4.30990+ 4 9.80566+ 1 1 0 0 24331 1451 1 0.00000+ 0 0.00000+ 0 0 0 0 04331 1451 2 0.00000+ 0 0.00000+ 0 0 0 227 544331 1451 3 43-TC- 99 JNDC EVAL-MAR90 JNDC FP NUCLEAR DATA W.G. 4331 1451 4 DIST-SEP90 REV2-NOV93 4331 1451 5 HISTORY 4331 1451 6 84-10 EVALUATION FOR JENDL-2 WAS MADE BY JNDC FPND W.G./1/ 4331 1451 7 90-03 MODIFICATION FOR JENDL-3 WAS MADE/2/. 4331 1451 8 93-11 JENDL-3.2 WAS MADE BY JNDC FPND W.G. 4331 1451 9 4331 1451 10 ***** MODIFIED PARTS FOR JENDL-3.2 ******************** 4331 1451 11 (2,151) RESOLVED RESONANCE PARAMETERS 4331 1451 12 *********************************************************** 4331 1451 13 4331 1451 14 4331 1451 15 MF = 1 GENERAL INFORMATION 4331 1451 16 MT=451 COMMENTS AND DICTIONARY 4331 1451 17 4331 1451 18 MF = 2 RESONANCE PARAMETERS 4331 1451 19 MT=151 RESOLVED AND UNRESOLVED RESONANCE PARAMETERS 4331 1451 20 RESOLVED RESONANCE REGION (MLBW FORMULA) : BELOW 4.219 KEV 4331 1451 21 RESONANCE PARAMETERS WERE TAKEN FROM JENDL-2 WITH SLIGHT 4331 1451 22 MODIFICATION. 4331 1451 23 EVALUATION FOR JENDL-2 WAS MADE BY KIKUCHI /3/. 4331 1451 24 PARAMETERS OF THE 1ST AND 2ND RESONANCES WERE ADOPTED FROM 4331 1451 25 RECOMMENDED VALUES OF FISCHER ET AL./4/, AND SLIGHTLY 4331 1451 26 ADJUSTED SO AS TO REPRODUCE THE CAPTURE CROSS SECTION OF 4331 1451 27 20+-1 BARNS AT 0.0253 EV AND THE RESONANCE INTEGRAL OF 4331 1451 28 340+-20 BARNS /5/. PARAMETERS OF LEVELS BETWEEN 40 EV AND 4331 1451 29 1.5 KEV WERE EVALUATED ON THE BASIS OF DATA MEASURED BY 4331 1451 30 ADAMCHUK ET AL. /6/ AND BY LITTLE AND BLOCK/7/. IN THE 4331 1451 31 ENERGY RANGE FROM 1.0 TO 2.6 KEV, ARTIFICIAL LEVELS WERE 4331 1451 32 GENERATED WITH STAT /8/ BY ASSUMING D=0.04 EV, S0= 0.17E-4, 4331 1451 33 S1=11.12E-4 AND THE AVERAGE RADIATION WIDTH OF 0.17 EV. FOR 4331 1451 34 THE RESONANCES OF WHICH ENERGY WAS ONLY MEASURED BY LITTLE 4331 1451 35 AND BLOCK, THEIR PARAMETERS WERE ALSO ESTIMATED WITH STAT. 4331 1451 36 ABOVE 2.66 KEV, EVALUATION WAS BASED ON THE CAPTURE AREAS 4331 1451 37 MEASURED BY MACKLIN /9/. SCATTERING RADIUS WAS TAKEN FROM 4331 1451 38 THE COMPILATION OF MUGHABGHAB ET AL./5/ 4331 1451 39 FOR JENDL-3, TOTAL SPIN J OF SOME RESONANCES WAS TENTATIVE-4331 1451 40 LY ESTIMATED WITH A RANDOM NUMBER METHOD. IN THIS PROCEDURE, 4331 1451 41 NEUTRON WIDTHS FOR RESONANCES ABOVE 2.66 KEV WERE DETERMINED 4331 1451 42 TO REPRODUCE THE CAPTURE AREAS MEASURED BY MACKLIN/9/. 4331 1451 43 FOR JENDL-3.2, NEUTRON OR RADIATIVE CAPTURE WIDTHS FOR 4331 1451 44 LEVELS BETWEEN 111 EV AND 754 EV WERE MODIFIED SO AS TO 4331 1451 45 REPRODUCE THE CAPTURE AREA MEASURED BY LITTLE AND BLOCK/7/. 