JAERI ... JENDL High-Energy File (upto 3 GeV) ... Feb. 2004 0 0 0 0 9.423900+4 2.369990+2 1 1 0 19437 1451 1 0.00000+ 0 1.00000+ 0 0 0 0 69437 1451 2 1.000000+0 3.000000+9 0 0 10 19437 1451 3 0.00000+ 0 0.00000+ 0 0 0 953 1289437 1451 4 94-Pu-239 JAERI EVAL-AUG01 T.Fukahori, A.Yu.Konobeyev 9437 1451 5 DIST- REV1- 9437 1451 6 ----JENDL-HE MATERIAL 9437 REVISION 1 9437 1451 7 -----INCIDENT NEUTRON DATA 9437 1451 8 ------ENDF-6 FORMAT 9437 1451 9 9437 1451 10 ************************************************** 9437 1451 11 * * 9437 1451 12 * JENDL-HE HIGH ENERGY FILE * 9437 1451 13 * * 9437 1451 14 ************************************************** 9437 1451 15 9437 1451 16 NEUTRON EVALUATION UP TO 3 GEV 9437 1451 17 __________________________________________________________________9437 1451 18 9437 1451 19 ************************************************** 9437 1451 20 * * 9437 1451 21 * JENDL-HE HIGH ENERGY FILE * 9437 1451 22 * * 9437 1451 23 ************************************************** 9437 1451 24 9437 1451 25 Neutron Evaluation up to 250 MeV 9437 1451 26 9437 1451 27 History 9437 1451 28 87-03 Evaluation was made by 9437 1451 29 M.Kawai and K.Hida(naig) : cross sections above 9437 1451 30 resonance region and other quantities, 9437 1451 31 T.Yoshida(naig) : resonance parameters and background 9437 1451 32 cross sections, 9437 1451 33 Data were compiled by T.Nakagawa (jaeri). 9437 1451 34 88-08 Partly modified. 9437 1451 35 Nu-bar, resolved resons., (n,2n). 9437 1451 36 89-02 FP yields were taken from JNDC FP decay data file version-2.9437 1451 37 89-03 Unresolved resonance parameters were slightly modified. 9437 1451 38 93-02 JENDL-3.2. 9437 1451 39 Resonance parameters evaluated by H.Derrien (jaeri)/1/. 9437 1451 40 Fission spectra calculated by T.Ohsawa (kinki univ.) 9437 1451 41 Compiled by T.Nakagawa (ndc/jaeri) 9437 1451 42 9437 1451 43 ***** modified parts for JENDL-3.2 ******************** 9437 1451 44 (2,151) Resolved resonance parameters up to 2.5 keV 9437 1451 45 (5,18) 9437 1451 46 *********************************************************** 9437 1451 47 9437 1451 48 2000-03 JENDL-3.3 compiled by K.Shibata (jaeri) 9437 1451 49 ***** modified parts for JENDL-3.3 ******************** 9437 1451 50 (1,451), (1,455), (2,151), (3,2), (3,18), (3,102), 9437 1451 51 (5,16), (5,17), (5,91), (5,455) 9437 1451 52 ************************************************************ 9437 1451 53 9437 1451 54 2000-05 Fission spectra were re-evaluated by T.Ohsawa (Kinki U.). 9437 1451 55 JENDL-3.2 was adopted at 14 and 20 MeV. 9437 1451 56 9437 1451 57 2001-06 Fission spectra were replaced with the calculations by 9437 1451 58 Kawano et al./2/ above 10 MeV. 9437 1451 59 9437 1451 60 2001-08 JENDL-HE 9437 1451 61 Prepared by T.Fukahori and A.Yu.Konobeyev 9437 1451 62 9437 1451 63 9437 1451 64 ********************** JENDL-HE ****************************** 9437 1451 65 9437 1451 66 File contains nuclear data for transport, heating, nuclide 9437 1451 67 production and other applications in the entire energy region 9437 1451 68 of primary neutrons from 1E-5 eV to 250 MeV. 9437 1451 69 Below 20 MeV data are taken from JENDL-3.3 file for Pu-239 9437 1451 70 prepared by M.Kawai et al. 9437 1451 71 The evaluation above 20 MeV was performed basing on the 9437 1451 72 modified GNASH code [1] and the available experimental data. 9437 1451 73 The description of nuclear level density was obtained on the 9437 1451 74 basis of the generalized superfluid model [2]. Spin and tempe- 9437 1451 75 rature dependent fission barriers were introduced in the 9437 1451 76 calculation. The nuclear dissipation effects were taken into 9437 1451 77 account according to Ref.[3]. 9437 1451 78 The particle transmission coefficients, total cross-sections, 9437 1451 79 elastic and inelastic scattering angular distributions were 9437 1451 80 obtained with the help of the ECIS code [4]. 9437 1451 81 The fission neutron and gamma-spectra were calculated using 9437 1451 82 the modified ALICE code [5,6] incorporating the fission algorithm 9437 1451 83 [7]. 9437 1451 84 The pre-equilibrium alpha-particle emission spectra were 9437 1451 85 calculated in the framework of coalescence pick-up model [8] 9437 1451 86 combined with the knock-out model [9]. The multiple pre- 9437 1451 87 equilibrium emission was taken into consideration. For deuteron, 9437 1451 88 triton and He-3 spectra calculation the exciton pick-up model 9437 1451 89 [10] was applied. The contribution of the direct mechanism to 9437 1451 90 the deuteron emission was considered on the basis of 9437 1451 91 phenomenological approach [11]. 9437 1451 92 The comments for the evaluated data: 9437 1451 93 9437 1451 94 MF=1 MT=452,456 Total number of neutrons and number of prompt 9437 1451 95 neutrons per fission. 9437 1451 96 Above 20 MeV all prefission neutrons were included in 9437 1451 97 MF=3/6, MT=201 and the corresponding amount was subtracted 9437 1451 98 from the total number of neutrons per fission. It results 9437 1451 99 in the jump in the data of MT=452,456 at 20 MeV, but not 9437 1451 100 in the total neutron production. 9437 1451 101 9437 1451 102 MF=3 MT= 1,2 Total and elastic cross-sections 9437 1451 103 Evalution was performed with the help of the coupled- 9437 1451 104 channels model. 9437 1451 105 9437 1451 106 MF=3 MT=4,16,17,37,102 Nuclear reaction cross-sections 9437 1451 107 Data are cut above 20 MeV and the corresponding nuclide 9437 1451 108 production yields above 20 MeV are written in MF=6, MT=5 9437 1451 109 section. 