4.40990+ 4 9.80562+ 1 1 0 0 24434 1451 1 0.00000+ 0 0.00000+ 0 0 0 0 04434 1451 2 0.00000+ 0 0.00000+ 0 0 0 210 554434 1451 3 44-RU- 99 JNDC EVAL-MAR90 JNDC FP NUCLEAR DATA W.G. 4434 1451 4 DIST-SEP90 REV2-OCT93 4434 1451 5 HISTORY 4434 1451 6 90-03 NEW EVALUATION FOR JENDL-3 WAS COMPLETED BY JNDC FPND 4434 1451 7 W.G./1/ 4434 1451 8 93-10 JENDL-3.2 WAS MADE BY JNDC FPND W.G. 4434 1451 9 4434 1451 10 ***** MODIFIED PARTS FOR JENDL-3.2 ******************** 4434 1451 11 (2,151) RESOLVED RESONANCE PARAMETERS 4434 1451 12 *********************************************************** 4434 1451 13 4434 1451 14 4434 1451 15 MF = 1 GENERAL INFORMATION 4434 1451 16 MT=451 COMMENTS AND DICTIONARY 4434 1451 17 4434 1451 18 MF = 2 RESONANCE PARAMETERS 4434 1451 19 MT=151 RESOLVED AND UNRESOLVED RESONANCE PARAMETERS 4434 1451 20 RESOLVED RESONANCE REGION (MLBW FORMULA) : BELOW 1 KEV 4434 1451 21 RESONANCE PARAMETERS WERE EVALUATED AS FOLLOWS: RESONANCE 4434 1451 22 ENERGIES, NEUTRON AND RADIATION WIDTHS WERE TAKEN FROM THE 4434 1451 23 MEASUREMENT OF POPOV ET AL./2/ AS FOR LOWEST TWO LEVES, THE 4434 1451 24 PARAMETERS WERE TAKEN FROM THE COMPILATION OF MUGHABGHAB ET 4434 1451 25 AL./3/. TOTAL SPIN J FOR RESONANCES MEASURED BY POPOV ET AL. 4434 1451 26 WAS TENTATIVELY ESTIMATED WITH A RANDOM NUMBER METHOD. 4434 1451 27 NEUTRON ORBITAL ANGULAR MOMENTUM L WAS ESTIMATED WITH A METHOD4434 1451 28 OF BOLLINGER AND THOMAS/4/. AVERAGE RADIATION WIDTH OF 199 4434 1451 29 MEV WAS DEDUCED AND ADOPTED TO THE LEVELS WHOSE RADIATION 4434 1451 30 WIDTH WAS UNKNOWN. SCATTERING RADIUS OF 6.1 FM WAS ASSUMED 4434 1451 31 FROM THE SYSTEMATICS OF MEASURED VALUES FOR NEIGHBORING 4434 1451 32 NUCLIDES. 4434 1451 33 4434 1451 34 FOR JENDL-3.2, TOTAL SPIN J WAS DETERMINED BASED ON THE 4434 1451 35 MEASUREMENTS OF COCEVA ET AL./5/ AND WITH A RANDUM NUMBER 4434 1451 36 METHOD. 4434 1451 37 4434 1451 38 UNRESOLVED RESONANCE REGION : 1 KEV - 100 KEV 4434 1451 39 THE NEUTRON STRENGTH FUNCTIONS, S0, S1 AND S2 WERE CALCULATED 4434 1451 40 WITH OPTICAL MODEL CODE CASTHY/6/. THE OBSERVED LEVEL 4434 1451 41 SPACING WAS DETERMINED TO REPRODUCE THE CAPTURE CROSS SECTION 4434 1451 42 CALCULATED WITH CASTHY. THE EFFECTIVE SCATTERING RADIUS WAS 4434 1451 43 OBTAINED FROM FITTING TO THE CALCULATED TOTAL CROSS SECTION 4434 1451 44 AT 100 KEV. THE RADIATION WIDTH GG WAS BASED ON THE 4434 1451 45 COMPILATION OF MUGHABGHAB ET AL./3/ 4434 1451 46 4434 1451 47 TYPICAL VALUES OF THE PARAMETERS AT 70 KEV: 4434 1451 48 S0 = 0.440E-4, S1 = 4.200E-4, S2 = 0.600E-4, SG = 79.2E-4, 4434 1451 49 GG = 0.195 EV, R = 6.224 FM. 4434 1451 50 4434 1451 51 CALCULATED 2200-M/S CROSS SECTIONS AND RES. INTEGRALS (BARNS) 4434 1451 52 2200 M/S RES. INTEG. 