JENDL-3 FISSION PRODUCT NUCLIDE DATA (1990-11) 311 0 0 0 6.11490+ 4 1.47639+ 2 1 0 0 16104 1451 1 0.0 + 0 0.0 + 0 0 0 0 06104 1451 2 0.0 + 0 0.0 + 0 0 0 200 616104 1451 3 61-PM-149 JNDC EVAL-MAR90 JNDC FP NUCLEAR DATA W.G. 6104 1451 4 DIST-NOV90 6104 1451 5 HISTORY 6104 1451 6 90-03 NEW EVALUATION FOR JENDL-3 WAS COMPLETED BY JNDC FPND 6104 1451 7 W.G./1/ 6104 1451 8 6104 1451 9 MF = 1 GENERAL INFORMATION 6104 1451 10 MT=451 COMMENTS AND DICTIONARY 6104 1451 11 6104 1451 12 MF = 2 RESONANCE PARAMETERS 6104 1451 13 MT=151 RESOLVED AND UNRESOLVED RESONANCE PARAMETERS 6104 1451 14 NO RESOLVED RESONANCE PARAMETERS 6104 1451 15 6104 1451 16 UNRESOLVED RESONANCE REGION : 2.6 EV - 100 KEV 6104 1451 17 THE NEUTRON STRENGTH FUNCTIONS, S0, S1 AND S2 WERE CALCULATED 6104 1451 18 WITH OPTICAL MODEL CODE CASTHY/2/. THE OBSERVED LEVEL SPACING6104 1451 19 WAS DETERMINED TO REPRODUCE THE CAPTURE CROSS SECTION 6104 1451 20 CALCULATED WITH CASTHY. THE EFFECTIVE SCATTERING RADIUS WAS 6104 1451 21 OBTAINED FROM FITTING TO THE CALCULATED TOTAL CROSS SECTION AT6104 1451 22 100 KEV. THE RADIATION WIDTH GG WAS BASED ON THE SYSTEMATICS 6104 1451 23 OF MEASURED VALUES FOR NEIGHBORING NUCLIDES. 6104 1451 24 6104 1451 25 TYPICAL VALUES OF THE PARAMETERS AT 70 KEV: 6104 1451 26 S0 = 3.400E-4, S1 = 0.930E-4, S2 = 2.300E-4, SG = 137.E-4, 6104 1451 27 GG = 0.068 EV, R = 3.970 FM. 6104 1451 28 6104 1451 29 CALCULATED 2200-M/S CROSS SECTIONS AND RES. INTEGRALS (BARNS) 6104 1451 30 2200 M/S RES. INTEG. 6104 1451 31 TOTAL 1403 - 6104 1451 32 ELASTIC 3.200 - 6104 1451 33 CAPTURE 1400 1570 6104 1451 34 6104 1451 35 MF = 3 NEUTRON CROSS SECTIONS 6104 1451 36 BELOW 2.6 EV, THE CAPTURE AND ELASTIC SCATTERING CROSS SECTIONS 6104 1451 37 WERE ASSUMED TO BE IN 1/V FORM AND CONSTANT, RESPECTIVELY. THE 6104 1451 38 CAPTURE CROSS SECTION AT 0.0253 EV WAS TAKEN FROM REF./3/, AND 6104 1451 39 THE ELASTIC SCATTERING CROSS SECTION WAS ESTIMATED BY ASSUMING 6104 1451 40 R = 5.0 FM. UNRESOLVED RESONANCE PARAMETERS WERE GIVEN IN THE 6104 1451 41 ENERGY RANGE FROM 2.6 EV TO 100 KEV. 6104 1451 42 6104 1451 43 ABOVE 100 KEV, THE SPHERICAL OPTICAL AND STATISTICAL MODEL 6104 1451 44 CALCULATION WAS PERFORMED WITH CASTHY, BY TAKING ACCOUNT OF 6104 1451 45 COMPETING REACTIONS, OF WHICH CROSS SECTIONS WERE CALCULATED 6104 1451 46 WITH PEGASUS/4/ STANDING ON A PREEQUILIBRIUM AND MULTI-STEP 6104 1451 47 EVAPORATION MODEL. THE OMP'S FOR NEUTRON GIVEN IN TABLE 1 WERE 