9437 1451 110 9437 1451 111 MF=3 MT=5 9437 1451 112 Sum of all individual reaction cross-sections except fission9437 1451 113 above 20 MeV. 9437 1451 114 9437 1451 115 MF=3 MT=18 Fission cross-sections 9437 1451 116 Calculated above 20 MeV using GNASH code and slightly 9437 1451 117 changed to fit the available experimental data. 9437 1451 118 9437 1451 119 MF=3 MT=51-68,91 Inelastic scattering cross-sections 9437 1451 120 At the energies above 20 MeV data are included in MF=3/6, 9437 1451 121 MT=201. 9437 1451 122 9437 1451 123 MF=3 MT=201 Neutron production cross-section 9437 1451 124 Data include the contributions of (n,xnypza) reactions as 9437 1451 125 all prefission reactions at the energies above 20 MeV. 9437 1451 126 9437 1451 127 MF=3 MT=202 Gamma production cross-section 9437 1451 128 Data presented are sum of gamma yields for the reactions 9437 1451 129 without fission, prefission reactions and from the 9437 1451 130 fission fragments at the primary energies above 20 MeV. 9437 1451 131 9437 1451 132 MF=3 MT=203-207 p,d,t,He3 and alpha production cross-sections 9437 1451 133 The evaluation was performed beginning from the reaction 9437 1451 134 threshold including the energies below 20 MeV. 9437 1451 135 9437 1451 136 MF=5 MT=16,17,37,91 Energy distributions of secondary neutrons 9437 1451 137 Data above 20 MeV are presented only to complete format 9437 1451 138 data representation. The corresponding cross-sections in 9437 1451 139 file MF=3 have zero values above 20 MeV and the data have 9437 1451 140 no physical meaning. 9437 1451 141 9437 1451 142 MF=5 MT=18 Fission neutron spectra 9437 1451 143 Calculated above 20 MeV with the help of the modified 9437 1451 144 ALICE code. 9437 1451 145 No contribution of prefission neutrons is given at 9437 1451 146 the energies above 20 MeV. These neutrons are included 9437 1451 147 in MF=6, MT=201. 9437 1451 148 9437 1451 149 MF=6 MT=5 9437 1451 150 Yields of the nuclei producing in nuclear reactions. 9437 1451 151 For some reactions (e.g. (n,2n)) the data complete 9437 1451 152 corresponding MF=3, MT-sections. 9437 1451 153 9437 1451 154 MF=6 MT=18 9437 1451 155 Charged particle yields and differential cross-sections 9437 1451 156 for the postfission evaporation 9437 1451 157 9437 1451 158 MF=6 MT=201-207 n,gamma,p,d,t,He3 and alpha-particle double- 9437 1451 159 differential cross-sections 9437 1451 160 Data for neutrons and charged particles presented here 9437 1451 161 do not include the contribution from the postfission 9437 1451 162 evaporation. Data for photons (MT=202) include contribu- 9437 1451 163 tions from all processes. 9437 1451 164 9437 1451 165 MF=12-15 Emitted photon characteristics 9437 1451 166 The values presented at the primary neutron energies 9437 1451 167 above 20 MeV are only to complete format data 9437 1451 168 representation. The corresponding characteristics at the 9437 1451 169 primary neutron energy above 20 MeV are given in MF=6, 9437 1451 170 MT=202. 9437 1451 171 9437 1451 172 9437 1451 173 REFERENCES 9437 1451 174 9437 1451 175 [1] P.G.Young, E.D.Arthur, M.B.Chadwick, Proc. Int. Atomic 9437 1451 176 Energy Workshop on Nuclear Reaction Data and Nuclear 9437 1451 177 Reactors, Trieste, April 15-May 17, 1996, p.227. 9437 1451 178 [2] A.V.Ignatyuk, IAEA-TECDOC-1034, 1998, Chapter 5. 9437 1451 179 [3] E.M.Rastopchin, S.I.Mulgin, Yu.V.Ostapenko, V.V.Pashkevich 9437 1451 180 et al, Sov. J. Nucl. Phys. 53 (1991) 741. 9437 1451 181 [4] J.Raynal, ECIS96 code, unpublished 9437 1451 182 [5] A.Yu.Konobeyev, Yu.A.Korovin, P.E.Pereslavtsev, Code "ALICE/ 9437 1451 183 ASH" for Calculation of Excitation Functions, Energy and An- 9437 1451 184 gular Distributions of Emitted Particles in Nuclear Reacti- 9437 1451 185 ons, Report INPE, Obninsk, February 1997 9437 1451 186 [6] A.I.Dityuk, A.Yu.Konobeyev, V.P.Lunev, Yu.N.Shubin, Report 9437 1451 187 IAEA INDC(CCP)-410, 1998 9437 1451 188 [7] A.Yu.Konobeyev, Yu.A.Korovin, M.Vecchi, Kerntechnik, 64 (1999)9437 1451 189 216. 9437 1451 190 [8] A.Iwamoto, K.Harada, Phys. Rev. C26 (1982) 1821. 9437 1451 191 [9] A.Yu.Konobeyev, V.P.Lunev, Yu.N.Shubin, Acta Physica Slovaca, 9437 1451 192 45 (1995) 705. 9437 1451 193 [10] N.Sato, A.Iwamoto, K.Harada, Phys. Rev. C28 (1983) 1527. 9437 1451 194 [11] A.Yu.Konobeyev, Yu.A.Korovin, Kerntechnik 61 (1996) 45. 9437 1451 195 9437 1451 196 9437 1451 197 *************Comments to JENDL-3.3 ****************************** 9437 1451 198 9437 1451 199 mf=1 General information 9437 1451 200 mt=451 Descriptive data and dictionary 9437 1451 201 mt=452 Number of neutrons per fission 9437 1451 202 Sum of nu-p (mt=456) and nu-d (mt=455). 9437 1451 203 mt=455 delayed neutron data 9437 1451 204 Evaluated data by Tuttle /3/ were adopted. 9437 1451 205 Decay constants were adopted from Keepin et al./4/ 9437 1451 206 mt=456 Number of prompt neutrons per fission 9437 1451 207 Standard Cf-252 sf nu-p was taken to be 3.756. Thermal nu-p 9437 1451 208 was 2.8781 that was a mean value of experimental data. The 9437 1451 209 energy dependent nu-p was obtained from 9437 1451 210 below 10 eV : ref./5/ multiplied by 1.001 9437 1451 211 10 eV 8 MeV 9437 1451 257 Ws = 3.6 + 0.4*En (MeV), En < 7 MeV 9437 1451 258 6.4 + 0.1*(En-7) (MeV), En > 7 MeV 9437 1451 259 Vso = 6.2 (mev) 9437 1451 260 r: rv = 1.26 , rs= 1.24 rso= 1.12 (fm) 9437 1451 261 a: av = 0.615, as= 0.50 , aso= 0.47 (fm) 9437 1451 262 beta-2= 0.21, beta-4= 0.065 9437 1451 263 The compound component was calculated with optical and 9437 1451 264 statistical model code casthy /21/, taking into account 9437 1451 265 level fluctuation and interference effects. The fission, 9437 1451 266 (n,2n), (n,3n), and (n,4n) reactions were considered as 9437 1451 267 competing processes. 