4434 1451 53 TOTAL 10.985 - 4434 1451 54 ELASTIC 3.676 - 4434 1451 55 CAPTURE 7.309 171 4434 1451 56 4434 1451 57 MF = 3 NEUTRON CROSS SECTIONS 4434 1451 58 BELOW 100 KEV, RESONANCE PARAMETERS WERE GIVEN. 4434 1451 59 ABOVE 100 KEV, THE SPHERICAL OPTICAL AND STATISTICAL MODEL 4434 1451 60 CALCULATION WAS PERFORMED WITH CASTHY, BY TAKING ACCOUNT OF 4434 1451 61 COMPETING REACTIONS, OF WHICH CROSS SECTIONS WERE CALCULATED 4434 1451 62 WITH PEGASUS/7/ STANDING ON A PREEQUILIBRIUM AND MULTI-STEP 4434 1451 63 EVAPORATION MODEL. THE OMP'S FOR NEUTRON GIVEN IN TABLE 1 WERE 4434 1451 64 DETERMINED TO REPRODUCE A SYSTEMATIC TREND OF THE TOTAL CROSS 4434 1451 65 SECTION BY CHANGING RSO OF IIJIMA-KAWAI POTENTIAL/8/. THE 4434 1451 66 OMP'S FOR CHARGED PARTICLES ARE AS FOLLOWS: 4434 1451 67 PROTON = PEREY/9/ 4434 1451 68 ALPHA = HUIZENGA AND IGO/10/ 4434 1451 69 DEUTERON = LOHR AND HAEBERLI/11/ 4434 1451 70 HELIUM-3 AND TRITON = BECCHETTI AND GREENLEES/12/ 4434 1451 71 PARAMETERS FOR THE COMPOSITE LEVEL DENSITY FORMULA OF GILBERT 4434 1451 72 AND CAMERON/13/ WERE EVALUATED BY IIJIMA ET AL./14/ MORE 4434 1451 73 EXTENSIVE DETERMINATION AND MODIFICATION WERE MADE IN THE 4434 1451 74 PRESENT WORK. TABLE 2 SHOWS THE LEVEL DENSITY PARAMETERS USED 4434 1451 75 IN THE PRESENT CALCULATION. ENERGY DEPENDENCE OF SPIN CUT-OFF 4434 1451 76 PARAMETER IN THE ENERGY RANGE BELOW E-JOINT IS DUE TO GRUPPELAAR4434 1451 77 /15/. 4434 1451 78 4434 1451 79 MT = 1 TOTAL 4434 1451 80 SPHERICAL OPTICAL MODEL CALCULATION WAS ADOPTED. 4434 1451 81 4434 1451 82 MT = 2 ELASTIC SCATTERING 4434 1451 83 CALCULATED AS (TOTAL - SUM OF PARTIAL CROSS SECTIONS). 4434 1451 84 4434 1451 85 MT = 4, 51 - 91 INELASTIC SCATTERING 4434 1451 86 SPHERICAL OPTICAL AND STATISTICAL MODEL CALCULATION WAS 4434 1451 87 ADOPTED. THE LEVEL SCHEME WAS TAKEN FROM REF./16/. 4434 1451 88 4434 1451 89 NO. ENERGY(MEV) SPIN-PARITY 4434 1451 90 GR. 0.0 5/2 + 4434 1451 91 1 0.0894 3/2 + 4434 1451 92 2 0.3221 5/2 + 4434 1451 93 3 0.3404 7/2 + 4434 1451 94 4 0.4420 3/2 + 4434 1451 95 5 0.5755 5/2 + 4434 1451 96 6 0.6180 7/2 + 4434 1451 97 7 0.7192 9/2 + 4434 1451 98 8 1.0480 11/2 + 4434 1451 99 9 1.0700 11/2 - 4434 1451 100 10 1.3130 11/2 + 4434 1451 101 11 1.4960 13/2 + 4434 1451 102 12 1.5720 15/2 - 4434 1451 103 LEVELS ABOVE 1.7 MEV WERE ASSUMED TO BE OVERLAPPING. 