ENDF/B-VI Release 5 142 0 0 0 9.423900+4 2.369986+2 1 1 0 39437 1451 1 0.000000+0 1.000000+0 0 0 0 69437 1451 2 1.000000+0 2.000000+7 5 0 10 69437 1451 3 0.000000+0 0.000000+0 0 0 790 1019437 1451 4 94-Pu-239 LANL EVAL-APR89 P.YOUNG, L.WESTON, W.POENITZ 9437 1451 5 DIST-SEP98 REV2-AUG97 19980921 9437 1451 6 ----ENDF/B-VI MATERIAL 9437 REVISION 2 9437 1451 7 -----INCIDENT NEUTRON DATA 9437 1451 8 ------ENDF-6 FORMAT 9437 1451 9 9437 1451 10 **************************************************************** 9437 1451 11 9437 1451 12 ENDF/B-VI MOD 3 Revision, August 1997, V. McLane (NNDC) 9437 1451 13 9437 1451 14 MF=1 changes 9437 1451 15 MF=455: Updated TAB1 bookkeeping (Minor revision). 9437 1451 16 MF=2 changes 9437 1451 17 MT=151: Corrected l-dependent scattering radius to equal 9437 1451 18 scattering radius 9437 1451 19 9437 1451 20 **************************************************************** 9437 1451 21 9437 1451 22 ENDF/B-VI MOD 2 Revision, January 1993, H. Derrien (ORNL), 9437 1451 23 T. Nakagawa (JAERI) 9437 1451 24 9437 1451 25 Resonance region evaluation by H.Derrien and T. Nakagawa 9437 1451 26 discussed below. This evaluation extended resonance region to 9437 1451 27 2.5 kev. 9437 1451 28 9437 1451 29 **************************************************************** 9437 1451 30 9437 1451 31 ENDF/B-VI MOD 1 Evaluation, April 1989, P.G. Young (LANL), 9437 1451 32 L.W.Weston (ORNL), W.P.Poenitz (ANL) 9437 1451 33 9437 1451 34 1. Prompt nubar evaluation obtained from work of E.Fort (Nuc. 9437 1451 35 Sci.Eng.99, 375 (1988). 9437 1451 36 2. Delayed nubar evaluation (En89). 9437 1451 37 3. Energy range above unresolved resonances (0.03 - 20 MeV) was 9437 1451 38 evaluated by P.Young, using results from W.Poenitz, G.Hale, 9437 1451 39 R.Peelle, and A.Carlson from the simultaneous standards 9437 1451 40 evaluation [11], and with contributions from R. MacFarlane 9437 1451 41 and L.Weston. More details are given below, and full 9437 1451 42 documentation will be issued later. 9437 1451 43 9437 1451 44 PU239 RESONANCE DATA 0 Kev TO 2.5 Kev ************************** 9437 1451 45 (H.Derrien, T.Nakagawa) 9437 1451 46 9437 1451 47 The present file contains the resonance parameters obtained 9437 1451 48 from a SAMMY fit analysis of high resolution experimental data, 9437 1451 49 performed at ORNL (Oak Ridge Nationnal Laboratory, USA) by 9437 1451 50 H.Derrien and G.De Saussure and at JAERI (Tokai-Mura Research 9437 1451 51 Establishment, Japan) by H.Derrien and T.Nakagawa. 9437 1451 52 The file contains three independant sections: 9437 1451 53 1) the first corresponds to the energy range 0 keV to 1 keV. 9437 1451 54 The corresponding set of resonance parametres contains 398 9437 1451 55 resonances in the energy range 0 keV to 1 keV, 4 ficticious 9437 1451 56 negative energy resonances and 3 ficticious resonances above 9437 1451 57 1 keV; 9437 1451 58 2) the second corresponds to the energy range 1 keV to 2 keV. 9437 1451 59 The corresponding set of resonance parameters contains 435 9437 1451 60 resonances in the energy range 0.980 keV to 2.02 keV, 3 9437 1451 61 ficticious resonances below 0.9 keV and 3 ficticious resonances 9437 1451 62 above 2.02 keV; 9437 1451 63 3) the third corresponds to the energy range 2 keV to 2.5 keV. 9437 1451 64 The corresponding set of resonance parameters contains 218 9437 1451 65 resonances in the energy range 1.98 keV to 2.53 keV, 3 9437 1451 66 ficticious resonances below 1.98 keV and 3 ficticious resonances9437 1451 67 above 2.53 keV. 9437 1451 68 In all sections the ficticious resonance parameters take 9437 1451 69 into account the contribution of all the external truncated 9437 1451 70 resonances in such a way that no total, scattering, fission and 9437 1451 71 capture smooth files are needed in the corresponding energy 9437 1451 72 ranges for the reproduction of the cross sections within the 9437 1451 73 experimental errors. 9437 1451 74 The following experimental data base has been used in the 9437 1451 75 SAMMY fits: 9437 1451 76 - absorption and fission from R. Gwin et al. [1,4]; 9437 1451 77 - fission from R. Gwin et al. [5,7], J. Blons [3], L.W. Weston 9437 1451 78 et al. [8,15]; 9437 1451 79 - transmission from R.R. Spencer et al. [10], J.A. Harvey et al.9437 1451 80 [9]. 9437 1451 81 Prior to the fits the experimental fission and absorption cross 9437 1451 82 sections were normalised,directly or indirectly to the 0.0253 eV 9437 1451 83 values obtained by the ENDF/B-VI standard evaluation group [11]. 9437 1451 84 The transmission data were considered as accurate absolute 9437 1451 85 measurements (R.R.Spencer total cross section at 0.0253 eV is 9437 1451 86 1025.0 b in excellent agreement with 1027.3 b standard value). 9437 1451 87 Details on the analysis are found in [14],[16],[17]. 9437 1451 88 9437 1451 89 ---------------------------------------------------------------- 9437 1451 90 COMMENTS ON THE THERMAL AND LOW ENERGY RANGES 9437 1451 91 9437 1451 92 The thermal cross-section values calculated at 293 K by the 9437 1451 93 resonance parameters of the first section are given in the 9437 1451 94 following table at 293 K and in barns. 9437 1451 95 9437 1451 96 SAMMY RESENDD Proposed standard [11] 9437 1451 97 ------- -------- ---------------------- 9437 1451 98 Fission 747.64 747.90 747.99+-1.87 9437 1451 99 Capture 271.10 270.73 271.43+-2.14 9437 1451 100 Scattering 7.97 7.99 7.88+-0.97 9437 1451 101 ------- -------- ---------------------- 9437 1451 102 Total 1026.71 1026.62 1027.30+-5.00 9437 1451 103 9437 1451 104 One should note that the 293 K cross sections calculated at 9437 1451 105 0.0253 eV depend on the way the Doppler broadening calculation 9437 1451 106 is performed. For instance using a Gaussian broadening function 9437 1451 107 will give a fission cross section about 2.5 barns larger than the9437 1451 108 one obtained from the accurate calculation which conserves the 9437 1451 109 1/v shape of the thermal cross section. The values given in the 9437 1451 110 table above were obtained from SAMMY (Leal-Hwang method) [13,18] 9437 1451 111 and from RESENDD with 0.1% for the interpolation accuracy [20]. 