JENDL/AC-2008 Pa-231 0 0 0 0 9.123100+4 2.290510+2 1 1 6 19131 1451 1 0.000000+0 1.000000+0 0 0 0 69131 1451 2 1.000000+0 2.000000+7 1 0 10 19131 1451 3 0.000000+0 0.000000+0 0 0 353 859131 1451 4 91-Pa-231 JAEA+ EVAL-OCT07 O.Iwamoto, T.Nakagawa, et al. 9131 1451 5 DIST-MAR08 20071022 9131 1451 6 ----JENDL/AC-2008 MATERIAL 9131 9131 1451 7 -----INCIDENT NEUTRON DATA 9131 1451 8 ------ENDF-6 FORMAT 9131 1451 9 9131 1451 10 History 9131 1451 11 05-11 Fission cross section was evaluated with GMA code. 9131 1451 12 06-08 Resonance parameters were revised. 9131 1451 13 07-10 Theoretical calculation was performed with CCONE code. 9131 1451 14 Data were compiled. 9131 1451 15 9131 1451 16 9131 1451 17 MF=1 General information 9131 1451 18 MT=452 Number of Neutrons per fission 9131 1451 19 Sum of MT's=455 and 456. 9131 1451 20 9131 1451 21 MT=455 Delayed neutron data 9131 1451 22 Estimated from systematics by Tuttle/1/, Benedetti et al./2/ 9131 1451 23 and Waldo et al./3/ 9131 1451 24 Decay constants were evaluated by Brady and England/4/. 9131 1451 25 9131 1451 26 MT=456 Number of prompt neutrons per fission 9131 1451 27 Estimated from Howerton's systematics/5/. 9131 1451 28 9131 1451 29 9131 1451 30 MF= 2 Resonance parameters 9131 1451 31 MT=151 9131 1451 32 Resolved resonance parameters (below 115 eV) 9131 1451 33 The resonance parameters of JENDL-3.3 were based on the 9131 1451 34 following data: 9131 1451 35 Resonance energies, neutron and gamma widths: 9131 1451 36 Hussein et al./6/ 9131 1451 37 Fission area: Plattard et al./7/ 9131 1451 38 Resonances below 1.24 eV: Mughabghab/8/ 9131 1451 39 9131 1451 40 Those data were revised for the present file by comparing with9131 1451 41 the total cross section of Simpson et al./9/ and the fission 9131 1451 42 cross section of Kobayashi et al./10/. 9131 1451 43 The resonance formula was changed to MLBW. Total spin of each 9131 1451 44 level was assumed with JCONV code/11/. 9131 1451 45 Thermal cross section and resonance integral calculated from 9131 1451 46 the present resonance parameters are given in the following 9131 1451 47 table. The thermal cross sections to be reproduced were 9131 1451 48 determined from experimental data: 9131 1451 49 Total = 211.0+-3.1 b 9131 1451 50 Simpson et al./9/ 9131 1451 51 9131 1451 52 Fission = 0.0239+-0.0007 b 9131 1451 53 Wagemans et al./12,13/, Kobayashi et al./14/ 9131 1451 54 9131 1451 55 Capture = 202.2+-5.3 b 9131 1451 56 Smith et al./15/, Aleksandrov et al./16/, 9131 1451 57 Gryntakis et al./17/, Kobayashi/18/ 9131 1451 58 9131 1451 59 The capture resonance integrals reported by Jurova et al./19/ 9131 1451 60 and Aleksandrov et al./16/ were 1044b and 1180b, respectively.9131 1451 61 9131 1451 62 Unresolved resonance parameters (115 eV - 10 keV) 9131 1451 63 Cross sections were reproduced with average resonance 9131 1451 64 parameters determined by ASREP code/20/. These parameters 9131 1451 65 are used only for self-shielding effects. 9131 1451 66 9131 1451 67 Thermal cross sections and resonance integrals (at 300K) 9131 1451 68 ------------------------------------------------------- 9131 1451 69 0.0253 eV reson. integ.(*) 9131 1451 70 (barns) (barns) 9131 1451 71 ------------------------------------------------------- 9131 1451 72 total 212.32 9131 1451 73 elastic 10.59 9131 1451 74 fission 0.0236 3.24 9131 1451 75 capture 201.71 542 9131 1451 76 ------------------------------------------------------- 9131 1451 77 (*) In the energy range from 0.5 eV to 10 MeV. 9131 1451 78 9131 1451 79 9131 1451 80 MF= 3 Neutron cross sections 9131 1451 81 Cross sections above the resolved resonance region except for 9131 1451 82 elastic scattering and fission cross sections (MT's =2, 18-21, 9131 1451 83 38) were calculated with CCONE code/21/. 9131 1451 84 9131 1451 85 MT= 1 Total cross section 9131 1451 86 The cross section was calculated with CC OMP of Soukhovitskii 9131 1451 87 et al./22/ with modification of the quadrupole deformation 9131 1451 88 parameter. 