9437 1451 268 9437 1451 269 The neutron transmission coefficients for the incident 9437 1451 270 channel were generated with ecis, whereas those for the exit 9437 1451 271 channel were calculated with casthy using spherical optical 9437 1451 272 potential parameters adopted for JENDL-2 evaluation: 9437 1451 273 V = 40.72 - 0.05*En (MeV) 9437 1451 274 Ws = 6.78 - 0.29*En (MeV) 9437 1451 275 Vso= 7.0 (MeV) 9437 1451 276 r = rso= 1.32, rs =1.357 (fm) 9437 1451 277 a = aso= b = 0.47 (fm) 9437 1451 278 The surface absorption is of derivative Woods-Saxon type. 9437 1451 279 The level scheme was taken from ref./22/: 9437 1451 280 no. energy(keV) spin-parity coupled level 9437 1451 281 g.s. 0.0 1/2 + * 9437 1451 282 1 7.86 3/2 + * 9437 1451 283 2 57.28 5/2 + * 9437 1451 284 3 75.71 7/2 + * 9437 1451 285 4 163.76 9/2 + * 9437 1451 286 5 194. 11/2 + * 9437 1451 287 6 285.46 5/2 + 9437 1451 288 7 317. 13/2 + * 9437 1451 289 8 330.13 7/2 + 9437 1451 290 9 360. 15/2 + * 9437 1451 291 10 387.41 9/2 + 9437 1451 292 11 391.6 7/2 - 9437 1451 293 12 435. 9/2 - 9437 1451 294 13 462. 11/2 + 9437 1451 295 14 469.8 1/2 - 9437 1451 296 15 488. 11/2 - 9437 1451 297 16 492.1 3/2 - 9437 1451 298 17 505.5 5/2 - 9437 1451 299 18 511.84 7/2 + 9437 1451 300 9437 1451 301 Continuum levels were assumed above 538 keV. 9437 1451 302 9437 1451 303 mt= 16, 17, 37 (n,2n), (n,3n), and (n,4n) 9437 1451 304 Calculated with a modified version of gnash /23/. The 9437 1451 305 neutron transmission coefficients were generated with ecis 9437 1451 306 /19/ and optical model code eliese-3 /24/, respectively, 9437 1451 307 using the above-mentioned deformed and spherical potentials. 9437 1451 308 The level schemes for pu-236, -237, -238, -239 and -240 were 9437 1451 309 taken from refs. /22,25,26,27,28/. The Gilbert-Cameron's 9437 1451 310 composite formula /29/ was used to represent the level 9437 1451 311 density. Level density parameters were determined from the 9437 1451 312 observed s-wave resonance spacing /30/ and the level schemes.9437 1451 313 the spin cut-off factors in the constant temperature model 9437 1451 314 were represented by Gruppelaar's prescription /31/. 9437 1451 315 9437 1451 316 pu-236 pu-237 pu-238 pu-239 pu-240 9437 1451 317 a (1/MeV) 25.50 28.00 26.23 29.44 26.96 9437 1451 318 t (MeV) 0.442 0.416 0.422 0.398 0.412 9437 1451 319 c (1/MeV) 3.06 14.5 2.88 15.0 3.30 9437 1451 320 E-joint(MeV) 4.71 4.09 4.38 3.97 4.26 9437 1451 321 sigma**2 8.63 8.18 6.47 11.6 9.69 9437 1451 322 no. levels 4.0 19.0 22.0 19.0 28.0 9437 1451 323 E-max (MeV) 0.307 0.4735 1.3103 0.5118 1.2621 9437 1451 324 D-obs (eV) 0.395 10.7 0.383 9.0 2.3 9437 1451 325 Gamma-g(eV) 0.043 0.027 0.043 0.034 0.043 9437 1451 326 9437 1451 327 D-obs of pu-236, -237 and -238 were not available from ref. 9437 1451 328 /30/, and hence the parameters "a" for these nuclei were 9437 1451 329 determined assuming its linear dependence on the mass a: 9437 1451 330 a = 0.365*a - 60.64 for even-even pu isotopes 9437 1451 331 a = 0.659*a - 128.18 for odd-mass pu isotopes 9437 1451 332 which were derived by analyzing the data of pu-241, -242, 9437 1451 333 -243, and -244 as well as pu-239 and -240. Low-lying levels 9437 1451 334 were hardly observed for pu-236 and it was assumed to be 9437 1451 335 identical to that of pu-238 to determine the constant 9437 1451 336 temperature parameters. 9437 1451 337 9437 1451 338 Evaluated fission cross section described below was fed to 9437 1451 339 gnash as a competing process/32/. The preequilibrium process9437 1451 340 was taken into account. Though the parameter f2 was 9437 1451 341 adjusted, the calculated (n,2n) cross section failed to well 9437 1451 342 reproduce the measured data. Therefore, the measured (n,2n) 9437 1451 343 cross section of Frehaut et al./33/ was adopted in place of 9437 1451 344 the calculated one. 9437 1451 345 9437 1451 346 mt=18 Fission 9437 1451 347 Below 30 keV 9437 1451 348 Based on measurements of ref./34/ and ref./35/. 9437 1451 349 Above 30 keV 9437 1451 350 New simultaneous evaluation was performed by 9437 1451 351 Kawano et al./36/ 9437 1451 352 9437 1451 353 mt=102 Capture 9437 1451 354 The cross section in the energy range below 1 MeV was derived9437 1451 355 as a product of the evaluated fission cross section and alpha9437 1451 356 value. The alpha values are identical to those of JENDL-2. 9437 1451 357 Above 1 MeV the results of the statistical model calculation 9437 1451 358 with casthy /21/ linked with ecis /19/ were adopted. The 9437 1451 359 photon strength function was normalized in the casthy 9437 1451 360 calculation so as to reproduce the capture cross section of 9437 1451 361 280 mb at 100 keV. 9437 1451 362 Direct and semi-direct calculations were performed by Kawano 9437 1451 363 /37/ above 500 keV. 9437 1451 364 9437 1451 365 mf=4 Angular distributions of secondary neutrons 9437 1451 366 mt=2,51-68,91 Calculated with ecis /19/ and casthy /21/. 9437 1451 367 mt=16,17,18,37 Isotropic in the laboratory system. 9437 1451 368 9437 1451 369 mf=5 Energy distributions secondary neutrons 9437 1451 370 mt=16,17,37,91 9437 1451 371 Calculated with threshold cross section calculation code 9437 1451 372 pegasus /38/ on the basis of preequilibrium and multi-step 9437 1451 373 evaporation model. 9437 1451 374 Data for mt=16,17,91 were replaced with gnash calculations 9437 1451 375 performed by Kawano/37/. 9437 1451 376 mt=18 9437 1451 377 Distributions were calculated with a modified Madland-Nix 9437 1451 378 model with consideration for multimodal nature of the fission9437 1451 379 process/39,40/. The compound nucleus formation cross sec- 9437 1451 380 tions for fission fragments were calculated using Becchetti- 9437 1451 381 Greenlees potential/41/. Up to 3rd-chance-fission were 9437 1451 382 considered at high incident neutron energies. 