TAPE 135 135 0 0 0 9.424101+4 2.389780+2 1 1 0 39443 1451 1 0.000000+0 1.000000+0 0 0 0 69443 1451 2 1.000000+0 0.000000+0 0 0 10 69443 1451 3 0.000000+0 0.000000+0 0 0 365 679443 1451 4 94-PU-241 ORNL EVAL-OCT88 L.WESTON,R.WRIGHT,H.DERRIEN + 9443 1451 5 DIST-SEP91 REV2-AUG94 950427 9443 1451 6 ----ENDF/B-VI MATERIAL 9443 REVISION 2 9443 1451 7 -----INCIDENT NEUTRON DATA 9443 1451 8 ------ENDF-6 FORMAT 9443 1451 9 * * * * * 9443 1451 10 CHANGES FOR REVISION 2 WERE INSERTION OF REVISED RESONANCE REGION9443 1451 11 PARAMETERS BY DERRIEN; RENORMALIZATION OF CAPTURE ABOVE THE 9443 1451 12 RESOLVED RESONANCE REGION TO BE 4.8% LOWER THAN VERSION 5 AND 9443 1451 13 UPWARD FROM 14% DOWN IN ORIGINAL VERSION 6. SCATTERING WAS 9443 1451 14 ADJUSTED TO MAKE UP DIFFERENCE. THE RENORMALIZATION WAS THE 9443 1451 15 SUGGESTION OF DERRIEN AFTER STUDY OF THE NEW MEASUREMENTS BY 9443 1451 16 WAGEMANS ET AL., REF 1. 9443 1451 17 * * * * * 9443 1451 18 PU-241 WAS REVISED FOR VERSION VI BY L.W.WESTON. THE 9443 1451 19 CHANGES WERE THE ADOPTION OF THE RECOMMENDED VALUES OF THE 9443 1451 20 STANDARDS COMMITTEE FOR THE THERMAL CONSTANTS; THE ADOPTION 9443 1451 21 OF THE REICH-MOORE RESONANCE PARAMETER EVALUATION OF THE 9443 1451 22 RESOLVED RESONANCE REGION BY H.DERRIEN,REF 2., OF CADARACHE, 9443 1451 23 FRANCE; RENORMALIZATION OF CAPTURE ABOVE 300EV BY 14% DOWNWARD 9443 1451 24 AS RECOMMENDED BY H.DERRIEN. THE TOTALS ABOVE 100 KEV WERE MADE 9443 1451 25 SAME AS PU-239. CAPTURE REVISED DOWNWARD ABOVE 1.5 MEV. 9443 1451 26 COVARIANCES WERE STRIPED OFF BECAUSE THEY WERE DEPENDANT ON 9443 1451 27 U-235 COVARIANCES WHICH ARE NOT COMPLETED. 9443 1451 28 ******************************************************************9443 1451 29 MF=1 MT=452 THERMAL NUBAR OF 2.9453 RECOMMENDED BY STANDARDS 9443 1451 30 COMMITTEE. PROMPT RATIOS TO CF ABOVE .47 MEV FROM 9443 1451 31 FREHAUT,REF.3. NUBAR PROMPT OF CF OF 3.7676. 9443 1451 32 MF=1 MT=455 TABULATION OF NU DELAYED (REF.4) EXCEPT THERMAL. 9443 1451 33 MF=1 MT=456 SEE MT=452 9443 1451 34 MF=2 MT=151 RESOLVED RESONANCE REGION 10-5 TO 300EV,REICH-MOORE 9443 1451 35 $$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$9443 1451 36 REVISED RESONANCE DATA ,JAERI MAY 1993 9443 1451 37 ***************************************************************** 9443 1451 38 Revision of the 241Pu Reich-Moore resonance parameters 9443 1451 39 by comparison with recent fission cross section measurements. 9443 1451 40 9443 1451 41 Herve Derrien 9443 1451 42 Japanese Atomic Energy Research Institute 9443 1451 43 9443 1451 44 I-INTRODUCTION. 9443 1451 45 The resonance parameters of the neutron cross sections 9443 1451 46 of 241Pu were obtained by Derrien and de Saussure(2) in the energy9443 1451 47 range from thermal to 300 eV by a Bayesian fit of selected 9443 1451 48 experimental effective total cross sections, fission and capture 9443 1451 49 cross sections by using the Reich-Moore fitting code SAMMY(5). 9443 1451 50 The results of this work were used in the ENDF/B-VI evaluated data9443 1451 51 file. Some difficulties were encountered in the normalization of 9443 1451 52 the experimental fission cross sections due to the discrepancies 9443 1451 53 in the shape of the available experimental data both in thermal 9443 1451 54 and high energy ranges. The consistency among the experimental 9443 1451 55 data base could not be obtained without large renormalization and 9443 1451 56 background correction parameters in the SAMMY fits. Particularly,9443 1451 57 it was shown that the discrepancy between the fission cross 9443 1451 58 sections in the thermal energy range was due to a deviation from 9443 1451 59 the 1/v shape below about 0.05 eV. 9443 1451 60 New fission cross section measurements were recently 9443 1451 61 performed by Wagemans et al.