9131 1451 89 9131 1451 90 MT=2 Elastic scattering cross section 9131 1451 91 Calculated as total - non-elstic scattering cross sections 9131 1451 92 9131 1451 93 MT=18 Fission cross section (Above 115 eV) 9131 1451 94 The following experimental data were analyzed in the energy 9131 1451 95 ranges from 115 eV to 12 keV, and from 110 keV to 12 MeV with 9131 1451 96 the GMA code/23/: 9131 1451 97 9131 1451 98 Authors Energy range Data points Reference 9131 1451 99 Plattard+ 0.112 - 16.9 MeV 4120 /24/ 9131 1451 100 Fursov+ 0.135 - 7.4 MeV 69 /25/(*1) 9131 1451 101 Kobayashi+ 0.089 - 12.6 keV 44 /10/ 9131 1451 102 Oberstedt+ 0.76 - 3.46 MeV 15 /26/ 9131 1451 103 (*1) The data were measured relatively to Pu-239 fission. 9131 1451 104 They were converted to Pa-231 fission by using JENDL-9131 1451 105 3.3 data. 9131 1451 106 The results of the analysis were adopted in the energy ranges 9131 1451 107 from 115 eV to 10 keV and from 120 keV to 9.5 MeV. 9131 1451 108 9131 1451 109 CCONE calculation was adopted in the energy ranges from 10 to 9131 1451 110 120 keV and above 9.5 MeV. 9131 1451 111 9131 1451 112 The results of GMA below 10 MeV, the preliminary experimental 9131 1451 113 data of IRMM/27/ above 15 MeV, and the experimental data of 9131 1451 114 Birgul and Lyle/28/ at 15 MeV were used to determine the 9131 1451 115 parameters in the CCONE calculation. 9131 1451 116 9131 1451 117 MT=19, 20, 21, 38 Multi-chance fission cross sections 9131 1451 118 Calculated with CCONE code, and renormalized to the total 9131 1451 119 fission cross section (MT=18). 9131 1451 120 9131 1451 121 9131 1451 122 MF= 4 Angular distributions of secondary neutrons 9131 1451 123 MT=2 Elastic scattering 9131 1451 124 Calculated with CCONE code/21/. 9131 1451 125 9131 1451 126 MT=18 Fission 9131 1451 127 Isotropic distributions in the laboratory system were assumed.9131 1451 128 9131 1451 129 MF= 5 Energy distributions of secondary neutrons 9131 1451 130 MT=18 Prompt neutrons 9131 1451 131 Calculated with CCONE code/21/. 9131 1451 132 9131 1451 133 MT=455 Delayed neutrons 9131 1451 134 Calculated by Brady and England/4/. 9131 1451 135 9131 1451 136 MF= 6 Energy-angle distributions 9131 1451 137 Calculated with CCONE code/21/. 9131 1451 138 Distributions from fission (MT=18) are not included. 9131 1451 139 9131 1451 140 9131 1451 141 ***************************************************************** 9131 1451 142 Calculation with CCONE code 9131 1451 143 ***************************************************************** 9131 1451 144 9131 1451 145 Models and parameters used in the CCONE/21/ calculation 9131 1451 146 1) Coupled channel optical model 9131 1451 147 Levels in the rotational band were included. Optical model 9131 1451 148 potential and coupled levels are shown in Table 1. 9131 1451 149 9131 1451 150 2) Two-component exciton model/29/ 9131 1451 151 * Global parametrization of Koning-Duijvestijn/30/ 9131 1451 152 was used. 9131 1451 153 * Gamma emission channel/31/ was added to simulate direct 9131 1451 154 and semi-direct capture reaction. 9131 1451 155 9131 1451 156 3) Hauser-Feshbach statistical model 9131 1451 157 * Moldauer width fluctuation correction/32/ was included. 9131 1451 158 * Neutron, gamma and fission decay channel were included. 9131 1451 159 * Transmission coefficients of neutrons were taken from 9131 1451 160 coupled channel calculation in Table 1. 9131 1451 161 * The level scheme of the target is shown in Table 2. 9131 1451 162 * Level density formula of constant temperature and Fermi-gas 9131 1451 163 model were used with shell energy correction and collective 9131 1451 164 enhancement factor. Parameters are shown in Table 3. 9131 1451 165 * Fission channel: 9131 1451 166 Double humped fission barriers were assumed. 9131 1451 167 Fission barrier penetrabilities were calculated with 9131 1451 168 Hill-Wheler formula/33/. Fission barrier parameters were 9131 1451 169 shown in Table 4. Transition state model was used and 9131 1451 170 continuum levels are assumed above the saddles. The level 9131 1451 171 density parameters for inner and outer saddles are shown in 9131 1451 172 Tables 5 and 6, respectively. 