 and Furutaka et al./7/ deduced from emission cross 4331 1451 53 sections of 540- and 591-keV decay gamma rays in Ru-100 4331 1451 54 using the recent gamma-ray emission probabilities for the 4331 1451 55 gamma rays/8/, and the corresponding values reported by 4331 1451 56 Harada et al./9/ recalculated with the new emission 4331 1451 57 probabilities. 4331 1451 58 The scattering radius of 6.7 fm was adopted. 4331 1451 59 4331 1451 60 Unresolved resonance region : 6.0 keV - 100 keV 4331 1451 61 Unresolved resonance parameters were adjusted with ASREP/10/4331 1451 62 to reproduce the capture and total cross sections calculated4331 1451 63 with CASTHY. The parameters should be used only for self- 4331 1451 64 shileding calculation. 4331 1451 65 4331 1451 66 Thermal cross sections and resonance integrals at 300 K 4331 1451 67 ---------------------------------------------------------- 4331 1451 68 0.0253 eV res. integ. (*) 4331 1451 69 (barns) (barns) 4331 1451 70 ---------------------------------------------------------- 4331 1451 71 Total 2.8261E+01 4331 1451 72 Elastic 4.6567E+00 4331 1451 73 n,gamma 2.3605E+01 3.2384E+02 4331 1451 74 ---------------------------------------------------------- 4331 1451 75 (*) Integrated from 0.5 eV to 10 MeV. 4331 1451 76 4331 1451 77 MF = 3 Neutron cross sections 4331 1451 78 Below 6 keV, resonance parameters were given. 4331 1451 79 Above 6 keV, the spherical optical and statistical model 4331 1451 80 calculation was performed with CASTHY/11/, by taking account of 4331 1451 81 competing reactions, of which cross sections were calculated 4331 1451 82 with PEGASUS/12/ standing on a preequilibrium and multi-step 4331 1451 83 evaporation model. The OMP's for neutron given in Table 1 were 4331 1451 84 determined to reproduce the total cross section measured by 4331 1451 85 Foster and Glasgow/13/ in the MeV region, and total cross 4331 1451 86 section of about 8 - 9 b in the 10-100 keV region. The OMP's 4331 1451 87 for charged particles are as follows: 4331 1451 88 Proton = Perey/14/ 4331 1451 89 Alpha = Huizenga and Igo/15/ 4331 1451 90 Deuteron = Lohr and Haeberli/16/ 4331 1451 91 Helium-3 and triton = Becchetti and Greenlees/17/ 4331 1451 92 4331 1451 93 Parameters for the composite level density formula of Gilbert 4331 1451 94 and Cameron/18/ were evaluated by Iijima et al./19/ More 4331 1451 95 extensive determination and modification were made in the 4331 1451 96 previous work/2/. Table 2 shows the level density parameters 4331 1451 97 used in the calculation. Energy dependence of spin cut-off 4331 1451 98 parameter in the energy range below E-joint is due to Gruppelaar4331 1451 99 /20/. 4331 1451 100 4331 1451 101 MT = 1 Total 4331 1451 102 Spherical optical model calculation was adopted. 4331 1451 103 4331 1451 104 MT = 2 Elastic scattering 4331 1451 105 Calculated as (total - sum of partial cross sections). 