6104 1451 48 ADOPTED FROM MOLDAUER/5/, WHICH REPRODUCED WELL THE PM-147 TOTAL6104 1451 49 CROSS SECTION MEASURED BY FOSTER AND GLASGOW/6/. THE OMP'S FOR 6104 1451 50 CHARGED PARTICLES ARE AS FOLLOWS: 6104 1451 51 PROTON = PEREY/7/ 6104 1451 52 ALPHA = HUIZENGA AND IGO/8/ 6104 1451 53 DEUTERON = LOHR AND HAEBERLI/9/ 6104 1451 54 HELIUM-3 AND TRITON = BECCHETTI AND GREENLEES/10/ 6104 1451 55 PARAMETERS FOR THE COMPOSITE LEVEL DENSITY FORMULA OF GILBERT 6104 1451 56 AND CAMERON/11/ WERE EVALUATED BY IIJIMA ET AL./12/ MORE 6104 1451 57 EXTENSIVE DETERMINATION AND MODIFICATION WERE MADE IN THE 6104 1451 58 PRESENT WORK. TABLE 2 SHOWS THE LEVEL DENSITY PARAMETERS USED 6104 1451 59 IN THE PRESENT CALCULATION. ENERGY DEPENDENCE OF SPIN CUT-OFF 6104 1451 60 PARAMETER IN THE ENERGY RANGE BELOW E-JOINT IS DUE TO GRUPPELAAR6104 1451 61 /13/. 6104 1451 62 6104 1451 63 MT = 1 TOTAL 6104 1451 64 SPHERICAL OPTICAL MODEL CALCULATION WAS ADOPTED. 6104 1451 65 6104 1451 66 MT = 2 ELASTIC SCATTERING 6104 1451 67 CALCULATED AS (TOTAL - SUM OF PARTIAL CROSS SECTIONS). 6104 1451 68 6104 1451 69 MT = 4, 51 - 91 INELASTIC SCATTERING 6104 1451 70 SPHERICAL OPTICAL AND STATISTICAL MODEL CALCULATION WAS 6104 1451 71 ADOPTED. THE LEVEL SCHEME WAS BASED ON EVALUATED NUCLEAR 6104 1451 72 STRUCTURE DATA FILE (1987 VERSION)/14/ AND NUCLEAR DATA 6104 1451 73 SHEETS/15/. 6104 1451 74 6104 1451 75 NO. ENERGY(MEV) SPIN-PARITY 6104 1451 76 GR. 0.0 7/2 + 6104 1451 77 1 0.1143 5/2 + 6104 1451 78 2 0.1886 5/2 + 6104 1451 79 3 0.2113 5/2 + 6104 1451 80 4 0.2402 11/2 - 6104 1451 81 5 0.2702 7/2 - 6104 1451 82 6 0.2882 5/2 + 6104 1451 83 7 0.3600 5/2 + 6104 1451 84 8 0.3876 1/2 + 6104 1451 85 9 0.3968 5/2 + 6104 1451 86 10 0.4253 5/2 + 6104 1451 87 11 0.4622 3/2 - 6104 1451 88 12 0.5156 9/2 + 6104 1451 89 13 0.5379 5/2 - 6104 1451 90 14 0.6548 7/2 - 6104 1451 91 LEVELS ABOVE 0.7 MEV WERE ASSUMED TO BE OVERLAPPING. 6104 1451 92 6104 1451 93 MT = 102 CAPTURE 6104 1451 94 SPHERICAL OPTICAL AND STATISTICAL MODEL CALCULATION WITH 6104 1451 95 CASTHY WAS ADOPTED. DIRECT AND SEMI-DIRECT CAPTURE CROSS 6104 1451 96 SECTIONS WERE ESTIMATED ACCORDING TO THE PROCEDURE OF BENZI 6104 1451 97 AND REFFO/16/ AND NORMALIZED TO 1 MILLI-BARN AT 14 MEV. 6104 1451 98 6104 1451 99 THE GAMMA-RAY STRENGTH FUNCTION (1.30E-02) WAS DETERMINED FROM6104 1451 100 THE SYSTEMATICS OF RADIATION WIDTH (0.068 EV) AND THE AVERAGE 6104 1451 101 S-WAVE RESONANCE LEVEL SPACING (5.22 EV) CALCULATED FROM THE 6104 1451 102 LEVEL DENSITY PARAMETERS. 