pu-241 jendl-3.2 with covariances 0 0 9.42410+ 4 2.38986+ 2 1 1 0 39443 1451 1 0.00000+ 0 1.00000+ 0 0 0 0 69443 1451 2 1.00000+ 0 2.00000+ 7 0 0 10 39443 1451 3 0.00000+ 0 0.00000+ 0 0 0 461 749443 1451 4 94-PU-241 JAERI EVAL-OCT87 Y.KIKUCHI,N.SEKINE,T.NAKAGAWA 9443 1451 5 DIST-SEP89 REV2-MAY93 9443 1451 6 ----JENDL-3.2 MATERIAL 9443 9443 1451 7 -----INCIDENT NEUTRON DATA 9443 1451 8 ------ENDF-6 FORMAT 9443 1451 9 HISTORY 9443 1451 10 79-10 NEW EVALUATION WAS MADE BY Y.KIKUCHI (JAERI) AND N.SEKINE 9443 1451 11 (HEC) /1/. DATA OF JENDL-1 /2/ WERE SUPERSEDED. 9443 1451 12 79-12 FILES 2, 3 AND 4 WERE RELEASED AS JENDL-2B /3/. 9443 1451 13 87-03 THE FISSION CROSS SECTION WAS REVISED BY ADOPTING RESULTS OF9443 1451 14 SIMULTANEOUS EVALUATION /4/ FOR JENDL-3. 9443 1451 15 89-02 FP YIELDS WERE ADDED. 9443 1451 16 90-07 FP YIELD DATA WERE MODIFIED. 9443 1451 17 93-05 JENDL-3.2. 9443 1451 18 RESOLVED RESONANCE PARAMETERS EVALUATED BY DERRIEN AND 9443 1451 19 DE SAUSSURE/5/ (ADOPTED IN ENDF/B-VI) WERE MODIFIED BY 9443 1451 20 H.DERRIEN (JAERI)/6/. 9443 1451 21 COMPILED BY T.NAKAGAWA (NDC/JAERI) 9443 1451 22 9443 1451 23 ***** MODIFIED PARTS FOR JENDL-3.2 ******************** 9443 1451 24 (2,151) RESOLVED RESONANCE PARAMETERS UP TO 300 EV 9443 1451 25 *********************************************************** 9443 1451 26 01-11 MF31, 32, 33, AND 34 WERE ADDED BY K.SHIBATA. 9443 1451 27 9443 1451 28 9443 1451 29 MF=1 GENERAL INFORMATION 9443 1451 30 MT=451 COMMENT AND DICTIONARY 9443 1451 31 MT=452 NUMBER OF NEUTRONS PER FISSION 9443 1451 32 SUM OF NU-P (MT=456) AND NU-D (MT=455). 9443 1451 33 MT=455 DELAYED NEUTRON DATA 9443 1451 34 DATA OF BENEDETTI+ /7/ 9443 1451 35 MT=456 NUMBER OF PROMPT NEUTRONS PER FISSION 9443 1451 36 DATA OF BOLDEMAN AND FREHAUT /8/ FOR THERMAL FISSION WERE 9443 1451 37 ADOPTED AT LOW ENERGIES BY ASSUMING NU-P(CF-252 SPONTANEOUS 9443 1451 38 FISSION) = 3.753 FOR JENDL-2. FOR JENDL-3, DATA WERE 9443 1451 39 INCREASED BY A FACTOR OF 3.756/3.753. AN ENERGY DEPENDENT 9443 1451 40 TERM WAS BASED ON FREHAUT+ /9/ 9443 1451 41 9443 1451 42 MF=2,MT=151 RESONANCE PARAMETERS 9443 1451 43 RESOLVED RESONANCES : 1 - 300 EV (REICH-MOORE FORMULA) 9443 1451 44 PARAMETERS WERE EVALUATED BY DERRIEN AND DE SAUSSURE/5/, 9443 1451 45 AND MODIFIED BY DERRIEN /6/. DETAILS OF THE MODIFICATION 9443 1451 46 ARE GIVEN IN APPENDIX. 9443 1451 47 9443 1451 48 UNRESOLVED RESONANCES : 300 EV - 30 KEV 9443 1451 49 OBTAINED BY FITTING EVALUATED FISSION AND CAPTURE CROSS 9443 1451 50 SECTIONS. 9443 1451 51 ENERGY DEPENDENT PARAMETERS : SO, S1 AND GAM-F. 9443 1451 52 FIXED PARAMETERS : R=9.8 FM , GAM-G = 0.040 EV, 9443 1451 53 D-OBS = 0.85 EV 9443 1451 54 9443 1451 55 2200-M/SEC CROSS SECTIONS AND CALCULATED RESONANCE INTEGRALS. 9443 1451 56 2200 M/SEC RES. INTEG. 9443 1451 57 TOTAL 1384.9 B - 9443 1451 58 ELASTIC 11.35 B - 9443 1451 59 FISSION 1012.0 B 572.6 B 9443 1451 60 CAPTURE 361.53 B 179.9 B 9443 1451 61 9443 1451 62 MF=3 NEUTRON CROSS SECTIONS 9443 1451 63 ABOVE 300 EV, SMOOTH CROSS SECTIONS WERE GIVEN AS FOLLOWS. 9443 1451 64 BETWEEN 300 EV AND 30 KEV, CROSS SECTIONS WERE REPRESENTED WITH 9443 1451 65 THE UNRESOLVED RESONANCE PARAMETES. 9443 1451 66 9443 1451 67 MT=1, 2, 4, 51-61, 91, 251 : TOTAL, ELASTIC, INELASTIC 9443 1451 68 SCATTERING CROSS SECTIONS AND MU-BAR 9443 1451 69 CALCULATED WITH OPTICAL AND STATISTICAL MODELS. OPTICAL 9443 1451 70 POTENTIAL PARAMETERS USED WERE OBTAINED FROM SYSTEMATICS/10/ 9443 1451 71 V = 40.25 - 0.05*EN , WS = 6.5 , VSO = 7.0 (MEV) 9443 1451 72 R = RSO = 1.32 , RS = 1.38 (FM) 9443 1451 73 A = B = ASO = 0.47 (FM) 9443 1451 74 STATISTICAL MODEL CALCULATION WAS PERFORMED WITH CASTHY CODE 9443 1451 75 /11/. COMPETING PROCESSES (FISSION, (N,2N), (N,3N), (N,4N)) 9443 1451 76 AND LEVEL FLUCTUATION WERE TAKEN INTO THE CALCULATION. THE 9443 1451 77 LEVEL SCHEME TAKEN FROM REF./12/. 