4331 1451 46 4331 1451 47 UNRESOLVED RESONANCE REGION : 4.219 KEV - 100 KEV 4331 1451 48 UNRESOLVED RESONANCE PARAMETERS WERE ADOPTED FROM JENDL-2. 4331 1451 49 THE PARAMETERS WERE ADJUSTED TO REPRODUCE THE CAPTURE CROSS 4331 1451 50 SECTION MEASURED BY MACKLIN /9/. THE EFFECTIVE SCATTERING 4331 1451 51 RADIUS WAS OBTAINED FROM FITTING TO THE CALCULATED TOTAL CROSS4331 1451 52 SECTION AT 100 KEV. 4331 1451 53 4331 1451 54 TYPICAL VALUES OF THE PARAMETERS AT 70 KEV: 4331 1451 55 S0 = 0.414E-4, S1 = 4.241E-4, S2 = 0.488 E-4, SG = 90.4E-4, 4331 1451 56 GG = 0.186 EV, R = 6.215 FM. 4331 1451 57 4331 1451 58 CALCULATED 2200-M/S CROSS SECTIONS AND RES. INTEGRALS (BARNS) 4331 1451 59 2200 M/S RES. INTEG. 4331 1451 60 TOTAL 23.063 - 4331 1451 61 ELASTIC 3.422 - 4331 1451 62 CAPTURE 19.641 312 4331 1451 63 4331 1451 64 MF = 3 NEUTRON CROSS SECTIONS 4331 1451 65 BELOW 100 KEV, RESONANCE PARAMETERS WERE GIVEN. 4331 1451 66 ABOVE 100 KEV, THE SPHERICAL OPTICAL AND STATISTICAL MODEL 4331 1451 67 CALCULATION WAS PERFORMED WITH CASTHY/10/, BY TAKING ACCOUNT OF 4331 1451 68 COMPETING REACTIONS, OF WHICH CROSS SECTIONS WERE CALCULATED 4331 1451 69 WITH PEGASUS/11/ STANDING ON A PREEQUILIBRIUM AND MULTI-STEP 4331 1451 70 EVAPORATION MODEL. THE OMP'S FOR NEUTRON GIVEN IN TABLE 1 WERE 4331 1451 71 DETERMINED TO REPRODUCE A SYSTEMATIC TREND OF THE TOTAL CROSS 4331 1451 72 SECTION BY CHANGING RSO OF IIJIMA-KAWAI POTENTIAL/12/. THE 4331 1451 73 OMP'S FOR CHARGED PARTICLES ARE AS FOLLOWS: 4331 1451 74 PROTON = PEREY/13/ 4331 1451 75 ALPHA = HUIZENGA AND IGO/14/ 4331 1451 76 DEUTERON = LOHR AND HAEBERLI/15/ 4331 1451 77 HELIUM-3 AND TRITON = BECCHETTI AND GREENLEES/16/ 4331 1451 78 PARAMETERS FOR THE COMPOSITE LEVEL DENSITY FORMULA OF GILBERT 4331 1451 79 AND CAMERON/17/ WERE EVALUATED BY IIJIMA ET AL./18/ MORE 4331 1451 80 EXTENSIVE DETERMINATION AND MODIFICATION WERE MADE IN THE 4331 1451 81 PRESENT WORK. TABLE 2 SHOWS THE LEVEL DENSITY PARAMETERS USED 4331 1451 82 IN THE PRESENT CALCULATION. ENERGY DEPENDENCE OF SPIN CUT-OFF 4331 1451 83 PARAMETER IN THE ENERGY RANGE BELOW E-JOINT IS DUE TO GRUPPELAAR4331 1451 84 /19/. 4331 1451 85 4331 1451 86 MT = 1 TOTAL 4331 1451 87 SPHERICAL OPTICAL MODEL CALCULATION WAS ADOPTED. 4331 1451 88 4331 1451 89 MT = 2 ELASTIC SCATTERING 4331 1451 90 CALCULATED AS (TOTAL - SUM OF PARTIAL CROSS SECTIONS). 