6104 1451 103 6104 1451 104 MT = 16 (N,2N) CROSS SECTION 6104 1451 105 MT = 17 (N,3N) CROSS SECTION 6104 1451 106 MT = 22 (N,N'A) CROSS SECTION 6104 1451 107 MT = 28 (N,N'P) CROSS SECTION 6104 1451 108 MT = 32 (N,N'D) CROSS SECTION 6104 1451 109 MT = 33 (N,N'T) CROSS SECTION 6104 1451 110 MT =103 (N,P) CROSS SECTION 6104 1451 111 MT =104 (N,D) CROSS SECTION 6104 1451 112 MT =105 (N,T) CROSS SECTION 6104 1451 113 MT =107 (N,ALPHA) CROSS SECTION 6104 1451 114 THESE REACTION CROSS SECTIONS WERE CALCULATED WITH THE 6104 1451 115 PREEQUILIBRIUM AND MULTI-STEP EVAPORATION MODEL CODE PEGASUS. 6104 1451 116 6104 1451 117 THE KALBACH'S CONSTANT K (= 128.4) WAS ESTIMATED BY THE 6104 1451 118 FORMULA DERIVED FROM KIKUCHI-KAWAI'S FORMALISM/17/ AND LEVEL 6104 1451 119 DENSITY PARAMETERS. 6104 1451 120 6104 1451 121 FINALLY, THE (N,P) AND (N,ALPHA) CROSS SECTIONS WERE 6104 1451 122 NORMALIZED TO THE FOLLOWING VALUES AT 14.5 MEV: 6104 1451 123 (N,P) 4.17 MB (SYSTEMATICS OF FORREST/18/) 6104 1451 124 (N,ALPHA) 1.71 MB (SYSTEMATICS OF FORREST) 6104 1451 125 6104 1451 126 MT = 251 MU-BAR 6104 1451 127 CALCULATED WITH CASTHY. 6104 1451 128 6104 1451 129 MF = 4 ANGULAR DISTRIBUTIONS OF SECONDARY NEUTRONS 6104 1451 130 LEGENDRE POLYNOMIAL COEFFICIENTS FOR ANGULAR DISTRIBUTIONS ARE 6104 1451 131 GIVEN IN THE CENTER-OF-MASS SYSTEM FOR MT=2 AND DISCRETE INELAS-6104 1451 132 TIC LEVELS, AND IN THE LABORATORY SYSTEM FOR MT=91. THEY WERE 6104 1451 133 CALCULATED WITH CASTHY. FOR OTHER REACTIONS, ISOTROPIC DISTRI- 6104 1451 134 BUTIONS IN THE LABORATORY SYSTEM WERE ASSUMED. 6104 1451 135 6104 1451 136 MF = 5 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS 6104 1451 137 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS WERE CALCULATED WITH 6104 1451 138 PEGASUS FOR INELASTIC SCATTERING TO OVERLAPPING LEVELS AND FOR 6104 1451 139 OTHER NEUTRON EMITTING REACTIONS. 6104 1451 140 6104 1451 141 TABLE 1 NEUTRON OPTICAL POTENTIAL PARAMETERS 6104 1451 142 6104 1451 143 DEPTH (MEV) RADIUS(FM) DIFFUSENESS(FM) 6104 1451 144 ---------------------- ------------ --------------- 6104 1451 145 V = 46.0 R0 = 6.75 A0 = 0.62 6104 1451 146 WS = 7.0 RS = 6.75 AS = 1.0 6104 1451 147 VSO= 7.0 RSO= 6.75 ASO= 0.62 6104 1451 148 THE FORM OF SURFACE ABSORPTION PART IS GAUSSIAN TYPE. 6104 1451 149 6104 1451 150 TABLE 2 LEVEL DENSITY PARAMETERS 6104 1451 151 6104 1451 152 NUCLIDE SYST