5.91430+ 4 1.41683+ 2 1 0 0 15931 1451 1 0.0 + 0 0.0 + 0 0 0 0 05931 1451 2 0.0 + 0 0.0 + 0 0 0 199 545931 1451 3 59-PR-143 JNDC EVAL-MAR90 JNDC FP NUCLEAR DATA W.G. 5931 1451 4 DIST-NOV90 5931 1451 5 HISTORY 5931 1451 6 90-03 NEW EVALUATION FOR JENDL-3 WAS COMPLETED BY JNDC FPND 5931 1451 7 W.G./1/ 5931 1451 8 5931 1451 9 MF = 1 GENERAL INFORMATION 5931 1451 10 MT=451 COMMENTS AND DICTIONARY 5931 1451 11 5931 1451 12 MF = 2 RESONANCE PARAMETERS 5931 1451 13 MT=151 RESOLVED AND UNRESOLVED RESONANCE PARAMETERS 5931 1451 14 NO RESOLVED RESONANCE PARAMETERS BECAUSE NO EXPERIMENTAL DATA 5931 1451 15 WERE AVAILABLE. 5931 1451 16 5931 1451 17 UNRESOLVED RESONANCE REGION : 4 EV - 100 KEV 5931 1451 18 THE LOWER BOUNDARY OF 4 EV WAS DETERMINED SO AS TO REPRODUCE 5931 1451 19 WELL THE CAPTURE RESONANCE INTEGRAL OF 190+-25 BARNS/2/. THE5931 1451 20 NEUTRON STRENGTH FUNCTIONS, S0, S1 AND S2 WERE CALCULATED WITH5931 1451 21 OPTICAL MODEL CODE CASTHY/3/. THE OBSERVED LEVEL SPACING WAS 5931 1451 22 DETERMINED TO REPRODUCE THE CAPTURE CROSS SECTION CALCULATED 5931 1451 23 WITH CASTHY. THE EFFECTIVE SCATTERING RADIUS WAS OBTAINED 5931 1451 24 FROM FITTING TO THE CALCULATED TOTAL CROSS SECTION AT 100 KEV.5931 1451 25 THE RADIATION WIDTH GG WAS BASED ON THE SYSTEMATICS OF 5931 1451 26 MEASURED VALUES FOR NEIGHBORING NUCLIDES. 5931 1451 27 5931 1451 28 TYPICAL VALUES OF THE PARAMETERS AT 70 KEV: 5931 1451 29 S0 = 2.300E-4, S1 = 1.100E-4, S2 = 1.700E-4, SG = 5.98E-4, 5931 1451 30 GG = 0.065 EV, R = 4.479 FM. 5931 1451 31 5931 1451 32 CALCULATED 2200-M/S CROSS SECTIONS AND RES. INTEGRALS (BARNS) 5931 1451 33 2200 M/S RES. INTEG. 5931 1451 34 TOTAL 92.90 - 5931 1451 35 ELASTIC 2.900 - 5931 1451 36 CAPTURE 90.00 185 5931 1451 37 5931 1451 38 MF = 3 NEUTRON CROSS SECTIONS 5931 1451 39 BELOW 4 EV, THE CAPTURE AND ELASTIC SCATTERING CROSS SECTIONS 5931 1451 40 WERE ASSUMED TO BE IN 1/V FORM AND CONSTANT, RESPECTIVELY. THE 5931 1451 41 CAPTURE CROSS SECTION AT 0.0253 EV WAS TAKEN FROM REF./2/, AND 5931 1451 42 THE ELASTIC SCATTERING CROSS SECTION WAS ESTIMATED BY ASSUMING 5931 1451 43 R = 4.8 FM. UNRESOLVED RESONANCE PARAMETERS WERE GIVEN IN THE 5931 1451 44 ENERGY RANGE FROM 4 EV TO 100 KEV. 5931 1451 45 5931 1451 46 ABOVE 100 KEV, THE SPHERICAL OPTICAL AND STATISTICAL MODEL 5931 1451 47 CALCULATION WAS PERFORMED WITH CASTHY, BY TAKING ACCOUNT OF 5931 1451 48 COMPETING REACTIONS, OF WHICH CROSS SECTIONS WERE CALCULATED 5931 1451 49 WITH PEGASUS/4/ STANDING ON A PREEQUILIBRIUM AND MULTI-STEP 5931 1451 50 EVAPORATION MODEL. THE OMP'S FOR NEUTRON GIVEN IN TABLE 1 WERE 5931 1451 51 ADOPTED FROM MOLDAUER/5/ SINCE THE PARAMETERS REPRODUCED WELL 5931 1451 52 THE TOTAL CROSS SECTION MEASURED BY FOSTER AND GLASGOW/6/. THE 5931 1451 53 OMP'S FOR CHARGED PARTICLES ARE AS FOLLOWS: 5931 1451 54 PROTON = PEREY/7/ 5931 1451 55 ALPHA = HUIZENGA AND IGO/8/ 5931 1451 56 DEUTERON = LOHR AND HAEBERLI/9/ 5931 1451 57 HELIUM-3 AND TRITON = BECCHETTI AND GREENLEES/10/ 5931 1451 58 PARAMETERS FOR THE COMPOSITE LEVEL DENSITY FORMULA OF GILBERT 5931 1451 59 AND CAMERON/11/ WERE EVALUATED BY IIJIMA ET AL./12/ MORE 5931 1451 60 EXTENSIVE DETERMINATION AND MODIFICATION WERE MADE IN THE 5931 1451 61 PRESENT WORK. TABLE 2 SHOWS THE LEVEL DENSITY PARAMETERS USED 5931 1451 62 IN THE PRESENT CALCULATION. ENERGY DEPENDENCE OF SPIN CUT-OFF 5931 1451 63 PARAMETER IN THE ENERGY RANGE BELOW E-JOINT IS DUE TO GRUPPELAAR5931 1451 64 /13/. 5931 1451 65 5931 1451 66 MT = 1 TOTAL 5931 1451 67 SPHERICAL OPTICAL MODEL CALCULATION WAS ADOPTED. 5931 1451 68 5931 1451 69 MT = 2 ELASTIC SCATTERING 5931 1451 70 CALCULATED AS (TOTAL - SUM OF PARTIAL CROSS SECTIONS). 5931 1451 71 5931 1451 72 MT = 4, 51 - 91 INELASTIC SCATTERING 5931 1451 73 SPHERICAL OPTICAL AND STATISTICAL MODEL CALCULATION WAS 5931 1451 74 ADOPTED. THE LEVEL SCHEME WAS BASED ON EVALUATED NUCLEAR 5931 1451 75 STRUCTURE DATA FILE (1987 VERSION)/14/ AND NUCLEAR DATA 5931 1451 76 SHEETS/15/. 5931 1451 77 5931 1451 78 NO. ENERGY(MEV) SPIN-PARITY 5931 1451 79 GR. 0.0 7/2 + 5931 1451 80 1 0.0574 5/2 + 5931 1451 81 2 0.3506 3/2 + 5931 1451 82 3 0.4904 7/2 + 5931 1451 83 4 0.7219 5/2 + 5931 1451 84 5 0.7401 1/2 - 5931 1451 85 6 0.9378 3/2 + 5931 1451 86 7 1.0603 5/2 + 5931 1451 87 8 1.1604 3/2 + 5931 1451 88 9 1.3820 3/2 + 5931 1451 89 10 1.3977 1/2 - 5931 1451 90 LEVELS ABOVE 1.526 MEV WERE ASSUMED TO BE OVERLAPPING. 5931 1451 91 5931 1451 92 MT = 102 CAPTURE 5931 1451 93 SPHERICAL OPTICAL AND STATISTICAL MODEL CALCULATION WITH 5931 1451 94 CASTHY WAS ADOPTED. DIRECT AND SEMI-DIRECT CAPTURE CROSS 5931 1451 95 SECTIONS WERE ESTIMATED ACCORDING TO THE PROCEDURE OF BENZI 5931 1451 96 AND REFFO/16/ AND NORMALIZED TO 1 MILLI-BARN AT 14 MEV. 5931 1451 97 5931 1451 98 THE GAMMA-RAY STRENGTH FUNCTION (6.24E-04) WAS DETERMINED FROM5931 1451 99 THE SYSTEMATICS OF RADIATION WIDTH (0.065 EV) AND THE AVERAGE 5931 1451 100 S-WAVE RESONANCE LEVEL SPACING (104 EV) CALCULATED FROM THE 5931 1451 101 LEVEL DENSITY PARAMETERS. 5931 1451 102 5931 1451 103 MT = 16 (N,2N) CROSS SECTION 5931 1451 104 MT = 17 (N,3N) CROSS SECTION 5931 1451 105 MT = 22 (N,N'A) CROSS SECTION 5931 1451 106 MT = 28 (N,N'P) CROSS SECTION 5931 1451 107 MT = 32 (N,N'D) CROSS SECTION 5931 1451 108 MT = 33 (N,N'T) CROSS SECTION 5931 1451 109 MT =103 (N,P) CROSS SECTION 5931 1451 110 MT =104 (N,D) CROSS SECTION 5931 1451 111 MT =105 (N,T) CROSS SECTION 5931 1451 112 MT =106 (N,HE3) CROSS SECTION 5931 1451 113 MT =107 (N,ALPHA) CROSS SECTION 5931 1451 114 THESE REACTION CROSS SECTIONS WERE CALCULATED WITH THE 5931 1451 115 PREEQUILIBRIUM AND MULTI-STEP EVAPORATION MODEL CODE PEGASUS. 