9131 1451 173 * Gamma-ray strength function of Kopecky et al/34/,/35/ 9131 1451 174 was used. The prameters are shown in Table 7. 9131 1451 175 9131 1451 176 9131 1451 177 ------------------------------------------------------------------9131 1451 178 Tables 9131 1451 179 ------------------------------------------------------------------9131 1451 180 9131 1451 181 Table 1. Coupled channel calculation 9131 1451 182 -------------------------------------------------- 9131 1451 183 * rigid rotor model was applied 9131 1451 184 * coupled levels = 0,1,2,3,9,14 (see Table 2) 9131 1451 185 * optical potential parameters /22/ 9131 1451 186 Volume: 9131 1451 187 V_0 = 49.97 MeV 9131 1451 188 lambda_HF = 0.01004 1/MeV 9131 1451 189 C_viso = 15.9 MeV 9131 1451 190 A_v = 12.04 MeV 9131 1451 191 B_v = 81.36 MeV 9131 1451 192 E_a = 385 MeV 9131 1451 193 r_v = 1.2568 fm 9131 1451 194 a_v = 0.633 fm 9131 1451 195 Surface: 9131 1451 196 W_0 = 17.2 MeV 9131 1451 197 B_s = 11.19 MeV 9131 1451 198 C_s = 0.01361 1/MeV 9131 1451 199 C_wiso = 23.5 MeV 9131 1451 200 r_s = 1.1803 fm 9131 1451 201 a_s = 0.601 fm 9131 1451 202 Spin-orbit: 9131 1451 203 V_so = 5.75 MeV 9131 1451 204 lambda_so = 0.005 1/MeV 9131 1451 205 W_so = -3.1 MeV 9131 1451 206 B_so = 160 MeV 9131 1451 207 r_so = 1.1214 fm 9131 1451 208 a_so = 0.59 fm 9131 1451 209 Coulomb: 9131 1451 210 C_coul = 1.3 9131 1451 211 r_c = 1.2452 fm 9131 1451 212 a_c = 0.545 fm 9131 1451 213 Deformation: 9131 1451 214 beta_2 = 0.19 9131 1451 215 beta_4 = 0.066 9131 1451 216 beta_6 = 0.0015 9131 1451 217 9131 1451 218 * Calculated strength function 9131 1451 219 S0= 0.81e-4 S1= 2.50e-4 R'= 9.64 fm (En=1 keV) 9131 1451 220 -------------------------------------------------- 9131 1451 221 9131 1451 222 Table 2. Level Scheme of Pa-231 9131 1451 223 ------------------- 9131 1451 224 No. Ex(MeV) J PI 9131 1451 225 ------------------- 9131 1451 226 0 0.00000 3/2 - * 9131 1451 227 1 0.00921 1/2 - * 9131 1451 228 2 0.05857 7/2 - * 9131 1451 229 3 0.07769 5/2 - * 9131 1451 230 4 0.08421 5/2 + 9131 1451 231 5 0.10141 7/2 + 9131 1451 232 6 0.10227 3/2 + 9131 1451 233 7 0.11165 9/2 + 9131 1451 234 8 0.13400 11/2 + 9131 1451 235 9 0.16860 11/2 - * 9131 1451 236 10 0.17150 11/2 + 9131 1451 237 11 0.17416 5/2 - 9131 1451 238 12 0.18350 5/2 + 9131 1451 239 13 0.18890 13/2 + 9131 1451 240 14 0.19350 9/2 - * 9131 1451 241 15 0.21824 7/2 - 9131 1451 242 16 0.24732 7/2 + 9131 1451 243 17 0.27200 9/2 - 9131 1451 244 18 0.27380 1/2 + 9131 1451 245 19 0.29660 17/2 + 9131 1451 246 20 0.30070 15/2 + 9131 1451 247 21 0.30400 9/2 + 9131 1451 248 22 0.31150 5/2 + 9131 1451 249 23 0.31680 17/2 + 9131 1451 250 24 0.31795 3/2 + 9131 1451 251 25 0.32021 3/2 - 9131 1451 252 26 0.32870 15/2 - 9131 1451 253 27 0.34000 11/2 - 9131 1451 254 28 0.35150 13/2 - 9131 1451 255 29 0.35184 5/2 - 9131 1451 256 30 0.38500 23/2 + 9131 1451 257 ------------------- 9131 1451 258 *) Coupled levels in CC calculation 9131 1451 259 9131 1451 260 Table 3. Level density parameters 9131 1451 261 -------------------------------------------------------- 9131 1451 262 Nuclide a* Pair Eshell T E0 Ematch 9131 1451 263 1/MeV MeV MeV MeV MeV MeV 9131 1451 264 -------------------------------------------------------- 9131 1451 265 Pa-232 17.9699 0.0000 2.9784 0.2779 -0.6740 1.0000 9131 1451 266 Pa-231 17.9034 0.7895 3.1164 0.4176 -1.2470 3.5007 9131 1451 267 Pa-230 17.8368 0.0000 2.9470 0.2794 -0.6728 1.0000 9131 1451 268 Pa-229 17.7702 0.7930 3.0707 0.3881 -0.8689 3.0597 9131 1451 269 Pa-228 17.7035 0.0000 2.9095 0.2810 -0.6716 1.0000 9131 1451 270 -------------------------------------------------------- 9131 1451 271 9131 1451 272 Table 4. Fission barrier parameters 9131 1451 273 ---------------------------------------- 9131 1451 274 Nuclide V_A hw_A V_B hw_B 9131 1451 275 MeV MeV MeV MeV 9131 1451 276 ---------------------------------------- 9131 1451 277 Pa-232 5.800 0.800 6.180 0.400 9131 1451 278 Pa-231 6.000 0.800 5.750 0.520 9131 1451 279 Pa-230 5.800 0.800 6.180 0.400 9131 1451 280 Pa-229 6.000 0.800 5.800 0.520 