9443 1451 78 NO ENERGY(KEV) SPIN-PARITY 9443 1451 79 G.S. 0 5/2 + 9443 1451 80 1 41.8 7/2 + 9443 1451 81 2 94.0 9/2 + 9443 1451 82 3 161.5 1/2 + 9443 1451 83 4 170.8 3/2 + 9443 1451 84 5 223.1 5/2 + 9443 1451 85 6 230.0 9/2 + 9443 1451 86 7 242.7 7/2 + 9443 1451 87 8 300 11/2 + 9443 1451 88 9 335 9/2 + 9443 1451 89 10 368 13/2 + 9443 1451 90 11 445 11/2 - 9443 1451 91 CONTINUUM LEVELS ASSUMED ABOVE 490 KEV. 9443 1451 92 THE LEVEL DENSITY PARAMETERS: GILBERT AND CAMERON /13/. 9443 1451 93 9443 1451 94 MT=16, 17, 37 (N,2N), (N,3N), (N,4N) 9443 1451 95 CALCULATED WITH EVAPORATION MODEL. 9443 1451 96 9443 1451 97 MT=18 FISSION 9443 1451 98 ABOVE 70 KEV, SIMULTANEOUS EVALUATION WITH U-235, U-238, 9443 1451 99 PU-240, PU-241 /4/ WERE ADOPTED. THE EXPERIMENTAL DATA 9443 1451 100 TAKEN INTO ACCOUNT ARE THOSE BY SZABO+ /14,15/, CARLSON+ 9443 1451 101 /16,17/, FURSOV+ /18/AND KEAPPELER+ /19/. BELOW 45 KEV, 9443 1451 102 JENDL-2 WAS ADOPTED. THESE TWO SETS OF DATA WERE CONNECTED9443 1451 103 SMOOTHLY BETWEEN 45 AND 70 KEV. 9443 1451 104 9443 1451 105 MT=102 CAPTURE 9443 1451 106 BASED ON THE DATA OF ALPHA BY WESTON+ /20/ UP TO 250 KEV. 9443 1451 107 CALCULATED WITH CASTHY ABOVE 250 KEV. THE GAMMA-RAY 9443 1451 108 STRENGTH FUNCTION WAS DETERMINED SO THAT THE CAPTURE CROSS9443 1451 109 SECTION WAS 269 MB AT 250 KEV. 9443 1451 110 9443 1451 111 MF=4 ANGULAR DISTRIBUTIONS OF SECONDARY NEUTRONS 9443 1451 112 MT=2, 51-61 : CALCULATED WITH CASTHY. 9443 1451 113 MT=16,17,18,37,91 : ISOTROPIC IN THE LABORATORY SYSTEM. 9443 1451 114 9443 1451 115 MF=5 ENERGY DISTRIBUTIONS OF SECONDARY NEUTRONS 9443 1451 116 MT=16,17,18,37,91 9443 1451 117 CALCULATED WITH PRE-EQUILIBRIUM AND MULTI-STEP EVAPORATION 9443 1451 118 CODE PEGASUS/21/. 9443 1451 119 MT=18 PROMPT FISSION NEUTRON SPECTRUM. 9443 1451 120 DETERMINED FROM Z**2/A SYSTEMATICS BY SMITH ET AL. /22/. 9443 1451 121 MT=455 DELAYED NEUTRON SPECTRUM. 9443 1451 122 EVALUATION BY SAPHIER ET AL. /23/ WAS ADOPTED. 9443 1451 123 9443 1451 124 MF=31 COVARIANCES OF AVERAGE NUMBER OF NEUTRONS PER FISSION 9443 1451 125 MT=452 9443 1451 126 CONSTRUCTED FROM MT=455 AND 456. 9443 1451 127 MT=455 9443 1451 128 BASED ON EXPERIMENTAL DATA. 9443 1451 129 MT=456 9443 1451 130 BASED ON EXPERIMENTAL DATA. A CHI-VALUE WAS 1.06. 9443 1451 131 9443 1451 132 MF=32 COVARIANCES OF RESONANCE PAREMETERS 9443 1451 133 MT=151 9443 1451 134 RESOLVED RESONANCE 9443 1451 135 BASED ON EXPERIMENTAL DATA /6/. 9443 1451 136 UNRESOLVED RESONANCE 9443 1451 137 THE COVARIANCES WERE OBTAINED BY USING KALMAN./24/ 9443 1451 138 9443 1451 139 MF=33 COVARIANCES OF CROSS SECTIONS (REF.24) 9443 1451 140 MT=1 9443 1451 141 THE COVARIANCES WERE OBTAINED BY USING KALMAN. 9443 1451 142 MT=2 9443 1451 143 CONSTRUCTED FROM MT=1, 4, 16, 17, 18, 37, AND 102. 9443 1451 144 MT=4, 51-61, 91 9443 1451 145 THE COVARIANCES WERE OBTAINED BY USING KALMAN /24/. 9443 1451 146 A CHI-VALUE WAS 0.97. 9443 1451 147 MT=16 9443 1451 148 SYSTEMATICS. 9443 1451 149 MT=17 9443 1451 150 SYSTEMATICS. 9443 1451 151 MT=18 9443 1451 152 BASED ON SIMULTANEOUS EVALUATION /4/. 9443 1451 153 MT=37 9443 1451 154 SYSTEMATICS. 9443 1451 155 MT=102 9443 1451 156 THE COVARIANCES WERE OBTAINED BY USING KALMAN /24/. 9443 1451 157 A CHI-VALUE WAS 0.97. 9443 1451 158 9443 1451 159 MF=34 COVARIANCES OF ANGULAR DISTRIBUTIONS (REF.24) 9443 1451 160 MT=2 9443 1451 161 THE COVARIANCES OF P1 COEFFICIENTS WERE OBTAINED BY USING 9443 1451 162 KALMAN. 9443 1451 163 9443 1451 164 9443 1451 165 REFERENCES 9443 1451 166 1) KIKUCHI Y. AND SEKINE N.: JAERI-M 84-111 (1984). 9443 1451 167 2) KIKUCHI Y.: J. NUCL. SCI. TECHNOL., 14, 467 (1977). 9443 1451 168 3) KIKUCHI Y. ET AL.: J. NUCL. SCI. TECHNOL., 17, 567 (1980). 9443 1451 169 4) KANDA Y. ET AL.: 1985 SANTA FE, 2, 1567 (1986). 9443 1451 170 5) DERRIEN H. AND DE SAUSSURE G.: NUCL. SCI. ENG., 106, 415 9443 1451 171 (1990). 