4331 1451 91 4331 1451 92 MT = 4, 51 - 91 INELASTIC SCATTERING 4331 1451 93 SPHERICAL OPTICAL AND STATISTICAL MODEL CALCULATION WAS 4331 1451 94 ADOPTED. THE LEVEL SCHEME WAS TAKEN FROM REF./20/ 4331 1451 95 4331 1451 96 NO. ENERGY(MEV) SPIN-PARITY 4331 1451 97 GR. 0.0 9/2 + 4331 1451 98 1 0.1405 7/2 + 4331 1451 99 2 0.1426 1/2 - 4331 1451 100 3 0.1811 5/2 + 4331 1451 101 4 0.5091 3/2 - 4331 1451 102 5 0.5343 5/2 - 4331 1451 103 6 0.6254 7/2 + 4331 1451 104 7 0.6715 5/2 - 4331 1451 105 8 0.7263 11/2 + 4331 1451 106 9 0.7616 5/2 + 4331 1451 107 10 0.7620 13/2 + 4331 1451 108 LEVELS ABOVE 0.9 MEV WERE ASSUMED TO BE OVERLAPPING. 4331 1451 109 4331 1451 110 MT = 102 CAPTURE 4331 1451 111 SPHERICAL OPTICAL AND STATISTICAL MODEL CALCULATION WITH 4331 1451 112 CASTHY WAS ADOPTED. DIRECT AND SEMI-DIRECT CAPTURE CROSS 4331 1451 113 SECTIONS WERE ESTIMATED ACCORDING TO THE PROCEDURE OF BENZI 4331 1451 114 AND REFFO/21/ AND NORMALIZED TO 1 MILLI-BARN AT 14 MEV. 4331 1451 115 4331 1451 116 THE GAMMA-RAY STRENGTH FUNCTION (8.37E-03) WAS ADJUSTED TO 4331 1451 117 REPRODUCE THE CAPTURE CROSS SECTION OF 380 MILLI-BARNS AT 100 4331 1451 118 KEV MEASURED BY MACKLIN/22/. 4331 1451 119 4331 1451 120 MT = 16 (N,2N) CROSS SECTION 4331 1451 121 MT = 17 (N,3N) CROSS SECTION 4331 1451 122 MT = 22 (N,N'A) CROSS SECTION 4331 1451 123 MT = 28 (N,N'P) CROSS SECTION 4331 1451 124 MT = 32 (N,N'D) CROSS SECTION 4331 1451 125 MT = 33 (N,N'T) CROSS SECTION 4331 1451 126 MT =103 (N,P) CROSS SECTION 4331 1451 127 MT =104 (N,D) CROSS SECTION 4331 1451 128 MT =105 (N,T) CROSS SECTION 4331 1451 129 MT =106 (N,HE3) CROSS SECTION 4331 1451 130 MT =107 (N,ALPHA) CROSS SECTION 4331 1451 131 THESE REACTION CROSS SECTIONS WERE CALCULATED WITH THE 4331 1451 132 PREEQUILIBRIUM AND MULTI-STEP EVAPORATION MODEL CODE PEGASUS. 4331 1451 133 4331 1451 134 THE KALBACH'S CONSTANT K (= 101.5) WAS ESTIMATED BY THE 4331 1451 135 FORMULA DERIVED FROM KIKUCHI-KAWAI'S FORMALISM/23/ AND LEVEL 4331 1451 136 DENSITY PARAMETERS. 4331 1451 137 4331 1451 138 FINALLY, THE (N,2N), (N,P) AND (N,ALPHA) CROSS SECTIONS WERE 4331 1451 139 NORMALIZED TO THE FOLLOWING VALUES AT 14.5 MEV: 4331 1451 140 (N,2N) 1230.00 MB (RECOMMENDED BY BYCHKOV ET AL./24/) 4331 1451 141 (N,P) 14.00 MB (RECOMMENDED BY FORREST/25/) 4331 1451 142 (N,ALPHA) 7.00 MB (RECOMMENDED BY FORREST) 4331 1451 143 4331 1451 144 MT = 251 MU-BAR 4331 1451 145 CALCULATED WITH CASTHY. 