9131 1451 281 Pa-228 5.800 0.800 6.180 0.400 9131 1451 282 ---------------------------------------- 9131 1451 283 9131 1451 284 Table 5. Level density above inner saddle 9131 1451 285 -------------------------------------------------------- 9131 1451 286 Nuclide a* Pair Eshell T E0 Ematch 9131 1451 287 1/MeV MeV MeV MeV MeV MeV 9131 1451 288 -------------------------------------------------------- 9131 1451 289 Pa-232 20.6654 0.0000 2.6000 0.3415 -2.6081 2.2000 9131 1451 290 Pa-231 20.5889 0.9211 2.6000 0.3276 -1.4734 2.9211 9131 1451 291 Pa-230 20.5123 0.0000 2.6000 0.3428 -2.6080 2.2000 9131 1451 292 Pa-229 20.4357 0.9251 2.6000 0.3435 -1.6829 3.1251 9131 1451 293 Pa-228 20.3591 0.0000 2.6000 0.3442 -2.6080 2.2000 9131 1451 294 -------------------------------------------------------- 9131 1451 295 9131 1451 296 Table 6. Level density above outer saddle 9131 1451 297 -------------------------------------------------------- 9131 1451 298 Nuclide a* Pair Eshell T E0 Ematch 9131 1451 299 1/MeV MeV MeV MeV MeV MeV 9131 1451 300 -------------------------------------------------------- 9131 1451 301 Pa-232 20.6654 0.0000 -0.0800 0.4050 -2.1087 2.5000 9131 1451 302 Pa-231 20.5889 0.9211 -0.1200 0.3706 -0.7702 2.9211 9131 1451 303 Pa-230 20.5123 0.0000 -0.1600 0.3867 -1.8562 2.2000 9131 1451 304 Pa-229 20.4357 0.9251 -0.2000 0.3880 -0.9302 3.1251 9131 1451 305 Pa-228 20.3591 0.0000 -0.2400 0.3894 -1.8544 2.2000 9131 1451 306 -------------------------------------------------------- 9131 1451 307 9131 1451 308 Table 7. Gamma-ray strength function for Pa-232 9131 1451 309 -------------------------------------------------------- 9131 1451 310 K0 = 1.502 E0 = 4.500 (MeV) 9131 1451 311 * E1: ER = 11.03 (MeV) EG = 2.71 (MeV) SIG = 302.00 (mb) 9131 1451 312 ER = 13.87 (MeV) EG = 4.77 (MeV) SIG = 449.00 (mb) 9131 1451 313 * M1: ER = 6.67 (MeV) EG = 4.00 (MeV) SIG = 2.79 (mb) 9131 1451 314 * E2: ER = 10.25 (MeV) EG = 3.33 (MeV) SIG = 6.39 (mb) 9131 1451 315 -------------------------------------------------------- 9131 1451 316 9131 1451 317 9131 1451 318 References 9131 1451 319 1) R.J.Tuttle: INDC(NDS)-107/G+Special, p.29 (1979). 9131 1451 320 2) G.Benedetti et al.: Nucl. Sci. Eng., 80, 379 (1982). 9131 1451 321 3) R.Waldo et al.: Phys. Rev., C23, 1113 (1981). 9131 1451 322 4) M.C.Brady, T.R.England: Nucl. Sci. Eng., 103, 129 (1989). 9131 1451 323 5) R.J.Howerton: Nucl. Sci. Eng., 62, 438 (1977). 9131 1451 324 6) A.Z.Hussein et al.: Nucl. Sci. Eng., 78, 370 (1981). 9131 1451 325 7) S.Plattard et al.: 1979 Koxville, p.491 (1979). 9131 1451 326 8) S.F.Mughabghab: "Neutron Cross Sections," Vol.1, Part B, 9131 1451 327 Academic Press (1984). 9131 1451 328 9) F.B.Simpson et al.: Nucl. Sci. Eng., 12, 243 (1962). 9131 1451 329 10) K.Kobayashi et al.: Nucl. Sci. Eng., 139, 273 (2001). 9131 1451 330 11) T.Nakagawa et al.: JAERI-Data/Code 99-030 (1999). 9131 1451 331 12) C.Wagemans et al.: Nucl. Phys., A285, 32 (1977). 9131 1451 332 13) C.Wagemans et al.: Ann. Nucl. Energy, 5, 267 (1978). 9131 1451 333 14) K.Kobayashi et al.: Nucl. Sci. Technol., 36, 549 (1999). 9131 1451 334 15) R.R.Smith et al.: Phys. Rev., 101, 1053 (1956). 9131 1451 335 16) B.M.Aleksandrov et al.: At. Energy, 32, 178 (1972). 9131 1451 336 17) E.Gryntakis, J.I.Kim: J. Inorg. Nucl. Chem., 36, 1447 (1974). 9131 1451 337 18) K.Kobayashi: NEANDC(J)-36L, p.40 (1974). 9131 1451 338 19) L.N.Jurova et al.: Yadernye Konstanty, 1/55, 3 (1984). 9131 1451 339 20) Y.Kikuchi et al.: JAERI-Data/Code 99-025 (1999) in Japanese. 9131 1451 340 21) O.Iwamoto: J. Nucl. Sci. Technol., 44, 687 (2007). 9131 1451 341 22) E.Sh.Soukhovitskii et al.: Phys. Rev. C72, 024604 (2005). 9131 1451 342 23) W.P.Poenitz: BNL-NCS-51363, Vol.I, p.249 (1981). 9131 1451 343 S.Chiba, D.L.Smith: ANL/NDM-121 (1991). 9131 1451 344 24) S.Plattard, et al.: Phys. Rev. Lett., 46, 633 (1981). 9131 1451 345 25) B.I.Fursov, et al.: Sov. At. Energy, 59, 899 (1985). 9131 1451 346 26) S.Oberstedt, et al.: Ann. Nucl. Energy, 32, 1867 (2005). 9131 1451 347 27) P.Schillebeeckx, A.Trkov: INDC(NDS)-0494 (2006). 