9443 1451 172 6) DERRIEN H.: JAERI-M 93-251 (1994). 9443 1451 173 7) BENEDETTI G. ET.AL.: NUCL. SCI. ENG., 80, 379 (1982). 9443 1451 174 8) BOLDEMAN J.W. AND FREHAUT J.: NUCL. SCI. ENG., 76, 49 (1980). 9443 1451 175 9) FREHAUT J. ET.AL.: CEA-R-4626 (1974). 9443 1451 176 10) MATSUNOBU H. ET.AL.: 1979 KNOXVILLE CONF., P.715, NBS SPECIAL 9443 1451 177 PUBLICATION 594 (1980). 9443 1451 178 11) IGARASI S. AND FUKAHORI T.: JAERI 1321 (1991). 9443 1451 179 12) LEDERER C.M. AND SHIRLEY V.S.: TABLE OF ISOTOPES, 7TH ED. 9443 1451 180 (1978). 9443 1451 181 13) GILBERT A. AND CAMERON A.G.W.: CAN. J. PHYS., 43, 1446(1965). 9443 1451 182 14) SZABO I. ET.AL.: CONF-701002, P.257 (1971). 9443 1451 183 15) SZABO I. ET.AL.: 1973 KIEV CONF, VOL.3, P.27 (1973). 9443 1451 184 16) CARLSON G.W. ET AL.: NUCL. SCI. ENG., 63, 149 (1977). 9443 1451 185 17) CARLSON G.W. AND BEHRENS J.W.: NUCL. SCI. ENG., 68, 128 9443 1451 186 (1978). 9443 1451 187 18) FURSOV B.I. ET.AL.: SOV. AT. ENERGY, 44, 262 (1978). 9443 1451 188 19) KAEPPELER F. AND PFLETSCHINGER E.: NUC. SCI. ENG., 51, 124 9443 1451 189 (1973). 9443 1451 190 20) WESTON L.W. AND TODD J.H.: NUCL.SCI.ENG.,65,454 (1978). 9443 1451 191 21) IIJIMA S. ET AL.: JAERI-M 87-025, 337 (1987). 9443 1451 192 22) SMITH A. ET AL.: ANL/NDM-50 (1979). 9443 1451 193 23) SAPHIER D. ET AL.: NUCL. SCI. ENG., 62, 660 (1977). 9443 1451 194 24) SHIBATA K. ET AL.: JAERI-RESEARCH 98-045 (1998). 9443 1451 195 9443 1451 196 9443 1451 197 ================================================================= 9443 1451 198 APPENDIX REVISED RESONANCE DATA ,JAERI MAY 1993 9443 1451 199 ================================================================= 9443 1451 200 9443 1451 201 REVISION OF THE 241PU REICH-MOORE RESONANCE PARAMETERS 9443 1451 202 BY COMPARISON WITH RECENT FISSION CROSS SECTION MEASUREMENTS. 9443 1451 203 9443 1451 204 HERVE DERRIEN 9443 1451 205 JAPANESE ATOMIC ENERGY RESEARCH INSTITUTE 9443 1451 206 9443 1451 207 I-INTRODUCTION. 9443 1451 208 9443 1451 209 THE RESONANCE PARAMETERS OF THE NEUTRON CROSS SECTIONS OF 9443 1451 210 241PU WERE OBTAINED BY DERRIEN AND DE SAUSSURE/1/ IN THE ENERGY 9443 1451 211 RANGE FROM THERMAL TO 300 EV BY A BAYESIAN FIT OF SELECTED 9443 1451 212 EXPERIMENTAL EFFECTIVE TOTAL CROSS SECTIONS, FISSION AND CAPTURE 9443 1451 213 CROSS SECTIONS BY USING THE REICH-MOORE FITTING CODE SAMMY/2/. 9443 1451 214 THE RESULTS OF THIS WORK WERE USED IN THE ENDF/B-VI EVALUATED DATA9443 1451 215 FILE. SOME DIFFICULTIES WERE ENCOUNTERED IN THE NORMALIZATION OF 9443 1451 216 THE EXPERIMENTAL FISSION CROSS SECTIONS DUE TO THE DISCREPANCIES 9443 1451 217 IN THE SHAPE OF THE AVAILABLE EXPERIMENTAL DATA BOTH IN THERMAL 9443 1451 218 AND HIGH ENERGY RANGES. THE CONSISTENCY AMONG THE EXPERIMENTAL 9443 1451 219 DATA BASE COULD NOT BE OBTAINED WITHOUT LARGE RENORMALIZATION AND 9443 1451 220 BACKGROUND CORRECTION PARAMETERS IN THE SAMMY FITS. PARTICULARLY, 9443 1451 221 IT WAS SHOWN THAT THE DISCREPANCY BETWEEN THE FISSION CROSS 9443 1451 222 SECTIONS IN THE THERMAL ENERGY RANGE WAS DUE TO A DEVIATION FROM 9443 1451 223 THE 1/V SHAPE BELOW ABOUT 0.05 EV. 9443 1451 224 NEW FISSION CROSS SECTION MEASUREMENTS WERE RECENTLY 9443 1451 225 PERFORMED BY WAGEMANS ET AL./3,4/ IN THE ENERGY RANGE FROM 0.002 9443 1451 226 EV TO 20 EV IN ORDER TO CHECK THE SHAPE OF THE CROSS SECTION IN 9443 1451 227 THE THERMAL ENERGY RANGE. THEY SHOWED THAT THE SHAPE OF THE 9443 1451 228 FISSION CROSS SECTION WAS CLEARLY COMPATIBLE WITH THE 1/V LAW, IN 9443 1451 229 CONTRADICTION TO ALL THE PREVIOUS MEASUREMENTS REPORTED IN THE 9443 1451 230 LITTERATURE. CONSEQUENTLY, THE NORMALIZATION OF ALL THE PREVIOUS 9443 1451 231 RESULTS USING THE LOW ENERGY REGION COULD BE ERRONEOUS. 