9437 1451 112 The following table shows experimental cross sections 9437 1451 113 averaged over the energy ranges 0.02 eV to 0.06eV and 0.02 ev 9437 1451 114 to 0.65 eV, compared to the calculated values: 9437 1451 115 9437 1451 116 References Average Cross Sections (barns) 9437 1451 117 [1-10] 0.02 - 0.06 eV 0.02 - 0.65 eV 9437 1451 118 ---------------- ----------------------- ----------------------- 9437 1451 119 Exp Calc (293K) Exp Calc (293K) 9437 1451 120 Gwin71 fiss 631.41 843.71 9437 1451 121 Gwin76 fiss 631.41 838.39 9437 1451 122 Gwin84 fiss(*) 631.41 631.75(+0.05%) 837.18 838.69(+0.18%) 9437 1451 123 Deruyter70 fiss 631.41 859.43 9437 1451 124 Wagemans80 fiss 631.41 862.56 9437 1451 125 Wagemans88 fiss 631.41 841.80 9437 1451 126 Gwin71 capture 243.84 243.22(-0.25%) 524.75 518.13(-1.26%) 9437 1451 127 Gwin76 absorpt(*) 875.90 874.29(-0.18%) 1359.96 1357.14(-0.21%) 9437 1451 128 Spencer84 tot(*) 883.20 882.86(-0.04%) 1361.69 1367.6 (+0.43%) 9437 1451 129 ----------------- ---------------------- ----------------------- 9437 1451 130 (*)These data had the largest weight in the thermal fit. The 9437 1451 131 values between the parentheses give the percentage deviation 9437 1451 132 between the calculated data and the experimental data. 9437 1451 133 9437 1451 134 The value of 631.4 barns for all the averaged experimental 9437 1451 135 fission cross sections in the energy range 0.02 eV to 0.06 eV 9437 1451 136 corresponds to the renormalisation of the fission experiments to 9437 1451 137 748.0+-1. barns at 0.0253 eV. ORNL data are consistent within 9437 1451 138 0.8% over the energy range 0.02 ev to 0.65 ev (i.e. over the 0.3 9437 1451 139 eV resonance). Deruyter 1970 and Wagemans 1980 data are about 9437 1451 140 2.5% larger and were not included in the SAMMY fit. 9437 1451 141 When normalized on the standard value at 0.0253 eV, Gwin 76 9437 1451 142 absorption agrees with the absorption obtained from Spencer total9437 1451 143 cross section within 0.7% over the 0.3 eV resonance. The present 9437 1451 144 evaluation is essentially the result of a consistent SAMMY 9437 1451 145 analysis of all the available ORNL data with a larger weight on 9437 1451 146 Gwin 1984 fission, Gwin 1976 absorption and Spencer transmission 9437 1451 147 data. 9437 1451 148 After renormalization of the calculated fission cross section9437 1451 149 on the preliminary 1991 Weston and Todd fission data (see next 9437 1451 150 section) a slight adjustment of the negative resonance parameters9437 1451 151 was performed to keep the values calculated at 0.0253 eV in close9437 1451 152 agreement with the standard values. The 1988 data of Wagemans et 9437 1451 153 al.[21] agree within 0.4% with the calculated values over the 9437 1451 154 energy range from 0.02 eV to 0.65 eV after adjustment of the 9437 1451 155 energy scale to the ORNL scale (the difference was 0.27 eV at 9437 1451 156 20 eV between 1988 Wagemans and ORNL SAMMY fit energy scales). 9437 1451 157 9437 1451 158 ---------------------------------------------------------------- 9437 1451 159 COMMENTS ON THE 0 keV TO 1 keV ENERGY RANGE. 9437 1451 160 9437 1451 161 At the end of 1987, an analysis was completed up to 1 kev. 9437 1451 162 In a preliminary step, a correlated fit of Harvey transmission 9437 1451 163 data, Weston 84 fission data, and Blons fission data was 9437 1451 164 performed with possible adjustment of the normalization 9437 1451 165 coefficients and of the background corrections. This preliminary 9437 1451 166 step has shown that this adjustment was not necessary to have 9437 1451 167 consistency between Harvey data and Weston data. The Blons data 9437 1451 168 needed a large readjustment of the background and normalization. 9437 1451 169 Therefore, the final fit was performed only on the Harvey 9437 1451 170 transmission data, Gwin 84 fission data (below 30 eV), and 9437 1451 171 Weston 84 fission data, with no background and normalization 9437 1451 172 adjustment. Blons data, which have better resolution than Weston 9437 1451 173 84 data, were used only to obtain more accurate fission widths 9437 1451 174 of some narrow resonances in the high energy range. 9437 1451 175 In 1989, preliminary results of the 1988 Weston fission 9437 1451 176 measurement [15] were included in the SAMMY experimental data 9437 1451 177 base. One expected from this measurement, which was performed by 9437 1451 178 using a 86-m flight path with a resolution comparable to that of 9437 1451 179 Harvey transmission, a confirmation of the excellent quality of 9437 1451 180 the 1984 measurement. A consistent SAMMY fit of Harvey transmis- 9437 1451 181 sion, Weston 84 fission and preliminary Weston 88 fission was re-9437 1451 182 started from the parameter and covariance files obtained in 1987.9437 1451 183 It appeared that large background and normalisation corrections 9437 1451 184 were needed on the new Weston fission to obtain consistency with 9437 1451 185 Harvey transmission data. These corrections were comparable to 9437 1451 186 those found on Blons data and were not understood by the authors 9437 1451 187 of the experiment. The last SAMMY runs were performed by not 9437 1451 188 allowing background and normalization variations on Harvey trans-9437 1451 189 mission and Weston 84 fission (very small error bars were 9437 1451 190 assigned to the corresponding parameters in the covariance 9437 1451 191 matrix) and by allowing these variations on Weston 88 data. A 9437 1451 192 new set of resonance parameters was obtained, which was improved 9437 1451 193 compared to the previous set due to the very high resolution of 9437 1451 194 the new Weston fission measurement. 