4331 1451 146 4331 1451 147 MF = 4 ANGULAR DISTRIBUTIONS OF SECONDARY NEUTRONS 4331 1451 148 LEGENDRE POLYNOMIAL COEFFICIENTS FOR ANGULAR DISTRIBUTIONS ARE 4331 1451 149 GIVEN IN THE CENTER-OF-MASS SYSTEM FOR MT=2 AND DISCRETE INELAS-4331 1451 150 TIC LEVELS, AND IN THE LABORATORY SYSTEM FOR MT=91. THEY WERE 4331 1451 151 CALCULATED WITH CASTHY. FOR OTHER REACTIONS, ISOTROPIC DISTRI- 4331 1451 152 BUTIONS IN THE LABORATORY SYSTEM WERE ASSUMED. 4331 1451 153 4331 1451 154 MF = 5 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS 4331 1451 155 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS WERE CALCULATED WITH 4331 1451 156 PEGASUS FOR INELASTIC SCATTERING TO OVERLAPPING LEVELS AND FOR 4331 1451 157 OTHER NEUTRON EMITTING REACTIONS. 4331 1451 158 4331 1451 159 TABLE 1 NEUTRON OPTICAL POTENTIAL PARAMETERS 4331 1451 160 4331 1451 161 DEPTH (MEV) RADIUS(FM) DIFFUSENESS(FM) 4331 1451 162 ---------------------- ------------ --------------- 4331 1451 163 V = 47.5 R0 = 5.972 A0 = 0.62 4331 1451 164 WS = 9.74 RS = 6.594 AS = 0.35 4331 1451 165 VSO= 7.0 RSO= 5.97 ASO= 0.62 4331 1451 166 THE FORM OF SURFACE ABSORPTION PART IS DER. WOODS-SAXON TYPE. 4331 1451 167 4331 1451 168 TABLE 2 LEVEL DENSITY PARAMETERS 4331 1451 169 4331 1451 170 NUCLIDE A(1/MEV) T(MEV) C(1/MEV) EX(MEV) PAIRING 4331 1451 171 --------------------------------------------------------------- 4331 1451 172 41-NB- 95 1.277E+01 7.500E-01 2.121E+00 5.782E+00 1.120E+00 4331 1451 173 41-NB- 96 1.331E+01 5.880E-01 3.406E+00 2.530E+00 0.0 4331 1451 174 41-NB- 97 1.337E+01 6.710E-01 9.771E-01 5.026E+00 1.290E+00 4331 1451 175 41-NB- 98 1.380E+01 5.110E-01 2.350E+00 1.731E+00 0.0 4331 1451 176 4331 1451 177 42-MO- 96 1.403E+01 7.410E-01 6.991E-01 7.645E+00 2.400E+00 4331 1451 178 42-MO- 97 1.517E+01 6.800E-01 2.769E+00 6.036E+00 1.280E+00 4331 1451 179 42-MO- 98 1.594E+01 6.900E-01 7.358E-01 7.888E+00 2.570E+00 4331 1451 180 42-MO- 99 1.774E+01 6.200E-01 4.294E+00 6.058E+00 1.280E+00 4331 1451 181 4331 1451 182 43-TC- 97 1.600E+01 6.700E-01 4.756E+00 6.089E+00 1.120E+00 4331 1451 183 43-TC- 98 1.659E+01 6.120E-01 1.776E+01 4.176E+00 0.0 4331 1451 184 43-TC- 99 1.600E+01 6.550E-01 2.973E+00 5.984E+00 1.290E+00 4331 1451 185 43-TC-100 1.637E+01 5.850E-01 1.189E+01 3.635E+00 0.0 4331 1451 186 --------------------------------------------------------------- 4331 1451 187 4331 1451 188 SPIN CUTOFF PARAMETERS WERE CALCULATED AS 0.146*SQRT(A)*A**(2/3).4331 1451 189 IN THE CASTHY CALCULATION, SPIN CUTOFF FACTORS AT 0 MEV WERE 4331 1451 190 ASSUMED TO BE 7.899 FOR TC- 99 AND 5.0 FOR TC-100. 4331 1451 191 4331 1451 192 REFERENCES 4331 1451 193 1) AOKI, T. ET AL.: PROC. INT. CONF. ON NUCLEAR DATA FOR BASIC 4331 1451 194 AND APPLIED SCIENCE, SANTA FE., VOL. 2, P.1627 (1985). 