(1,6) in the energy range from 0.002 9443 1451 62 eV to 20 eV in order to check the shape of the cross section in 9443 1451 63 the thermal energy range. They showed that the shape of the 9443 1451 64 fission cross section was clearly compatible with the 1/v law,in 9443 1451 65 contradiction to all the previous measurements reported in the 9443 1451 66 literature. Consequently, the normalization of all the 9443 1451 67 previous results using the low energy region could be erroneous. 9443 1451 68 Particularly,the discrepancy observed in the average fission 9443 1451 69 cross section over the 0.26 eV resonance could be due to the 9443 1451 70 errors of normalization in the thermal region. Wagemans et al. 9443 1451 71 compared the ENDF/B-VI data to their new results and concluded 9443 1451 72 that the evaluated data files using the evaluation of Derrien and 9443 1451 73 de Saussure should be revised in the energy range up to 300 eV. 9443 1451 74 9443 1451 75 II-COMMENTS ON ENDF/B-VI EVALUATION. 9443 1451 76 9443 1451 77 In the energy range from 0.01 eV to 3 eV the new data of 9443 1451 78 Wagemans et al. are on average 2.2% smaller than ENDF/B-VI. This 9443 1451 79 difference is mainly due a difference of 3% between the 1976 data 9443 1451 80 of Wagemans et al.(7) and the new values of Wagemans et al. The 9443 1451 81 1976 data of Wagemans et al. were used in the evaluation of 9443 1451 82 Derrien and de Saussure in the low energy region. 9443 1451 83 In the intermediate energy range from 3 eV to 12 eV,the 9443 1451 84 average fission of ENDF/B-VI is in excellent agreement with the 9443 1451 85 new data of Wagemans et al. In this energy range,the SAMMY fits of9443 1451 86 Derrien and de Saussure were performed on the fission cross 9443 1451 87 section of Weston and Todd(8),of Blons(9) and of Migneco et al. 9443 1451 88 (10) with an adjustment of the normalization factor and of the 9443 1451 89 background correction parameters of all the experimental data; the9443 1451 90 agreement between the new data of Wagemans et al. and ENDF/B-VI 9443 1451 91 shows that, at least in this energy range, SAMMY performed on the 9443 1451 92 data of Weston and Todd a renormalization equivalent to that 9443 1451 93 recommended by Wagemans et al.(1). 9443 1451 94 In the higher range up to 300 eV,the SAMMY fits relied 9443 1451 95 mainly on the high resolution measurements of Blons and of 9443 1451 96 Migneco et al. for the accurate determination of the resonance 9443 1451 97 parameters. Quite large normalization coefficients and background9443 1451 98 correction parameters were also needed in this energy range to 9443 1451 99 obtain the consistency between the calculated cross sections and 9443 1451 100 the experimental data. However,the result of the fits was in quite9443 1451 101 good agreement with the data of Weston and Todd normalized to the 9443 1451 102 1976 data of Wagemans et al.in the low energy region, which is 9443 1451 103 also equivalent to the normalization to the 1983 data of Wagemans 9443 1451 104 et al.(11). Since the earlier data of Wagemans et al. should 9443 1451 105 decrease by 3% to be consistent with the new data, it is likely 9443 1451 106 that the ENDF/B-VI fission cross section could be too large by 9443 1451 107 about 3% in the energy range above 12 eV. 9443 1451 108 9443 1451 109 III-REVISION OF THE RESONANCE PARAMETERS. 