9437 1451 195 The calculated average fission cross section in the energy 9437 1451 196 range from 0.1 kev to 1.0 kev was 3.7% smaller than the values 9437 1451 197 obtained by the ENDF/B-VI standard evaluation group due to the 9437 1451 198 fact that Weston 84 data were 3.1% lower than the average 9437 1451 199 standard value. A new measurement was performed by Weston and 9437 1451 200 Todd in 1991 [22] in order to check their 1984 data. A careful 9437 1451 201 normalization of the data in the thermal energy range showed 9437 1451 202 that the 1984 data should be renormalized by about +3%. To take 9437 1451 203 into account this renormalization, the 1989 resonance parameters 9437 1451 204 were modified at JAERI [17] in the following way: 9437 1451 205 1) increase of the fission width by 3% and decrease of the 9437 1451 206 capture width by a quantity equal to the variation of the 9437 1451 207 fission width in the narrow resonances(mainly 1+ resonances); 9437 1451 208 that does not modify the total cross section in the correspond- 9437 1451 209 ing resonances; 9437 1451 210 2) adjustment of the neutron width of the 0+ resonances by a 9437 1451 211 refit of the transmission data and of the renormalized Weston 9437 1451 212 and Todd 1984 data in energy ranges where the contribution of 9437 1451 213 the 0+ resonances is dominant, and increase of the other(small) 9437 1451 214 0+ neutron widths by 3%. No severe inconsistency was observed 9437 1451 215 between the transmission data and the new fission data over the 9437 1451 216 dominant 0+ resonances; the differences between the 1989 fits of 9437 1451 217 the transmission and the new fits were consistent within the 9437 1451 218 experimental error bars. 9437 1451 219 The following table shows the fission cross sections calculat-9437 1451 220 ed from the resonance parameters, the experimental values and 9437 1451 221 the results of the ENDF/B-VI standard evaluation group averaged 9437 1451 222 in the same energy intervals. Weston 1991 data are preliminary. 9437 1451 223 Weston 1984 data are normalized on preliminary Weston 1991. 9437 1451 224 9437 1451 225 Energy Cross Sections (barn) 9437 1451 226 (eV) Calc. Weston 1991 Weston 1984 Standard 9437 1451 227 ---------- ------ ----------- ----------- -------- 9437 1451 228 0.010-10. 80.12 79.98 9437 1451 229 9-20 94.74 94.91 9437 1451 230 20-40 17.52 17.76 17.97 9437 1451 231 40-60 50.64 50.90 50.87 9437 1451 232 60-100 54.42 54.38 54.33 9437 1451 233 100-200 18.63 18.59 18.56 18.66 9437 1451 234 200-300 17.85 17.89 17.88 9437 1451 235 300-400 8.31 8.34 8.43 9437 1451 236 400-500 9.59 9.58 9.57 9437 1451 237 ---------- ------ ----------- ----------- -------- 9437 1451 238 200-500 11.92 11.93 11.93 11.96 9437 1451 239 ---------- ------ ----------- ----------- -------- 9437 1451 240 500-600 15.39 15.57 15.86 9437 1451 241 600-700 4.37 4.30 4.46 9437 1451 242 700-800 5.51 5.53 5.63 9437 1451 243 800-900 4.84 4.89 4.98 9437 1451 244 900-1000 8.33 8.38 8.30 9437 1451 245 ---------- ------ ----------- ----------- -------- 9437 1451 246 500-1000 7.69 7.73 7.73 7.79 9437 1451 247 ---------- ------ ----------- ----------- -------- 9437 1451 248 20-1000 13.09 13.11 13.11 9437 1451 249 -------------------------------------------------------- 9437 1451 250 9437 1451 251 Gwin 1971 and 1976 absorption data were not included in the 9437 1451 252 SAMMY fit in the energy range above 1 ev. Accurate absorption 9437 1451 253 cross sections should be calculated from the parameters obtained 9437 1451 254 from the analysis of the transmission and fission data. The 9437 1451 255 following table shows the calculated average values of the 9437 1451 256 capture, absorption and alpha compared to Gwin 1971 and Gwin 9437 1451 257 1976 data. The calculations were performed with RESENDD, 1% 9437 1451 258 accuracy. 9437 1451 259 9437 1451 260 Energy (eV) Cross Sections (barn) 9437 1451 261 calc. values (293 K) Gwin data 9437 1451 262 ------------ --------------------- ------------------ 9437 1451 263 CAPT ABSORP ALPHA ABSORP ALPHA 9437 1451 264 7.3- 16.0 76.61 196.04 0.64 208.00 0.74(*) 9437 1451 265 16.0- 37.5 20.51 44.55 0.85 46.50 0.89(*) 9437 1451 266 37.5- 50.0 48.72 70.00 2.29 83.15 2.96(*) 9437 1451 267 50.0-100.0 33.60 92.13 0.57 92.84 0.63 9437 1451 268 100.0-200.0 15.58 34.29 0.83 33.66 0.87 9437 1451 269 200.0-300.0 15.85 33.68 0.89 34.69 0.94 9437 1451 270 300.0-400.0 9.69 18.01 1.16 18.31 1.16 9437 1451 271 400.0-500.0 3.96 13.56 0.41 13.56 0.44 9437 1451 272 500.0-600.0 10.87 26.30 0.70 26.54 0.72 9437 1451 273 600.0-700.0 6.53 10.90 1.49 11.57 1.54 9437 1451 274 700.0-800.0 4.95 10.47 0.90 10.52 0.97 9437 1451 275 800.0-900.0 3.65 8.50 0.75 9.30 0.82 9437 1451 276 900.0-999.9 5.06 13.51 0.60 13.23 0.70 9437 1451 277 ------------------------------------------------------ 9437 1451 278 (*) Gwin 1971 data 9437 1451 279 9437 1451 280 If one excepts the energy range 37.5-50 eV, the calculated 9437 1451 281 absorption values agree well with Gwin experimental data; they 9437 1451 282 are on average 1.2% lower in the energy range from 50 eV to 9437 1451 283 1000 eV. 9437 1451 284 9437 1451 285 ---------------------------------------------------------------- 9437 1451 286 COMMENTS ON THE 1 kev TO 2 kev ENERGY RANGE 9437 1451 287 9437 1451 288 Preliminary resonance parameters were obtained in 1989 from 9437 1451 289 the analysis of the Harvey thick sample transmission data and of 9437 1451 290 the preliminary results of Weston 88 fission measurement. Due to 9437 1451 291 lack of time, the medium and thin sample transmission data were 9437 1451 292 not included in the SAMMY data base, and the contribution of the 9437 1451 293 truncated external resonances was not carefully investigated. 9437 1451 294 Nevertheless, the results were used in the ENDF/B-VI file, along 9437 1451 295 with a smooth file in order to agree with the average values of 9437 1451 296 a previous ENDF/B-VI evaluation (this preliminary set of 9437 1451 297 parameters was considered as more useful than the statistical 9437 1451 298 parameters in the energy range 1 kev to 2 kev for the 9437 1451 299 calculation of the self-shielding factors). 9437 1451 300 The analysis was restarted in April 1991 at JAERI with an 9437 1451 301 updated version of SAMMY adapted by T. Nakagawa to the FACOM 780.9437 1451 302 The preliminary set of parameters obtained at Oak Ridge in 1989 9437 1451 303 was used as prior information to start the SAMMY calculations. 9437 1451 304 Also prior to the analysis, the contribution of the external 9437 1451 305 resonances was calculated by using the set of the 0 kev to 1 keV 9437 1451 306 known resonances, shifted in the energy ranges -1 kev to 0 kev, 9437 1451 307 2 kev to 3kev, and 3 kev to 4 kev; equivalent contribution was 9437 1451 308 obtained by using 3 ficticious resonances below 1 kev and 3 9437 1451 309 ficticious resonances above 2 kev [17]. The analysis was 9437 1451 310 performed on the thick and medium sample transmissions of Harvey 9437 1451 311 (the thin sample data was not useful in the high energy range) 9437 1451 312 and on the 1988 fission data released by Weston at the beginning 9437 1451 313 of 1991 [15]. The definitive SAMMY fits were performed in April 9437 1451 314 1992 after renormalization of the 1988 data of Weston to the 9437 1451 315 ENDF/B-VI standard values between 1 keV and 2 kev, in agreement 9437 1451 316 with the 1991 new measurements of Westin and Todd. 9437 1451 317 The average cross sections calculated from the resonance 9437 1451 318 parameters are compared to the experimental values in the 9437 1451 319 following table. 