4.40980+ 4 9.70642+ 1 1 0 0 14431 1451 1 0.0 + 0 0.0 + 0 0 0 0 04431 1451 2 0.0 + 0 0.0 + 0 0 0 210 584431 1451 3 44-RU- 98 JNDC EVAL-MAR90 JNDC FP NUCLEAR DATA W.G. 4431 1451 4 DIST-NOV90 4431 1451 5 HISTORY 4431 1451 6 90-03 NEW EVALUATION FOR JENDL-3 WAS COMPLETED BY JNDC FPND 4431 1451 7 W.G./1/ 4431 1451 8 4431 1451 9 MF = 1 GENERAL INFORMATION 4431 1451 10 MT=451 COMMENTS AND DICTIONARY 4431 1451 11 4431 1451 12 MF = 2 RESONANCE PARAMETERS 4431 1451 13 MT=151 RESOLVED AND UNRESOLVED RESONANCE PARAMETERS 4431 1451 14 NO RESOLVED RESONANCE PARAMETERS 4431 1451 15 4431 1451 16 UNRESOLVED RESONANCE REGION : 140 EV - 100 KEV 4431 1451 17 THE NEUTRON STRENGTH FUNCTIONS, S0, S1 AND S2 WERE CALCULATED 4431 1451 18 WITH OPTICAL MODEL CODE CASTHY/2/. THE OBSERVED LEVEL SPACING4431 1451 19 WAS DETERMINED TO REPRODUCE THE CAPTURE CROSS SECTION 4431 1451 20 CALCULATED WITH CASTHY. THE EFFECTIVE SCATTERING RADIUS WAS 4431 1451 21 OBTAINED FROM FITTING TO THE CALCULATED TOTAL CROSS SECTION AT4431 1451 22 100 KEV. THE RADIATION WIDTH GG WAS BASED ON THE SYSTEMATICS 4431 1451 23 OF MEASURED VALUES FOR NEIGHBORING NUCLIDES. 4431 1451 24 4431 1451 25 TYPICAL VALUES OF THE PARAMETERS AT 70 KEV: 4431 1451 26 S0 = 0.440E-4, S1 = 4.300E-4, S2 = 0.610E-4, SG = 4.88E-4, 4431 1451 27 GG = 0.130 EV, R = 6.187 FM. 4431 1451 28 4431 1451 29 CALCULATED 2200-M/S CROSS SECTIONS AND RES. INTEGRALS (BARNS) 4431 1451 30 2200 M/S RES. INTEG. 4431 1451 31 TOTAL 13.10 - 4431 1451 32 ELASTIC 5.100 - 4431 1451 33 CAPTURE 8.000 11.5 4431 1451 34 4431 1451 35 MF = 3 NEUTRON CROSS SECTIONS 4431 1451 36 BELOW 140 EV, THE CAPTURE AND ELASTIC SCATTERING CROSS SECTIONS 4431 1451 37 WERE ASSUMED TO BE IN 1/V FORM AND CONSTANT, RESPECTIVELY. THE 4431 1451 38 CAPTURE CROSS SECTION AT 0.0253 EV WAS TAKEN FROM REF./3/, AND 4431 1451 39 THE ELASTIC SCATTERING CROSS SECTION WAS ESTIMATED BY ASSUMING 4431 1451 40 R = 6.3 FM. UNRESOLVED RESONANCE PARAMETERS WERE GIVEN IN THE 4431 1451 41 ENERGY RANGE FROM 140 EV TO 100 KEV. 4431 1451 42 4431 1451 43 ABOVE 100 KEV, THE SPHERICAL OPTICAL AND STATISTICAL MODEL 4431 1451 44 CALCULATION WAS PERFORMED WITH CASTHY, BY TAKING ACCOUNT OF 4431 1451 45 COMPETING REACTIONS, OF WHICH CROSS SECTIONS WERE CALCULATED 4431 1451 46 WITH PEGASUS/4/ STANDING ON A PREEQUILIBRIUM AND MULTI-STEP 4431 1451 47 EVAPORATION MODEL. THE OMP'S FOR NEUTRON GIVEN IN TABLE 1 WERE 4431 1451 48 DETERMINED TO REPRODUCE A SYSTEMATIC TREND OF THE TOTAL CROSS 4431 1451 49 