9443 1451 232 PARTICULARLY, THE DISCREPANCY OBSERVED IN THE AVERAGE FISSION 9443 1451 233 CROSS SECTION OVER THE 0.26 EV RESONANCE COULD BE DUE TO THE 9443 1451 234 ERRORS OF NORMALIZATION IN THE THERMAL REGION. WAGEMANS ET AL. 9443 1451 235 COMPARED THE ENDF/B-VI DATA TO THEIR NEW RESULTS AND CONCLUDED 9443 1451 236 THAT THE EVALUATED DATA FILES USING THE EVALUATION OF DERRIEN AND 9443 1451 237 DE SAUSSURE SHOULD BE REVISED IN THE ENERGY RANGE UP TO 300 EV. 9443 1451 238 9443 1451 239 II-COMMENTS ON ENDF/B-VI EVALUATION. 9443 1451 240 9443 1451 241 IN THE ENERGY RANGE FROM 0.01 EV TO 3 EV THE NEW DATA OF 9443 1451 242 WAGEMANS ET AL. ARE ON AVERAGE 2.2 % SMALLER THAN ENDF/B-VI. THIS 9443 1451 243 DIFFERENCE IS MAINLY DUE A DIFFERENCE OF 3% BETWEEN THE 1976 DATA 9443 1451 244 OF WAGEMANS ET AL./5/ AND THE NEW VALUES OF WAGEMANS ET AL. THE 9443 1451 245 1976 DATA OF WAGEMANS ET AL. WERE USED IN THE EVALUATION OF 9443 1451 246 DERRIEN AND DE SAUSSURE IN THE LOW ENERGY REGION. 9443 1451 247 IN THE INTERMEDIATE ENERGY RANGE FROM 3 EV TO 12 EV, THE 9443 1451 248 AVERAGE FISSION OF ENDF/B-VI IS IN EXCELLENT AGREEMENT WITH THE 9443 1451 249 NEW DATA OF WAGEMANS ET AL. IN THIS ENERGY RANGE, THE SAMMY FITS 9443 1451 250 OF DERRIEN AND DE SAUSSURE WERE PERFORMED ON THE FISSION CROSS 9443 1451 251 SECTION OF WESTON AND TODD/6/, OF BLONS/7/ AND OF MIGNECO ET 9443 1451 252 AL./8/ WITH AN ADJUSTMENT OF THE NORMALIZATION FACTOR AND OF THE 9443 1451 253 BACKGROUND CORRECTION PARAMETERS OF ALL THE EXPERIMENTAL DATA; THE9443 1451 254 AGREEMENT BETWEEN THE NEW DATA OF WAGEMANS ET AL. AND ENDF/B-VI 9443 1451 255 SHOWS THAT, AT LEAST IN THIS ENERGY RANGE, SAMMY PERFORMED ON THE 9443 1451 256 DATA OF WESTON AND TODD A RENORMALIZATION EQUIVALENT TO THAT 9443 1451 257 RECOMMENDED BY WAGEMANS ET AL./4/. 9443 1451 258 IN THE HIGHER RANGE UP TO 300 EV, THE SAMMY FITS RELIED 9443 1451 259 MAINLY ON THE HIGH RESOLUTION MEASUREMENTS OF BLONS AND OF MIGNECO9443 1451 260 ET AL. FOR THE ACCURATE DETERMINATION OF THE RESONANCE PARAMETERS.9443 1451 261 QUITE LARGE NORMALIZATION COEFFICIENTS AND BACKGROUND CORRECTION 9443 1451 262 PARAMETERS WERE ALSO NEEDED IN THIS ENERGY RANGE TO OBTAIN THE 9443 1451 263 CONSISTENCY BETWEEN THE CALCULATED CROSS SECTIONS AND THE 9443 1451 264 EXPERIMENTAL DATA. HOWEVER, THE RESULT OF THE FITS WAS IN QUITE 9443 1451 265 GOOD AGREEMENT WITH THE DATA OF WESTON AND TODD NORMALIZED TO THE 9443 1451 266 1976 DATA OF WAGEMANS ET AL. IN THE LOW ENERGY REGION,WHICH IS 9443 1451 267 ALSO EQUIVALENT TO THE NORMALIZATION TO THE 1983 DATA OF WAGEMANS 9443 1451 268 ET AL./9/. SINCE THE EARLIER DATA OF WAGEMANS ET AL. SHOULD 9443 1451 269 DECREASE BY 3% TO BE CONSISTENT WITH THE NEW DATA, IT IS LIKELY 9443 1451 270 THAT THE ENDF/B-VI FISSION CROSS SECTION COULD BE TOO LARGE BY 9443 1451 271 ABOUT 3% IN THE ENERGY RANGE ABOVE 12 EV. 9443 1451 272 9443 1451 273 III-REVISION OF THE RESONANCE PARAMETERS. 9443 1451 274 9443 1451 275 AN ACCURATE UP-DATING OF THE 241PU RESONANCE PARAMETERS COULD9443 1451 276 BE OBTAINED BY RENORMALIZING THE FISSION EXPERIMENTAL DATA BASE 9443 1451 277 ACCORDING TO THE NEW DATA OF WAGEMANS ET AL. AND BY RESTARTING THE9443 1451 278 SAMMY FITS OF THE NEW EXPERIMENTAL DATA BASE, INCLUDING THE HIGH 9443 1451 279 RESOLUTION TRANSMISSION DATA OF HARVEY AND SIMPSON/10/. DUE TO 9443 1451 280 LACK OF TIME A NEW SAMMY ANALYSIS WAS PERFORMED ONLY IN THE ENERGY9443 1451 281 RANGE FROM 0.002 EV TO 3 EV. IN THE ENERGY RANGE ABOVE 3 EV THE 9443 1451 282 UP-DATING WAS PERFORMED BY APPLYING SOME SMALL CORRECTIONS TO THE 9443 1451 283 RESONANCE PARAMETERS. 