9443 1451 110 9443 1451 111 An accurate up-dating of the 241Pu resonance parameters 9443 1451 112 could be obtained by renormalizing the fission experimental data 9443 1451 113 base according to the new data of Wagemans et al. and by 9443 1451 114 restarting the SAMMY fits of the new experimental data base, 9443 1451 115 including the high resolution transmission data of Harvey and 9443 1451 116 Simpson(12). Due to lack of time a new SAMMY analysis was 9443 1451 117 performed only in the energy range from 0.002 eV to 3 eV. In the 9443 1451 118 energy range above 3 eV the up-dating was performed by applying 9443 1451 119 some small corrections to the resonance parameters. 9443 1451 120 The SAMMY analysis of the new Wagemans et al. data was 9443 1451 121 performed along with the total cross section of Young and 9443 1451 122 Smith(13) in the energy range from 0.002 eV to 3 eV,by starting 9443 1451 123 with the ENDF/B-VI resonance parameters. Only the parameters of 9443 1451 124 the 3+ resonances at -0.122 eV and at 0.265 eV were adjusted in 9443 1451 125 this energy range. The values of the cross sections calculated 9443 1451 126 at 0.0253 eV are compared to the standard data(14) in Table 1. The9443 1451 127 average total,fission and capture cross sections calculated with 9443 1451 128 the new resonance parameters are displayed on Table 2,3 and 4 with9443 1451 129 the corresponding experimental data and the values obtained from 9443 1451 130 ENDF/B-VI. One should point out that an energy shift of 9443 1451 131 dE/E=+0.00384 was applied to the data of Young and Smith in order 9443 1451 132 to achieve a good consistency with the energy scale of the 9443 1451 133 fission data of Wagemans et al. over the resonance at 0.0265 eV. 9443 1451 134 In the energy range above 3 eV the small corrections 9443 1451 135 applied to the resonance parameters result in a decrease of the 9443 1451 136 average fission cross section and in an increase of the average 9443 1451 137 capture cross section,with a variation of the average total cross 9443 1451 138 section smaller than the errors of the experimental data of Harvey9443 1451 139 and Simpson. The average values of the fission and capture cross 9443 1451 140 sections calculated with the new resonance parameters are shown in9443 1451 141 Table 5 and 6 along with the renormalized fission cross section of9443 1451 142 Weston and Todd and the values calculated from ENDF/B-VI. 9443 1451 143 9443 1451 144 IV-CONCLUSION. 9443 1451 145 9443 1451 146 The results of the recent measurement of the 241Pu fission9443 1451 147 cross section in the energy range from 0.002 eV to 4 eV of 9443 1451 148 Wagemans et al. were used in a new evaluation of the resonance 9443 1451 149 parameters. The accuracy of the calculated cross sections was 9443 1451 150 greatly improved in the resonance at 0.265 eV. The cross sections 9443 1451 151 averaged over this resonance should have the same accuracy as 9443 1451 152 the standard values at 0.0253 eV. In the high energy region up 9443 1451 153 to 300 eV the SAMMY analysis of the new experimental data base 9443 1451 154 obtained by the renormalization of the experimental data is 9443 1451 155 recommended in order to improve the corrections to the resonance 9443 1451 156 parameters performed in the present work. 9443 1451 157 9443 1451 158 9443 1451 159 Table 1 9443 1451 160 9443 1451 161 Cross sections at 0.0253 eV 9443 1451 162 9443 1451 163 ------------------------------------------------------------- 9443 1451 164 Present results ENDF/B-VI Standard(14) 9443 1451 165 ------------------------------------------------------------- 9443 1451 166 Fission 1012.50(-0.0%) 1012.68+-6.58 9443 1451 167 Capture 361.52(+0.1%) 361.29+-4.95 