SECTION BY CHANGING RSO OF IIJIMA-KAWAI POTENTIAL/5/. THE 4431 1451 50 OMP'S FOR CHARGED PARTICLES ARE AS FOLLOWS: 4431 1451 51 PROTON = PEREY/6/ 4431 1451 52 ALPHA = HUIZENGA AND IGO/7/ 4431 1451 53 DEUTERON = LOHR AND HAEBERLI/8/ 4431 1451 54 HELIUM-3 AND TRITON = BECCHETTI AND GREENLEES/9/ 4431 1451 55 PARAMETERS FOR THE COMPOSITE LEVEL DENSITY FORMULA OF GILBERT 4431 1451 56 AND CAMERON/10/ WERE EVALUATED BY IIJIMA ET AL./11/ MORE 4431 1451 57 EXTENSIVE DETERMINATION AND MODIFICATION WERE MADE IN THE 4431 1451 58 PRESENT WORK. TABLE 2 SHOWS THE LEVEL DENSITY PARAMETERS USED 4431 1451 59 IN THE PRESENT CALCULATION. ENERGY DEPENDENCE OF SPIN CUT-OFF 4431 1451 60 PARAMETER IN THE ENERGY RANGE BELOW E-JOINT IS DUE TO GRUPPELAAR4431 1451 61 /12/. 4431 1451 62 4431 1451 63 MT = 1 TOTAL 4431 1451 64 SPHERICAL OPTICAL MODEL CALCULATION WAS ADOPTED. 4431 1451 65 4431 1451 66 MT = 2 ELASTIC SCATTERING 4431 1451 67 CALCULATED AS (TOTAL - SUM OF PARTIAL CROSS SECTIONS). 4431 1451 68 4431 1451 69 MT = 4, 51 - 91 INELASTIC SCATTERING 4431 1451 70 SPHERICAL OPTICAL AND STATISTICAL MODEL CALCULATION WAS 4431 1451 71 ADOPTED. THE LEVEL SCHEME WAS BASED ON EVALUATED NUCLEAR 4431 1451 72 STRUCTURE DATA FILE (1987 VERSION)/13/ AND NUCLEAR DATA 4431 1451 73 SHEETS/14/. 4431 1451 74 4431 1451 75 NO. ENERGY(MEV) SPIN-PARITY DWBA CAL. 4431 1451 76 GR. 0.0 0 + 4431 1451 77 1 0.6524 2 + * 4431 1451 78 2 1.3211 0 + 4431 1451 79 3 1.3978 4 + 4431 1451 80 4 1.4146 2 + 4431 1451 81 5 1.7972 3 + 4431 1451 82 6 1.8169 1 + 4431 1451 83 7 2.0133 3 + 4431 1451 84 8 2.2226 6 + 4431 1451 85 9 2.2670 4 + 4431 1451 86 10 2.2850 4 + 4431 1451 87 11 2.4350 3 - 4431 1451 88 12 2.5469 4 + 4431 1451 89 13 2.6570 5 - 4431 1451 90 LEVELS ABOVE 2.671 MEV WERE ASSUMED TO BE OVERLAPPING. 4431 1451 91 4431 1451 92 FOR THE LEVELS WITH AN ASTERISK, THE CONTRIBUTION OF DIRECT 4431 1451 93 INELASTIC SCATTERING CROSS SECTIONS WAS CALCULATED BY THE 4431 1451 94 DWUCK-4 CODE/15/. DEFORMATION PARAMETER (BETA2 = 0.1947) WAS 4431 1451 95 BASED ON THE DATA COMPILED BY RAMAN ET AL./16/ 4431 1451 96 4431 1451 97 MT = 102 CAPTURE 4431 1451 98 SPHERICAL OPTICAL AND STATISTICAL MODEL CALCULATION WITH 4431 1451 99 CASTHY WAS ADOPTED. DIRECT AND SEMI-DIRECT CAPTURE CROSS 4431 1451 100 SECTIONS WERE ESTIMATED ACCORDING TO THE PROCEDURE OF BENZI 4431 1451 101 AND REFFO/17/ AND NORMALIZED TO 1 MILLI-BARN AT 14 MEV. 4431 1451 102 4431 1451 103 THE GAMMA-RAY STRENGTH FUNCTION (4.61E-04) WAS DETERMINED FROM4431 1451 104 THE SYSTEMATICS OF RADIATION WIDTH (0.13 EV) AND THE AVERAGE 4431 1451 105 S-WAVE RESONANCE LEVEL SPACING (282 EV) CALCULATED FROM THE 4431 1451 106 LEVEL DENSITY PARAMETERS. 