9131 1451 348 28) O.Birgul, S.J.Lyle: Radiochimica Acta, 11, 108 (1969). 9131 1451 349 29) C.Kalbach: Phys. Rev. C33, 818 (1986). 9131 1451 350 30) A.J.Koning, M.C.Duijvestijn: Nucl. Phys. 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C47, 312 (1990). 9131 1451 356 9131 1451 357 1 451 442 19131 1451 358 1 452 5 19131 1451 359 1 455 7 19131 1451 360 1 456 4 19131 1451 361 2 151 231 19131 1451 362 3 1 63 19131 1451 363 3 2 63 19131 1451 364 3 4 36 19131 1451 365 3 16 13 19131 1451 366 3 17 9 19131 1451 367 3 18 60 19131 1451 368 3 19 49 19131 1451 369 3 20 22 19131 1451 370 3 21 13 19131 1451 371 3 38 9 19131 1451 372 3 51 36 19131 1451 373 3 52 34 19131 1451 374 3 53 33 19131 1451 375 3 54 33 19131 1451 376 3 55 32 19131 1451 377 3 56 32 19131 1451 378 3 57 32 19131 1451 379 3 58 31 19131 1451 380 3 59 30 19131 1451 381 3 60 30 19131 1451 382 3 61 29 19131 1451 383 3 62 29 19131 1451 384 3 63 29 19131 1451 385 3 64 28 19131 1451 386 3 65 28 19131 1451 387 3 66 27 19131 1451 388 3 67 27 19131 1451 389 3 68 26 19131 1451 390 3 69 26 19131 1451 391 3 70 25 19131 1451 392 3 71 25 19131 1451 393 3 72 25 19131 1451 394 3 73 24 19131 1451 395 3 74 24 19131 1451 396 3 75 24 19131 1451 397 3 76 23 19131 1451 398 3 77 23 19131 1451 399 3 78 23 19131 1451 400 3 79 22 19131 1451 401 3 80 22 19131 1451 402 3 91 33 19131 1451 403 3 102 40 19131 1451 404 4 2 524 19131 1451 405 4 18 2 19131 1451 406 5 18 3974 19131 1451 407 5 455 579 19131 1451 408 6 16 1748 19131 1451 409 6 17 580 19131 1451 410 6 51 209 19131 1451 411 6 52 313 19131 1451 412 6 53 308 19131 1451 413 6 54 205 19131 1451 414 6 55 204 19131 1451 415 6 56 207 19131 1451 416 6 57 202 19131 1451 417 6 58 199 19131 1451 418 6 59 293 19131 1451 419 6 60 191 19131 1451 420 6 61 193 19131 1451 421 6 62 191 19131 1451 422 6 63 185 19131 1451 423 6 64 278 19131 1451 424 6 65 181 19131 1451 425 6 66 188 19131 1451 426 6 67 182 19131 1451 427 6 68 177 19131 1451 428 6 69 180 19131 1451 429 6 70 171 19131 1451 430 6 71 177 19131 1451 431 6 72 158 19131 1451 432 6 73 168 19131 1451 433 6 74 156 19131 1451 434 6 75 168 19131 1451 435 6 76 158 19131 1451 436 6 77 162 19131 1451 437 6 78 154 19131 1451 438 6 79 152 19131 1451 439 6 80 148 19131 1451 440 6 91 6369 19131 1451 441 6 102 3539 19131 1451 442 9131 1 099999 9.123100+4 2.290510+2 0 2 0 09131 1452 1 0.000000+0 0.000000+0 0 0 1 59131 1452 2 5 2 0 0 0 09131 1452 3 1.000000-5 2.245230+0 2.530000-2 2.245230+0 5.500000+6 2.828230+09131 1452 4 7.000000+6 2.983860+0 2.000000+7 4.361860+0 9131 1452 5 9131 1 099999 9.123100+4 2.290510+2 0 2 0 09131 1455 1 0.000000+0 0.000000+0 0 0 6 09131 1455 2 1.290000-2 3.470000-2 1.150000-1 2.856000-1 6.706000-1 2.311100+09131 1455 3 0.000000+0 0.000000+0 0 0 1 59131 1455 4 5 2 0 0 0 09131 1455 5 1.000000-5 1.083000-2 2.530000-2 1.083000-2 5.500000+6 1.083000-29131 1455 6 7.000000+6 7.460000-3 2.000000+7 7.460000-3 9131 1455 7 9131 1 099999 9.123100+4 2.290510+2 0 2 0 09131 1456 1 0.000000+0 0.000000+0 0 0 1 29131 1456 2 2 2 0 0 0 09131 1456 3 1.000000-5 2.234400+0 2.000000+7 4.354400+0 9131 1456 4 9131 1 099999 9131 0 0 0 9.123100+4 2.290510+2 0 0 1 09131 2151 1 9.123100+4 1.000000+0 0 0 2 09131 2151 2 1.000000-5 1.150000+2 1 2 0 09131 2151 3 1.500000+0 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5 18 1807 352 2 0 0 0 09131 5 18 1808 0.000000+0 0.000000+0 1.000000-5 1.88319-12 1.200000-5 2.06293-129131 5 18 1809 1.400000-5 2.22822-12 1.600000-5 2.38207-12 1.800000-5 2.52657-129131 5 18 1810 2.200000-5 2.79323-12 2.500000-5 2.97759-12 2.900000-5 3.20697-129131 5 18 1811 3.400000-5 3.47244-12 4.000000-5 3.76640-12 4.600000-5 4.03901-129131 5 18 1812 5.400000-5 4.37617-12 6.300000-5 4.72680-12 7.400000-5 5.12287-129131 5 18 1813 8.600000-5 5.52265-12 1.000000-4 5.95523-12 1.200000-4 6.52364-129131 5 18 1814 1.400000-4 7.04635-12 1.600000-4 7.53287-12 1.800000-4 7.98983-129131 5 18 1815 2.200000-4 8.83311-12 2.500000-4 9.41614-12 2.900000-4 1.01415-119131 5 18 1816 3.400000-4 1.09811-11 4.000000-4 1.19107-11 4.600000-4 1.27728-119131 5 18 1817 5.400000-4 1.38390-11 6.300000-4 1.49479-11 