9443 1451 168 Scattering 11.36(-7.1%) 12.17+-2.62 9443 1451 169 Total 1385.38(-0.1%) 1386.14+-8.64 9443 1451 170 ------------------------------------------------------------- 9443 1451 171 9443 1451 172 9443 1451 173 Table 2 9443 1451 174 9443 1451 175 The total cross section integral in the energy range from 9443 1451 176 0.0021 eV to 3 eV. 9443 1451 177 9443 1451 178 ------------------------------------------------------------------9443 1451 179 Energy range Present work ENDF/B-VI Young and Smith(13) 9443 1451 180 (eV) (b.eV) (b.eV) (b.eV) 9443 1451 181 ------------------------------------------------------------------9443 1451 182 0.0021-0.020 43.54 43.09(-1.0%) 43.25(-0.7%) 9443 1451 183 0.0200-0.030 14.03 14.02(-0.1%) 14.01(-0.1%) 9443 1451 184 0.0300-0.100 65.09 66.17(+1.7%) 64.99(-0.1%) 9443 1451 185 0.1000-0.500 378.38 385.27(+1.8%) 380.10(+0.4%) 9443 1451 186 0.5000-1.000 29.74 29.41(-1.1%) 31.19(+4.4%) 9443 1451 187 1.0000-3.000 83.36 83.92(+0.7%) 82.50(-1.0%) 9443 1451 188 ------------------------------------------------------------------9443 1451 189 0.0021-3.000 614.14 621.88(+1.3%) 616.04(+0.3%) 9443 1451 190 ------------------------------------------------------------------9443 1451 191 9443 1451 192 9443 1451 193 Table 3 9443 1451 194 9443 1451 195 The fission cross section integral in the energy range 9443 1451 196 from 0.0021 eV to 3 eV. 9443 1451 197 9443 1451 198 ------------------------------------------------------------------9443 1451 199 Energy range This work ENDF/B-VI Wagemans et al. Weston and Todd9443 1451 200 (eV) (b.eV) (b.eV) (b.eV)(1) (b.eV)(8) 9443 1451 201 ------------------------------------------------------------------9443 1451 202 0.0021-0.020 31.06 30.61(-1.5%) 31.09(+0.1%) 9443 1451 203 0.0200-0.030 10.24 10.22(-0.2%) 10.24( 0.0%) 9443 1451 204 0.0300-0.100 49.02 50.02(+2.0%) 48.70(-0.6%) 9443 1451 205 0.1000-0.500 262.76 270.84(+3.1%) 264.58(+0.7%) 262.53(-0.1%) 9443 1451 206 0.5000-1.000 17.93 17.64(-1.6%) 17.60(-1.8%) 17.67(-1.4%) 9443 1451 207 1.0000-3.000 54.88 55.62(+1.3%) 54.40(-0.9%) 55.06(+0.3%) 9443 1451 208 ------------------------------------------------------------------9443 1451 209 0.0021-3.000 425.89 434.95(+2.1%) 426.61(+0.2%) 9443 1451 210 ------------------------------------------------------------------9443 1451 211 0.1000-3.000 335.57 344.10(+2.5%) 336.58(+0.3%) 335.26(-0.1%) 9443 1451 212 ------------------------------------------------------------------9443 1451 213 Weston and Todd experimental data were normalized to Wagemans et 9443 1451 214 al.(1) in the energy range from 0.1 eV to 12 eV (original EXFOR 9443 1451 215 data multiplied by 0.952). 9443 1451 216 9443 1451 217 9443 1451 218 Table 4 9443 1451 219 9443 1451 220 The capture cross section integral in the energy range from 9443 1451 221 from 0.0021 eV to3 eV. 9443 1451 222 9443 1451 223 -------------------------------------------------------------- 9443 1451 224 Energy range Present work ENDF/B-VI Weston and Todd(8) 9443 1451 225 (eV) (b.eV) (b.eV) (b.eV) 9443 1451 226 -------------------------------------------------------------- 9443 1451 227 0.0021-0.020 12.25 12.28(+0.2%) 9443 1451 228 0.0200-0.030 3.67 3.68(+0.3%) 9443 1451 229 0.0300-0.100 15.28 15.39(+0.7%) 15.27(-0.1%) 9443 1451 230 0.1000-0.500 110.58 109.47(-1.0%) 110.49(-0.1%) 9443 1451 231 0.5000-1.000 5.90 5.87(-0.5%) 6.51 9443 1451 232 1.0000-3.000 7.30 7.14(-2.2%) 8.96 9443 1451 233 -------------------------------------------------------------- 9443 1451 234 0.0021-3.000 154.98 153.83(-0.7%) 9443 1451 235 -------------------------------------------------------------- 9443 1451 236 0.0300-3.000 139.06 137.87(-0.9%) 141.29(+1.6%) 9443 1451 237 -------------------------------------------------------------- 9443 1451 238 Weston and Todd experimental data were normalized to the cal- 9443 1451 239 culated average capture cross section over the resonance at 9443 1451 240 0.264 eV (original EXFOR data multiplied by 0.914); in the 9443 1451 241 energy range from 0.5 eV to 3 eV the experimental data are not 9443 1451 242 accurate due to large corrections for the impurities. 