A(1/MEV) T(MEV) C(1/MEV) EX(MEV) PAIRING 6104 1451 153 --------------------------------------------------------------- 6104 1451 154 59-PR-145 * 2.088E+01 5.411E-01 7.911E+00 5.258E+00 9.200E-01 6104 1451 155 59-PR-146 * 2.263E+01 5.387E-01 8.918E+01 4.815E+00 0.0 6104 1451 156 59-PR-147 2.440E+01 4.420E-01 3.742E+00 4.298E+00 9.900E-01 6104 1451 157 59-PR-148 1.996E+01 4.690E-01 1.108E+01 2.807E+00 0.0 6104 1451 158 6104 1451 159 60-ND-146 2.019E+01 5.660E-01 1.121E+00 6.714E+00 2.100E+00 6104 1451 160 60-ND-147 2.398E+01 4.850E-01 5.510E+00 5.235E+00 1.180E+00 6104 1451 161 60-ND-148 2.359E+01 5.150E-01 1.328E+00 6.751E+00 2.170E+00 6104 1451 162 60-ND-149 2.657E+01 4.750E-01 1.192E+01 5.636E+00 1.180E+00 6104 1451 163 6104 1451 164 61-PM-147 2.192E+01 4.913E-01 4.801E+00 4.589E+00 9.200E-01 6104 1451 165 61-PM-148 2.227E+01 4.300E-01 1.420E+01 2.672E+00 0.0 6104 1451 166 61-PM-149 2.377E+01 4.890E-01 8.141E+00 5.075E+00 9.900E-01 6104 1451 167 61-PM-150 2.270E+01 3.800E-01 7.943E+00 1.973E+00 0.0 6104 1451 168 --------------------------------------------------------------- 6104 1451 169 SYST: * = LDP'S WERE DETERMINED FROM SYSTEMATICS. 6104 1451 170 6104 1451 171 SPIN CUTOFF PARAMETERS WERE CALCULATED AS 0.146*SQRT(A)*A**(2/3).6104 1451 172 IN THE CASTHY CALCULATION, SPIN CUTOFF FACTORS AT 0 MEV WERE 6104 1451 173 ASSUMED TO BE 6.071 FOR PM-149 AND 5.0 FOR PM-150. 6104 1451 174 6104 1451 175 REFERENCES 6104 1451 176 1) KAWAI, M. ET AL.: PROC. INT. CONF. ON NUCLEAR DATA FOR SCIENCE6104 1451 177 AND TECHNOLOGY, MITO, P. 569 (1988). 6104 1451 178 2) IGARASI, S.: J. NUCL. SCI. TECHNOL., 12, 67 (1975). 6104 1451 179 3) MUGHABGHAB, S.F.: "NEUTRON CROSS SECTIONS, VOL. I, PART B", 6104 1451 180 ACADEMIC PRESS (1984). 6104 1451 181 4) IIJIMA, S. ET AL.: JAERI-M 87-025, P. 337 (1987). 6104 1451 182 5) MOLDAUER, P. A.: NUCL. PHYS., 47, 65 (1963). 6104 1451 183 6) FOSTER, D.G. JR. AND GLASGOW, D.W.: PHYS. REV., C3, 576 6104 1451 184 (1971). 6104 1451 185 7) PEREY, F.G: PHYS. REV. 131, 745 (1963). 6104 1451 186 8) HUIZENGA, J.R. AND IGO, G.: NUCL. PHYS. 29, 462 (1962). 6104 1451 187 9) LOHR, J.M. AND HAEBERLI, W.: NUCL. PHYS. A232, 381 (1974). 6104 1451 188 10) BECCHETTI, F.D., JR. AND GREENLEES, G.W.: POLARIZATION 6104 1451 189 PHENOMENA IN NUCLEAR REACTIONS ((EDS) H.H. BARSHALL AND 6104 1451 190 W. HAEBERLI), P. 682, THE UNIVERSITY OF WISCONSIN PRESS. 6104 1451 191 (1971). 6104 1451 192 11) GILBERT, A. AND CAMERON, A.G.W.: CAN. J. PHYS., 43, 1446 6104 1451 193 (1965). 