9437 1451 383 A preequilibrium emission was taken into account above 10 MeV9437 1451 384 as described in Ref./2/. The prefission neutron spectrum 9437 1451 385 was calculated with the Feshbach-Kerman-Koonin theory /42/. 9437 1451 386 The Ignatyuk formula/43/ were used to generate the level 9437 1451 387 density parameters. 9437 1451 388 Parameters adopted for thermal-neutron fission/40/: 9437 1451 389 (S1: standard-1, S2: standard-2, S3: standard-3 modes) 9437 1451 390 total average fragment kinetic energy 9437 1451 391 = 190.4 MeV for S1 9437 1451 392 = 174.2 MeV for S2 9437 1451 393 = 164.2 MeV for S3 9437 1451 394 average energy release = 205.400 MeV for S1 9437 1451 395 = 196.279 MeV for S2 9437 1451 396 = 182.123 MeV for S3 9437 1451 397 average mass number of light ff = 105 for S1 9437 1451 398 = 99 for S2 9437 1451 399 = 83 for s3 9437 1451 400 average mass number of heavy ff = 135 for S1 9437 1451 401 = 141 for S2 9437 1451 402 = 157 for s3 9437 1451 403 level density of the light ff = 11.236(S1), 9437 1451 404 10.764(S2), 6.669(S3) 9437 1451 405 level density of the heavy ff = 9.577(S1), 9437 1451 406 13.104(S1),16.284(S3) 9437 1451 407 mode branching ratio = 0.248(S1), 0.742(S2), 0.01(S3) 9437 1451 408 These data are essentially based on Schillebeeckx et al. 9437 1451 409 /44/. 9437 1451 410 Note that the parameters vary with the incident energy. 9437 1451 411 Energy-dependent mode branching ratio data of Brosa et al.9437 1451 412 /45/ was used. 9437 1451 413 mt=455 9437 1451 414 Taken from Brady and England /46/. Group abundance parameters9437 1451 415 were adjusted so as to reproduce total delayed neutron 9437 1451 416 emission rate measured by Keepin et al./4/, Besant et al. 9437 1451 417 /47/ and Maksyutenko /48/ 9437 1451 418 9437 1451 419 mf=12 Photon production multiplicities and transition 9437 1451 420 probability arrays 9437 1451 421 mt=16,17,37,91,102 (n,2n),(n,3n),(n,4n),inelastic scattering 9437 1451 422 to the continuum, and capture 9437 1451 423 Data calculated with gnash /23/ were stored under option-1 9437 1451 424 (multiplicities). The photon branching data were taken from9437 1451 425 refs. /22/ and /25,26,27,28/. Some assumptions were made 9437 1451 426 for levels of pu-237 and -239 which had no information on 9437 1451 427 branching: if e1 transitions were allowed to lower levels, 9437 1451 428 the transition probabilities were equally shared among them.9437 1451 429 If not, equally shared collective E2 transitions were 9437 1451 430 assumed. The photon strength functions were represented by 9437 1451 431 the Brink-Axel type giant dipole resonance with conventional9437 1451 432 resonance positions and widths. They were normalized to 9437 1451 433 input values at the thermal energy. The pygmy resonance was9437 1451 434 introduced only for pu-240. The parameters were assumed to 9437 1451 435 be the same as those of u-238 /49/. 9437 1451 436 9437 1451 437 mt=18 Fission 9437 1451 438 Stored under option-1 (multiplicities). The thermal neutron9437 1451 439 induced fission gamma spectrum measured by Verbinski /50/ 9437 1451 440 was adopted and used up to 20 MeV neutron. Since no data 9437 1451 441 were given for the photons below 0.14 MeV, it was assumed to9437 1451 442 be the same as that of the photons between 0.14 and 0.3 MeV.9437 1451 443 9437 1451 444 mt=51-68 Inelastic scattering 9437 1451 445 Stored under option-2 (transition probability arrays). Data9437 1451 446 were taken from ref./22/, and the same assumptions as 9437 1451 447 described above were applied to the levels to which no data 9437 1451 448 were given. 9437 1451 449 9437 1451 450 mf=14 Photon angular distributions 9437 1451 451 mt=16,17,18,37,51-68,91,102 Isotropic. 9437 1451 452 9437 1451 453 mf=15 Continuous photon energy spectra 9437 1451 454 mt=16,17,37,91,102 Calculated with gnash /23/ 9437 1451 455 mt=18 Experimental data by Verbinski /50/ 9437 1451 456 were adopted. 9437 1451 457 9437 1451 458 References 9437 1451 459 1) Derrien H.: J. Nucl. Sci. Technol., 30, 845 (1993). 9437 1451 460 2) Kawano T. et al.: Phys. Rev., C63, 034601 (2001). 9437 1451 461 3) Tuttle R.J.: INDC(NDS)-107/G + special, 29 (1980). 9437 1451 462 4) Keepin G.R. et al.: Phy. Rev., 107, 1044 (1957). 9437 1451 463 5) Gwin R. et al.: Nucl. Sci. Eng., 94, 365 (1986). 9437 1451 464 6) Frehaut J.: NEANDC(E)-238/L (1986). 9437 1451 465 7) Gwin R. et al.: Nucl. Sci. 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Nucl. energy, 7, 495 (1980). 9437 1451 494 36) Kawano T. et al.: JAERI-Research 2000-004 (2000). 9437 1451 495 37) Kawano T.: Private communication (1999). 9437 1451 496 38) Iijima S. et al.: JAERI-M 87-025, p.337 (1987). 9437 1451 497 39) Madland D.G. and Nix J.R.: Nucl. Sci. Eng., 81, 213 (1982). 9437 1451 498 40) Ohsawa, T. et al.: Nucl. Phys. A665, 3 (2000). 9437 1451 499 41) Becchetti Jr.F.D. and Greenlees G.W.: Phys. Rev., 182, 1190 9437 1451 500 (1969). 9437 1451 501 42) Feshbach H., et al.: Ann. Phys. (N.Y.) 125, 429 (1980). 9437 1451 502 43) Ignatyuk A.V.: Sov. J. Nucl. Phys., 29, 450 (1979). 9437 1451 503 44) Schillebeeckx P. et al.: Nucl. Phys. A545, 623 (1992). 9437 1451 504 45) Brosa U. et al.: Phys. Rev. C59, 767 (1999). 9437 1451 505 46) Brady M.C. and England T.R.: Nucl. Sci. Eng., 103, 129 (1989).9437 1451 506 47) Besant C.B. et al.: J. Br. Nucl. Energy Soc., 16, 161 9437 1451 507 (1977) 9437 1451 508 48) Maksyutenko B.P.: Yad. Fiz. 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Rev., C7, 1173 (1973). 