9443 1451 243 9443 1451 244 9443 1451 245 Table 5 9443 1451 246 9443 1451 247 The fission cross section integral in the energy range from 9443 1451 248 3 eV to 300 eV. 9443 1451 249 9443 1451 250 ------------------------------------------------------------------9443 1451 251 Energy range Present work ENDF/B-VI Weston and Todd(8) 9443 1451 252 (eV) (b.eV) (b.eV) (b.eV) 9443 1451 253 ------------------------------------------------------------------9443 1451 254 3- 20 3038.63 3066.37(+0.9%) 3036.23(-0.1%) 9443 1451 255 20- 50 1683.69 1739.68(+3.3%) 1705.50(+1.3%) 9443 1451 256 50-100 1971.15 2030.10(+3.0%) 1931.50(-2.0%) 9443 1451 257 100-200 2554.85 2628.39(+2.9%) 2531.00(-0.9%) 9443 1451 258 200-300 2741.23 2820.75(+2.9%) 2747.00(+0.2%) 9443 1451 259 ------------------------------------------------------------------9443 1451 260 3-300 11989.55 12285.29(+2.5%) 11951.23(-0.3%) 9443 1451 261 ------------------------------------------------------------------9443 1451 262 Weston and Todd experimental data were normalized to Wagemans et 9443 1451 263 al.(1) in the energy range from 0.1 eV to 12 eV (original EXFOR 9443 1451 264 data multiplied by 0.952). 9443 1451 265 9443 1451 266 9443 1451 267 Table 6 9443 1451 268 9443 1451 269 The capture cross section integral in the energy range from 9443 1451 270 3 eV to 300 eV. 9443 1451 271 9443 1451 272 ------------------------------------------------------------------9443 1451 273 Energy range Present work ENDF/B-VI Weston and Todd(8) 9443 1451 274 (eV) (b.eV) (b.eV) (b.eV) 9443 1451 275 ------------------------------------------------------------------9443 1451 276 3- 20 1213.07 1138.52(-6.5%) 1192.90(-1.7%) 9443 1451 277 20- 50 330.34 307.48(-7.5%) 338.09(+2.3%) 9443 1451 278 50-100 605.40 585.88(-3.2%) 594.83(-1.8%) 9443 1451 279 100-200 609.83 581.77(-4.8%) 652.68(+7.0%) 9443 1451 280 200-300 684.97 661.12(-3.6%) 700.53(+2.3%) 9443 1451 281 ------------------------------------------------------------------9443 1451 282 3-300 3443.36 3274.77(-5.1%) 3479.04(+1.0%) 9443 1451 283 ------------------------------------------------------------------9443 1451 284 Weston and Todd experimental data normalized to the calculated 9443 1451 285 average capture cross section over the resonance at 0.265 eV 9443 1451 286 (original EXFOR data multiplied by 0.914). 9443 1451 287 9443 1451 288 ***************************************************************** 9443 1451 289 9443 1451 290 $$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$9443 1451 291 9443 1451 292 UNRESOLVED RESONANCE PARAMETERS START AT 300EV. 9443 1451 293 SAME AS VERSION V EXCEPT CAPTURE DOWN BY 4.8% AS 9443 1451 294 PER THE RECOMMENDATION OF H. DERRIEN AFTER THE STUDY9443 1451 295 OF THE WAGEMANS ET AL. DATA, REF 1. REVISION 1 HAD 9443 1451 296 CAPTURE DOWN BY 14% WHICH WAS DECIDED TO BE AN 9443 1451 297 OVERCORRECTION. FISSION IS UNCHANGED FROM VERSION 5 9443 1451 298 WHICH WAS BASED ON DATA OF SIMPSON, REF. 16, JAMES, 9443 1451 299 REF. 17, MIGNECO, REF. 10, BLONS, REF. 9, WESTON, 9443 1451 300 REF. 8, AND CARLSON, REF. 18. 9443 1451 301 MF=3 MT=1 TOTALS WERE REVISED FROM VERSION 5 TO REFLECT MORE 9443 1451 302 PHYSICAL SHAPE AS COMPARED TO PU239. 