5931 1451 116 5931 1451 117 THE KALBACH'S CONSTANT K (= 324.5) WAS ESTIMATED BY THE 5931 1451 118 FORMULA DERIVED FROM KIKUCHI-KAWAI'S FORMALISM/17/ AND LEVEL 5931 1451 119 DENSITY PARAMETERS. 5931 1451 120 5931 1451 121 FINALLY, THE (N,P) AND (N,ALPHA) CROSS SECTIONS WERE 5931 1451 122 NORMALIZED TO THE FOLLOWING VALUES AT 14.5 MEV: 5931 1451 123 (N,P) 5.29 MB (SYSTEMATICS OF FORREST/18/) 5931 1451 124 (N,ALPHA) 2.22 MB (SYSTEMATICS OF FORREST) 5931 1451 125 5931 1451 126 MT = 251 MU-BAR 5931 1451 127 CALCULATED WITH CASTHY. 5931 1451 128 5931 1451 129 MF = 4 ANGULAR DISTRIBUTIONS OF SECONDARY NEUTRONS 5931 1451 130 LEGENDRE POLYNOMIAL COEFFICIENTS FOR ANGULAR DISTRIBUTIONS ARE 5931 1451 131 GIVEN IN THE CENTER-OF-MASS SYSTEM FOR MT=2 AND DISCRETE INELAS-5931 1451 132 TIC LEVELS, AND IN THE LABORATORY SYSTEM FOR MT=91. THEY WERE 5931 1451 133 CALCULATED WITH CASTHY. FOR OTHER REACTIONS, ISOTROPIC DISTRI- 5931 1451 134 BUTIONS IN THE LABORATORY SYSTEM WERE ASSUMED. 5931 1451 135 5931 1451 136 MF = 5 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS 5931 1451 137 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS WERE CALCULATED WITH 5931 1451 138 PEGASUS FOR INELASTIC SCATTERING TO OVERLAPPING LEVELS AND FOR 5931 1451 139 OTHER NEUTRON EMITTING REACTIONS. 5931 1451 140 5931 1451 141 TABLE 1 NEUTRON OPTICAL POTENTIAL PARAMETERS 5931 1451 142 5931 1451 143 DEPTH (MEV) RADIUS(FM) DIFFUSENESS(FM) 5931 1451 144 ---------------------- ------------ --------------- 5931 1451 145 V = 46.0 R0 = 6.666 A0 = 0.62 5931 1451 146 WS = 7.0 RS = 6.666 AS = 1.0 5931 1451 147 VSO= 7.0 RSO= 6.666 ASO= 0.62 5931 1451 148 THE FORM OF SURFACE ABSORPTION PART IS GAUSSIAN TYPE. 5931 1451 149 5931 1451 150 TABLE 2 LEVEL DENSITY PARAMETERS 5931 1451 151 5931 1451 152 NUCLIDE A(1/MEV) T(MEV) C(1/MEV) EX(MEV) PAIRING 5931 1451 153 --------------------------------------------------------------- 5931 1451 154 57-LA-139 1.380E+01 6.500E-01 1.653E+00 4.468E+00 8.500E-01 5931 1451 155 57-LA-140 1.558E+01 5.900E-01 7.912E+00 3.425E+00 0.0 5931 1451 156 57-LA-141 1.894E+01 5.130E-01 3.056E+00 4.024E+00 7.600E-01 5931 1451 157 57-LA-142 2.026E+01 4.610E-01 1.125E+01 2.749E+00 0.0 5931 1451 158 5931 1451 159 58-CE-140 1.413E+01 6.541E-01 3.376E-01 5.852E+00 2.020E+00 5931 1451 160 58-CE-141 1.714E+01 5.150E-01 7.134E-01 3.957E+00 1.170E+00 5931 1451 161 58-CE-142 1.600E+01 6.000E-01 4.210E-01 5.674E+00 1.930E+00 5931 1451 162 58-CE-143 1.900E+01 5.500E-01 2.613E+00 5.094E+00 1.170E+00 5931 1451 163 5931 1451 164 59-PR-141 1.400E+01 6.500E-01 1.810E+00 4.559E+00 8.500E-01 5931 1451 165 59-PR-142 1.595E+01 6.150E-01 1.201E+01 3.974E+00 0.0 5931 1451 166 59-PR-143 1.500E+01 6.280E-01 2.607E+00 4.558E+00 7.600E-01 5931 1451 167 59-PR-144 1.600E+01 6.000E-01 1.045E+01 3.744E+00 0.0 5931 1451 168 --------------------------------------------------------------- 5931 1451 169 5931 1451 170 SPIN CUTOFF PARAMETERS WERE CALCULATED AS 0.146*SQRT(A)*A**(2/3).5931 1451 171 IN THE CASTHY CALCULATION, SPIN CUTOFF FACTORS AT 0 MEV WERE 5931 1451 172 ASSUMED TO BE 3.050 FOR PR-143 AND 5.0 FOR PR-144. 