9437 1451 512 9437 1451 513 ================================================================= 9437 1451 514 APPENDIX RESONANCE DATA 9437 1451 515 ================================================================= 9437 1451 516 9437 1451 517 THE PRESENT FILE CONTAINS THE RESONANCE PARAMETERS OBTAINED 9437 1451 518 FROM A SAMMY FIT ANALYSIS OF HIGH RESOLUTION EXPERIMENTAL DATA, 9437 1451 519 PERFORMED AT ORNL(OAK RIDGE NATIONNAL LABORATORY,USA) BY H.DERRIEN9437 1451 520 AND G.DE SAUSSURE AND AT JAERI(TOKAI-MURA RESEARCH ESTABLISHMENT, 9437 1451 521 JAPAN) BY H.DERRIEN. 9437 1451 522 THE FILE CONTAINS THREE INDEPENDANT SECTIONS: 9437 1451 523 1/ THE FIRST CORRESPONDS TO THE ENERGY RANGE 0 KEV TO 1 KEV. 9437 1451 524 THE CORRESPONDING SET OF RESONANCE PARAMETRES CONTAINS 398 RESO- 9437 1451 525 NANCES IN THE ENERGY RANGE 0 KEV TO 1 KEV, 4 FICTICIOUS NEGATIVE 9437 1451 526 ENERGY RESONANCES AND 3 FICTICIOUS RESONANCES ABOVE 1 KEV; 9437 1451 527 2/ THE SECOND CORRESPONDS TO THE ENERGY RANGE 1 KEV TO 2 KEV. 9437 1451 528 THE CORRESPONDING SET OF RESONANCE PARAMETERS CONTAINS 435 RESON- 9437 1451 529 ANCES IN THE ENERGY RANGE 0.980 KEV TO 2.02 KEV, 3 FICTICIOUS 9437 1451 530 RESONANCES BELOW 0.9 KEV AND 3 FICTICIOUS RESONANCES ABOVE 2.02 9437 1451 531 KEV; 9437 1451 532 3/ THE THIRD CORRESPONDS TO THE ENERGY RANGE 2 KEV TO 2.5 KEV. 9437 1451 533 THE CORRESPONDING SET OF RESONANCE PARAMETERS CONTAINS 218 RESO- 9437 1451 534 NANCES IN THE ENERGY RANGE 1.98 KEV TO 2.53 KEV, 3 FICTICIOUS 9437 1451 535 RESONANCES BELOW 1.98 KEV AND 3 FICTICIOUS RESONANCES ABOVE 2.53 9437 1451 536 KEV. 9437 1451 537 IN ALL SECTIONS THE FICTICIOUS RESONANCE PARAMETERS TAKE INTO 9437 1451 538 ACCOUNT THE CONTRIBUTION OF ALL THE EXTERNAL TRUNCATED RESONANCES 9437 1451 539 IN SUCH A WAY THAT NO TOTAL, SCATTERING, FISSION AND CAPTURE 9437 1451 540 SMOOTH FILES ARE NEEDED IN THE CORRESPONDING ENERGY RANGES FOR THE9437 1451 541 REPRODUCTION OF THE CROSS SECTIONS WITHIN THE EXPERIMENTAL ERRORS.9437 1451 542 THE FOLLOWING EXPERIMENTAL DATA BASE HAS BEEN USED IN THE SAMMY9437 1451 543 FITS: 9437 1451 544 -ABSORPTION AND FISSION FROM R.GWIN ET AL./1,2/; 9437 1451 545 -FISSION FROM R.GWIN ET AL./3,4/, J.BLONS/5/, L.W.WESTON ET 9437 1451 546 AL./6,7/; 9437 1451 547 -TRANSMISSION FROM R.R.SPENCER ET AL./8/, J.A.HARVEY ET AL./9/ 9437 1451 548 PRIOR TO THE FITS THE EXPERIMENTAL FISSION AND ABSORPTION CROSS 9437 1451 549 SECTIONS WERE NORMALISED, DIRECTLY OR INDIRECTLY TO THE 0.0253 EV 9437 1451 550 VALUES OBTAINED BY THE ENDF/B-VI STANDARD EVALUATION GROUP/10/. 9437 1451 551 THE TRANSMISSION DATA WERE CONSIDERED AS ACCURATE ABSOLUTE MEASU- 9437 1451 552 REMENTS(R.R.SPENCER TOTAL CROSS SECTION AT 0.0253 EV IS 1025.0 B 9437 1451 553 IN EXCELLENT AGREEMENT WITH THE 1027.3 B STANDARD VALUE). 9437 1451 554 DETAILS ON THE ANALYSIS ARE FOUND IN REFERENCES/11,12,13/ 9437 1451 555 9437 1451 556 ***************************************************************** 9437 1451 557 COMMENTS ON THE THERMAL AND LOW ENERGY RANGES 9437 1451 558 ***************************************************************** 9437 1451 559 9437 1451 560 THE THERMAL CROSS SECTION VALUES CALCULATED AT 293 K BY THE 9437 1451 561 RESONANCE PARAMETERS OF THE FIRST SECTION ARE GIVEN IN THE FOLLO- 9437 1451 562 WING TABLE: 9437 1451 563 9437 1451 564 9437 1451 565 SAMMY RESENDD PROPOSED 9437 1451 566 293 K (BARN) STANDARD VALUES(BARN)/10/ 9437 1451 567 **************************************************************** 9437 1451 568 FISSION 747.64 747.90 747.99+-1.87 9437 1451 569 CAPTURE 271.10 270.73 271.43+-2.14 9437 1451 570 SCATTERING 7.97 7.99 7.88+-0.97 9437 1451 571 TOTAL 1026.71 1026.62 1027.30+-5.00 9437 1451 572 **************************************************************** 9437 1451 573 9437 1451 574 ONE SHOULD NOTE THAT THE 293 K CROSS SECTIONS CALCULATED AT 9437 1451 575 0.0253 EV DEPEND ON THE WAY THE DOPPLER BROADENING CALCULATION IS 9437 1451 576 PERFORMED. FOR INSTANCE USING A GAUSSIAN BROADENING FUNCTION WILL 9437 1451 577 GIVE A FISSION CROSS SECTION ABOUT 2.5 BARNS LARGER THAN THE ONE 9437 1451 578 OBTAINED FROM THE ACCURATE CALCULATION WHICH CONSERVES THE 1/V 9437 1451 579 SHAPE OF THE THERMAL CROSS SECTION. THE VALUES GIVEN IN THE TABLE 9437 1451 580 ABOVE WERE OBTAINED FROM SAMMY (LEAL-HWANG METHOD)/14,15/ AND FROM9437 1451 581 RESENDD WITH 0.1% FOR THE INTERPOLATION ACCURACY/16/. 9437 1451 582 THE FOLLOWING TABLE SHOWS EXPERIMENTAL CROSS SECTIONS AVE- 9437 1451 583 RAGED OVER THE ENERGY RANGES 0.02 EV TO 0.06 EV AND 0.02 EV TO 9437 1451 584 0.65 EV, COMPARED TO THE CALCULATED VALUES: 9437 1451 585 9437 1451 586 9437 1451 587 AVERAGE CROSS-SECTIONS(BARN) 9437 1451 588 **************************************************************** 9437 1451 589 REFERENCES(1-10) 0.02 TO 0.06 EV 0.02 TO 0.65 EV 9437 1451 590 **************************************************************** 9437 1451 591 EXP CALC (293K) EXP CALC (293K) 9437 1451 592 GWIN71 FISS 631.41 843.71 9437 1451 593 GWIN76 FISS 631.41 838.39 9437 1451 594 GWIN84 FISS(*) 631.41 631.75(+0.05%) 837.18 838.69(+0.18%) 9437 1451 595 DERUYTER70 FISS 631.41 859.43 9437 1451 596 WAGEMANS80 FISS 631.41 862.56 9437 1451 597 WAGEMANS88 FISS 631.41 841.80 9437 1451 598 GWIN71 CAPTURE 243.84 243.22(-0.25%) 524.75 518.13(-1.26%) 9437 1451 599 GWIN76 ABSORPT(*) 875.90 874.29(-0.18%) 1359.96 1357.14(-0.21%) 9437 1451 600 SPENCER84 TOT(*) 883.20 882.86(-0.04%) 1361.69 1367.6 (+0.43%) 9437 1451 601 **************************************************************** 9437 1451 602 (*)THESE DATA HAD THE LARGIEST WEIGHT IN THE THERMAL FIT. THE VA- 9437 1451 603 LUES BETWEEN THE PARENTHESES GIVE THE PERCENTAGE DEVIATION BETWEEN9437 1451 604 THE CALCULATED DATA AND THE EXPERIMENTAL DATA. 9437 1451 605 ***************************************************************** 9437 1451 606 9437 1451 607 THE VALUE OF 631.4 BARNS FOR ALL THE AVERAGED EXPERIMENTAL 