4434 1451 104 4434 1451 105 MT = 102 CAPTURE 4434 1451 106 SPHERICAL OPTICAL AND STATISTICAL MODEL CALCULATION WITH 4434 1451 107 CASTHY WAS ADOPTED. DIRECT AND SEMI-DIRECT CAPTURE CROSS 4434 1451 108 SECTIONS WERE ESTIMATED ACCORDING TO THE PROCEDURE OF BENZI 4434 1451 109 AND REFFO/17/ AND NORMALIZED TO 1 MILLI-BARN AT 14 MEV. 4434 1451 110 4434 1451 111 THE GAMMA-RAY STRENGTH FUNCTION (7.80E-03) WAS DETERMINED FROM4434 1451 112 THE RADIATION WIDTH (0.195+-0.020 EV) AND AVERAGE S-WAVE 4434 1451 113 RESONANCE LEVEL SPACING (25+-2 EV/3/). 4434 1451 114 4434 1451 115 MT = 16 (N,2N) CROSS SECTION 4434 1451 116 MT = 17 (N,3N) CROSS SECTION 4434 1451 117 MT = 22 (N,N'A) CROSS SECTION 4434 1451 118 MT = 28 (N,N'P) CROSS SECTION 4434 1451 119 MT = 32 (N,N'D) CROSS SECTION 4434 1451 120 MT =103 (N,P) CROSS SECTION 4434 1451 121 MT =104 (N,D) CROSS SECTION 4434 1451 122 MT =105 (N,T) CROSS SECTION 4434 1451 123 MT =106 (N,HE3) CROSS SECTION 4434 1451 124 MT =107 (N,ALPHA) CROSS SECTION 4434 1451 125 THESE REACTION CROSS SECTIONS WERE CALCULATED WITH THE 4434 1451 126 PREEQUILIBRIUM AND MULTI-STEP EVAPORATION MODEL CODE PEGASUS. 4434 1451 127 4434 1451 128 THE KALBACH'S CONSTANT K (= 126.7) WAS ESTIMATED BY THE 4434 1451 129 FORMULA DERIVED FROM KIKUCHI-KAWAI'S FORMALISM/18/ AND LEVEL 4434 1451 130 DENSITY PARAMETERS. 4434 1451 131 4434 1451 132 FINALLY, THE (N,P) AND (N,ALPHA) CROSS SECTIONS WERE 4434 1451 133 NORMALIZED TO THE FOLLOWING VALUES AT 14.5 MEV: 4434 1451 134 (N,P) 49.40 MB (SYSTEMATICS OF FORREST/19/) 4434 1451 135 (N,ALPHA) 12.30 MB (SYSTEMATICS OF FORREST) 4434 1451 136 4434 1451 137 MT = 251 MU-BAR 4434 1451 138 CALCULATED WITH CASTHY. 4434 1451 139 4434 1451 140 MF = 4 ANGULAR DISTRIBUTIONS OF SECONDARY NEUTRONS 4434 1451 141 LEGENDRE POLYNOMIAL COEFFICIENTS FOR ANGULAR DISTRIBUTIONS ARE 4434 1451 142 GIVEN IN THE CENTER-OF-MASS SYSTEM FOR MT=2 AND DISCRETE INELAS-4434 1451 143 TIC LEVELS, AND IN THE LABORATORY SYSTEM FOR MT=91. THEY WERE 4434 1451 144 CALCULATED WITH CASTHY/6/. 4434 1451 145 4434 1451 146 MF = 5 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS 4434 1451 147 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS WERE CALCULATED WITH 4434 1451 148 PEGASUS FOR INELASTIC SCATTERING TO OVERLAPPING LEVELS AND FOR 4434 1451 149 OTHER NEUTRON EMITTING REACTIONS. 