7.400000-4 1.62004-119131 5 18 1818 8.600000-4 1.74647-11 1.000000-3 1.88328-11 1.200000-3 2.06304-119131 5 18 1819 1.400000-3 2.22834-11 1.600000-3 2.38221-11 1.800000-3 2.52673-119131 5 18 1820 2.200000-3 2.79342-11 2.500000-3 2.97781-11 2.900000-3 3.20722-119131 5 18 1821 3.400000-3 3.47274-11 4.000000-3 3.76675-11 4.600000-3 4.03942-119131 5 18 1822 5.400000-3 4.37664-11 6.300000-3 4.72736-11 7.400000-3 5.12352-119131 5 18 1823 8.600000-3 5.52340-11 1.000000-2 5.95611-11 1.200000-2 6.52469-119131 5 18 1824 1.400000-2 7.04757-11 1.600000-2 7.53427-11 1.800000-2 7.99140-119131 5 18 1825 2.200000-2 8.83503-11 2.500000-2 9.41833-11 2.900000-2 1.01441-109131 5 18 1826 3.400000-2 1.09840-10 4.000000-2 1.19142-10 4.600000-2 1.27768-109131 5 18 1827 5.400000-2 1.38437-10 6.300000-2 1.49534-10 7.400000-2 1.62069-109131 5 18 1828 8.600000-2 1.74722-10 1.000000-1 1.88415-10 1.200000-1 2.06409-109131 5 18 1829 1.400000-1 2.22957-10 1.600000-1 2.38361-10 1.800000-1 2.52830-109131 5 18 1830 2.200000-1 2.79535-10 2.500000-1 2.98000-10 2.900000-1 3.20976-109131 5 18 1831 3.400000-1 3.47572-10 4.000000-1 3.77025-10 4.600000-1 4.04344-109131 5 18 1832 5.400000-1 4.38136-10 6.300000-1 4.73287-10 7.400000-1 5.13000-109131 5 18 1833 8.600000-1 5.53093-10 1.000000+0 5.96486-10 1.200000+0 6.53520-109131 5 18 1834 1.400000+0 7.05983-10 1.600000+0 7.54828-10 1.800000+0 8.00716-109131 5 18 1835 2.200000+0 8.85429-10 2.500000+0 9.44021-10 2.900000+0 1.016940-99131 5 18 1836 3.400000+0 1.101380-9 4.000000+0 1.194920-9 4.600000+0 1.281710-99131 5 18 1837 5.400000+0 1.389100-9 6.300000+0 1.500860-9 7.400000+0 1.627170-99131 5 18 1838 8.600000+0 1.754760-9 1.000000+1 1.892910-9 1.200000+1 2.074590-99131 5 18 1839 1.400000+1 2.241830-9 1.600000+1 2.397620-9 1.800000+1 2.544060-99131 5 18 1840 2.200000+1 2.814610-9 2.500000+1 3.001890-9 2.900000+1 3.235160-99131 5 18 1841 3.400000+1 3.505490-9 4.000000+1 3.805280-9 4.600000+1 4.083730-99131 5 18 1842 5.400000+1 4.428650-9 6.300000+1 4.788040-9 7.400000+1 5.194800-99131 5 18 1843 8.600000+1 5.606240-9 1.000000+2 6.052420-9 1.200000+2 6.640260-99131 5 18 1844 1.400000+2 7.182390-9 1.600000+2 7.688340-9 1.800000+2 8.164720-99131 5 18 1845 2.200000+2 9.046830-9 2.500000+2 9.658970-9 2.900000+2 1.042320-89131 5 18 1846 3.400000+2 1.131120-8 4.000000+2 1.229900-8 4.600000+2 1.321920-89131 5 18 1847 5.400000+2 1.436300-8 6.300000+2 1.555900-8 7.400000+2 1.691790-89131 5 18 1848 8.600000+2 1.829820-8 1.000000+3 1.980150-8 1.200000+3 2.179220-89131 5 18 1849 1.400000+3 2.363810-8 1.600000+3 2.536940-8 1.800000+3 2.700700-89131 5 18 1850 2.200000+3 3.005840-8 2.500000+3 3.219020-8 2.900000+3 3.486760-89131 5 18 1851 3.400000+3 3.800120-8 4.000000+3 4.151410-8 4.600000+3 4.481260-89131 5 18 1852 5.400000+3 4.894540-8 6.300000+3 5.330610-8 7.400000+3 5.830810-89131 5 18 1853 8.600000+3 6.343840-8 1.000000+4 6.908140-8 1.200000+4 7.663970-89131 5 18 1854 1.400000+4 8.373310-8 1.600000+4 9.045730-8 1.800000+4 9.687880-89131 5 18 1855 2.200000+4 1.089960-7 2.500000+4 1.175740-7 2.900000+4 1.284710-79131 5 18 1856 3.400000+4 1.413920-7 4.000000+4 1.560790-7 4.600000+4 1.700500-79131 5 18 1857 5.400000+4 1.877890-7 6.300000+4 2.067650-7 7.400000+4 2.288340-79131 5 18 1858 8.600000+4 2.517770-7 1.000000+5 2.773380-7 2.000000+5 3.602230-79131 5 18 1859 3.000000+5 3.657330-7 4.000000+5 3.466030-7 5.000000+5 3.341890-79131 5 18 1860 6.000000+5 3.295020-7 7.000000+5 3.282260-7 8.000000+5 3.268080-79131 5 18 1861 9.000000+5 3.240050-7 1.000000+6 3.195230-7 1.100000+6 3.134710-79131 5 18 1862 1.200000+6 3.060600-7 1.300000+6 2.975610-7 1.400000+6 2.882680-79131 5 18 1863 1.500000+6 2.784180-7 1.600000+6 2.682010-7 1.700000+6 2.577710-79131 5 18 1864 1.800000+6 2.472520-7 1.900000+6 2.367440-7 2.000000+6 2.263260-79131 5 18 1865 2.100000+6 2.160620-7 2.200000+6 2.060020-7 2.300000+6 1.961850-79131 5 18 1866 2.400000+6 1.866410-7 2.500000+6 1.773910-7 2.600000+6 1.684520-79131 5 18 1867 2.700000+6 1.598350-7 2.800000+6 1.515450-7 2.900000+6 1.435870-79131 5 18 1868 3.000000+6 1.359580-7 3.100000+6 