4331 1451 195 2) KAWAI, M. ET AL.: J. NUCL. SCI. TECHNOL., 29, 195 (1992). 4331 1451 196 3) KIKUCHI, Y. ET AL.: JAERI-M 86-030 (1986). 4331 1451 197 4) FISCHER, P., ET AL.: "PROC. INT. CONF. ON NEUTRON PHYS. AND 4331 1451 198 NUCL. DATA FOR REACTORS AND OTHER APPLIED PURPOSES, HARWELL 4331 1451 199 1978", 718. 4331 1451 200 5) MUGHABGHAB, S.F. ET AL.: "NEUTRON CROSS SECTIONS, VOL. I, 4331 1451 201 PART A", ACADEMIC PRESS (1981). 4331 1451 202 6) ADAMCHUK, JU.V.,ET AL.: IAE-2335 (1973). 4331 1451 203 7) LITTLE, R.C., BLOCK, R.L.: TRANS. AM. NUCL. SOC., 26, 574 4331 1451 204 (1977). 4331 1451 205 8) KIKUCHI, Y.: JAERI-M 6248 (1975). 4331 1451 206 9) MACKLIN, R.L.: NUCL. SCI. ENG., 81, 520 (1982). 4331 1451 207 10) IGARASI, S. AND FUKAHORI, T.: JAERI 1321 (1991). 4331 1451 208 11) IIJIMA, S. ET AL.: JAERI-M 87-025, P. 337 (1987). 4331 1451 209 12) IIJIMA, S. AND KAWAI, M.: J. NUCL. SCI. TECHNOL., 20, 77 4331 1451 210 (1983). 4331 1451 211 13) PEREY, F.G: PHYS. REV. 131, 745 (1963). 4331 1451 212 14) HUIZENGA, J.R. AND IGO, G.: NUCL. PHYS. 29, 462 (1962). 4331 1451 213 15) LOHR, J.M. AND HAEBERLI, W.: NUCL. PHYS. A232, 381 (1974). 4331 1451 214 16) BECCHETTI, F.D., JR. AND GREENLEES, G.W.: POLARIZATION 4331 1451 215 PHENOMENA IN NUCLEAR REACTIONS ((EDS) H.H. BARSHALL AND 4331 1451 216 W. HAEBERLI), P. 682, THE UNIVERSITY OF WISCONSIN PRESS. 4331 1451 217 (1971). 4331 1451 218 17) GILBERT, A. AND CAMERON, A.G.W.: CAN. J. PHYS., 43, 1446 4331 1451 219 (1965). 4331 1451 220 18) IIJIMA, S., ET AL.: J. NUCL. SCI. TECHNOL. 21, 10 (1984). 4331 1451 221 19) GRUPPELAAR, H.: ECN-13 (1977). 4331 1451 222 20) MATSUMOTO, J., ET AL.: JAERI-M 7734 (1978). 4331 1451 223 21) BENZI, V. AND REFFO, G.: CCDN-NW/10 (1969). 4331 1451 224 22) MACKLIN, R.L.: NUCL. SCI. ENG., 81, 520 (1982). 4331 1451 225 23) KIKUCHI, K. AND KAWAI, M.: "NUCLEAR MATTER AND NUCLEAR 4331 1451 226 REACTIONS", NORTH HOLLAND (1968). 4331 1451 227 24) BYCHKOV, V.M. ET AL.: INDC(CCP)-146/LJ (1980). 4331 1451 228 25) FORREST, R.A.: AERE-R 12419 (1986). 4331 1451 229 4331 1451 230 1 451 284 14331 1451 231 2 151 532 24331 1451 232 3 1 25 14331 1451 233 3 2 25 14331 1451 234 3 4 16 14331 1451 235 3 16 9 14331 1451 236 3 17 5 14331 1451 237 3 22 13 14331 1451 238 3 28 11 14331 1451 239 3 32 7 14331 1451 240 3 33 7 14331 1451 241 3 51 16 14331 1451 242 3 52 16 14331 1451 243 3 53 15 14331 1451 244 3 54 13 14331 1451 245 3 55 13 14331 1451 246 3 56 13 14331 1451 247 3 57 12 14331 1451 248 3 58 12 14331 1451 249 3 59 11 14331 