4434 1451 150 4434 1451 151 TABLE 1 NEUTRON OPTICAL POTENTIAL PARAMETERS 4434 1451 152 4434 1451 153 DEPTH (MEV) RADIUS(FM) DIFFUSENESS(FM) 4434 1451 154 ---------------------- ------------ --------------- 4434 1451 155 V = 47.5 R0 = 5.972 A0 = 0.62 4434 1451 156 WS = 9.74 RS = 6.594 AS = 0.35 4434 1451 157 VSO= 7.0 RSO= 5.97 ASO= 0.62 4434 1451 158 THE FORM OF SURFACE ABSORPTION PART IS DER. WOODS-SAXON TYPE. 4434 1451 159 4434 1451 160 TABLE 2 LEVEL DENSITY PARAMETERS 4434 1451 161 4434 1451 162 NUCLIDE A(1/MEV) T(MEV) C(1/MEV) EX(MEV) PAIRING 4434 1451 163 --------------------------------------------------------------- 4434 1451 164 42-MO- 95 1.360E+01 7.150E-01 1.847E+00 5.835E+00 1.280E+00 4434 1451 165 42-MO- 96 1.403E+01 7.410E-01 6.991E-01 7.645E+00 2.400E+00 4434 1451 166 42-MO- 97 1.517E+01 6.800E-01 2.769E+00 6.036E+00 1.280E+00 4434 1451 167 42-MO- 98 1.594E+01 6.900E-01 7.358E-01 7.888E+00 2.570E+00 4434 1451 168 4434 1451 169 43-TC- 96 1.741E+01 5.640E-01 1.503E+01 3.650E+00 0.0 4434 1451 170 43-TC- 97 1.600E+01 6.700E-01 4.756E+00 6.089E+00 1.120E+00 4434 1451 171 43-TC- 98 1.659E+01 6.120E-01 1.776E+01 4.176E+00 0.0 4434 1451 172 43-TC- 99 1.600E+01 6.550E-01 2.973E+00 5.984E+00 1.290E+00 4434 1451 173 4434 1451 174 44-RU- 97 1.510E+01 6.390E-01 1.567E+00 5.300E+00 1.280E+00 4434 1451 175 44-RU- 98 1.382E+01 7.400E-01 6.070E-01 7.507E+00 2.400E+00 4434 1451 176 44-RU- 99 1.650E+01 6.570E-01 4.016E+00 6.235E+00 1.280E+00 4434 1451 177 44-RU-100 1.520E+01 7.200E-01 7.835E-01 8.078E+00 2.570E+00 4434 1451 178 --------------------------------------------------------------- 4434 1451 179 4434 1451 180 SPIN CUTOFF PARAMETERS WERE CALCULATED AS 0.146*SQRT(A)*A**(2/3).4434 1451 181 IN THE CASTHY CALCULATION, SPIN CUTOFF FACTORS AT 0 MEV WERE 4434 1451 182 ASSUMED TO BE 12.66 FOR RU- 99 AND 4.062 FOR RU-100. 4434 1451 183 4434 1451 184 REFERENCES 4434 1451 185 1) KAWAI, M. ET AL.: J. NUCL. SCI. TECHNOL., 29, 195 (1992). 4434 1451 186 2) POPOV, JU.P., ET AL.: YAD. FIZ., 29, 561 (1979). 4434 1451 187 3) MUGHABGHAB, S.F. ET AL.: "NEUTRON CROSS SECTIONS, VOL. I, 4434 1451 188 PART A", ACADEMIC PRESS (1981). 4434 1451 189 4) BOLLINGER, L.M. AND THOMAS, G.E.: PHYS. REV., 171,1293(1968). 4434 1451 190 5) COCEVA, C., ET AL.: NUCL. PHYS., A 117, 586 (1968). 4434 1451 191 6) IGARASI, S. AND FUKAHORI, T.: JAERI 1321 (1991). 4434 1451 192 7) IIJIMA, S. ET AL.: JAERI-M 87-025, P. 337 (1987). 4434 1451 193 8) IIJIMA, S. AND KAWAI, M.: J. NUCL. SCI. TECHNOL., 20, 77 4434 1451 194 (1983). 4434 1451 195 9) PEREY, F.G: PHYS. REV. 131, 745 (1963). 4434 1451 196 10) HUIZENGA, J.R. AND IGO, G.: NUCL. PHYS. 29, 462 (1962). 4434 1451 197 11) LOHR, J.M. AND HAEBERLI, W.: NUCL. PHYS. A232, 381 (1974). 4434 1451 198 12) BECCHETTI, F.D., JR. AND GREENLEES, G.W.: POLARIZATION 4434 1451 199 PHENOMENA IN NUCLEAR REACTIONS ((EDS) H.H. BARSHALL AND 4434 1451 200 W. HAEBERLI), P. 682, THE UNIVERSITY OF WISCONSIN PRESS. 