4431 1451 107 4431 1451 108 MT = 16 (N,2N) CROSS SECTION 4431 1451 109 MT = 17 (N,3N) CROSS SECTION 4431 1451 110 MT = 22 (N,N'A) CROSS SECTION 4431 1451 111 MT = 28 (N,N'P) CROSS SECTION 4431 1451 112 MT = 32 (N,N'D) CROSS SECTION 4431 1451 113 MT =103 (N,P) CROSS SECTION 4431 1451 114 MT =104 (N,D) CROSS SECTION 4431 1451 115 MT =105 (N,T) CROSS SECTION 4431 1451 116 MT =106 (N,HE3) CROSS SECTION 4431 1451 117 MT =107 (N,ALPHA) CROSS SECTION 4431 1451 118 MT =111 (N,2P) CROSS SECTION 4431 1451 119 THESE REACTION CROSS SECTIONS WERE CALCULATED WITH THE 4431 1451 120 PREEQUILIBRIUM AND MULTI-STEP EVAPORATION MODEL CODE PEGASUS. 4431 1451 121 4431 1451 122 THE KALBACH'S CONSTANT K (= 96.1) WAS ESTIMATED BY THE 4431 1451 123 FORMULA DERIVED FROM KIKUCHI-KAWAI'S FORMALISM/18/ AND LEVEL 4431 1451 124 DENSITY PARAMETERS. 4431 1451 125 4431 1451 126 FINALLY, THE (N,2N), (N,P) AND (N,ALPHA) CROSS SECTIONS WERE 4431 1451 127 NORMALIZED TO THE FOLLOWING VALUES AT 14.5 MEV: 4431 1451 128 (N,2N) 1050.00 MB (RECOMMENDED BY BYCHKOV+/19/) 4431 1451 129 (N,P) 70.70 MB (SYSTEMATICS OF FORREST/20/) 4431 1451 130 (N,ALPHA) 17.20 MB (SYSTEMATICS OF FORREST) 4431 1451 131 4431 1451 132 MT = 251 MU-BAR 4431 1451 133 CALCULATED WITH CASTHY. 4431 1451 134 4431 1451 135 MF = 4 ANGULAR DISTRIBUTIONS OF SECONDARY NEUTRONS 4431 1451 136 LEGENDRE POLYNOMIAL COEFFICIENTS FOR ANGULAR DISTRIBUTIONS ARE 4431 1451 137 GIVEN IN THE CENTER-OF-MASS SYSTEM FOR MT=2 AND DISCRETE INELAS-4431 1451 138 TIC LEVELS, AND IN THE LABORATORY SYSTEM FOR MT=91. THEY WERE 4431 1451 139 CALCULATED WITH CASTHY. CONTRIBUTION OF DIRECT INELASTIC 4431 1451 140 SCATTERING WAS CALCULATED WITH DWUCK-4. FOR OTHER REACTIONS, 4431 1451 141 ISOTROPIC DISTRIBUTIONS IN THE LABORATORY SYSTEM WERE ASSUMED. 4431 1451 142 4431 1451 143 MF = 5 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS 4431 1451 144 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS WERE CALCULATED WITH 4431 1451 145 PEGASUS FOR INELASTIC SCATTERING FROM OVERLAPPING LEVELS AND FOR4431 1451 146 OTHER NEUTRON EMITTING REACTIONS. 