4331 1451 106 4331 1451 107 MT = 4, 51 - 91 Inelastic scattering 4331 1451 108 4331 1451 109 The level scheme was taken from Ref./21/ 4331 1451 110 4331 1451 111 No. Energy(MeV) Spin-parity 4331 1451 112 GR. 0.0 9/2 + 4331 1451 113 1 0.1405 7/2 + * 4331 1451 114 2 0.1427 1/2 - 4331 1451 115 3 0.1811 5/2 + * 4331 1451 116 4 0.5091 3/2 - 4331 1451 117 5 0.5344 3/2 - 4331 1451 118 6 0.5369 5/2 + 4331 1451 119 7 0.6125 5/2 - * 4331 1451 120 8 0.6254 9/2 + * 4331 1451 121 9 0.6715 3/2 - 4331 1451 122 10 0.7198 7/2 + * 4331 1451 123 11 0.7267 11/2 + * 4331 1451 124 12 0.7617 5/2 + * 4331 1451 125 13 0.7619 13/2 + * 4331 1451 126 14 0.9206 1/2 + 4331 1451 127 15 0.9861 7/2 - * 4331 1451 128 16 1.0041 3/2 - 4331 1451 129 4331 1451 130 Levels above 1.0175 MeV were assumed to be overlapping. 4331 1451 131 The compound inelastic scattering was calculated with CASTHY. 4331 1451 132 For the levels with "*", direct inelastic scattering was 4331 1451 133 calculated with DWUCK /22,23/. Deformation parameters were 4331 1451 134 based on the recommendation by Raman et al./24/ 4331 1451 135 4331 1451 136 MT = 102 Capture 4331 1451 137 Spherical optical and statistical model calculation with 4331 1451 138 CASTHY was adopted. Direct and semi-direct capture cross 4331 1451 139 sections were estimated according to the procedure of Benzi 4331 1451 140 and Reffo/25/ and normalized to 9 mb at 14.7 MeV /26/. 4331 1451 141 4331 1451 142 The gamma-ray strength function (8.01E-03) was adjusted to 4331 1451 143 reproduce the capture cross section of 630 mb at 50 keV. 4331 1451 144 4331 1451 145 MT = 16 (n,2n) Cross Section 4331 1451 146 MT = 17 (n,3n) Cross Section 4331 1451 147 MT = 22 (n,n'a) Cross Section 4331 1451 148 MT = 28 (n,n'p) Cross Section 4331 1451 149 MT = 32 (n,n'd) Cross Section 4331 1451 150 MT = 33 (n,n't) Cross Section 4331 1451 151 MT =103 (n,p) Cross Section 4331 1451 152 MT =104 (n,d) Cross Section 4331 1451 153 MT =105 (n,t) Cross Section 4331 1451 154 MT =106 (n,He3) Cross Section 4331 1451 155 MT =107 (n,alpha) Cross Section 4331 1451 156 These reaction cross sections were calculated with the 4331 1451 157 preequilibrium and multi-step evaporation model code PEGASUS. 4331 1451 158 4331 1451 159 The Kalbach's constant K (= 101.5) was estimated by the 4331 1451 160 formula derived from Kikuchi-Kawai's formalism/27/ and level 4331 1451 161 density parameters. 4331 1451 162 4331 1451 163 Finally, the (n,2n) and (n,p) cross sections were normalized 4331 1451 164 to the following values at 14.5 MeV: 4331 1451 165 (n,2n) 1230.00 mb (recommended by Bychkov et al./28/) 4331 1451 166 (n,p) 14.00 mb (recommended by Forrest/29/) 4331 1451 167 The (n,alpha) and (n,n'alpha) cross section was normalized to 4331 1451 168 the data of Ikdeda et al. /30/ 4331 1451 169 4331 1451 170 MF = 4 Angular Distributions of Secondary Neutrons 4331 1451 171 Legendre polynomial coefficients for angular distributions are 4331 1451 172 given in the center-of-mass system for MT=2 and discrete inelas-4331 1451 173 tic levels, and in the laboratory system for MT=91. They were 4331 1451 174 calculated with CASTHY. Those of direct inelastic scttering 4331 1451 175 were calculated with DWUCK, and added to the rusults of CASTHY 4331 1451 176 calculation. 4331 1451 177 4331 1451 178 For other reactions, isotropic distributions in the laboratory 4331 1451 179 system were assumed. 