9437 1451 608 FISSION CROSS SECTIONS IN THE ENERGY RANGE 0.02 EV TO 0.06 EV 9437 1451 609 CORRESPONDS TO THE RENORMALISATION OF THE FISSION EXPERIMENTS TO 9437 1451 610 748.0+-1. BARNS AT 0.0253 EV. ORNL DATA ARE CONSISTENT WITHIN 0.8%9437 1451 611 OVER THE ENERGY RANGE 0.02 EV TO 0.65 EV (I.E. OVER THE 0.3 EV 9437 1451 612 RESONANCE). DERUYTER 1970 AND WAGEMANS 1980 DATA ARE ABOUT 2.5% 9437 1451 613 LARGER AND WERE NOT INCLUDED IN THE SAMMY FIT. WHEN NORMALIZED ON 9437 1451 614 THE STANDARD VALUE AT 0.0253 EV, GWIN 76 ABSORPTION AGREES WITH 9437 1451 615 THE ABSORPTION OBTAINED FROM SPENCER TOTAL CROSS SECTION WITHIN 9437 1451 616 0.7% OVER THE 0.3 EV RESONANCE. THE PRESENT EVALUATION IS 9437 1451 617 ESSENTIALLY THE RESULT OF A CONSISTENT SAMMY ANALYSIS OF ALL THE 9437 1451 618 AVAILABLE ORNL DATA WITH A LARGER WEIGHT ON GWIN 1984 FISSION, 9437 1451 619 GWIN 1976 ABSORPTION AND SPENCER TRANSMISSION DATA. 9437 1451 620 AFTER RENORMALIZATION OF THE CALCULATED FISSION CROSS SECTION9437 1451 621 ON THE PRELIMINARY 1991 WESTON AND TODD FISSION DATA(SEE NEXT 9437 1451 622 SECTION) A SLIGHT ADJUSTMENT OF THE NEGATIVE RESONANCE PARAMETERS 9437 1451 623 WAS PERFORMED TO KEEP THE VALUES CALCULATED AT 0.0253 EV IN CLOSE 9437 1451 624 AGREEMENT WITH THE STANDARD VALUES. THE 1988 DATA OF WAGEMANS ET 9437 1451 625 AL./17/ AGREE WITHIN 0.4% WITH THE CALCULATED VALUES OVER THE 9437 1451 626 ENERGY RANGE FROM 0.02 EV TO 0.65 EV AFTER ADJUSTMENT OF THE 9437 1451 627 ENERGY SCALE TO THE ORNL SCALE (THE DIFFERENCE WAS 0.27 EV AT 20 9437 1451 628 EV BETWEEN 1988 WAGEMANS AND ORNL SAMMY FIT ENERGY SCALES). 9437 1451 629 9437 1451 630 ***************************************************************** 9437 1451 631 COMMENTS ON THE 0 KEV TO 1 KEV ENERGY RANGE. 9437 1451 632 ***************************************************************** 9437 1451 633 9437 1451 634 AT THE END OF 1987, AN ANALYSIS WAS COMPLETED UP TO 1 KEV. IN A9437 1451 635 PRELIMINARY STEP, A CORRELATED FIT OF HARVEY TRANSMISSION DATA, 9437 1451 636 WESTON 84 FISSION DATA AND BLONS FISSION DATA WAS PERFORMED, WITH 9437 1451 637 POSSIBLE ADJUSTMENT OF THE NORMALIZATION COEFFICIENTS AND OF THE 9437 1451 638 BACKGROUND CORRECTIONS. THIS PRELIMINARY STEP HAS SHOWN THAT THIS 9437 1451 639 ADJUSTMENT WAS NOT NECESSARY TO HAVE CONSISTENCY BETWEEN HARVEY 9437 1451 640 DATA AND WESTON DATA. BLONS DATA NEEDED A LARGE READJUSTMENT OF 9437 1451 641 THE BACKGROUND AND OF THE NORMALIZATION. THEREFORE, THE FINAL FIT 9437 1451 642 WAS PERFORMED ONLY ON HARVEY TRANSMISSION DATA, GWIN 84 FISSION 9437 1451 643 DATA (BELOW 30 EV) AND WESTON 84 FISSION DATA, WITH NO BACKGROUND 9437 1451 644 AND NORMALISATION ADJUSTMENT. BLONS DATA, WHICH HAVE BETTER 9437 1451 645 RESOLUTION THAN WESTON 84 DATA, WERE USED ONLY TO OBTAIN MORE 9437 1451 646 ACCURATE FISSION WIDTHS OF SOME NARROW RESONANCES IN THE HIGH 9437 1451 647 ENERGY RANGE. 9437 1451 648 IN 1989, PRELIMINARY RESULTS OF THE 1988 WESTON FISSION 9437 1451 649 MEASUREMENT/7/ WERE INCLUDED IN THE SAMMY EXPERIMENTAL DATA 9437 1451 650 BASE. ONE EXPECTED FROM THIS MEASUREMENT, WHICH WAS PERFORMED BY 9437 1451 651 USING A 86 M FLIGHT PATH WITH A RESOLUTION COMPARABLE TO THE 9437 1451 652 RESOLUTION OF HARVEY TRANSMISSION, A CONFIRMATION OF THE EXCELLENT9437 1451 653 QUALITY OF THE 1984 MEASUREMENT. A CONSISTENT SAMMY FIT OF HARVEY 9437 1451 654 TRANSMISSION, WESTON 84 FISSION AND PRELIMINARY WESTON 88 FISSION 9437 1451 655 WAS RESTARTED FROM THE PARAMETER AND COVARIANCE FILES OBTAINED IN 9437 1451 656 1987. IT APPEARED THAT LARGE BACKGROUND AND NORMALISATION 9437 1451 657 CORRECTIONS WERE NEEDED ON THE NEW WESTON FISSION TO OBTAIN 9437 1451 658 CONSISTENCY WITH HARVEY TRANSMISSION DATA. THESE CORRECTIONS WERE 9437 1451 659 COMPARABLE TO THOSE FOUND ON BLONS DATA AND WERE NOT UNDERSTOOD BY9437 1451 660 THE AUTHORS OF THE EXPERIMENT. THE LAST SAMMY RUNS WERE PERFORMED 9437 1451 661 BY NOT ALLOWING BACKGROUND AND NORMALIZATION VARIATIONS ON HARVEY 9437 1451 662 TRANSMISSION AND WESTON 84 FISSION(VERY SMALL ERROR BARS WERE 9437 1451 663 ASSIGNED TO THE CORRESPONDING PARAMETERS IN THE COVARIANCE MATRIX)9437 1451 664 AND BY ALLOWING THESE VARIATIONS ON WESTON 88 DATA. A NEW SET OF 9437 1451 665 RESONANCE PARAMETERS WAS OBTAINED,WHICH WAS IMPROVED COMPARED TO 9437 1451 666 THE PREVIOUS SET DUE TO THE VERY HIGH RESOLUTION OF THE NEW WESTON9437 1451 667 FISSION MEASUREMENT. 9437 1451 668 THE CALCULATED AVERAGE FISSION CROSS SECTION IN THE ENERGY 9437 1451 669 RANGE FROM 0.1 KEV TO 1.0 KEV WAS 3.7% SMALLER THAN THE VALUES 9437 1451 670 OBTAINED BY THE ENDF/B-VI STANDARD EVALUATION GROUP, DUE TO THE 9437 1451 671 FACT THAT WESTON 84 DATA WERE 3.1% LOWER THAN THE AVERAGE STANDARD9437 1451 672 VALUE. A NEW MEASUREMENT WAS PERFORMED BY WESTON AND TODD IN 1991 9437 1451 673 /18/ IN ORDER TO CHECK THEIR 1984 DATA. A CAREFUL NORMALIZATION 9437 1451 674 OF THE DATA IN THE THERMAL ENERGY RANGE SHOWED THAT THE 1984 DATA 9437 1451 675 SHOULD BE RENORMALIZED BY ABOUT +3%. TO TAKE INTO ACCOUNT THIS 9437 1451 676 RENORMALIZATION, THE 1989 RESONANCE PARAMETERS WERE MODIFIED AT 9437 1451 677 JAERI/13/ IN THE FOLLOWING WAY: 9437 1451 678 1/ INCREASE OF THE FISSION WIDTH BY 3% AND DECREASE OF THE 9437 1451 679 CAPTURE WIDTH BY A QUANTITY EQUAL TO THE VARIATION OF THE FISSION 9437 1451 680 WIDTH, IN THE NARROW RESONANCES(MAINLY 1+ RESONANCES); THAT DOES 9437 1451 681 NOT MODIFY THE TOTAL CROSS SECTION IN THE CORRESPONDING 9437 1451 682 RESONANCES; 9437 1451 683 2/ ADJUSTMENT OF THE NEUTRON WIDTH OF THE 0+ RESONANCES BY A 9437 1451 684 REFIT OF THE TRANSMISSION DATA AND OF THE RENORMALIZED WESTON AND 9437 1451 685 TODD 1984 DATA IN ENERGY RANGES WHERE THE CONTRIBUTION