9443 1451 303 MF=3 MT=2 ADJUSTED TO BE CONSISTENT WITH TOTAL AND OTHER 9443 1451 304 PARTIAL CROSS SECTIONS. 9443 1451 305 MF=3 MT=18 ABOVE 40.2KEV SAME AS VERSION V AND BASED ON BEHRENS9443 1451 306 ,REF.15, KAPPELAR,REF.19, AND SZABO,REF.20, RATIOS 9443 1451 307 TO U235 WITH USE OF ENDF V EVALUATION OF U235. 9443 1451 308 MF=3 MT=102 RENORMALIZED DOWNWARD BY 4.8% FROM VERSION V. SEE 9443 1451 309 UNRESOLVED REGION ABOVE FOR EXPLAINATION. 9443 1451 310 MF=5 MT=16 REVISED BY R.J. HOWERTON FOR VERSION V. 9443 1451 311 MF=5 MT=17 REVISED BY R.J. HOWERTON FOR VERSION V. 9443 1451 312 MF=5 MT=18 FISSION NEUTRON ENERGY DISTRIBUTION GIVEN 9443 1451 313 AS SIMPLE FISSION SPECTRUM PLUS A 9443 1451 314 MAXWELLIAN (AWRE O-101/64) 9443 1451 315 MF=5 MT=91 REVISED BY R.J. HOWERTON FOR VERSION V. 9443 1451 316 MF=5,MT=455 DELAYED NEUTRON SECONDARY ENERGY DISTRIBUTION 9443 1451 317 SEE REF. 21. 9443 1451 318 MF=12 MT=18 USED DATA OF PEELE AND MAIENSCHEIN, REF 22, FOR 9443 1451 319 235-U THERMAL FISSION. 9443 1451 320 MF=12 MT=102 USED 238-U SPECTRUM ADJUSTED FOR MULTIPLICITY AND 9443 1451 321 ENERGY CONSERVATION. 9443 1451 322 MF=13 MT=3 CALCULATED BY R.J. HOWERTON 9443 1451 323 MF=15 MT=3 CALCULATED BY R.J. HOWERTON 9443 1451 324 MF=15 MT=18 CALCULATED BY R.J. HOWERTON. USED PEELE AND 9443 1451 325 MAIENSCHEIN DATA, REF 22, AND METHOD DESCRIBED 9443 1451 326 IN REF 23. 9443 1451 327 MF=15 MT=102 CALCULATED BY R.J. HOWERTON. 9443 1451 328 MF=33 MT=18,102 REPLACED BY L.WESTON DEC.1982 REF.24. 9443 1451 329 9443 1451 330 REFERENCES. 9443 1451 331 9443 1451 332 1. WAGEMANS,C. ET AL., Proc. Int. Conf. Nuc. Data for Sci. and 9443 1451 333 Tech., May 13-17, 1991, Julich, p. 35(1992). 9443 1451 334 2. DERRIEN,H. and de SAUSSURE,G.,Nuc.Sci.Eng.106,415(1990). 9443 1451 335 3. FREHAUT ET AL., CEA-R-4626, BRC(1974). 9443 1451 336 4. KAISER, R.E., CARPENTER, S.G.,(ANL-WEST) private comm.(1977).9443 1451 337 5. LARSON,N.M. and PEREY,F.G.,ORNL/TM-9719(1985). 9443 1451 338 6. WAGEMANS,C.,SCHILLEBEECKX,P.,DERUYTTER,A. and 9443 1451 339 BARTHELEMY,R.,Proc.Int.Conf.,PHYSOR 90,Marseille,France, 9443 1451 340 Vol.1,III-9(1990). 9443 1451 341 7. WAGEMANS,C. and DERUYTTER,A.,Nucl.Sci.Eng.60,44(1976). 9443 1451 342 8. WESTON,L.W. and TODD,J.H.,Nucl.Sci.Eng.65,454(1978). 9443 1451 343 9. BLONS,J.,Nucl.Sci.Eng.51,130(1973). 9443 1451 344 10. MIGNECO,E.,THEOBALD,J.P. and WARTENA,J.A.,Proc.Conf.Nuclear 9443 1451 345 Data for Reactors, Helsinki, Finland, June 15-19, 1970, 9443 1451 346 Vol.I,p.437,IAEA(1970). 9443 1451 347 11. WAGEMANS,C. and DERUYTTER,A.,Proc.Conf. on Nuclear Data for 9443 1451 348 Science and Technology,Antwerp,Belgium,69(1983). 9443 1451 349 12. HARVEY,J.A. and SIMPSON,O.D.,Oak-Ridge National 9443 1451 350 Laboratory(1973), unpublished. 9443 1451 351 13. YOUNG,T.B. and SMITH,J.R.,WASH-1093,p.60(1968). 9443 1451 352 14. CARLSON,A. et al.,ENDF/B-VI standard evaluation,private 9443 1451 353 communication from PEELLE,R.W.(1987). 9443 1451 354 15. J.W.BEHRENS AND G.W.CARLSON,UCRL-51925(1975). 9443 1451 355 16. SIMPSON, O.D., ET AL., Proc. Cross Sections and Tech. Conf., 9443 1451 356 Washington, II,910(1966). 9443 1451 357 17. JAMES, G.D., Helsinki Conf., Vol. 1, 267 (1970). 9443 1451 358 18. CARLSON, G.W., BEHRENS, J.W., and CZIRR, J.B., Nucl. Sci. 9443 1451 359 Eng. 63, 149(1977). 9443 1451 360 19. F.KAPPELAR AND E.PFLETSCHINGER, NUCL.SCI.ENG.,51,124(1973). 9443 1451 361 20. I.SZABO ET AL.,SYMP. NEUTRON STANDARDS,ARGONNE,257(1970). 