4331 1451 180 4331 1451 181 MF = 5 Energy Distributions of Secondary Neutrons 4331 1451 182 Energy distributions of secondary neutrons were calculated with 4331 1451 183 PEGASUS for inelastic scattering to overlapping levels and for 4331 1451 184 other neutron emitting reactions. 4331 1451 185 4331 1451 186 Interpolation of 22 (unit base interpolation) was adopted. 4331 1451 187 4331 1451 188 4331 1451 189 Table 1 Neutron Optical Potential Parameters 4331 1451 190 4331 1451 191 Depth (MeV) Radius(fm) Diffuseness(fm) 4331 1451 192 ---------------------- ------------ --------------- 4331 1451 193 V = 45.5-0.48*En r0 = 1.350 a0 = 0.60 4331 1451 194 Ws = 6.79+0.83*En rs = 1.330 as = 0.40 4331 1451 195 Vso= 7.0 rso= 1.350 aso= 0.60 4331 1451 196 The form of surface absorption part is der. Woods-Saxon type. 4331 1451 197 4331 1451 198 Table 2 Level Density Parameters 4331 1451 199 4331 1451 200 Nuclide a(1/MeV) T(MeV) C(1/MeV) EX(MeV) Pairing 4331 1451 201 --------------------------------------------------------------- 4331 1451 202 41-Nb- 95 1.277E+01 7.500E-01 2.121E+00 5.782E+00 1.120E+00 4331 1451 203 41-Nb- 96 1.331E+01 5.880E-01 3.406E+00 2.530E+00 0.0 4331 1451 204 41-Nb- 97 1.337E+01 6.710E-01 9.771E-01 5.026E+00 1.290E+00 4331 1451 205 41-Nb- 98 1.380E+01 5.110E-01 2.350E+00 1.731E+00 0.0 4331 1451 206 4331 1451 207 42-Mo- 96 1.403E+01 7.410E-01 6.991E-01 7.645E+00 2.400E+00 4331 1451 208 42-Mo- 97 1.517E+01 6.800E-01 2.769E+00 6.036E+00 1.280E+00 4331 1451 209 42-Mo- 98 1.594E+01 6.900E-01 7.358E-01 7.888E+00 2.570E+00 4331 1451 210 42-Mo- 99 1.774E+01 6.200E-01 4.294E+00 6.058E+00 1.280E+00 4331 1451 211 4331 1451 212 43-Tc- 97 1.600E+01 6.700E-01 4.756E+00 6.089E+00 1.120E+00 4331 1451 213 43-Tc- 98 1.659E+01 6.120E-01 1.776E+01 4.176E+00 0.0 4331 1451 214 43-Tc- 99 1.600E+01 6.550E-01 2.973E+00 5.984E+00 1.290E+00 4331 1451 215 43-Tc-100 1.637E+01 5.850E-01 1.189E+01 3.635E+00 0.0 4331 1451 216 --------------------------------------------------------------- 4331 1451 217 4331 1451 218 Spin cutoff parameters were calculated as 0.146*SQRT(a)*A**(2/3).4331 1451 219 In the CASTHY calculation, spin cutoff factors at 0 MeV were 4331 1451 220 assumed to be 7.899 for Tc- 99 and 5.0 for Tc-100. 4331 1451 221 4331 1451 222 References 4331 1451 223 1) Aoki T. et al.: Proc. Int. Conf. on Nuclear Data for Basic 4331 1451 224 and Applied Science, Santa Fe., Vol. 2, p.1627 (1985). 4331 1451 225 2) Kawai M. et al.: J. Nucl. Sci. Technol., 29, 195 (1992). 4331 1451 226 3) Kawai M., et al.: J. Nucl. Sci. Technol., 38, 261 (2001). 4331 1451 227 4) Shibata K. et al.: J. Nucl. Sci. Technol., 39, 1125 (2002). 4331 1451 228 5) Gunsing F., et al.: Phys. Rev., C61, 054608 (2000). 4331 1451 229 6) Molnar G., et al.: Radiochim. Acta 90, 479 (2002). 4331 1451 230 7) Furutaka K. et al.: J. Nucl. Sci. Technol., 41, 1033 (2004). 4331 1451 231 8) Furutaka K. et al.: J. Nucl. Sci. Technol., 38, 1035 (2001). 4331 1451 232 9) Harada H. et al.: J. Nucl. Sci. Technol., 32, 395 (1995). 4331 1451 233 10) Kikuchi Y., et al.: JAERI-Data/Code 99-025 (1999). 4331 1451 234 [in Japanese] 4331 1451 235 11) Igarasi S. and Fukahori, T.: JAERI 1321 (1991). 4331 1451 236 12) Nakagawa T., et al.: JAERI-Data/Code 99-031 (1999). 4331 1451 237 13) Foster D.G. Jr., Glasgow D.W.: Phys. Rev., C3, 576 (1971). 