9437 1451 320 9437 1451 321 Energy Cross Sections (barn) 9437 1451 322 (keV) Total Fission Capture 9437 1451 323 -------- ---------------- ---------------- --------------- 9437 1451 324 CALC(a) EXP(b) CALC(a) EXP(c) CALC(a) EXP(d) 9437 1451 325 1.0-1.1 24.47 24.95 5.549 5.581 4.728 5.04 9437 1451 326 1.1-1.2 22.82 23.10 5.985 6.017 3.757 2.95 9437 1451 327 1.2-1.3 22.29 22.90 4.601 4.501 4.287 4.00 9437 1451 328 1.3-1.4 22.63 22.85 6.997 6.997 3.012 2.52 9437 1451 329 1.4-1.5 20.42 20.95 4.041 4.059 3.450 3.57 9437 1451 330 1.5-1.6 18.30 18.95 2.564 2.613 3.521 3.89 9437 1451 331 1.6-1.7 21.82 21.90 3.952 3.955 3.833 4.36 9437 1451 332 1.7-1.8 21.26 21.35 3.400 3.425 4.091 4.37 9437 1451 333 1.8-1.9 23.76 23.30 5.178 5.187 3.639 3.14 9437 1451 334 1.9-2.0 18.48 18.90 2.152 2.180 3.205 4.06 9437 1451 335 -------- ---------------- ---------------- --------------- 9437 1451 336 1.0-2.0 21.63 21.92 4.442 4.446 3.752 3.79 9437 1451 337 ------------------------------------------------------------- 9437 1451 338 (a) total,fission and capture cross sections calculated by 9437 1451 339 RESEND from the resonance parameters. 9437 1451 340 (b) experimental total cross sections from Derrien [23]. 9437 1451 341 (c) Weston and Todd 1988 high resolution fission cross sections 9437 1451 342 [15] normalized to ENDF/B-VI standard in the energy range 9437 1451 343 from 1.0 kev to 2.0 kev. 9437 1451 344 (d) Gwin 1971 experimental data normalized to Gwin 1976 data. 9437 1451 345 9437 1451 346 The difference of 1.3% between the average calculated total 9437 1451 347 cross section and the average experimental cross section in the 9437 1451 348 energy range from 1.0 keV and 2.0 keV is mainly due to the method9437 1451 349 of evaluating the total cross section from the effective cross 9437 1451 350 section of Derrien [23]. The accuracy of the Sammy fit of the 9437 1451 351 experimental transmission data is better than 0.5% on the cross 9437 1451 352 section. The calculated fission cross sections are in very good 9437 1451 353 agreement with the experimental data. The capture data [1] are 9437 1451 354 average values obtained from the data available in the EXFOR 9437 1451 355 file and normalized to Gwin 1976 average values; there are large 9437 1451 356 differences between the calculated data and the experimental 9437 1451 357 data averaged over 0.1kev intervals; but on the interval from 9437 1451 358 1.0 keV to 2.0 keV the average values are consistent within 1.0%.9437 1451 359 9437 1451 360 ---------------------------------------------------------------- 9437 1451 361 COMMENTS ON THE 2.0 keV TO 2.5 keV REGION 9437 1451 362 9437 1451 363 This energy range was also analysed at JAERI [17]. No 9437 1451 364 preliminary set of resonance parameters was available prior to 9437 1451 365 the analysis. More than 90% of the resonances, compared to the 9437 1451 366 low energy range, could still be identified in the transmission 9437 1451 367 data between 2 keV and 2.5 keV. Therefore, the correlated SAMMY 9437 1451 368 analysis of Harvey transmissions and Weston fission was still 9437 1451 369 feasible in this energy range. The resonance parameters obtained 9437 1451 370 are consistent and have nearly the same statistical properties 9437 1451 371 as those of the resonances in the 0 to 2 keV energy range. A 9437 1451 372 quite good fit of the transmission and fission data was obtained 9437 1451 373 without background and normalization adjustment. However, the 9437 1451 374 calculated fission cross sections are, on average, 1.4% lower 9437 1451 375 than the experimental values. This difference, which however is 9437 1451 376 not larger than the systematic errors on the experimental data, 9437 1451 377 could be due to the difficulties of identifying the wide j=0+ 9437 1451 378 resonances in the experimental data, because the effects of the 9437 1451 379 increasing resolution and Doppler widths. Prior to the SAMMY 9437 1451 380 fits, the fission data of Weston and Todd (1988 high resolution 9437 1451 381 data) were normalized to the ENDF/B-VI standard in the energy 9437 1451 382 range from 1 kev to 2 kev. 9437 1451 383 The cross sections, calculated from the resonance parameters 9437 1451 384 and averaged over 0.1 keV intervals, are given in the following 9437 1451 385 table. 9437 1451 386 9437 1451 387 Energy Cross Sections (barn) 9437 1451 388 (keV) TOTAL FISSION CAPTURE 9437 1451 389 --------- ---------------- ---------------- ------- 9437 1451 390 CALC(a) EXP(b) CALC(a) EXP(c) CALC(a) 9437 1451 391 2.0-2.1 17.34 17.30 2.034 2.062 3.223 9437 1451 392 2.1-2.2 20.27 19.80 2.949 2.999 4.051 9437 1451 393 2.2-2.3 19.34 19.10 2.357 2.393 3.324 9437 1451 394 2.3-2.4 21.28 21.20 3.646 3.679 3.640 9437 1451 395 2.4-2.5 20.03 20.60 3.956 4.024 3.128 9437 1451 396 --------- ---------------- ---------------- ----------- 9437 1451 397 2.0-2.5 19.65 19.60 2.989 3.031 3.473 9437 1451 398 ----------------------------------------------------------- 9437 1451 399 (a) total,fission and capture cross sections calculated by 9437 1451 400 RESENDD, 1% accuracy at 300 K, from the resonance 9437 1451 401 parameters. 9437 1451 402 (b) average total cross sections obtained from the average 9437 1451 403 experimental effective cross sections of Derrien [23]. 