4431 1451 147 4431 1451 148 TABLE 1 NEUTRON OPTICAL POTENTIAL PARAMETERS 4431 1451 149 4431 1451 150 DEPTH (MEV) RADIUS(FM) DIFFUSENESS(FM) 4431 1451 151 ---------------------- ------------ --------------- 4431 1451 152 V = 47.5 R0 = 5.972 A0 = 0.62 4431 1451 153 WS = 9.74 RS = 6.594 AS = 0.35 4431 1451 154 VSO= 7.0 RSO= 5.97 ASO= 0.62 4431 1451 155 THE FORM OF SURFACE ABSORPTION PART IS DER. WOODS-SAXON TYPE. 4431 1451 156 4431 1451 157 TABLE 2 LEVEL DENSITY PARAMETERS 4431 1451 158 4431 1451 159 NUCLIDE SYST A(1/MEV) T(MEV) C(1/MEV) EX(MEV) PAIRING 4431 1451 160 --------------------------------------------------------------- 4431 1451 161 42-MO- 94 1.301E+01 6.850E-01 3.417E-01 5.770E+00 2.000E+00 4431 1451 162 42-MO- 95 1.360E+01 7.150E-01 1.847E+00 5.835E+00 1.280E+00 4431 1451 163 42-MO- 96 1.403E+01 7.410E-01 6.991E-01 7.645E+00 2.400E+00 4431 1451 164 42-MO- 97 1.517E+01 6.800E-01 2.769E+00 6.036E+00 1.280E+00 4431 1451 165 4431 1451 166 43-TC- 95 * 1.159E+01 6.842E-01 1.101E+00 3.745E+00 7.200E-01 4431 1451 167 43-TC- 96 1.741E+01 5.640E-01 1.503E+01 3.650E+00 0.0 4431 1451 168 43-TC- 97 1.600E+01 6.700E-01 4.756E+00 6.089E+00 1.120E+00 4431 1451 169 43-TC- 98 1.659E+01 6.120E-01 1.776E+01 4.176E+00 0.0 4431 1451 170 4431 1451 171 44-RU- 96 1.343E+01 6.680E-01 3.373E-01 5.719E+00 2.000E+00 4431 1451 172 44-RU- 97 1.510E+01 6.390E-01 1.567E+00 5.300E+00 1.280E+00 4431 1451 173 44-RU- 98 1.382E+01 7.400E-01 6.070E-01 7.507E+00 2.400E+00 4431 1451 174 44-RU- 99 1.650E+01 6.570E-01 4.016E+00 6.235E+00 1.280E+00 4431 1451 175 --------------------------------------------------------------- 4431 1451 176 SYST: * = LDP'S WERE DETERMINED FROM SYSTEMATICS. 4431 1451 177 4431 1451 178 SPIN CUTOFF PARAMETERS WERE CALCULATED AS 0.146*SQRT(A)*A**(2/3).4431 1451 179 IN THE CASTHY CALCULATION, SPIN CUTOFF FACTORS AT 0 MEV WERE 4431 1451 180 ASSUMED TO BE 7.894 FOR RU- 98 AND 12.66 FOR RU- 99. 4431 1451 181 4431 1451 182 REFERENCES 4431 1451 183 1) KAWAI, M. ET AL.: PROC. INT. CONF. ON NUCLEAR DATA FOR SCIENCE4431 1451 184 AND TECHNOLOGY, MITO, P. 569 (1988). 4431 1451 185 2) IGARASI, S.: J. NUCL. SCI. TECHNOL., 12, 67 (1975). 4431 1451 186 3) MUGHABGHAB, S.F. ET AL.: "NEUTRON CROSS SECTIONS, VOL. I, 4431 1451 187 PART A", ACADEMIC PRESS (1981). 4431 1451 188 4) IIJIMA, S. ET AL.: JAERI-M 87-025, P. 337 (1987). 4431 1451 189 5) IIJIMA, S. AND KAWAI, M.: J. NUCL. SCI. TECHNOL., 20, 77 4431 1451 190 (1983). 4431 1451 191 6) PEREY, F.G: PHYS. REV. 131, 745 (1963). 4431 1451 192 7) HUIZENGA, J.R. AND IGO, G.: NUCL. PHYS. 29, 462 (1962). 4431 1451 193 8) LOHR, J.M. AND HAEBERLI, W.: NUCL. PHYS. A232, 381 (1974). 