4331 1451 238 14) Perey F.G: Phys. Rev. 131, 745 (1963). 4331 1451 239 15) Huizenga J.R. and Igo G.: Nucl. Phys. 29, 462 (1962). 4331 1451 240 16) Lohr, J.M. and Haeberli W.: Nucl. Phys. A232, 381 (1974). 4331 1451 241 17) Becchetti F.D., Jr. and Greenlees G.W.: Polarization 4331 1451 242 Phenomena in Nuclear Reactions ((eds) H.H. Barshall and 4331 1451 243 W. Haeberli), p. 682, The university of Wisconsin Press. 4331 1451 244 (1971). 4331 1451 245 18) Gilbert A. and Cameron A.G.W.: Can. J. Phys., 43, 1446 4331 1451 246 (1965). 4331 1451 247 19) Iijima S., et al.: J. Nucl. Sci. Technol. 21, 10 (1984). 4331 1451 248 20) Gruppelaar H.: ECN-13 (1977). 4331 1451 249 21) Firestone R.B.: "Table of Isotopes, 8th Ed.", Wiley- 4331 1451 250 Interscience Publication (1998). 4331 1451 251 22) Kunz P.D.: private communication. 4331 1451 252 23) Yamamuro N.: JAERI-M 88-140 (1988) [in Japanese] 4331 1451 253 24) Raman S., et al.: Atom. Data and Nucl. Data Tables 36, 1 4331 1451 254 (1987) 4331 1451 255 25) Benzi V. and Reffo, G.: CCDN-NW/10 (1969). 4331 1451 256 26) Qaim S.: J. Inorg. Nucl. Chem., 35, 3669 (1973). 4331 1451 257 27) Kikuchi K. and Kawai, M.: "Nuclear Matter and Nuclear 4331 1451 258 Reactions", North Holland (1968). 4331 1451 259 28) Bychkov V.M. et al.: INDC(CCP)-146/LJ (1980). 4331 1451 260 29) Forrest R.A.: AERE-R 12419 (1986). 4331 1451 261 30) Ikeda Y., et al.: Nucl. Sci. Eng., 116, 28 (1994). 4331 1451 262 4331 1451 263 1 451 328 14331 1451 264 2 151 863 14331 1451 265 3 1 79 14331 1451 266 3 2 31 14331 1451 267 3 4 19 04331 1451 268 3 16 9 04331 1451 269 3 17 5 04331 1451 270 3 22 13 04331 1451 271 3 28 11 04331 1451 272 3 32 7 04331 1451 273 3 33 7 04331 1451 274 3 51 19 04331 1451 275 3 52 18 04331 1451 276 3 53 18 04331 1451 277 3 54 15 04331 1451 278 3 55 15 04331 1451 279 3 56 15 04331 1451 280 3 57 14 04331 1451 281 3 58 14 04331 1451 282 3 59 14 04331 1451 283 3 60 13 04331 1451 284 3 61 13 04331 1451 285 3 62 12 04331 1451 286 3 63 12 04331 1451 287 3 64 11 04331 1451 288 3 65 11 04331 1451 289 3 66 10 04331 1451 290 3 91 10 04331 1451 291 3 102 62 14331 1451 292 3 103 14 04331 1451 293 3 104 12 04331 1451 294 3 105 11 04331 1451 295 3 106 10 04331 1451 296 3 107 15 04331 1451 297 4 2 187 04331 1451 298 4 16 2 04331 1451 299 4 17 2 04331 1451 300 4 22 2 04331 1451 301 4 28 2 04331 1451 302 4 32 2 04331 1451 303 4 33 2 04331 1451 304 4 51 96 04331 1451 305 4 52 26 04331 1451 306 4 53 91 04331 1451 307 4 54 26 04331 1451 308 4 55 27 04331 1451 309 4 56 27 04331 1451 310 4 57 81 04331 1451 311 4 58 81 04331 1451 312 4 59 26 04331 1451 313 4 60 81 04331 1451 314 4 61 81 04331 1451 315 4 62 81 04331 1451 316 4 63 76 04331 1451 317 4 64 27 04331 1451 318 4 65 71 04331 1451 319 4 66 24 04331 1451 320 4 91 24 04331 1451 321 5 16 55 04331 1451 322 5 17 27 04331 1451 323 5 22 189 04331 1451 324 5 28 112 04331 1451 325 5 32 56 04331 1451 326 5 33 49 04331 1451 327 5 91 137 04331 1451 328 4331 1 099999 4331 0 0 0 4.309900+4 9.805660+1 0 0 1 04331 2151 1 4.309900+4 1.000000+0 0 0 2 04331 2151 2 1.000000-5 6.000000+3 1 2 0 04331 2151 3 4.500000+0 6.700000-1 0 0 2 04331 2151 4 9.805660+1 0.000000+0 0 0 3108 5184331 2151 5 -1.500000+1 5.000000+0 1.651000-1 1.510000-2 