9437 1451 404 (c) 1988 high resolution data of Weston and Todd [15] 9437 1451 405 normalized to ENDF/B-VI standard in the energy range 9437 1451 406 from 1 kev to 2 kev. 9437 1451 407 9437 1451 408 ---------------------------------------------------------------- 9437 1451 409 FISSION AND CAPTURE RESONANCE INTEGRALS 9437 1451 410 9437 1451 411 The fission and capture resonance integrals are compared to 9437 1451 412 JENDL3 data in the following table: 9437 1451 413 9437 1451 414 Energy range (eV) Fission(barn) Capture(barn) 9437 1451 415 ----------------- ----------------- ----------------- 9437 1451 416 JENDL3 present JENDL3 present 9437 1451 417 0.5 - 5.0 85.725 84.879 28.651 28.723 9437 1451 418 5.0 - 10.0 25.081 25.147 19.059 18.950 9437 1451 419 10.0 - 50.0 96.856 99.715 77.181 74.686 9437 1451 420 50.0 - 100.0 40.479 41.552 25.930 25.376 9437 1451 421 100.0 - 301.0 19.677 20.252 17.952 17.729 9437 1451 422 301.0 -1000.0 10.047 10.317 8.348 8.418 9437 1451 423 1000.0 -2000.0 3.484 3.206 2.840 2.634 9437 1451 424 2000.0 -2.E+07 17.783 (17.783) 5.224 (5.224) 9437 1451 425 ----------------- ----------------- ----------------- 9437 1451 426 Total 299.132 302.851 185.185 181.739 9437 1451 427 ---------------------------------------------------------- 9437 1451 428 9437 1451 429 The JENDL3 resonance parameters are those obtained in 1987 in 9437 1451 430 the energy range 0 keV to 1 keV. They are sligthly different from9437 1451 431 those published in 1989. Which explains the small differences 9437 1451 432 observed between JENDL3 and the present results in this energy 9437 1451 433 range. In the energy range 1 keV to 2 keV, JENDL3 is unresolved 9437 1451 434 range. The fission and capture resonance integrals calculated 9437 1451 435 from ENDF/B-V and those found in BNL-325 are the following: 9437 1451 436 9437 1451 437 ENDF/B-V Fission: 302.13 b Capture: 194.10 b 9437 1451 438 BNL-325 Fission: 310+-10 b Capture: 200+-20 b 9437 1451 439 9437 1451 440 The consequence of changing from the old sets of resonance 9437 1451 441 parameters(ENDF/B-V and previous sets) to the new set is that 9437 1451 442 the capture resonance integral will decrease by 6.7% compared 9437 1451 443 with the ENDF/B-V value. 9437 1451 444 9437 1451 445 ---------------------------------------------------------------- 9437 1451 446 UNRESOLVED RESONANCE REGION 9437 1451 447 9437 1451 448 The average resonance prameters are given in the energy range 9437 1451 449 2.5 keV to 30 keV for 70 energy points. They were obtained by 9437 1451 450 using the Cadarache statistical code FISINGA to fit the gross 9437 1451 451 structure of the Saclay experimental total cross sections [26] 9437 1451 452 below 4 keV and of selected experimental fission cross sections 9437 1451 453 normalized to ENDF/B-VI standard evaluation [11]. Above 4 keV no 9437 1451 454 high resolution total cross section data are available; average 9437 1451 455 total cross sections were calculated to be consistent with the 9437 1451 456 stastistical paramaters obtained in the resolved resonance 9437 1451 457 region [14] and with the Optical Model parameters of Lagrange 9437 1451 458 and Madland [24] obtained by fitting the experimental data in 9437 1451 459 the high energy range. A value of 9.46 Fm was used for the 9437 1451 460 effective radius. The values obtained for alpha are consistent 9437 1451 461 with the experimental data. 9437 1451 462 The competitive width is not used for the inelastic scattering9437 1451 463 cross section. In each energy point of the unresolved region the 9437 1451 464 neutron width corresponds only to the elastic scattering cross 9437 1451 465 section. The inelastic scattering cross section should be found 9437 1451 466 file 3. 9437 1451 467 The cross sections obtained at 0RNL by processing the 9437 1451 468 evaluated file using NJOY-87.1 are given in the following table, 9437 1451 469 'FISS' for the fission values and 'CAPT' for the capture values. 9437 1451 470 9437 1451 471 Energy Cross sections Energy Cross sections 9437 1451 472 (keV) (barn) (keV) (barn) 9437 1451 473 ------ ----------------- ------ ---------------- 9437 1451 474 FISS CAPT FISS CAPT 9437 1451 475 2.500 4.280 2.456 13.750 1.715 0.942 9437 1451 476 2.550 2.725 2.754 14.250 1.492 0.948 9437 1451 477 2.650 3.103 3.425 14.750 1.797 0.854 9437 1451 478 2.750 4.169 2.010 15.250 1.883 0.797 9437 1451 479 2.850 4.126 2.077 15.750 1.697 0.843 9437 1451 480 2.950 3.362 3.710 16.250 1.801 0.782 9437 1451 481 3.050 3.017 1.998 16.750 1.628 0.824 9437 1451 482 3.150 4.896 1.934 17.250 1.498 0.819 9437 1451 483 3.250 3.954 2.277 17.750 1.862 0.701 9437 1451 484 3.350 1.710 2.166 18.250 1.711 0.736 9437 1451 485 3.450 2.198 2.572 18.750 1.632 0.748 9437 1451 486 3.550 2.214 1.885 19.250 1.738 0.694 9437 1451 487 3.650 2.394 2.948 19.750 1.743 0.677 9437 1451 488 3.750 3.067 1.624 20.500 1.672 0.679 9437 1451 489 3.850 3.556 2.122 21.500 1.646 0.661 9437 1451 490 3.950 2.931 2.397 22.500 1.472 0.697 9437 1451 491 4.125 2.114 2.270 23.500 1.632 0.619 9437 1451 492 4.375 2.509 2.129 24.500 1.636 0.597 9437 1451 493 4.625 2.772 1.715 25.500 1.547 0.607 9437 1451 494 4.875 1.980 2.186 26.500 1.628 0.562 9437 1451 495 5.125 2.406 1.916 27.500 1.544 0.572 9437 1451 496 5.375 2.153 1.953 28.500 1.568 0.549 9437 1451 497 5.625 2.294 1.807 29.500 1.609 0.521 9437 1451 498 9437 1451 499 Average values of the fission cross sections compared to the 9437 1451 500 ENDF/B-VI standard evaluation [11] and alpha values compared to 9437 1451 501 some experimental data are given in the following table. 9437 1451 502 9437 1451 503 Energy Cross sections (barn) Alpha 9437 1451 504 (keV) (1) (2) (3) (4) (5) (6) (7) (8) 9437 1451 505 ------ ------------------------- -------------------------- 9437 1451 506 3- 4 2.992 3.000 2.213 2.20 0.740 0.720 0.895 0.820 9437 1451 507 4- 5 2.394 2.383 2.073 2.07 0.866 0.870 0.821 0.837 9437 1451 508 5- 6 2.266 2.301 1.863 1.91 0.822 0.820 0.867 0.834 9437 1451 509 6- 7 2.006 2.008 1.677 1.63 0.836 0.790 0.816 0.793 9437 1451 510 7- 8 2.134 2.054 1.409 1.34 0.660 0.640 0.630 0.605 9437 1451 511 8- 9 2.207 2.216 1.245 1.23 0.564 0.540 0.575 0.530 9437 1451 512 9-10 1.867 1.864 1.136 1.05 0.608 0.550 0.617 0.569 9437 1451 513 9437 1451 514 1-10 2.628 2.622 2.014 2.06 0.767 0.752 0.806 0.768 9437 1451 515 10-20 1.762 1.764 0.876 0.85 0.497 0.480 0.466 0.498 9437 1451 516 20-30 1.597 1.595 0.606 0.58 0.379 0.350 0.373 0.388 9437 1451 517 ------------------------------------------------------------- 9437 1451 518 (1) Fission cross section, present evaluation (0K) 9437 1451 519 (2) Fission cross section, ENDF/B-VI standard [11] 9437 1451 520 (3) Capture cross section, present evaluation (293 K) 9437 1451 521 (4) Capture cross section, Gwin et al. 1976 [4] 9437 1451 522 (5) Alpha value, present evaluation (293 K) 9437 1451 523 (6) Alpha value from Gwin et al. 1976 [4] 9437 1451 524 (7) Alpha value from Sowerby-Konshin evaluation 1971 [25] 9437 1451 525 (8) Average alpha value from experimental data 9437 1451 526 9437 1451 527 The fission and capture resonance integrals obtained at 0RNL are 9437 1451 528 compared to ENDF/B-5 data in the following table. 