OF THE 0+ 9437 1451 686 RESONANCES IS DOMINANT, AND INCREASE OF THE OTHER(SMALL) 0+ 9437 1451 687 NEUTRON WIDTHS BY 3%. NO SEVERE INCONSISTENCY WAS OBSERVED BETWEEN9437 1451 688 THE TRANSMISSION DATA AND THE NEW FISSION DATA OVER THE DOMINANT 9437 1451 689 0+ RESONANCES;THE DIFFERENCES BETWEEN THE 1989 FITS OF THE TRANS- 9437 1451 690 MISSION AND THE NEW FITS WERE CONSISTENT WITHIN THE EXPERIMENTAL 9437 1451 691 ERROR BARS. 9437 1451 692 THE FOLLOWING TABLE SHOWS THE FISSION CROSS SECTIONS CALCULA- 9437 1451 693 TED FROM THE RESONANCE PARAMETERS, THE EXPERIMENTAL VALUES AND THE9437 1451 694 RESULTS OF THE ENDF/B-VI STANDARD EVALUATION GROUP AVERAGED IN THE9437 1451 695 SAME ENERGY INTERVALS. WESTON 1991 DATA ARE PRELIMINARY. WESTON 9437 1451 696 1984 DATA ARE NORMALIZED ON PRELIMINARY WESTON 1991: 9437 1451 697 9437 1451 698 CROSS-SECTIONS(BARN) 9437 1451 699 ************************************************* 9437 1451 700 ENERGY CALCUL WESTON WESTON STANDARD 9437 1451 701 (EV) 1991 1984 9437 1451 702 ************************************************* 9437 1451 703 0.010-10. 80.12 79.98 9437 1451 704 9-20 94.74 94.91 9437 1451 705 20-40 17.52 17.76 17.97 9437 1451 706 40-60 50.64 50.90 50.87 9437 1451 707 60-100 54.42 54.38 54.33 9437 1451 708 100-200 18.63 18.59 18.56 18.66 9437 1451 709 200-300 17.85 17.89 17.88 9437 1451 710 300-400 8.31 8.34 8.43 9437 1451 711 400-500 9.59 9.58 9.57 9437 1451 712 ------------------------------------------------- 9437 1451 713 200-500 11.92 11.93 11.93 11.96 9437 1451 714 ------------------------------------------------- 9437 1451 715 500-600 15.39 15.57 15.86 9437 1451 716 600-700 4.37 4.30 4.46 9437 1451 717 700-800 5.51 5.53 5.63 9437 1451 718 800-900 4.84 4.89 4.98 9437 1451 719 900-1000 8.33 8.38 8.30 9437 1451 720 ------------------------------------------------- 9437 1451 721 500-1000 7.69 7.73 7.73 7.79 9437 1451 722 ------------------------------------------------- 9437 1451 723 20-1000 13.09 13.11 13.11 9437 1451 724 ************************************************** 9437 1451 725 9437 1451 726 9437 1451 727 GWIN 1971 AND 1976 ABSORPTION DATA WERE NOT INCLUDED IN THE 9437 1451 728 SAMMY FIT IN THE ENERGY RANGE ABOVE 1 EV. ACCURATE ABSORPTION 9437 1451 729 CROSS SECTIONS SHOULD BE CALCULATED FROM THE PARAMETERS OBTAINED 9437 1451 730 FROM THE ANALYSIS OF THE TRANSMISSION AND FISSION DATA. THE FOLLO-9437 1451 731 WING TABLE SHOWS THE CALCULATED AVERAGE VALUES OF THE CAPTURE, AB-9437 1451 732 SORPTION AND ALPHA COMPARED TO GWIN 1971 AND GWIN 1976 DATA. THE 9437 1451 733 CALCULATIONS WERE PERFORMED WITH RESENDD, 1.0 % ACCURACY: 9437 1451 734 9437 1451 735 CROSS-SECTIONS(BARN) 9437 1451 736 ******************************************************* 9437 1451 737 ENERGY(EV) CALC. VALUES (293K) GWIN DATA 9437 1451 738 ******************************************************* 9437 1451 739 CAPT ABSORP ALPHA ABSORP ALPHA 9437 1451 740 7.3- 16.0 76.61 196.04 0.64 208.00 0.74(*) 9437 1451 741 16.0- 37.5 20.51 44.55 0.85 46.50 0.89(*) 9437 1451 742 37.5- 50.0 48.72 70.00 2.29 83.15 2.96(*) 9437 1451 743 50.0-100.0 33.60 92.13 0.57 92.84 0.63 9437 1451 744 100.0-200.0 15.58 34.29 0.83 33.66 0.87 9437 1451 745 200.0-300.0 15.85 33.68 0.89 34.69 0.94 9437 1451 746 300.0-400.0 9.69 18.01 1.16 18.31 1.16 9437 1451 747 400.0-500.0 3.96 13.56 0.41 13.56 0.44 9437 1451 748 500.0-600.0 10.87 26.30 0.70 26.54 0.72 9437 1451 749 600.0-700.0 6.53 10.90 1.49 11.57 1.54 9437 1451 750 700.0-800.0 4.95 10.47 0.90 10.52 0.97 9437 1451 751 800.0-900.0 3.65 8.50 0.75 9.30 0.82 9437 1451 752 900.0-999.9 5.06 13.51 0.60 13.23 0.70 9437 1451 753 ****************************************************** 9437 1451 754 (*) GWIN 1971 DATA 9437 1451 755 9437 1451 756 IF ONE EXCEPTS THE ENERGY RANGE 37.5-50 EV, THE CALCULATED AB- 9437 1451 757 SORPTION VALUES AGREE WELL WITH GWIN EXPERIMENTAL DATA; THEY ARE 9437 1451 758 ON AVERAGE 1.2% LOWER IN THE ENERGY RANGE FROM 50 EV TO 1000 EV. 9437 1451 759 9437 1451 760 ***************************************************************** 9437 1451 761 COMMENTS ON THE 1 KEV TO 2 KEV ENERGY RANGE 9437 1451 762 ***************************************************************** 9437 1451 763 9437 1451 764 PRELIMINARY RESONANCE PARAMETERS WERE OBTAINED IN 1989 FROM THE9437 1451 765 ANALYSIS OF THE HARVEY THICK SAMPLE TRANSMISSION DATA AND OF THE 9437 1451 766 PRELIMINARY RESULTS OF WESTON 88 FISSION MEASUREMENT. DUE TO LACK9437 1451 767 OF TIME, THE MEDIUM AND THIN SAMPLE TRANSMISSION DATA WERE NOT 9437 1451 768 INCLUDED IN THE SAMMY DATA BASE, AND THE CONTRIBUTION OF THE 9437 1451 769 TRUNCATED EXTERNAL RESONANCES WAS NOT CAREFULLY INVESTIGATED. 9437 1451 770 NEVERTHELESS, THE RESULTS WERE USED IN THE ENDF/B-VI FILE, ALONG 9437 1451 771 WITH A SMOOTH FILE IN ORDER TO AGREE WITH THE AVERAGE VALUES OF A 9437 1451 772 PREVIOUS ENDF/B-VI EVALUATION (THIS PRELIMINARY SET OF PARAMETERS 9437 1451 773 WAS CONSIDERED AS MORE USEFUL THAN THE STATISTICAL PARAMETERS IN 9437 1451 774 THE ENERGY RANGE 1 KEV TO 2 KEV FOR THE CALCULATION OF THE SELF- 9437 1451 775 SHIELDING FACTORS). 