1451 250 3 60 11 14331 1451 251 3 91 10 14331 1451 252 3 102 20 14331 1451 253 3 103 14 14331 1451 254 3 104 12 14331 1451 255 3 105 11 14331 1451 256 3 106 10 14331 1451 257 3 107 15 14331 1451 258 3 251 23 14331 1451 259 4 2 243 14331 1451 260 4 16 10 14331 1451 261 4 17 10 14331 1451 262 4 22 10 14331 1451 263 4 28 10 14331 1451 264 4 32 10 14331 1451 265 4 33 10 14331 1451 266 4 51 27 14331 1451 267 4 52 25 14331 1451 268 4 53 27 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296 1.23700+ 2 4.00000+ 0 1.73215- 1 3.21500- 3 1.70000- 1 0.00000+ 04331 2151 297 1.62900+ 2 4.00000+ 0 1.94410- 1 6.11100- 2 1.33300- 1 0.00000+ 04331 2151 298 1.82200+ 2 4.00000+ 0 1.91190- 1 2.11900- 2 1.70000- 1 0.00000+ 04331 2151 299 1.91900+ 2 4.00000+ 0 1.90300- 1 2.03000- 2 1.70000- 1 0.00000+ 04331 2151 300 2.41300+ 2 5.00000+ 0 1.87550- 1 1.75500- 2 1.70000- 1 0.00000+ 04331 2151 301 2.79900+ 2 5.00000+ 0 1.78880- 1 8.88000- 3 1.70000- 1 0.00000+ 04331 2151 302 3.00200+ 2 4.00000+ 0 9.44100- 2 4.66500- 2 4.77600- 2 0.00000+ 04331 2151 303 3.07000+ 2 5.00000+ 0 1.80050- 1 1.00500- 2 1.70000- 1 0.00000+ 04331 2151 304 3.58700+ 2 5.00000+ 0 8.71100- 2 1.40600- 2 7.30500- 2 0.00000+ 04331 2151 305 3.65200+ 2 5.00000+ 0 2.17100- 1 1.63500- 1 5.36000- 2 0.00000+ 04331 2151 306 3.80200+ 2 4.00000+ 0 8.56600- 2 3.68700- 2 4.87900- 2 0.00000+ 04331 2151 307 4.17100+ 2 4.00000+ 0 1.35670- 1 8.63900- 2 4.92800- 2 0.00000+ 04331 2151 308 4.27100+ 2 4.00000+ 0 1.61620- 1 1.12700- 1 4.89200- 2 0.00000+ 04331 2151 309 4.60400+ 2 5.00000+ 0 8.12500- 2 4.72900- 2 3.39600- 2 0.00000+ 04331 2151 310 4.78900+ 2 4.00000+ 0 1.81940- 1 1.19400- 2 1.70000- 1 0.00000+ 04331 2151 311 5.17000+ 2 4.00000+ 0 1.85180- 1 1.51800- 2 1.70000- 1 0.00000+ 04331 2151 312 5.21000+ 2 4.00000+ 0 9.51100- 2 3.28000- 2 6.23100- 2 0.00000+ 04331 2151 313 5.37400+ 2 4.00000+ 0 8.55700- 2 3.87300- 2 4.68400- 2 0.00000+ 04331 2151 314 5.98300+ 2 4.00000+ 0 1.33030- 1 5.99500- 2 7.30799- 2 0.00000+ 04331 2151 315 6.07300+ 2 5.00000+ 0 8.13200- 2 3.81600- 2 4.31600- 2 0.00000+ 04331 2151 316 6.55300+ 2 4.00000+ 0 1.13680- 1 6.07000- 2 5.29800- 2 0.00000+ 04331 2151 317 6.72500+ 2 5.00000+ 0 1.89520- 1 1.95200- 2 1.70000- 1 0.00000+ 04331 2151 318 7.46200+ 2 5.00000+ 0 1.79750- 1 1.18200- 1 6.15500- 2 0.00000+ 04331 2151 319 7.54500+ 2 5.00000+ 0 1.04890- 1 6.00300- 2 4.48600- 2 0.00000+ 04331 2151 320 8.05800+ 2 5.00000+ 0 8.40800- 2 3.83000- 2 4.57800- 2 0.00000+ 04331 2151 321 8.16700+ 2 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