9443 1451 362 21. T.R.ENGLAND ET AL,LA-11151-MS(1988),LA-11534-T(1989) 9443 1451 363 LAURA-88-4118, TO BE PUBLISHED IN NSE(1989) 9443 1451 364 22. R.W. PEELE AND F.C. MAIENSCHEIN, NUCL.SCI. ENG.40,485 (1970).9443 1451 365 23. S.T. PERKINS,R.C. HAIGHT,AND R.J. HOWERTON, NUCL. SCI. ENG. 9443 1451 366 57,1 (1975). 9443 1451 367 24. L.W.WESTON P.C. TO B.A.MAGURNO NOV.12,1982 9443 1451 368 * * * * * *9443 1451 369 1 451 436 39443 1451 370 1 452 5 09443 1451 371 1 455 7 09443 1451 372 1 456 5 09443 1451 373 1 458 5 09443 1451 374 2 151 408 39443 1451 375 3 1 39 19443 1451 376 3 2 39 29443 1451 377 3 4 37 09443 1451 378 3 16 17 09443 1451 379 3 17 8 09443 1451 380 3 18 39 19443 1451 381 3 51 21 09443 1451 382 3 52 18 09443 1451 383 3 53 17 09443 1451 384 3 54 16 09443 1451 385 3 55 16 09443 1451 386 3 56 15 09443 1451 387 3 57 15 09443 1451 388 3 58 14 09443 1451 389 3 59 14 09443 1451 390 3 60 13 09443 1451 391 3 61 12 09443 1451 392 3 62 11 09443 1451 393 3 63 11 09443 1451 394 3 64 10 09443 1451 395 3 65 10 09443 1451 396 3 91 26 09443 1451 397 3 102 39 39443 1451 398 4 2 133 09443 1451 399 4 16 10 09443 1451 400 4 17 10 09443 1451 401 4 18 10 09443 1451 402 4 51 10 09443 1451 403 4 52 10 09443 1451 404 4 53 10 09443 1451 405 4 54 10 09443 1451 406 4 55 10 09443 1451 407 4 56 10 09443 1451 408 4 57 10 09443 1451 409 4 58 10 09443 1451 410 4 59 10 09443 1451 411 4 60 10 09443 1451 412 4 61 10 09443 1451 413 4 62 10 09443 1451 414 4 63 10 09443 1451 415 4 64 10 09443 1451 416 4 65 10 09443 1451 417 4 91 10 09443 1451 418 5 16 217 09443 1451 419 5 17 111 09443 1451 420 5 18 8 09443 1451 421 5 91 193 09443 1451 422 5 455 579 09443 1451 423 8 16 2 09443 1451 424 8 17 2 09443 1451 425 8 102 2 09443 1451 426 12 18 5 09443 1451 427 12 102 5 09443 1451 428 13 3 9 09443 1451 429 14 3 1 09443 1451 430 14 18 1 09443 1451 431 14 102 1 09443 1451 432 15 3 413 09443 1451 433 15 18 45 09443 1451 434 15 102 48 09443 1451 435 31 452 50 09443 1451 436 0.000000+0 0.000000+0 0 0 0 09443 1 0 437 9.424101+4 2.389780+2 0 2 0 09443 1452 438 0.000000+0 0.000000+0 0 0 1 59443 1452 439 5 2 9443 1452 440 1.000000-5 2.945300+0 4.721001+5 2.945300+0 4.000001+6 3.506500+09443 1452 441 7.000002+6 3.962200+0 2.000000+7 5.971200+0 9443 1452 442 0.000000+0 0.000000+0 0 0 0 09443 1 0 443 9.424101+4 2.389780+2 0 2 0 09443 1455 444 0.000000+0 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1.021000+7 2.66580-10 1.042000+7 2.18610-10 1.053000+7 1.97000-109443 5 16 1905 1.065000+7 1.75830-10 1.077000+7 1.56920-10 1.090000+7 1.38700-109443 5 16 1906 1.103000+7 1.22580-10 1.117000+7 1.07290-10 1.131000+7 9.38950-119443 5 16 1907 1.145000+7 8.21600-11 1.160000+7 7.11950-11 1.175000+7 6.16850-119443 5 16 1908 1.192000+7 5.24200-11 1.209000+7 4.45390-11 1.227000+7 3.74740-119443 5 16 1909 1.246000+7 3.12210-11 1.264000+7 2.62570-11 1.284000+7 2.16560-119443 5 16 1910 1.294000+7 1.96660-11 1.305000+7 1.76860-11 1.316000+7 1.59040-119443 5 16 1911 1.328000+7 1.41630-11 1.343000+7 1.22510-11 1.358000+7 1.05960-119443 5 16 1912 1.375000+7 8.98750-12 1.392000+7 7.62200-12 1.410000+7 6.40050-129443 5 16 1913 1.429000+7 5.32200-12 1.439000+7 4.82920-12 1.450000+7 4.33930-129443 5 16 1914 1.461000+7 3.89880-12 1.472000+7 3.50290-12 1.473000+7 1.71770-129443 5 16 1915 1.474000+7 0.000000+0 9443 5 16 1916 0.000000+0 0.000000+0 0 0 0 09443 5 0 1917 9.424101+4 2.389780+2 0 0 1 09443 5 17 1918 0.000000+0 0.000000+0 0 1 1 29443 5 17 1919 2 2 9443 5 17 1920 1.175000+7 1.000000+0 2.000000+7 1.000000+0 9443 5 17 1921 0.000000+0 0.000000+0 0 0 1 69443 5 17 1922 6 2 9443 5 17 1923 0.000000+0 1.175000+7 0 0 1 39443 5 17 1924 3 2 9443 5 17 1925 1.000000+2 0.000000+0 2.000000+2 1.000000-2 3.000000+2 0.000000+09443 5 17 1926 0.000000+0 1.200000+7 0 0 1 239443 5 17 1927 23 2 9443 