9437 1451 529 9437 1451 530 Energy range Fission (barn) Capture (barn) 9437 1451 531 (eV) ENDF/B-5 present ENDF/B-5 present 9437 1451 532 --------------- ----------------- ----------------- 9437 1451 533 0.5 - 5.0 86.02 85.71 32.31 28.65 9437 1451 534 5.0 - 10.0 26.03 25.08 20.14 19.06 9437 1451 535 10.0 - 50.0 100.25 96.87 78.66 77.19 9437 1451 536 50.0 - 100.0 40.32 40.47 27.23 25.93 9437 1451 537 100.0 - 301.0 19.98 19.68 19.52 17.95 9437 1451 538 301.0 -1000.0 10.15 10.05 8.54 8.35 9437 1451 539 --------------- ----------------- ----------------- 9437 1451 540 0.5 -1000.0 282.76 277.85 186.30 177.13 9437 1451 541 -------------------------------------------------------- 9437 1451 542 9437 1451 543 The fission and capture resonance integrals are obtained by 9437 1451 544 adding the ENDF/B-V value above 1 keV to the present evaluation. 9437 1451 545 These and the corresponding values from ENDF/B-V evaluation are: 9437 1451 546 Present - Fission: 297.22 b Capture: 184.93 b 9437 1451 547 ENDF/B-V - Fission: 302.13 b Capture: 194.10 b 9437 1451 548 9437 1451 549 ---------------------------------------------------------------- 9437 1451 550 REFERENCES 9437 1451 551 9437 1451 552 1. R. Gwin et al., Nucl.Sci.Eng. 45, 25 (1971). 9437 1451 553 2. A.J. Deruyter et al., J.Nucl.En. 26, 293 (1972). 9437 1451 554 3. J. Blons, Nucl.Sci.Eng. 51, 130 (1973). 9437 1451 555 4. R. Gwin et al., Nucl.Sci.Eng. 59, 79 (1976). 9437 1451 556 5. R. Gwin et al., Nucl.Sci.Eng. 61, 116 (1976). 9437 1451 557 6. W. Wagemans, Ann.Nucl.En. 7 #9, 495 (1980). 9437 1451 558 7. R. Gwin et al., Nucl.Sci.Eng. 88, 37 (1984). 9437 1451 559 8. L.W. Weston et al., Nucl.Sci.Eng. 88, 567 (1984). 9437 1451 560 9. J.A. Harvey et al., Nuclear Data for Sci. and Technol., Proc. 9437 1451 561 Int. Conf., May 30 - June 3, 1988, Mito, Japan (Saikon 9437 1451 562 Publishing Co., 1988) p.115. 9437 1451 563 10. R.R. Spencer et al., Nucl.Sci.Eng. 96, 318 (1987). 9437 1451 564 11. A. Carlson et al., preliminary results of the ENDF/B-6 9437 1451 565 standard evaluation (Sep.8, 1987); see W. P. Poenitz et al., 9437 1451 566 Argonne National Laboratory report ANL/NDM-139 [ENDF-358] 9437 1451 567 (1997) 9437 1451 568 12. A.J. Deruyter, J.Nucl.En. 26, 293 (1972). 9437 1451 569 13. N.M. Larson et al., Oak Ridge National Laboratory reports 9437 1451 570 ORNL/TM-7485, ORNL/TM-9179, and ORNL/TM-9719/R1 9437 1451 571 14. H. Derrien and G. DeSaussure, Oak Ridge National Laboratory 9437 1451 572 report ORNL-TM-10986 (1988). 9437 1451 573 15. L.W. Weston and J.H. Todd, Nucl.Sci.Eng. 111, 415 (1992). 9437 1451 574 16. H. Derrien et al., Nucl.Sci.Eng. 106, 434 (1990). 9437 1451 575 17. H. Derrien and T. Nakagawa, to be published. 9437 1451 576 18. L. Leal and R.N. Hwang, Trans.Am.Nucl.Soc. 55, 340 (1987). 9437 1451 577 19. H. Derrien et aL., Nucl.Sci.Eng. 106, 434 (1990). 9437 1451 578 20. T. Nakagawa, RESENDD a JAERI version of RESEND 9437 1451 579 21. C. Wagemans et al., Nuclear Data for Sci. and Technol., Proc. 9437 1451 580 Int. Conf., May 30 - June 3, 1988, Mito, Japan (Saikon 9437 1451 581 Publishing Co., 1988) p.91. 9437 1451 582 22. L.W. Weston et al., Nucl.Sci.Eng. 115, 164 (1993). 9437 1451 583 23. H. Derrien, to be published in J.Nucl.Sci.Technol. 9437 1451 584 24. Ch. Lagrange and D.G. Madland, Phys.Rev. C 33, 1616 (1986). 9437 1451 585 25. M.G. Sowerby et al., At.En.Rev. 10, 453 (1972) 9437 1451 586 26. H. Derrien, thesis, Univ. Paris - Sud, Orsay Serie A No. 1172 9437 1451 587 (1973). 9437 1451 588 9437 1451 589 ENERGY REGION 0.03 TO 20 MEV *********************************** 9437 1451 590 Principal LANL evaluators: P.G.Young, R.E.MacFarlane, E.D.Arthur 9437 1451 591 9437 1451 592 The evaluation above 10 keV is based on a detailed theoretical9437 1451 593 analysis utilizing the available experimental data. Coupled 9437 1451 594 channel optical model calculations with the ECIS code [Ra70] 9437 1451 595 were used to provide the total, elastic, and inelastic cross 9437 1451 596 sections to the first 7 members of the ground state rotational 9437 1451 597 band, as well as neutron elastic and inelastic angular distri- 9437 1451 598 butions to the rotational levels. The ECIS code was also 9437 1451 599 used to calculate neutron transmission coefficients. Hauser- 9437 1451 600 Feshbach statistical theory calculations were carried out with 9437 1451 601 the GNASH [Ar88,Yo77] and COMNUC [Du70] code systems, including 9437 1451 602 preequilibrium and fission. DWBA calculations were performed 9437 1451 603 with the DWUCK code [Ku70] for several vibrational levels, using 9437 1451 604 B(El) values inferred from (d,d') data on Pu238 and Pu240, as 9437 1451 605 well as Coulomb excitation measurements. A weak coupling 9437 1451 606 model [Pe69] was used to apply the Pu238 and Pu240 results to 9437 1451 607 states in Pu239. 9437 1451 608 This analysis is an extension of the calculations used for the 9437 1451 609 ENDF/B-V.2 evaluation, described in reference Ar82. 9437 1451 610 9437 1451 611 MF=1 Descriptive and Nubar Information ------------------------- 9437 1451 612 MT=452 Total Nubar. Sum of MT=455 and 456. 9437 1451 613 MT=455 Delayed Neutron Yields. England [En89]. 9437 1451 614 MT=456 Prompt Neutron Yields. From 10-5 to 650 eV, based on the9437 1451 615 evaluation of Fort [Fo88], after minor renormalization 9437 1451 616 for consistency with CSEWG standards. Fort's values 9437 1451 617 were multiplied by 1.000411 from 10-5 to 10 eV to 9437 1451 618 fall within 1/2 std. deviation of Pu239 thermal nubar 9437 1451 619 value, with the factor varying linearly to 1.00282 at 9437 1451 620 500 eV for consistency with Cf252 nubar. Fort's eval. 9437 1451 621 (renomalized) was used intact below 62.3 eV but higher 9437 1451 622 energy data were thinned with a thinning criterion of 9437 1451 623 0.036%, a factor of 5 less than the standard deviation 9437 1451 624 of the CSEWG standard value of Pu239 thermal nubar. 9437 1451 625 Above 650 eV, the evaluation is based on a covariance 9437 1451 626 analysis of all available exp. data from the CSISRS 9437 1451 627 data file at the NNDC, BNL, using the GLUCS analysis 9437 1451 628 code [He80]. A smooth curve was passed through the 9437 1451 629 GLUCS results with structure removed. All the exp. 9437 1451 630 data were renormalized to ENDF/B-VI standards 9437 1451 631 prior to the covariance analysis. 9437 1451 632 9437 1451 633 MF=3 Smooth Cross Sections ------------------------------------- 9437 1451 634 MT=1 Neutron Total Cross Section. 