9443 1451 284 THE SAMMY ANALYSIS OF THE NEW WAGEMANS ET AL. DATA WAS 9443 1451 285 PERFORMED ALONG WITH THE TOTAL CROSS SECTION OF YOUNG AND 9443 1451 286 SMITH/11/ IN THE ENERGY RANGE FROM 0.002 EV TO 3 EV, BY STARTING 9443 1451 287 WITH THE ENDF/B-VI RESONANCE PARAMETERS. ONLY THE PARAMETERS OF 9443 1451 288 THE 3+ RESONANCES AT -0.122 EV AND AT 0.265 EV WERE ADJUSTED IN 9443 1451 289 THIS ENERGY RANGE. THE VALUES OF THE CROSS SECTIONS CALCULATED AT 9443 1451 290 0.0253 EV ARE COMPARED TO THE STANDARD DATA/12/ IN TABLE 1. THE 9443 1451 291 AVERAGE TOTAL, FISSION AND CAPTURE CROSS SECTIONS CALCULATED WITH 9443 1451 292 THE NEW RESONANCE PARAMETERS ARE DISPLAYED ON TABLES 2, 3 AND 4 9443 1451 293 WITH THE CORRESPONDING EXPERIMENTAL DATA AND THE VALUES OBTAINED 9443 1451 294 FROM ENDF/B-VI. ONE SHOULD POINT OUT THAT AN ENERGY SHIFT OF 9443 1451 295 DE/E=+0.00384 WAS APPLIED TO THE DATA OF YOUNG AND SMITH IN ORDER 9443 1451 296 TO ACHIEVE A GOOD CONSISTENCY WITH THE ENERGY SCALE OF THE FISSION9443 1451 297 DATA OF WAGEMANS ET AL. OVER THE RESONANCE AT 0.0265 EV. 9443 1451 298 IN THE ENERGY RANGE ABOVE 3 EV THE SMALL CORRECTIONS APPLIED 9443 1451 299 TO THE RESONANCE PARAMETERS RESULT IN A DECREASE OF THE AVERAGE 9443 1451 300 FISSION CROSS SECTION AND IN AN INCREASE OF THE AVERAGE CAPTURE 9443 1451 301 CROSS SECTION, WITH A VARIATION OF THE AVERAGE TOTAL CROSS SECTION9443 1451 302 SMALLER THAN THE ERRORS OF THE EXPERIMENTAL DATA OF HARVEY AND 9443 1451 303 SIMPSON. THE AVERAGE VALUES OF THE FISSION AND CAPTURE CROSS 9443 1451 304 SECTIONS CALCULATED WITH THE NEW RESONANCE PARAMETERS ARE SHOWN IN9443 1451 305 TABLE 5 AND 6 ALONG WITH THE RENORMALIZED FISSION CROSS SECTION OF9443 1451 306 WESTON AND TODD AND THE VALUES CALCULATED FROM ENDF/B-VI. 9443 1451 307 9443 1451 308 IV-CONCLUSION. 9443 1451 309 9443 1451 310 THE RESULTS OF THE RECENT MEASUREMENT OF THE 241PU FISSION 9443 1451 311 CROSS SECTION IN THE ENERGY RANGE FROM 0.002 EV TO 4 EV OF 9443 1451 312 WAGEMANS ET AL. WERE USED IN A NEW EVALUATION OF THE RESONANCE 9443 1451 313 PARAMETERS. THE ACCURACY OF THE CALCULATED CROSS SECTIONS WAS 9443 1451 314 GREATLY IMPROVED IN THE RESONANCE AT 0.265 EV. THE CROSS SECTIONS 9443 1451 315 AVERAGED OVER THIS RESONANCE SHOULD HAVE THE SAME ACCURACY THAN 9443 1451 316 THE STANDARD VALUES AT 0.0253 EV. IN THE HIGH ENERGY REGION UP TO 9443 1451 317 300 EV THE SAMMY ANALYSIS OF THE NEW EXPERIMENTAL DATA BASE 9443 1451 318 OBTAINED BY THE RENORMALIZATION OF THE EXPERIMENTAL DATA IS 9443 1451 319 RECOMMENDED IN ORDER TO IMPROVE THE CORRECTIONS TO THE RESONANCE 9443 1451 320 PARAMETERS PERFORMED IN THE PRESENT WORK. 9443 1451 321 9443 1451 322 9443 1451 323 9443 1451 324 TABLE 1 CROSS SECTIONS AT 0.0253 EV 9443 1451 325 9443 1451 326 ------------------------------------------------------------- 9443 1451 327 PRESENT RESULTS ENDF/B-VI STANDARD/12/ 9443 1451 328 ------------------------------------------------------------- 9443 1451 329 FISSION 1012.50(-0.0%) 1012.68+-6.58 9443 1451 330 CAPTURE 361.52(+0.1%) 361.29+-4.95 9443 1451 331 SCATTERING 11.36(-7.1%) 12.17+-2.62 9443 1451 332 TOTAL 1385.38(-0.1%) 1386.14+-8.64 9443 1451 333 ------------------------------------------------------------- 9443 1451 334 9443 1451 335 9443 1451 336 TABLE 2 THE TOTAL CROSS SECTION INTEGRAL IN THE ENERGY RANGE9443 1451 337 FROM 0.0021 EV TO 3 EV. 9443 1451 338 9443 1451 339 ------------------------------------------------------------------9443 1451 340 ENERGY RANGE PRESENT WORK ENDF/B-VI YOUNG AND SMITH/11/ 9443 1451 341 (EV) (B*EV) (B*EV) (B*EV) 9443 1451 342 ------------------------------------------------------------------9443 1451 343 0.0021-0.020 43.54 43.09(-1.0%) 43.25(-0.7%) 9443 1451 344 0.0200-0.030 14.03 14.02(-0.1%) 14.01(-0.1%) 9443 1451 345 0.0300-0.100 65.09 66.17(+1.7%) 64.99(-0.1%) 9443 1451 346 0.1000-0.500 378.38 385.27(+1.8%) 380.10(+0.4%) 9443 1451 347 0.5000-1.000 29.74 29.41(-1.1%) 31.19(+4.4%) 9443 1451 348 1.0000-3.000 83.36 83.92(+0.7%) 82.50(-1.0%) 9443 1451 349 ------------------------------------------------------------------9443 1451 350 0.0021-3.000 614.14 621.88(+1.3%) 616.04(+0.3%) 9443 1451 351 ------------------------------------------------------------------9443 1451 352 