5 17 1928 1.000000+4 0.000000+0 2.000000+4 5.811700-6 3.000000+4 7.137000-69443 5 17 1929 4.000000+4 7.791300-6 5.000001+4 7.973700-6 6.000001+4 7.834000-69443 5 17 1930 7.000001+4 7.483000-6 8.000001+4 7.001700-6 1.200000+5 4.719000-69443 5 17 1931 1.300000+5 4.185700-6 1.400000+5 3.690300-6 1.500000+5 3.237400-69443 5 17 1932 1.600000+5 2.827200-6 1.700000+5 2.459400-6 1.800000+5 2.132000-69443 5 17 1933 1.900000+5 1.842500-6 2.000000+5 1.588000-6 2.100000+5 1.365100-69443 5 17 1934 2.200000+5 1.170800-6 2.300000+5 1.002200-6 2.400000+5 8.562000-79443 5 17 1935 2.500000+5 3.108800-7 2.600000+5 0.000000+0 9443 5 17 1936 0.000000+0 1.400000+7 0 0 1 639443 5 17 1937 63 2 9443 5 17 1938 1.000000+4 0.000000+0 2.000000+4 3.784300-7 3.000000+4 5.424000-79443 5 17 1939 4.000000+4 6.910600-7 5.000001+4 8.254600-7 6.000001+4 9.465300-79443 5 17 1940 7.000001+4 1.055300-6 9.000001+4 1.238800-6 1.000000+5 1.315300-69443 5 17 1941 1.200000+5 1.441200-6 1.500000+5 1.571900-6 1.800000+5 1.645700-69443 5 17 1942 2.200000+5 1.677100-6 2.400000+5 1.670600-6 2.700000+5 1.639800-69443 5 17 1943 3.200001+5 1.548400-6 3.700001+5 1.426300-6 5.000001+5 1.067500-69443 5 17 1944 5.700001+5 8.853000-7 6.400001+5 7.231000-7 7.000001+5 6.021300-79443 5 17 1945 7.600001+5 4.977000-7 7.900001+5 4.513700-7 8.300001+5 3.954000-79443 5 17 1946 8.600001+5 3.574700-7 9.000001+5 3.119000-7 9.400001+5 2.716000-79443 5 17 1947 9.800002+5 2.360800-7 1.020000+6 2.048700-7 1.070000+6 1.712200-79443 5 17 1948 1.120000+6 1.427900-7 1.170000+6 1.188400-7 1.220000+6 9.872300-89443 5 17 1949 1.250000+6 8.826000-8 1.280000+6 7.885600-8 1.310000+6 7.041600-89443 5 17 1950 1.340000+6 6.284700-8 1.370000+6 5.606300-8 1.410000+6 4.810700-89443 5 17 1951 1.440000+6 4.286700-8 1.480000+6 3.673300-8 1.510000+6 3.270100-89443 5 17 1952 1.550000+6 2.798700-8 1.590000+6 2.393600-8 1.630000+6 2.046000-89443 5 17 1953 1.670000+6 1.747600-8 1.720000+6 1.434000-8 1.760000+6 1.223500-89443 5 17 1954 1.810000+6 1.002400-8 1.860000+6 8.207000-9 1.910000+6 6.714300-99443 5 17 1955 1.940000+6 5.950300-9 1.980000+6 5.063300-9 2.020000+6 4.307000-99443 5 17 1956 2.060000+6 3.662000-9 2.100000+6 3.112400-9 2.140000+6 2.644500-99443 5 17 1957 2.170000+6 2.339700-9 2.190000+6 2.156100-9 2.220000+6 1.907000-99443 5 17 1958 2.240001+6 1.757000-9 2.250001+6 8.09300-10 2.260001+6 0.000000+09443 5 17 1959 0.000000+0 1.500000+7 0 0 1 489443 5 17 1960 48 2 9443 5 17 1961 1.000000+4 0.000000+0 2.000000+4 9.514400-8 3.000000+4 1.395800-79443 5 17 1962 4.000000+4 1.820100-7 5.000001+4 2.225200-7 6.000001+4 2.611600-79443 5 17 1963 8.000001+4 3.330700-7 1.000000+5 3.982400-7 1.300000+5 4.843400-79443 5 17 1964 1.600000+5 5.576400-7 1.900000+5 6.195000-7 2.200000+5 6.710400-79443 5 17 1965 2.500000+5 7.133700-7 3.100000+5 7.741700-7 3.800001+5 8.122700-79443 5 17 1966 4.500001+5 8.233400-7 5.500001+5 8.057700-7 6.700001+5 7.518400-79443 5 17 1967 7.800001+5 6.854400-7 1.120000+6 4.623400-7 1.240000+6 3.920700-79443 5 17 1968 1.350000+6 3.342700-7 1.450000+6 2.875000-7 1.550000+6 2.460800-79443 5 17 1969 1.650000+6 2.097600-7 1.750000+6 1.781400-7 1.810000+6 1.612500-79443 5 17 1970 1.880000+6 1.433600-7 1.950000+6 1.272800-7 2.020000+6 1.128500-79443 5 17 1971 2.090000+6 9.994100-8 2.160000+6 8.841000-8 2.240001+6 7.675000-89443 5 17 1972 2.320001+6 6.654700-8 2.410001+6 5.659700-8 2.510001+6 4.720000-89443 5 17 1973 2.610001+6 3.930000-8 2.720001+6 3.207500-8 2.780001+6 2.869000-89443 5 17 1974 2.840001+6 2.565000-8 2.900001+6 2.292300-8 2.960001+6 2.047700-89443 5 17 1975 3.020001+6 1.828400-8 3.090001+6 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