1.286590-7 3.200000+6 1.216830-79131 5 18 1869 3.300000+6 1.150240-7 3.400000+6 1.086770-7 3.500000+6 1.026320-79131 5 18 1870 3.600000+6 9.688140-8 3.700000+6 9.141500-8 3.800000+6 8.622320-89131 5 18 1871 3.900000+6 8.129600-8 4.000000+6 7.662340-8 4.100000+6 7.219510-89131 5 18 1872 4.200000+6 6.800080-8 4.300000+6 6.403070-8 4.400000+6 6.027470-89131 5 18 1873 4.500000+6 5.672310-8 4.600000+6 5.336650-8 4.700000+6 5.019560-89131 5 18 1874 4.800000+6 4.720130-8 4.900000+6 4.437510-8 5.000000+6 4.170860-89131 5 18 1875 5.100000+6 3.919360-8 5.200000+6 3.682240-8 5.300000+6 3.458760-89131 5 18 1876 5.400000+6 3.248190-8 5.500000+6 3.049850-8 5.600000+6 2.863080-89131 5 18 1877 5.700000+6 2.687270-8 5.800000+6 2.521810-8 5.900000+6 2.366130-89131 5 18 1878 6.000000+6 2.219700-8 6.100000+6 2.081990-8 6.200000+6 1.952530-89131 5 18 1879 6.300000+6 1.830830-8 6.400000+6 1.716460-8 6.500000+6 1.609010-89131 5 18 1880 6.600000+6 1.508070-8 6.700000+6 1.413260-8 6.800000+6 1.324240-89131 5 18 1881 6.900000+6 1.240670-8 7.000000+6 1.162220-8 7.100000+6 1.088590-89131 5 18 1882 7.200000+6 1.019500-8 7.300000+6 9.546870-9 7.400000+6 8.938860-99131 5 18 1883 7.500000+6 8.368610-9 7.600000+6 7.833860-9 7.700000+6 7.332470-99131 5 18 1884 7.800000+6 6.862430-9 7.900000+6 6.421840-9 8.000000+6 6.008910-99131 5 18 1885 8.100000+6 5.621950-9 8.200000+6 5.259390-9 8.300000+6 4.919730-99131 5 18 1886 8.400000+6 4.601550-9 8.500000+6 4.303550-9 8.600000+6 4.024470-99131 5 18 1887 8.700000+6 3.763140-9 8.800000+6 3.518460-9 8.900000+6 3.289390-99131 5 18 1888 9.000000+6 3.074970-9 9.100000+6 2.874280-9 9.200000+6 2.686460-99131 5 18 1889 9.300000+6 2.510710-9 9.400000+6 2.346260-9 9.500000+6 2.192400-99131 5 18 1890 9.600000+6 2.048470-9 9.700000+6 1.913830-9 9.800000+6 1.787910-99131 5 18 1891 9.900000+6 1.670140-9 1.000000+7 1.560010-9 1.010000+7 1.457040-99131 5 18 1892 1.020000+7 1.360760-9 1.030000+7 1.270750-9 1.040000+7 1.186620-99131 5 18 1893 1.050000+7 1.107970-9 1.060000+7 1.034460-9 1.070000+7 9.65766-109131 5 18 1894 1.080000+7 9.01570-10 1.090000+7 8.41585-10 1.100000+7 7.85538-109131 5 18 1895 1.110000+7 7.33176-10 1.120000+7 6.84260-10 1.130000+7 6.38566-109131 5 18 1896 1.140000+7 5.95886-10 1.150000+7 5.56024-10 1.160000+7 5.18796-109131 5 18 1897 1.170000+7 4.84030-10 1.180000+7 4.51567-10 1.190000+7 4.21256-109131 5 18 1898 1.200000+7 3.92957-10 1.210000+7 3.66537-10 1.220000+7 3.41873-109131 5 18 1899 1.230000+7 3.18850-10 1.240000+7 2.97361-10 1.250000+7 2.77305-109131 5 18 1900 1.260000+7 2.58587-10 1.270000+7 2.41119-10 1.280000+7 2.24819-109131 5 18 1901 1.290000+7 2.09609-10 1.300000+7 1.95418-10 1.310000+7 1.82177-109131 5 18 1902 1.320000+7 1.69825-10 1.330000+7 1.58303-10 1.340000+7 1.47554-109131 5 18 1903 1.350000+7 1.37528-10 1.360000+7 1.28177-10 1.370000+7 1.19456-109131 5 18 1904 1.380000+7 1.11322-10 1.390000+7 1.03737-10 1.400000+7 9.66647-119131 5 18 1905 1.410000+7 9.00698-11 1.420000+7 8.39207-11 1.430000+7 7.81878-119131 5 18 1906 1.440000+7 7.28430-11 1.450000+7 6.78604-11 1.460000+7 6.32156-119131 5 18 1907 1.470000+7 5.88861-11 1.480000+7 5.48506-11 1.490000+7 5.10893-119131 5 18 1908 1.500000+7 4.75837-11 1.510000+7 4.43168-11 1.520000+7 4.12723-119131 5 18 1909 1.530000+7 3.84352-11 1.540000+7 3.57916-11 1.550000+7 3.33284-119131 5 18 1910 1.560000+7 3.10334-11 1.570000+7 2.88952-11 1.580000+7 2.69032-119131 5 18 1911 1.590000+7 2.50474-11 1.600000+7 2.33187-11 1.610000+7 2.17084-119131 5 18 1912 1.620000+7 2.02084-11 1.630000+7 1.88114-11 1.640000+7 1.75102-119131 5 18 1913 1.650000+7 1.62983-11 1.660000+7 1.51697-11 1.670000+7 1.41187-119131 5 18 1914 1.680000+7 1.31400-11 1.690000+7 1.22287-11 1.700000+7 1.13801-119131 5 18 1915 1.710000+7 1.05901-11 1.720000+7 9.85443-12 1.730000+7 9.16956-129131 5 18 1916 1.740000+7 8.53197-12 1.750000+7 7.93841-12 1.760000+7 7.38587-129131 5 18 1917 1.770000+7 6.87153-12 1.780000+7 6.39278-12 1.790000+7 5.94716-129131 5 18 1918 1.800000+7 5.53241-12 1.810000+7 5.14639-12 1.820000+7 4.78714-129131 5 18 1919 1.830000+7 4.45280-12 1.840000+7 