9443 1451 353 9443 1451 354 TABLE 3 THE FISSION CROSS SECTION INTEGRAL IN THE ENERGY 9443 1451 355 RANGE FROM 0.0021 EV TO 3 EV. 9443 1451 356 9443 1451 357 ------------------------------------------------------------------9443 1451 358 ENERGY RANGE THIS WORK ENDF/B-VI WAGEMANS ET AL. WESTON AND TODD9443 1451 359 (EV) (B*EV) (B*EV) (B*EV)/4/ (B*EV)/6/ 9443 1451 360 ------------------------------------------------------------------9443 1451 361 0.0021-0.020 31.06 30.61(-1.5%) 31.09(+0.1%) 9443 1451 362 0.0200-0.030 10.24 10.22(-0.2%) 10.24( 0.0%) 9443 1451 363 0.0300-0.100 49.02 50.02(+2.0%) 48.70(-0.6%) 9443 1451 364 0.1000-0.500 262.76 270.84(+3.1%) 264.58(+0.7%) 262.53(-0.1%) 9443 1451 365 0.5000-1.000 17.93 17.64(-1.6%) 17.60(-1.8%) 17.67(-1.4%) 9443 1451 366 1.0000-3.000 54.88 55.62(+1.3%) 54.40(-0.9%) 55.06(+0.3%) 9443 1451 367 ------------------------------------------------------------------9443 1451 368 0.0021-3.000 425.89 434.95(+2.1%) 426.61(+0.2%) 9443 1451 369 ------------------------------------------------------------------9443 1451 370 0.1000-3.000 335.57 344.10(+2.5%) 336.58(+0.3%) 335.26(-0.1%) 9443 1451 371 ------------------------------------------------------------------9443 1451 372 WESTON AND TODD EXPERIMENTAL DATA WERE NORMALIZED TO WAGEMANS ET 9443 1451 373 AL./4/ IN THE ENERGY RANGE FROM 0.1 EV TO 12 EV (ORIGINAL EXFOR 9443 1451 374 DATA MULTIPLIED BY 0.952). 9443 1451 375 9443 1451 376 9443 1451 377 TABLE 4 THE CAPTURE CROSS SECTION INTEGRAL IN THE ENERGY RANGE9443 1451 378 FROM 0.0021 EV TO 3 EV. 9443 1451 379 9443 1451 380 -------------------------------------------------------------- 9443 1451 381 ENERGY RANGE PRESENT WORK ENDF/B-VI WESTON AND TODD/6/ 9443 1451 382 (EV) (B*EV) (B*EV) (B*EV) 9443 1451 383 -------------------------------------------------------------- 9443 1451 384 0.0021-0.020 12.25 12.28(+0.2%) 9443 1451 385 0.0200-0.030 3.67 3.68(+0.3%) 9443 1451 386 0.0300-0.100 15.28 15.39(+0.7%) 15.27(-0.1%) 9443 1451 387 0.1000-0.500 110.58 109.47(-1.0%) 110.49(-0.1%) 9443 1451 388 0.5000-1.000 5.90 5.87(-0.5%) 6.51 9443 1451 389 1.0000-3.000 7.30 7.14(-2.2%) 8.96 9443 1451 390 -------------------------------------------------------------- 9443 1451 391 0.0021-3.000 154.98 153.83(-0.7%) 9443 1451 392 -------------------------------------------------------------- 9443 1451 393 0.0300-3.000 139.06 137.87(-0.9%) 141.29(+1.6%) 9443 1451 394 -------------------------------------------------------------- 9443 1451 395 WESTON AND TODD EXPERIMENTAL DATA WERE NORMALIZED TO THE CAL- 9443 1451 396 CULATED AVERAGE CAPTURE CROSS SECTION OVER THE RESONANCE AT 9443 1451 397 0.264 EV(ORIGINAL EXFOR DATA MULTIPLIED BY 0.914); IN THE ENERGY9443 1451 398 RANGE FROM 0.5 EV TO 3 EV THE EXPERIMENTAL DATA ARE NOT ACCURATE9443 1451 399 DUE TO LARGE CORRECTIONS FOR THE IMPURITIES. 9443 1451 400 9443 1451 401 9443 1451 402 TABLE 5 THE FISSION CROSS SECTION INTEGRAL IN THE ENERGY RANGE9443 1451 403 FROM 3 EV TO 300 EV. 9443 1451 404 9443 1451 405 ------------------------------------------------------------------9443 1451 406 ENERGY RANGE PRESENT WORK ENDF/B-VI WESTON AND TODD/6/ 9443 1451 407 (EV) (B*EV) (B*EV) (B*EV) 9443 1451 408 ------------------------------------------------------------------9443 1451 409 3- 20 3038.63 3066.37(+0.9%) 3036.23(-0.1%) 9443 1451 410 20- 50 1683.69 1739.68(+3.3%) 1705.50(+1.3%) 9443 1451 411 50-100 1971.15 2030.10(+3.0%) 1931.50(-2.0%) 9443 1451 412 100-200 2554.85 2628.39(+2.9%) 2531.00(-0.9%) 9443 1451 413 200-300 2741.23 2820.75(+2.9%) 2747.00(+0.2%) 9443 1451 414 ------------------------------------------------------------------9443 1451 415 3-300 11989.55 12285.29(+2.5%) 11951.23(-0.3%) 9443 1451 416 ------------------------------------------------------------------9443 1451 417 WESTON AND TODD EXPERIMENTAL DATA WERE NORMALIZED TO WAGEMANS ET 9443 1451 418 AL./4/ IN THE ENERGY RANGE FROM 0.1 EV TO 12 EV (ORIGINAL EXFOR 9443 1451 419 DATA MULTIPLIED BY 0.952). 