1.500000-1 0.000000+04331 2151 6 5.580000+0 5.000000+0 1.504500-1 3.450000-3 1.470000-1 0.000000+04331 2151 7 2.027000+1 4.000000+0 1.633700-1 8.370000-3 1.550000-1 0.000000+04331 2151 8 3.984000+1 5.000000+0 1.240800-1 1.080000-3 1.230000-1 0.000000+04331 2151 9 5.668000+1 4.000000+0 1.449000-1 3.900000-3 1.410000-1 0.000000+04331 2151 10 1.112200+2 5.000000+0 1.439400-1 9.940000-3 1.340000-1 0.000000+04331 2151 11 1.237700+2 4.000000+0 1.491100-1 4.110000-3 1.450000-1 0.000000+04331 2151 12 1.630100+2 5.000000+0 2.018000-1 5.780000-2 1.440000-1 0.000000+04331 2151 13 1.820900+2 4.000000+0 2.273000-1 6.730000-2 1.600000-1 0.000000+04331 2151 14 1.917100+2 5.000000+0 1.854000-1 3.640000-2 1.490000-1 0.000000+04331 2151 15 2.064100+2 4.000000+0 1.476900-1 6.900000-4 1.470000-1 0.000000+04331 2151 16 2.148300+2 4.000000+0 1.481900-1 1.190000-3 1.470000-1 0.000000+04331 2151 17 2.206200+2 5.000000+0 1.474890-1 4.890000-4 1.470000-1 0.000000+04331 2151 18 2.412100+2 4.000000+0 1.849000-1 3.790000-2 1.470000-1 0.000000+04331 2151 19 2.731700+2 4.000000+0 1.477910-1 7.910000-4 1.470000-1 0.000000+04331 2151 20 2.799800+2 4.000000+0 1.620000-1 1.500000-2 1.470000-1 0.000000+04331 2151 21 2.999800+2 4.000000+0 1.839000-1 3.690000-2 1.470000-1 0.000000+04331 2151 22 3.068100+2 5.000000+0 1.613000-1 1.430000-2 1.470000-1 0.000000+04331 2151 23 3.432100+2 5.000000+0 1.486200-1 1.620000-3 1.470000-1 0.000000+04331 2151 24 3.586500+2 4.000000+0 1.666000-1 1.960000-2 1.470000-1 0.000000+04331 2151 25 3.614500+2 5.000000+0 1.480300-1 1.030000-3 1.470000-1 0.000000+04331 2151 26 3.626900+2 4.000000+0 1.489700-1 1.970000-3 1.470000-1 0.000000+04331 2151 27 3.649300+2 5.000000+0 2.890000-1 1.420000-1 1.470000-1 0.000000+04331 2151 28 3.798400+2 5.000000+0 1.679000-1 2.090000-2 1.470000-1 0.000000+04331 2151 29 4.168200+2 4.000000+0 2.114000-1 6.440000-2 1.470000-1 0.000000+04331 2151 30 4.265400+2 5.000000+0 2.079000-1 6.090000-2 1.470000-1 0.000000+04331 2151 31 4.477000+2 5.000000+0 1.492200-1 2.220000-3 1.470000-1 0.000000+04331 2151 32 4.599200+2 4.000000+0 1.888000-1 4.180000-2 1.470000-1 0.000000+04331 2151 33 4.787700+2 4.000000+0 1.597000-1 1.270000-2 1.470000-1 0.000000+04331 2151 34 4.865800+2 5.000000+0 1.523500-1 5.350000-3 1.470000-1 0.000000+04331 2151 35 5.164500+2 4.000000+0 1.602000-1 1.320000-2 1.470000-1 0.000000+04331 2151 36 5.205600+2 5.000000+0 1.765000-1 2.950000-2 1.470000-1 0.000000+04331 2151 37 5.366100+2 4.000000+0 1.775000-1 3.050000-2 1.470000-1 0.000000+04331 2151 38 5.632300+2 5.000000+0 1.549700-1 7.970000-3 1.470000-1 0.000000+04331 2151 39 5.937500+2 4.000000+0 1.532000-1 6.200000-3 1.470000-1 0.000000+04331 2151 40 5.981700+2 5.000000+0 1.731000-1 2.610000-2 1.470000-1 0.000000+04331 2151 41 5.995400+2 5.000000+0 1.502600-1 3.260000-3 1.470000-1 0.000000+04331 2151 42 6.067600+2 4.000000+0 1.846000-1 3.760000-2 1.470000-1 0.000000+04331 2151 43 6.234900+2 4.000000+0 1.524900-1 5.490000-3 1.470000-1 0.000000+04331 2151 44 6.325600+2 5.000000+0 1.493900-1 2.390000-3 1.470000-1 0.000000+04331 2151 45 6.547100+2 4.000000+0 1.935000-1 4.650000-2 1.470000-1 0.000000+04331 2151 46 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