4434 1451 201 (1971). 4434 1451 202 13) GILBERT, A. AND CAMERON, A.G.W.: CAN. J. PHYS., 43, 1446 4434 1451 203 (1965). 4434 1451 204 14) IIJIMA, S., ET AL.: J. NUCL. SCI. TECHNOL. 21, 10 (1984). 4434 1451 205 15) GRUPPELAAR, H.: ECN-13 (1977). 4434 1451 206 16) LEDERER, C.M., ET AL.: "TABLE OF ISOTOPES, 7TH ED.", WILEY- 4434 1451 207 INTERSCIENCE PUBLICATION (1978). 4434 1451 208 17) BENZI, V. AND REFFO, G.: CCDN-NW/10 (1969). 4434 1451 209 18) KIKUCHI, K. AND KAWAI, M.: "NUCLEAR MATTER AND NUCLEAR 4434 1451 210 REACTIONS", NORTH HOLLAND (1968). 4434 1451 211 19) FORREST, R.A.: AERE-R 12419 (1986). 4434 1451 212 4434 1451 213 1 451 268 14434 1451 214 2 151 302 24434 1451 215 3 1 28 14434 1451 216 3 2 27 14434 1451 217 3 4 17 14434 1451 218 3 16 10 14434 1451 219 3 17 5 14434 1451 220 3 22 13 14434 1451 221 3 28 9 14434 1451 222 3 32 7 14434 1451 223 3 51 17 14434 1451 224 3 52 15 14434 1451 225 3 53 15 14434 1451 226 3 54 14 14434 1451 227 3 55 14 14434 1451 228 3 56 13 14434 1451 229 3 57 13 14434 1451 230 3 58 11 14434 1451 231 3 59 11 14434 1451 232 3 60 10 14434 1451 233 3 61 10 14434 1451 234 3 62 9 14434 1451 235 3 91 9 14434 1451 236 3 102 21 14434 1451 237 3 103 15 14434 1451 238 3 104 11 14434 1451 239 3 105 10 14434 1451 240 3 106 10 14434 1451 241 3 107 15 14434 1451 242 3 251 23 14434 1451 243 4 2 249 14434 1451 244 4 16 10 14434 1451 245 4 17 10 14434 1451 246 4 22 10 14434 1451 247 4 28 10 14434 1451 248 4 32 10 14434 1451 249 4 51 27 14434 1451 250 4 52 27 14434 1451 251 4 53 27 14434 1451 252 4 54 27 14434 1451 253 4 55 26 14434 1451 254 4 56 26 14434 1451 255 4 57 26 14434 1451 256 4 58 22 14434 1451 257 4 59 22 14434 1451 258 4 60 22 14434 1451 259 4 61 22 14434 1451 260 4 62 22 14434 1451 261 4 91 22 14434 1451 262 5 16 66 14434 1451 263 5 17 22 14434 1451 264 5 22 200 14434 1451 265 5 28 96 14434 1451 266 5 32 49 14434 1451 267 5 91 120 14434 1451 268 4434 1 0 269 4434 0 0 270 4.40990+ 4 9.80562+ 1 0 0 1 04434 2151 271 4.40990+ 4 1.00000+ 0 0 0 2 04434 2151 272 1.00000- 5 1.00000+ 3 1 2 0 04434 2151 273 2.50000+ 0 6.10000- 1 0 0 1 04434 2151 274 9.80562+ 1 0.00000+ 0 0 0 240 404434 2151 275 1.00500+ 1 3.00000+ 0 1.85600- 1 3.59999- 3 1.82000- 1 0.00000+ 04434 2151 276 2.51000+ 1 3.00000+ 0 2.00000- 1 1.00000- 2 1.90000- 1 0.00000+ 04434 2151 277 5.71300+ 1 3.00000+ 0 2.10240- 1 1.22400- 2 1.98000- 1 0.00000+ 04434 2151 278 8.16500+ 1 2.00000+ 0 2.40760- 1 5.75999- 3 2.35000- 1 0.00000+ 04434 2151 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