9443 1451 420 9443 1451 421 9443 1451 422 TABLE 6 THE CAPTURE CROSS SECTION INTEGRAL IN THE ENERGY RANGE9443 1451 423 FROM 3 EV TO 300 EV. 9443 1451 424 9443 1451 425 ------------------------------------------------------------------9443 1451 426 ENERGY RANGE PRESENT WORK ENDF/B-VI WESTON AND TODD/6/ 9443 1451 427 (EV) (B*EV) (B*EV) (B*EV) 9443 1451 428 ------------------------------------------------------------------9443 1451 429 3- 20 1213.07 1138.52(-6.5%) 1192.90(-1.7%) 9443 1451 430 20- 50 330.34 307.48(-7.5%) 338.09(+2.3%) 9443 1451 431 50-100 605.40 585.88(-3.2%) 594.83(-1.8%) 9443 1451 432 100-200 609.83 581.77(-4.8%) 652.68(+7.0%) 9443 1451 433 200-300 684.97 661.12(-3.6%) 700.53(+2.3%) 9443 1451 434 ------------------------------------------------------------------9443 1451 435 3-300 3443.36 3274.77(-5.1%) 3479.04(+1.0%) 9443 1451 436 ------------------------------------------------------------------9443 1451 437 WESTON AND TODD EXPERIMENTAL DATA NORMALIZED TO THE CALCULATED 9443 1451 438 AVERAGE CAPTURE CROSS SECTION OVER THE RESONANCE AT 0.265 EV 9443 1451 439 (ORIGINAL EXFOR DATA MULTIPLIED BY 0.914). 9443 1451 440 9443 1451 441 9443 1451 442 REFERENCES OF APPENDIX 9443 1451 443 1) DERRIEN,H. AND DE SAUSSURE,G.:NUC. SCI. ENG. 106, 415(1990). 9443 1451 444 2) LARSON,N.M. AND PEREY,F.G.:ORNL/TM-9719(1985). 9443 1451 445 3) WAGEMANS,C., SCHILLEBEECKX,P., DERUYTTER,A. AND BARTHELEMY,R.:9443 1451 446 PROC. INT. CONF., PHYSOR 90, MARSEILLE, FRANCE, VOL.1, 9443 1451 447 III-9(1990). 9443 1451 448 4) WAGEMANS,C., SCHILLEBEECKX,P., DERUYTTER,A. AND BARTHELEMY,R.:9443 1451 449 PROC. CONF. ON NUCLEAR DATA FOR SCIENCE AND TECHNOLOGY, JUELICH9443 1451 450 13-17 MAY 1991, P.35(1991). 9443 1451 451 5) WAGEMANS,C. AND DERUYTTER,A.: NUCL. SCI. ENG. 60, 44(1976). 9443 1451 452 6) WESTON,L.W. AND TODD,J.H.: NUCL. SCI. ENG. 65, 454(1978). 9443 1451 453 7) BLONS,J.: NUCL. SCI. ENG. 51, 130(1973). 9443 1451 454 8) MIGNECO,E., THEOBALD,J.P. AND WARTENA,J.A.: PROC. CONF. NUCL.9443 1451 455 DATA FOR REACTORS, HELSINKI, FINLAND, JUNE 15-19, 1970, VOL.I, 9443 1451 456 P.437, IAEA(1970). 9443 1451 457 9) WAGEMANS,C. AND DERUYTTER,A.: PROC. CONF. ON NUCLEAR DATA FOR 9443 1451 458 SCIENCE AND TECHNOLOGY, ANTWERP, BELGIUM, 69(1983). 9443 1451 459 10) HARVEY,J.A. AND SIMPSON,O.D.: OAK-RIDGE NATIONAL 9443 1451 460 LABORATORY(1973), UNPUBLISHED. 9443 1451 461 11) YOUNG,T.B. AND SMITH,J.R.: WASH-1093, P.60(1968). 9443 1451 462 12) CARLSON,A. ET AL.: ENDF/B-VI STANDARD EVALUATION, PRIVATE 9443 1451 463 COMMUNICATION FROM PEELLE,R.W.(1987). 9443 1451 464 9443 1451 465 1 451 537 19443 1451 466 1 452 5 19443 1451 467 1 455 7 19443 1451 468 1 456 3 19443 1451 469 2 151 384 39443 1451 470 3 1 51 19443 1451 471 3 2 50 19443 1451 472 3 4 28 19443 1451 473 3 16 9 19443 1451 474 3 17 7 19443 1451 475 3 18 46 19443 1451 476 3 37 5 19443 1451 477 3 51 28 19443 1451 478 3 52 25 19443 1451 479 3 53 23 19443 1451 480 3 54 23 19443 1451 481 3 55 22 19443 1451 482 3 56 21 19443 1451 483 3 57 21 19443 1451 484 3 58 20 19443 1451 485 3 59 19 19443 1451 486 3 60 19 19443 1451 487 3 61 18 19443 1451 488 3 91 17 19443 1451 489 3 102 28 19443 1451 490 3 251 37 19443 1451 491 4 2 371 19443 1451 492 4 16 10 19443 1451 493 4 17 10 19443 1451 494 4 18 10 19443 1451 495 4 37 10 19443 1451 496 4 51 28 19443 1451 497 4 52 28 19443 1451 498 4 53 28 19443 1451 499 4 54 28 19443 1451 500 4 55 28 19443 1451 501 4 56 28 19443 1451 502 4 57 28 19443 1451 503 4 58 28 19443 1451 504 4 59 28 19443 1451 505 4 60 28 19443 1451 506 4 61 28 19443 1451 507 4 91 10 09443 1451 508 5 16 17 19443 1451 509 5 17 22 19443 1451 510 5 18 8 09443 1451 511 5 37 25 19443 1451 512 5 91 10 19443 1451 513 5 455 250 19443 1451 514 31 452 5 39443 1451 515 31 455 5 