4.14167-12 1.850000+7 3.85214-129131 5 18 1920 1.860000+7 3.58273-12 1.870000+7 3.33205-12 1.880000+7 3.09879-129131 5 18 1921 1.890000+7 2.88177-12 1.900000+7 2.67985-12 1.910000+7 2.49200-129131 5 18 1922 1.920000+7 2.31724-12 1.930000+7 2.15466-12 1.940000+7 2.00342-129131 5 18 1923 1.950000+7 1.86274-12 1.960000+7 1.73187-12 1.970000+7 1.61015-129131 5 18 1924 1.980000+7 1.49694-12 1.990000+7 1.39164-12 2.000000+7 1.29370-129131 5 18 1925 2.020000+7 0.000000+0 9131 5 18 1926 0.000000+0 6.500000+6 0 0 1 3529131 5 18 1927 352 2 0 0 0 09131 5 18 1928 0.000000+0 0.000000+0 1.000000-5 1.73805-12 1.200000-5 1.90393-129131 5 18 1929 1.400000-5 2.05649-12 1.600000-5 2.19848-12 1.800000-5 2.33184-129131 5 18 1930 2.200000-5 2.57795-12 2.500000-5 2.74810-12 2.900000-5 2.95980-129131 5 18 1931 3.400000-5 3.20481-12 4.000000-5 3.47611-12 4.600000-5 3.72772-129131 5 18 1932 5.400000-5 4.03888-12 6.300000-5 4.36250-12 7.400000-5 4.72804-129131 5 18 1933 8.600000-5 5.09701-12 1.000000-4 5.49625-12 1.200000-4 6.02085-129131 5 18 1934 1.400000-4 6.50327-12 1.600000-4 6.95230-12 1.800000-4 7.37404-129131 5 18 1935 2.200000-4 8.15233-12 2.500000-4 8.69043-12 2.900000-4 9.35990-129131 5 18 1936 3.400000-4 1.01347-11 4.000000-4 1.09927-11 4.600000-4 1.17884-119131 5 18 1937 5.400000-4 1.27724-11 6.300000-4 1.37959-11 7.400000-4 1.49519-119131 5 18 1938 8.600000-4 1.61187-11 1.000000-3 1.73813-11 1.200000-3 1.90404-119131 5 18 1939 1.400000-3 2.05661-11 1.600000-3 2.19862-11 1.800000-3 2.33200-119131 5 18 1940 2.200000-3 2.57814-11 2.500000-3 2.74832-11 2.900000-3 2.96006-119131 5 18 1941 3.400000-3 3.20512-11 4.000000-3 3.47647-11 4.600000-3 3.72813-119131 5 18 1942 5.400000-3 4.03937-11 6.300000-3 4.36306-11 7.400000-3 4.72870-119131 5 18 1943 8.600000-3 5.09778-11 1.000000-2 5.49715-11 1.200000-2 6.02193-119131 5 18 1944 1.400000-2 6.50453-11 1.600000-2 6.95373-11 1.800000-2 7.37565-119131 5 18 1945 2.200000-2 8.15430-11 2.500000-2 8.69267-11 2.900000-2 9.36249-119131 5 18 1946 3.400000-2 1.01378-10 4.000000-2 1.09963-10 4.600000-2 1.17925-109131 5 18 1947 5.400000-2 1.27773-10 6.300000-2 1.38015-10 7.400000-2 1.49585-109131 5 18 1948 8.600000-2 1.61264-10 1.000000-1 1.73903-10 1.200000-1 1.90512-109131 5 18 1949 1.400000-1 2.05787-10 1.600000-1 2.20005-10 1.800000-1 2.33361-109131 5 18 1950 2.200000-1 2.58011-10 2.500000-1 2.75057-10 2.900000-1 2.96266-109131 5 18 1951 3.400000-1 3.20817-10 4.000000-1 3.48005-10 4.600000-1 3.73225-109131 5 18 1952 5.400000-1 4.04421-10 6.300000-1 4.36871-10 7.400000-1 4.73534-109131 5 18 1953 8.600000-1 5.10549-10 1.000000+0 5.50611-10 1.200000+0 6.03269-109131 5 18 1954 1.400000+0 6.51708-10 1.600000+0 6.96808-10 1.800000+0 7.39179-109131 5 18 1955 2.200000+0 8.17403-10 2.500000+0 8.71508-10 2.900000+0 9.38850-109131 5 18 1956 3.400000+0 1.016830-9 4.000000+0 1.103220-9 4.600000+0 1.183380-99131 5 18 1957 5.400000+0 1.282570-9 6.300000+0 1.385800-9 7.400000+0 1.502490-99131 5 18 1958 8.600000+0 1.620360-9 1.000000+1 1.748000-9 1.200000+1 1.915880-99131 5 18 1959 1.400000+1 2.070420-9 1.600000+1 2.214410-9 1.800000+1 2.349760-99131 5 18 1960 2.200000+1 2.599850-9 2.500000+1 2.772990-9 2.900000+1 2.988670-99131 5 18 1961 3.400000+1 3.238670-9 4.000000+1 3.515940-9 4.600000+1 3.773520-99131 5 18 1962 5.400000+1 4.092650-9 6.300000+1 4.425230-9 7.400000+1 4.801720-99131 5 18 1963 8.600000+1 5.182630-9 1.000000+2 5.595810-9 1.200000+2 6.140320-99131 5 18 1964 1.400000+2 6.642650-9 1.600000+2 7.111570-9 1.800000+2 7.553210-99131 5 18 1965 2.200000+2 8.371290-9 2.500000+2 8.939220-9 2.900000+2 9.648460-99131 5 18 1966 3.400000+2 1.047300-8 4.000000+2 1.139060-8 4.600000+2 1.224590-89131 5 18 1967 5.400000+2 1.330940-8 6.300000+2 1.442210-8 7.400000+2 1.568720-89131 5 18 1968 8.600000+2 1.697300-8 1.000000+3 1.837430-8 1.200000+3 2.023130-89131 5 18 1969 1.400000+3 2.195480-8 1.600000+3 2.357250-8 1.800000+3 2.510370-89131 5 18 1970 2.200000+3 2.795960-8 2.500000+3 2.995690-8 2.900000+3 3.246760-89131 5 18 1971 3.400000+3 3.540920-8 4.000000+3 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