5931 1451 173 5931 1451 174 REFERENCES 5931 1451 175 1) KAWAI, M. ET AL.: PROC. INT. CONF. ON NUCLEAR DATA FOR SCIENCE5931 1451 176 AND TECHNOLOGY, MITO, P. 569 (1988). 5931 1451 177 2) MUGHABGHAB, S.F. ET AL.: "NEUTRON CROSS SECTIONS, VOL. I, 5931 1451 178 PART A", ACADEMIC PRESS (1981). 5931 1451 179 3) IGARASI, S.: J. NUCL. SCI. TECHNOL., 12, 67 (1975). 5931 1451 180 4) IIJIMA, S. ET AL.: JAERI-M 87-025, P. 337 (1987). 5931 1451 181 5) MOLDAUER, P. A.: NUCL. PHYS., 47, 65 (1963). 5931 1451 182 6) FOSTER, D.G. JR. AND GLASGOW, D.W.: PHYS. REV., C3, 576 5931 1451 183 (1971). 5931 1451 184 7) PEREY, F.G: PHYS. REV. 131, 745 (1963). 5931 1451 185 8) HUIZENGA, J.R. AND IGO, G.: NUCL. PHYS. 29, 462 (1962). 5931 1451 186 9) LOHR, J.M. AND HAEBERLI, W.: NUCL. PHYS. A232, 381 (1974). 5931 1451 187 10) BECCHETTI, F.D., JR. AND GREENLEES, G.W.: POLARIZATION 5931 1451 188 PHENOMENA IN NUCLEAR REACTIONS ((EDS) H.H. BARSHALL AND 5931 1451 189 W. HAEBERLI), P. 682, THE UNIVERSITY OF WISCONSIN PRESS. 5931 1451 190 (1971). 5931 1451 191 11) GILBERT, A. AND CAMERON, A.G.W.: CAN. J. PHYS., 43, 1446 5931 1451 192 (1965). 5931 1451 193 12) IIJIMA, S., ET AL.: J. NUCL. SCI. TECHNOL. 21, 10 (1984). 5931 1451 194 13) GRUPPELAAR, H.: ECN-13 (1977). 5931 1451 195 14) ENSDF: EVALUATED NUCLEAR STRUCTURE DATA FILE (JUNE 1987). 5931 1451 196 15) NUCLEAR DATA SHEETS, 48, 753 (1986). 5931 1451 197 16) BENZI, V. AND REFFO, G.: CCDN-NW/10 (1969). 5931 1451 198 17) KIKUCHI, K. AND KAWAI, M.: "NUCLEAR MATTER AND NUCLEAR 5931 1451 199 REACTIONS", NORTH HOLLAND (1968). 5931 1451 200 18) FORREST, R.A.: AERE-R 12419 (1986). 5931 1451 201 5931 1451 202 1 451 256 15931 1451 203 2 151 367 15931 1451 204 3 1 30 15931 1451 205 3 2 26 15931 1451 206 3 4 17 15931 1451 207 3 16 10 15931 1451 208 3 17 6 15931 1451 209 3 22 15 15931 1451 210 3 28 11 15931 1451 211 3 32 8 15931 1451 212 3 33 8 15931 1451 213 3 51 17 15931 1451 214 3 52 14 15931 1451 215 3 53 14 15931 1451 216 3 54 13 15931 1451 217 3 55 13 15931 1451 218 3 56 12 15931 1451 219 3 57 11 15931 1451 220 3 58 11 15931 1451 221 3 59 10 15931 1451 222 3 60 10 15931 1451 223 3 91 9 15931 1451 224 3 102 21 15931 1451 225 3 103 14 15931 1451 226 3 104 12 15931 1451 227 3 105 12 15931 1451 228 3 106 10 15931 1451 229 3 107 15 15931 1451 230 3 251 23 15931 1451 231 4 2 248 15931 1451 232 4 16 10 15931 1451 233 4 17 10 15931 1451 234 4 22 10 15931 1451 235 4 28 10 15931 1451 236 4 32 10 15931 1451 237 4 33 10 15931 1451 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