6104 1451 194 12) IIJIMA, S., ET AL.: J. NUCL. SCI. TECHNOL. 21, 10 (1984). 6104 1451 195 13) GRUPPELAAR, H.: ECN-13 (1977). 6104 1451 196 14) ENSDF: EVALUATED NUCLEAR STRUCTURE DATA FILE (JUNE 1987). 6104 1451 197 15) NUCLEAR DATA SHEETS, 46, 1 (1985). 6104 1451 198 16) BENZI, V. AND REFFO, G.: CCDN-NW/10 (1969). 6104 1451 199 17) KIKUCHI, K. AND KAWAI, M.: "NUCLEAR MATTER AND NUCLEAR 6104 1451 200 REACTIONS", NORTH HOLLAND (1968). 6104 1451 201 18) FORREST, R.A.: AERE-R 12419 (1986). 6104 1451 202 6104 1451 203 1 451 264 16104 1451 204 2 151 367 16104 1451 205 3 1 45 16104 1451 206 3 2 45 16104 1451 207 3 4 17 16104 1451 208 3 16 10 16104 1451 209 3 17 6 16104 1451 210 3 22 13 16104 1451 211 3 28 11 16104 1451 212 3 32 7 16104 1451 213 3 33 8 16104 1451 214 3 51 17 16104 1451 215 3 52 17 16104 1451 216 3 53 16 16104 1451 217 3 54 16 16104 1451 218 3 55 15 16104 1451 219 3 56 15 16104 1451 220 3 57 14 16104 1451 221 3 58 14 16104 1451 222 3 59 13 16104 1451 223 3 60 13 16104 1451 224 3 61 13 16104 1451 225 3 62 12 16104 1451 226 3 63 12 16104 1451 227 3 64 11 16104 1451 228 3 91 11 16104 1451 229 3 102 23 16104 1451 230 3 103 14 16104 1451 231 3 104 12 16104 1451 232 3 105 12 16104 1451 233 3 107 15 16104 1451 234 3 251 24 16104 1451 235 4 2 259 16104 1451 236 4 16 10 16104 1451 237 4 17 10 16104 1451 238 4 22 10 16104 1451 239 4 28 10 16104 1451 240 4 32 10 16104 1451 241 4 33 10 16104 1451 242 4 51 27 16104 1451 243 4 52 27 16104 1451 244 4 53 27 16104 1451 245 4 54 24 16104 1451 246 4 55 24 16104 1451 247 4 56 27 16104 1451 248 4 57 27 16104 1451 249 4 58 27 16104 1451 250 4 59 27 16104 1451 251 4 60 27 16104 1451 252 4 61 24 16104 1451 253 4 62 27 16104 1451 254 4 63 24 16104 1451 255 4 64 24 16104 1451 256 4 91 27 16104 1451 257 5 16 83 16104 1451 258 5 17 42 16104 1451 259 5 22 226 16104 1451 260 5 28 144 16104 1451 261 5 32 61 16104 1451 262 5 33 70 16104 1451 263 5 91 152 16104 1451 264 6104 1 0 265 6104 0 0 266 6.11490+ 4 1.47639+ 2 0 0 1 06104 2151 267 6.11490+ 4 1.00000+ 0 0 1 1 06104 2151 268 2.60000+ 0 1.00000+ 5 2 2 0 06104 2151 269 3.50000+ 0 3.96970- 1 0 0 3 06104 2151 270 1.47639+ 2 0.0 + 0 0 0 2 06104 2151 271 3.00000+ 0 0.0 + 0 5 0 174 286104 2151 272 0.0 + 0 0.0 + 0 0.0 + 0 1.00000+ 0 0.0 + 0 0.0 + 06104 2151 273 2.60000+ 0 6.68610+ 0 0.0 + 0 2.27330- 3 6.80000- 2 0.0 + 06104 2151 274 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