0.03 to 20 MeV, based on 9437 1451 635 coupled-channel optical calculations and the exp. data 9437 1451 636 of [Po81,Sh78,Po83,Sc74,Fo71,Sm73,Na73,Pe60,Ca73,Li90] 9437 1451 637 The experimental and theoretical results were combined 9437 1451 638 through a covariance analysis with the GLUCS code 9437 1451 639 system [He80]. The covariance analysis results, which 9437 1451 640 agreed well with Derrien's [De89] unresolved resonance 9437 1451 641 analysis at 30 keV, were smoothly joined to those 9437 1451 642 results between 30 and 50 keV. 9437 1451 643 MT=2 0.030 to 20 MeV, based on subtraction of MT=4,16,17,18, 9437 1451 644 37, and 102 from MT=1. 9437 1451 645 MT=4 Sum of MT=51-91 9437 1451 646 MT=16 GNASH Hauser-Feshbach statistical/preequilibrium calc. 9437 1451 647 MT=17 GNASH Hauser-Feshbach statistical/preequilibrium calc. 9437 1451 648 MT=18 The Pu239(n,f) cross section that resulted from the 9437 1451 649 simultaneous standards analysis for version 6 was 9437 1451 650 renormalized by a factor of 1.007 and used directly 9437 1451 651 from 50 keV to 1.25 MeV. Between 30 and 50 keV, the 9437 1451 652 evaluation was matched smoothly to the Derrien 9437 1451 653 unresolved resonance parameter analysis, requiring a 9437 1451 654 a reduction of about 4% near 30 keV. Above 1.25 MeV, 9437 1451 655 the evaluation is based on a new covariance analysis 9437 1451 656 of all available ratio and absolute Pu239(n,f) data, 9437 1451 657 including new measurements [Li88,Me88] that were not 9437 1451 658 available for the simul. standards analysis. The GLUCS 9437 1451 659 code was used for the covariance analysis, and a 9437 1451 660 smooth curve was drawn through the analysis results. 9437 1451 661 The new covariance analysis agrees reasonably with the 9437 1451 662 simultaneous standards results (both cross section and 9437 1451 663 standard deviation) at energies below the newer exp. 9437 1451 664 results. At higher energies, the effect of the new data 9437 1451 665 on the analysis is to raise the (n,f) cross section 9437 1451 666 somewhat at higher energies, particularly near 9 MeV 9437 1451 667 (about 4%) and above 15 MeV (few %). 9437 1451 668 MT=19 (n,f) first-chance fission cross section. 9437 1451 669 Ratio of first-chance to total fission obtained from 9437 1451 670 GNASH calculations. 9437 1451 671 MT=20 (n,nf) second-chance fission cross section. 9437 1451 672 Ratio of second-chance to total fission obtained from 9437 1451 673 GNASH calculations. 9437 1451 674 MT=21 (n,2nf) third-chance fission cross section. 9437 1451 675 Ratio of third-chance to total fission obtained from 9437 1451 676 GNASH calculations. 9437 1451 677 MT=37 GNASH Hauser-Feshbach statistical/preequilibrium calc. 9437 1451 678 MT=38 (n,3nf) fourth-chance fission cross section. 9437 1451 679 Ratio of fourth-chance to total fission obtained from 9437 1451 680 GNASH calculations. 9437 1451 681 MT=51-55,57 Thres. to 20 MeV, coupled-channel optical model 9437 1451 682 calculations (3/2+ to 13/2+ members of the K=1/2 ground 9437 1451 683 state rotational band) using the ECIS code. Compound 9437 1451 684 nucleus contributions, obtained from COMNUC calcula- 9437 1451 685 tions, are also included. 9437 1451 686 MT=56,58-69,71,72,74-77 Threshold to 6.0 MeV, Compound 9437 1451 687 nucleus reaction theory calculation with width fluctua- 9437 1451 688 tions, using the COMNUC code. 9437 1451 689 MT=70,73,78-81 Threshold to 20 MeV, distorted wave Born 9437 1451 690 approximation calculations with the DWUCK code for 9437 1451 691 l=2 and l=3 vibrational states. The l=2 states are 9437 1451 692 MT=78,80 and the l=3 states are MT=70,73,79, and 81. 9437 1451 693 Compound nucleus contributions were included in 9437 1451 694 the data for MT = 70 and 73. 9437 1451 695 MT=91 GNASH Hauser-Feshbach statistical/preequilibrium calc. 9437 1451 696 Note that the MT=78-81 vibrational states lie in the 9437 1451 697 MT=91 continuum region. 9437 1451 698 MT=102 0.030-20 MeV, obtained using the values of alpha (ratio 9437 1451 699 of capture to fission cross sections) from ENDF/B-V.2, 9437 1451 700 together with MT=18 from the present evaluation. 9437 1451 701 Between 40 and 100 MeV, structure in the cross section 9437 1451 702 was smoothed out. Below 50 keV, the results were 9437 1451 703 smoothly joined to the unresolved resonance result at 9437 1451 704 30 keV, requiring an increase of 0.2% at 30 keV. 9437 1451 705 9437 1451 706 MF=4 Neutron Angular Distributions ----------------------------- 9437 1451 707 MT=2 Elastic scattering angular distribution based on ECIS 9437 1451 708 coupled-channel calculations, with a compound elastic 9437 1451 709 component from COMNUC included below 6 MeV. 9437 1451 710 MT=51-55,57 Thres. to 20 MeV, Coupled-channel optical model 9437 1451 711 calculations plus compound-nucleus contributions. 9437 1451 712 MT=56,58-69,71,72,74-77 Threshold to 6.0 MeV, Compound 9437 1451 713 nucleus reaction theory calculation with width fluctua- 9437 1451 714 tions, using the COMNUC code. 9437 1451 715 MT=70,73,78-81 Thres. to 20 MeV, Distorted wave Born approx. 9437 1451 716 imation calculations with DWUCK code. Compound-nucleus 9437 1451 717 contributions are included for MT=70 and 73. 9437 1451 718 9437 1451 719 MF=5 Neutron Energy Distributions ------------------------------ 9437 1451 720 MF=18 Composite neutron energy distributions from fission. 9437 1451 721 Based on calculations by D.Madland [Ar84] using Madland-9437 1451 722 Nix formalism. The calculations include the first-, 9437 1451 723 second-, and third-chance fission neutron components. 9437 1451 724 These data are the same as were used for Revision 2 of 9437 1451 725 ENDF/B-V. Parameters for the calculation were adjusted 9437 1451 726 to give the same average fission neutron energy at 9437 1451 727 thermal as ENDF/B-V.0. Tabulated data (LF=1) used. 9437 1451 728 MT=455 Tal England [En89]. 9437 1451 729 9437 1451 730 MF=6 Correlated Energy-Angle Distributions --------------------- 9437 1451 731 MT=16 GNASH Hauser-Feshbach statistical/preequilibrium calc. 9437 1451 732 Updated Kalbach-Mann systematics used for specifying 9437 1451 733 neutron distributions [Ka87]. Only neutrons given. 9437 1451 734 MT=17 GNASH Hauser-Feshbach statistical/preequilibrium calc. 9437 1451 735 Updated Kalbach-Mann systematics used for specifying 9437 1451 736 neutron distributions [Ka87]. Only neutrons given. 