4431 1451 194 9) BECCHETTI, F.D., JR. AND GREENLEES, G.W.: POLARIZATION 4431 1451 195 PHENOMENA IN NUCLEAR REACTIONS ((EDS) H.H. BARSHALL AND 4431 1451 196 W. HAEBERLI), P. 682, THE UNIVERSITY OF WISCONSIN PRESS. 4431 1451 197 (1971). 4431 1451 198 10) GILBERT, A. AND CAMERON, A.G.W.: CAN. J. PHYS., 43, 1446 4431 1451 199 (1965). 4431 1451 200 11) IIJIMA, S., ET AL.: J. NUCL. SCI. TECHNOL. 21, 10 (1984). 4431 1451 201 12) GRUPPELAAR, H.: ECN-13 (1977). 4431 1451 202 13) ENSDF: EVALUATED NUCLEAR STRUCTURE DATA FILE (JUNE 1987). 4431 1451 203 14) NUCLEAR DATA SHEETS, 39, 467 (1983). 4431 1451 204 15) KUNZ, P.D.: PRIVATE COMMUNICATION. 4431 1451 205 16) RAMAN, S., ET AL.: ATOM. DATA AND NUCL. DATA TABLES 36, 1 4431 1451 206 (1987) 4431 1451 207 17) BENZI, V. AND REFFO, G.: CCDN-NW/10 (1969). 4431 1451 208 18) KIKUCHI, K. AND KAWAI, M.: "NUCLEAR MATTER AND NUCLEAR 4431 1451 209 REACTIONS", NORTH HOLLAND (1968). 4431 1451 210 19) BYCHKOV, V.M. ET AL.: INDC(CCP)-146/LJ (1980). 4431 1451 211 20) FORREST, R.A.: AERE-R 12419 (1986). 4431 1451 212 4431 1451 213 1 451 271 14431 1451 214 2 151 147 14431 1451 215 3 1 32 14431 1451 216 3 2 26 14431 1451 217 3 4 15 14431 1451 218 3 16 8 14431 1451 219 3 17 4 14431 1451 220 3 22 13 14431 1451 221 3 28 10 14431 1451 222 3 32 6 14431 1451 223 3 51 15 14431 1451 224 3 52 13 14431 1451 225 3 53 13 14431 1451 226 3 54 13 14431 1451 227 3 55 12 14431 1451 228 3 56 11 14431 1451 229 3 57 11 14431 1451 230 3 58 10 14431 1451 231 3 59 10 14431 1451 232 3 60 10 14431 1451 233 3 61 9 14431 1451 234 3 62 9 14431 1451 235 3 63 9 14431 1451 236 3 91 8 14431 1451 237 3 102 21 14431 1451 238 3 103 14 14431 1451 239 3 104 11 14431 1451 240 3 105 9 14431 1451 241 3 106 11 14431 1451 242 3 107 15 14431 1451 243 3 111 10 14431 1451 244 3 251 24 14431 1451 245 4 2 255 14431 1451 246 4 16 10 14431 1451 247 4 17 10 14431 1451 248 4 22 10 14431 1451 249 4 28 10 14431 1451 250 4 32 10 14431 1451 251 4 51 116 14431 1451 252 4 52 22 14431 1451 253 4 53 22 14431 1451 254 4 54 22 14431 1451 255 4 55 22 14431 1451 256 4 56 22 14431 1451 257 4 57 22 14431 1451 258 4 58 22 14431 1451 259 4 59 22 14431 1451 260 4 60 22 14431 1451 261 4 61 22 14431 1451 262 4 62 22 14431 1451 263 4 63 22 14431 1451 264 4 91 22 14431 1451 265 5 16 49 14431 1451 266 5 17 18 14431 1451 267 5 22 208 14431 1451 268 5 28 90 14431 1451 269 5 32 33 14431 1451 270 5 91 111 14431 1451 271 4431 1 0 272 4431 0 0 273 4.40980+ 4 9.70642+ 1 0 0 1 04431 2151 274 4.40980+ 4 1.00000+ 0 0 1 1 04431 2151 