39443 1451 516 31 456 8 39443 1451 517 32 151 79 39443 1451 518 33 1 62 39443 1451 519 33 2 12 39443 1451 520 33 4 10 39443 1451 521 33 16 13 39443 1451 522 33 17 8 39443 1451 523 33 18 1246 39443 1451 524 33 37 6 39443 1451 525 33 51 42 39443 1451 526 33 52 35 39443 1451 527 33 53 32 39443 1451 528 33 54 32 39443 1451 529 33 55 29 39443 1451 530 33 56 29 39443 1451 531 33 57 29 39443 1451 532 33 58 29 39443 1451 533 33 59 29 39443 1451 534 33 60 29 39443 1451 535 33 61 26 39443 1451 536 33 91 26 39443 1451 537 33 102 49 39443 1451 538 34 2 148 39443 1451 539 9443 1 099999 9.42410+ 4 2.38986+ 2 0 2 0 09443 1452 1 0.00000+ 0 0.00000+ 0 0 0 1 49443 1452 2 4 2 0 0 0 09443 1452 3 1.00000- 5 2.93130+ 0 5.00000+ 6 3.67680+ 0 7.00000+ 6 3.96811+ 09443 1452 4 2.00000+ 7 5.90641+ 0 9443 1452 5 9443 1 099999 9.42410+ 4 2.38986+ 2 0 2 0 09443 1455 1 0.00000+ 0 0.00000+ 0 0 0 6 09443 1455 2 1.28000- 2 2.99000- 2 1.24000- 1 3.52000- 1 1.61000+ 0 3.47000+ 09443 1455 3 0.00000+ 0 0.00000+ 0 0 0 1 49443 1455 4 4 2 0 0 0 09443 1455 5 1.00000- 5 1.60000- 2 5.00000+ 6 1.60000- 2 7.00000+ 6 9.11000- 39443 1455 6 2.00000+ 7 9.11000- 3 9443 1455 7 9443 1 099999 9.42410+ 4 2.38986+ 2 0 1 0 09443 1456 1 0.00000+ 0 0.00000+ 0 0 0 2 09443 1456 2 2.91530+ 0 1.49100- 7 9443 1456 3 9443 1 099999 9443 0 0 0 9.42410+ 4 2.38986+ 2 0 0 1 09443 2151 1 9.42410+ 4 1.00000+ 0 0 1 2 09443 2151 2 1.00000- 5 3.00000+ 2 1 3 0 09443 2151 3 2.50000+ 0 9.54000- 1 0 0 1 19443 2151 4 2.38986+ 2 0.00000+ 0 0 0 1458 2439443 2151 5 -5.95300+ 1 2.00000+ 0 5.96100- 1 4.45000- 2 4.15300- 1 4.29800- 29443 2151 6 -5.58000+ 0 3.00000+ 0 2.28900- 3 3.64400- 2 1.64800+ 0 1.57600- 29443 2151 7 -1.40500+ 0 3.00000+ 0 1.51300- 6 1.92500- 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7.98800- 3 3.39800- 2 7.37500- 2 2.82900- 29443 2151 21 1.59870+ 1 2.00000+ 0 1.72000- 3 4.00000- 2-4.08300- 1 7.85000- 39443 2151 22 1.66740+ 1 3.00000+ 0 1.07300- 3 3.66400- 2 2.06400- 1 1.54100- 39443 2151 23 1.78530+ 1 3.00000+ 0 2.96600- 3 3.60400- 2 5.95200- 4 1.87300- 29443 2151 24 1.82690+ 1 3.00000+ 0 1.30100- 4 4.09500- 2-3.14800- 2 1.51000- 49443 2151 25 2.07200+ 1 3.00000+ 0 3.45300- 4 3.97500- 2 1.21100- 2 4.40900- 29443 2151 26 2.19210+ 1 3.00000+ 0 9.96900- 5 3.32300- 2-1.17100- 2 0.00000+ 09443 2151 27 2.29950+ 1 3.00000+ 0 7.94200- 4 4.44600- 2 1.98400- 1 3.02700- 29443 2151 28 2.36790+ 1 2.00000+ 0 5.65100- 4 4.18600- 2 3.78800- 1-5.35800- 39443 2151 29 2.41030+ 1 3.00000+ 0 1.14700- 3 4.51600- 2-3.26500- 2-5.79800- 29443 2151 30 2.45290+ 1 2.00000+ 0 2.02000- 4 4.00000- 2 4.18900- 1 0.00000+ 09443 2151 31 2.64290+ 1 2.00000+ 0 5.32400- 3 4.45100- 2 1.04900- 2 2.52000- 19443 2151 32 2.74370+ 1 2.00000+ 0 2.06800- 4 4.00000- 2-4.63200- 1 0.00000+ 09443 2151 33 2.88570+ 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2151 46 4.08070+ 1 2.00000+ 0 2.56400- 3 4.07500- 2-9.96300- 1-1.66400- 29443 2151 47 4.28180+ 1 3.00000+ 0 2.32400- 4 4.53900- 2 1.79600- 1 0.00000+ 09443 2151 48 4.34780+ 1 3.00000+ 0 2.30700- 4 3.08500- 2 0.00000+ 0 2.84400- 29443 2151 49 4.65700+ 1 3.00000+ 0 1.23500- 3 3.85200- 2 0.00000+ 0-2.31300- 19443 2151 50 4.73480+ 1 3.00000+ 0 1.20500- 4 3.92200- 2 7.69900- 2 1.29200- 19443 2151 51 4.81030+ 1 2.00000+ 0 7.15000- 3 4.23700- 2-2.60300- 1 1.94400- 19443 2151 52 5.04050+ 1 3.00000+ 0 5.18300- 4 4.03400- 2 1.49300- 2 2.91700- 19443 2151 53 5.23430+ 1 2.00000+ 0 5.32800- 5 4.09300- 2 3.10400- 2 0.00000+ 09443 2151 54 5.42700+ 1 3.00000+ 0 3.00000- 5 4.04400- 2-1.45500- 2 0.00000+ 09443 2151 55 5.59000+ 1 3.00000+ 0 3.54900- 5 4.04400- 2 0.00000+ 0 1.45500- 29443 2151 56 5.72300+ 1 3.00000+ 0 3.20000- 5 4.01500- 2 4.85000- 3 0.00000+ 09443 2151 57 5.79500+ 1 2.00000+ 0 2.16000- 4 4.43600- 2 1.45500- 1 0.00000+ 09443 2151 58 5.81370+ 1 2.00000+ 0 1.20200- 3 4.00000- 2 1.54100- 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