9437 1451 737 MT=37 GNASH Hauser-Feshbach statistical/preequilibrium calc. 9437 1451 738 Updated Kalbach-Mann systematics used for specifying 9437 1451 739 neutron distributions [Ka87]. Only neutrons given. 9437 1451 740 MT=91 GNASH Hauser-Feshbach statistical/preequilibrium calc. 9437 1451 741 Updated Kalbach-Mann systematics used for specifying 9437 1451 742 neutron distributions [Ka87]. Only neutrons given. 9437 1451 743 9437 1451 744 MF=12,13,14,15 Photon-Production Data -------------------------- 9437 1451 745 All photon-production data were carried over from ENDF/B-V.2, 9437 1451 746 MAT=1399. Data are given for MF=12, MT=4,18,102; MF=13, MT=3; 9437 1451 747 MF=14, MT=3,4,18,102; and, MF=15, MT=3,4,18,102. 9437 1451 748 9437 1451 749 ---------------------------------------------------------------- 9437 1451 750 REFERENCES 9437 1451 751 9437 1451 752 [Ar84] E. Arthur et al., Nuc.Sci.Eng. 88, 56 (1984). 9437 1451 753 [Ar88] E.D. Arthur, report LA-UR-88-382 (1988). 9437 1451 754 [Ca73] J. Cabe et al., report CEA-R-4524 (1973). 9437 1451 755 [Ca85] A. Carlson et al., Nuclear Data for Basic and Applied 9437 1451 756 Science, Proc. Conf., Santa Fe, NM 13-17 May 1985 (Gordon and 9437 1451 757 Breach Science Publishers, 1986) p.1429. 9437 1451 758 [De89] H. Derrien and G. de Saussure, Oak Ridge National 9437 1451 759 Laboratory report ORNL-10986 (1989). 9437 1451 760 [Du70] C.L. Dunford, report AI-AEC-12931 (1970). 9437 1451 761 [En89] T.R. England et al, Los Alamos reports LA 11151-MS 9437 1451 762 (1988) and LA-11534-T (1989); M.C. Brady and T.R. England, 9437 1451 763 Nucl.Sci.Eng. 103, 129 (1989). 9437 1451 764 [Fo71] D. Foster and D. Glasgow, Phys.Rev. C3, 576 (1971). 9437 1451 765 [Fo88] E. Fort et al., Nuc.Sci.Eng. 99, 375 (1988). 9437 1451 766 [Fr86] J. Frehaut, report NEANDC(E) 238/L (1986). 9437 1451 767 [He80] D. Hetrick and C.Y. Fu, Oak Ridge National Laboratory 9437 1451 768 report ORNL/TM-7341 (1980). 9437 1451 769 [Ka87] C. Kalbach, Phys.Rev. C 37, 2350 (1988). 9437 1451 770 [Ku70] P.D. Kunz, DWUCK: A Distorted-Wave Born Approximation 9437 1451 771 Program, unpublished report. 9437 1451 772 [Li88] P. Lisowski et al., Nuclear Data for Sci. and Technol., 9437 1451 773 Proc. Int. Conf., May 30-June 3, 1988, Mito, Japan (Saikon 9437 1451 774 Publishing Co., 1988) p.97. 9437 1451 775 [Li90] P. Lisowski, private comm. of WNR data taken in 1985. 9437 1451 776 [Me88] J. Meadows, Ann.Nucl.Energy 15, 421 (1988). 9437 1451 777 [Na73] K. Nadolny et al., USNDC-9 (1973)p.170 9437 1451 778 [Pe60] J. Peterson et al., Phys.Rev. 120, 521 (1960). 9437 1451 779 [Pe69] R.J. Peterson, Ann.Phys. 53, 40 (1969). 9437 1451 780 [Po81] W. Poenitz et al., Nuc.Sci.Eng. 78, 333 (1981). 9437 1451 781 [Po83] W. Poenitz et al., Argonne National Laboratory report 9437 1451 782 ANL-NDM-80 (1983). 9437 1451 783 [Ra70] J. Raynal,IAEA SMR-9/8 (1970). 9437 1451 784 [Sc74] R. Schwartz et al., Nucl.Sci.Eng. 54, 322 (1974). 9437 1451 785 [Sh78] R. Shamu et al., private communication, 1978. 9437 1451 786 [Sm73] A. Smith et al., J.Nuc.En. 27, 317 (1973). 9437 1451 787 [Yo77] P.G. Young and E.D. Arthur, Los Alamos National 9437 1451 788 Laboratory report LA-6947 (1977). 9437 1451 789 [Yo88] P.G. Young and E.D. Arthur, Nuclear Data for Sci. and 9437 1451 790 Technol., Proc. Int. Conf., May 30-June 3, 1988, Mito, Japan 9437 1451 791 (Saikon Publishing Co., 1988) p.603. 9437 1451 792 9437 1451 793 ************************ C O N T E N T S *********************** 9437 1451 794 1 451 895 39437 1451 795 1 452 912 19437 1451 796 1 455 7 39437 1451 797 1 456 912 19437 1451 798 1 458 5 29437 1451 799 2 151 1445 39437 1451 800 3 1 117 19437 1451 801 3 2 110 19437 1451 802 3 4 43 19437 1451 803 3 16 17 19437 1451 804 3 17 9 19437 1451 805 3 18 104 19437 1451 806 3 19 104 19437 1451 807 3 20 47 19437 1451 808 3 21 32 19437 1451 809 3 37 5 19437 1451 810 3 38 15 19437 1451 811 3 51 41 19437 1451 812 3 52 38 19437 1451 813 3 53 37 19437 1451 814 3 54 36 19437 1451 815 3 55 35 19437 1451 816 3 56 23 19437 1451 817 3 57 34 19437 1451 818 3 58 22 19437 1451 819 3 59 22 19437 1451 820 3 60 21 19437 1451 821 3 61 21 19437 1451 822 3 62 20 19437 1451 823 3 63 20 19437 1451 824 3 64 19 19437 1451 825 3 65 19 19437 1451 826 3 66 19 19437 1451 827 3 67 18 19437 1451 828 3 68 18 19437 1451 829 3 69 18 19437 1451 830 3 70 29 19437 1451 831 3 71 17 19437 1451 832 3 72 16 19437 1451 833 3 73 28 19437 1451 834 3 74 15 19437 1451 835 3 75 15 19437 1451 836 3 76 14 19437 1451 837 3 77 14 19437 1451 838 3 78 25 19437 1451 839 3 79 24 19437 1451 840 3 80 24 19437 1451 841 3 81 23 19437 1451 842 3 91 26 19437 1451 843 3 102 46 19437 1451 844 4 2 111 19437 1451 845 4 18 2 19437 1451 846 4 51 109 19437 1451 847 4 52 105 19437 1451 848 4 53 103 19437 1451 849 4 54 101 19437 1451 850 4 55 101 19437 1451 851 4 56 56 19437 1451 852 4 57 97 19437 1451 853 4 58 54 19437 1451 854 4 59 54 19437 1451 855 4 60 54 19437 1451 856 4 61 54 19437 1451 857 4 62 52 19437 1451 858 4 63 52 19437 1451 859 4 64 52 19437 1451 860 4 65 52 19437 1451 861 4 66 52 19437 1451 862 4 67 52 19437 1451 863 4 68 52 19437 1451 864 4 69 52 19437 1451 865 4 70 91 19437 1451 866 4 71 50 19437 1451 867 4 72 50 19437 1451 868 4 73 91 19437 1451 869 4 74 50 19437 1451 870 4 75 50 19437 1451 871 4 76 48 19437 1451 872 4 77 47 19437 1451 873 4 78 85 19437 1451 874 4 79 82 19437 1451 875 4 80 79 19437 1451 876 4 81 79 19437 1451 877 5 18 1640 19437 1451 878 5 455 579 19437 1451 879 6 16 663 19437 1451 880 6 17 200 19437 1451 881 6 37 30 19437 1451 882 6 91 1341 19437 1451 883 12 4 65 09437 1451 884 12 18 5 09437 1451 885 12 102 5 09437 1451 886 13 3 7 09437 1451 887 14 3 1 09437 1451 888 14 4 1 09437 1451 889 14 18 1 09437 1451 890 14 102 1 09437 1451 891 15 3 136 09437 1451 892 15 4 41 09437 1451 893 15 18 58 09437 1451 894 15 102 56 09437 1451 895 0.000000+0 0.000000+0 0 0 0 09437 1 099999 9.423900+4 2.369986+2 0 2 0 09437 1452 1 0.000000+0 0.000000+0 0 0 1 27269437 1452 2 2726 2 9437 1452 3 1.000000-5 2.880712+0 3.000000-5 2.880710+0 4.999999-3 2.880383+09437 1452 4 2.530000-2 2.878900+0 3.125000-2 2.878465+0 3.515600-2 2.878225+09437 1452 5 5.078100-2 2.876840+0 6.640601-2 2.875400+0 7.812500-2 2.874373+09437 1452 6 9.375000-2 2.872725+0 1.054700-1 2.871565+0 1.171900-1 2.870327+09437 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