275 1.40000+ 2 1.00000+ 5 2 2 0 04431 2151 276 0.0 + 0 6.18690- 1 0 0 3 04431 2151 277 9.70642+ 1 0.0 + 0 0 0 1 04431 2151 278 5.00000- 1 0.0 + 0 5 0 162 264431 2151 279 0.0 + 0 0.0 + 0 0.0 + 0 1.00000+ 0 0.0 + 0 0.0 + 04431 2151 280 1.40000+ 2 2.81930+ 2 0.0 + 0 1.24050- 2 1.30000- 1 0.0 + 04431 2151 281 2.00000+ 2 2.82030+ 2 0.0 + 0 1.24090- 2 1.30000- 1 0.0 + 04431 2151 282 3.00000+ 2 2.82120+ 2 0.0 + 0 1.24130- 2 1.30000- 1 0.0 + 04431 2151 283 4.00000+ 2 2.82230+ 2 0.0 + 0 1.24180- 2 1.30000- 1 0.0 + 04431 2151 284 5.00000+ 2 2.82320+ 2 0.0 + 0 1.24220- 2 1.30000- 1 0.0 + 04431 2151 285 6.00000+ 2 2.82430+ 2 0.0 + 0 1.24270- 2 1.30000- 1 0.0 + 04431 2151 286 8.00000+ 2 2.82660+ 2 0.0 + 0 1.24370- 2 1.30000- 1 0.0 + 04431 2151 287 1.00000+ 3 2.82900+ 2 0.0 + 0 1.24480- 2 1.30000- 1 0.0 + 04431 2151 288 1.50000+ 3 2.82250+ 2 0.0 + 0 1.24190- 2 1.30000- 1 0.0 + 04431 2151 289 2.00000+ 3 2.83220+ 2 0.0 + 0 1.24620- 2 1.30000- 1 0.0 + 04431 2151 290 3.00000+ 3 2.85290+ 2 0.0 + 0 1.25530- 2 1.30000- 1 0.0 + 04431 2151 291 4.00000+ 3 2.86040+ 2 0.0 + 0 1.25860- 2 1.30000- 1 0.0 + 04431 2151 292 5.00000+ 3 2.86510+ 2 0.0 + 0 1.26060- 2 1.30000- 1 0.0 + 04431 2151 293 6.00000+ 3 2.86790+ 2 0.0 + 0 1.26190- 2 1.30000- 1 0.0 + 04431 2151 294 7.00000+ 3 2.86650+ 2 0.0 + 0 1.26130- 2 1.30000- 1 0.0 + 04431 2151 295 8.00000+ 3 2.86630+ 2 0.0 + 0 1.26120- 2 1.30000- 1 0.0 + 04431 2151 296 1.00000+ 4 2.86370+ 2 0.0 + 0 1.26000- 2 1.30000- 1 0.0 + 04431 2151 297 1.50000+ 4 2.85210+ 2 0.0 + 0 1.25490- 2 1.30000- 1 0.0 + 04431 2151 298 2.50000+ 4 2.82090+ 2 0.0 + 0 1.24120- 2 1.30000- 1 0.0 + 04431 2151 299 3.00000+ 4 2.80410+ 2 0.0 + 0 1.23380- 2 1.30000- 1 0.0 + 04431 2151 300 4.00000+ 4 2.77030+ 2 0.0 + 0 1.21890- 2 1.30000- 1 0.0 + 04431 2151 301 5.00000+ 4 2.73670+ 2 0.0 + 0 1.20410- 2 1.30000- 1 0.0 + 04431 2151 302 6.00000+ 4 2.69790+ 2 0.0 + 0 1.18710- 2 1.30000- 1 0.0 + 04431 2151 303 7.00000+ 4 2.66300+ 2 0.0 + 0 1.17170- 2 1.30000- 1 0.0 + 04431 2151 304 8.00000+ 4 2.62860+ 2 0.0 + 0 1.15660- 2 1.30000- 1 0.0 + 04431 2151 305 1.00000+ 5 2.51910+ 2 0.0 + 0 1.10840- 2 1.30000- 1 0.0 + 04431 2151 306 9.70642+ 1 0.0 + 0 1 0 2 04431 2151 307 5.00000- 1 0.0 + 0 5 0 162 264431 2151 308 0.0 + 0 0.0 + 0 0.0 + 0 1.00000+ 0 0.0 + 0 0.0 + 04431 2151 309 1.40000+ 2 2.81930+ 2 0.0 + 0 1.21230- 1 1.30000- 1 0.0 + 04431 2151 310 2.00000+ 2 2.82030+ 2 0.0 + 0 1.21270- 1 1.30000- 1 0.0 + 04431 2151 311 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