9437 1451 776 THE ANALYSIS WAS RESTARTED IN APRIL 1991 AT JAERI(TOKAI 9437 1451 777 RESEARCH ESTABLISHMENT) WITH AN UPDATED VERSION OF SAMMY ADAPTED 9437 1451 778 BY T.NAKAGAWA TO THE FACOM 780. THE PRELIMINARY SET OF PARAMETERS 9437 1451 779 OBTAINED AT OAK RIDGE IN 1989 WAS USED AS PRIOR INFORMATIONS TO 9437 1451 780 START THE SAMMY CALCULATIONS. ALSO PRIOR TO THE ANALYSIS, THE CON-9437 1451 781 TRIBUTION OF THE EXTERNAL RESONANCES WAS CALCULATED BY USING THE 9437 1451 782 SET OF THE 0 KEV TO 1 KEV KNOWN RESONANCES, SHIFTED IN THE ENERGY 9437 1451 783 RANGES -1 KEV TO 0 KEV, 2 KEV TO 3KEV AND 3 KEV TO 4 KEV; EQUIVA- 9437 1451 784 LENT CONTRIBUTION WAS OBTAINED BY USING 3 FICTICIOUS RESONANCES 9437 1451 785 BELOW 1 KEV AND 3 FICTICIOUS RESONANCES ABOVE 2 KEV(SEE DETAILS IN9437 1451 786 REF./13/). THE ANALYSIS WAS PERFORMED ON THE THICK AND MEDIUM 9437 1451 787 SAMPLE TRANSMISSIONS OF HARVEY DATA (THE THIN SAMPLE DATA WAS NOT 9437 1451 788 USEFUL IN THE HIGH ENERGY RANGE) AND ON THE 1988 FISSION DATA RE- 9437 1451 789 LEASED BY WESTON AT THE BEGINNING OF 1991/7/. THE DEFINITIVE 9437 1451 790 SAMMY FITS WERE PERFORMED IN APRIL 1992 AFTER RENORMALIZATION OF 9437 1451 791 THE 1988 DATA OF WESTON ON THE ENDF/B-VI STANDARD VALUES BETWEEN 19437 1451 792 KEV AND 2 KEV, IN AGREEMENT WITH THE 1991 NEW MEASUREMENTS OF 9437 1451 793 WESTON AND TODD. 9437 1451 794 THE AVERAGE CROSS SECTIONS CALCULATED FROM THE RESONANCE 9437 1451 795 PARAMETERS ARE COMPARED TO THE EXPERIMENTAL VALUES IN THE FOLLO- 9437 1451 796 WING TABLE: 9437 1451 797 9437 1451 798 9437 1451 799 ************************************************************** 9437 1451 800 CROSS-SECTIONS(BARN) 9437 1451 801 --------------------------------------------------- 9437 1451 802 TOTAL FISSION CAPTURE 9437 1451 803 ENERGY -------------- ------------- ------------- 9437 1451 804 KEV CALC(A) EXP(B) CALC(A) EXP(C) CALC(A) EXP(D) 9437 1451 805 ************************************************************** 9437 1451 806 1.0-1.1 24.47 24.95 5.549 5.581 4.728 5.04 9437 1451 807 1.1-1.2 22.82 23.10 5.985 6.017 3.757 2.95 9437 1451 808 1.2-1.3 22.29 22.90 4.601 4.501 4.287 4.00 9437 1451 809 1.3-1.4 22.63 22.85 6.997 6.997 3.012 2.52 9437 1451 810 1.4-1.5 20.42 20.95 4.041 4.059 3.450 3.57 9437 1451 811 1.5-1.6 18.30 18.95 2.564 2.613 3.521 3.89 9437 1451 812 1.6-1.7 21.82 21.90 3.952 3.955 3.833 4.36 9437 1451 813 1.7-1.8 21.26 21.35 3.400 3.425 4.091 4.37 9437 1451 814 1.8-1.9 23.76 23.30 5.178 5.187 3.639 3.14 9437 1451 815 1.9-2.0 18.48 18.90 2.152 2.180 3.205 4.06 9437 1451 816 ************************************************************** 9437 1451 817 1.0-2.0 21.63 21.92 4.442 4.446 3.752 3.79 9437 1451 818 ************************************************************** 9437 1451 819 (A) TOTAL, FISSION AND CAPTURE CROSS SECTIONS CALCULATED BY 9437 1451 820 RESENDD FROM THE RESONANCE PARAMETERS. 9437 1451 821 (B) EXPERIMENTAL TOTAL CROSS SECTIONS FROM REFERENCE/19/. 9437 1451 822 (C) WESTON AND TODD 1988 HIGH RESOLUTION FISSION CROSS SECTIONS 9437 1451 823 FROM REFERENCE/7/ NORMALIZED TO ENDF/B-VI STANDARD IN THE 9437 1451 824 ENERGY RANGE FROM 1.0 KEV TO 2.0 KEV. 9437 1451 825 (D) GWIN 1971 EXPERIMENTAL DATA NORMALIZED TO GWIN 1976 DATA. 9437 1451 826 ************************************************************** 9437 1451 827 9437 1451 828 THE DIFFERENCE OF 1.3% BETWEEN THE AVERAGE CALCULATED TOTAL 9437 1451 829 CROSS SECTION AND THE AVERAGE EXPERIMENTAL CROSS SECTION IN THE 9437 1451 830 ENERGY RANGE FROM 1.0 KEV AND 2.0 KEV IS MAINLY DUE TO THE METHOD 9437 1451 831 OF EVALUATING THE TOTAL CROSS SECTION FROM THE EFFECTIVE CROSS 9437 1451 832 SECTION IN REFERENCE/19/. THE ACCURACY OF THE SAMMY FIT OF THE 9437 1451 833 EXPERIMENTAL TRANSMISSION DATA IS BETTER THAN 0.5% ON THE CROSS 9437 1451 834 SECTION. THE CALCULATED FISSION CROSS SECTIONS ARE IN VERY GOOD 9437 1451 835 AGREEMENT WITH THE EXPERIMENTAL DATA. THE CAPTURE DATA /1/ ARE 9437 1451 836 AVERAGE VALUES OBTAINED FROM THE DATA AVAILABLE IN THE EXFOR FILE 9437 1451 837 AND NORMALIZED TO GWIN 1976 AVERAGE VALUES; THERE ARE LARGE 9437 1451 838 DIFFERENCES BETWEEN THE CALCULATED DATA AND THE EXPERIMENTAL DATA 9437 1451 839 AVERAGED OVER 0.1 KEV INTERVALS; BUT ON THE INTERVAL FROM 1.0 KEV 9437 1451 840 TO 2.0 KEV THE AVERAGE VALUES ARE CONSISTENT WITHIN 1.0%. 9437 1451 841 9437 1451 842 ***************************************************************** 9437 1451 843 COMMENTS ON THE 2.0 KEV TO 2.5 KEV REGION 9437 1451 844 ***************************************************************** 9437 1451 845 9437 1451 846 THIS ENERGY RANGE WAS ALSO ANALYSED AT JAERI /13/. NO 9437 1451 847 PRELIMINARY SET OF RESONANCE PARAMETERS WAS AVAILABLE PRIOR TO THE9437 1451 848 ANALYSIS. MORE THAN 90% OF THE RESONANCES, COMPARED TO THE LOW 9437 1451 849 ENERGY RANGE, COULD STILL BE IDENTIFIED IN THE TRANSMISSION DATA 9437 1451 850 BETWEEN 2 KEV AND 2.5 KEV. THEREFORE THE CORRELATED SAMMY ANALYSIS9437 1451 851 OF HARVEY TRANSMISSIONS AND WESTON FISSION WAS STILL FEASIBLE IN 9437 1451 852 THIS ENERGY RANGE. THE RESONANCE PARAMETERS OBTAINED ARE 9437 1451 853 CONSISTENT AND HAS NEARLY THE SAME STATISTICAL PROPERTIES AS THOSE9437 1451 854 OF THE RESONANCES IN THE 0 TO 2 KEV ENERGY RANGE. A QUITE GOOD FIT9437 1451 855 OF THE TRANSMISSION AND FISSION DATA WAS OBTAINED WITHOUT 9437 1451 856 BACKGROUND AND NORMALISATION ADJUSTMENT. HOWEVER, THE CALCULATED 9437 1451 857 FISSION CROSS SECTIONS ARE, ON AVERAGE, 1.4% LOWER THAN THE 9437 1451 858 EXPERIMENTAL VALUES. THIS DIFFERENCE,WHICH HOWEVER IS NOT LARGER 9437 1451 859 THAN THE SYSTEMATIC ERRORS ON THE EXPERIMENTAL DATA, COULD BE DUE 9437 1451 860 TO THE DIFFICULTIES OF IDENTIFYING THE WIDE J=0+ RESONANCES IN THE9437 1451 861 EXPERIMENTAL DATA, BECAUSE THE EFFECTS OF THE INCREASING 9437 1451 862 RESOLUTION AND DOPPLER WIDTHS. PRIOR TO THE SAMMY FITS, THE 9437 1451 863 FISSION DATA OF WESTON AND TODD (1988 HIGH RESOLUTION DATA) WERE 9437 1451 864 NORMALIZED TO THE ENDF/B-VI STANDARD IN THE ENERGY RANGE FROM 1 9437 1451 865 KEV TO 2 KEV. 9437 1451 866 THE CROSS SECTIONS,CALCULATED FROM THE RESONANCE PARAMETERS 9437 1451 867 AND AVERAGED OVER 0.1 KEV INTERVALS,ARE GIVEN IN THE FOLLOWING 9437 1451 868 TABLE: 9437 1451 869 9437 1451 870 ************************************************************** 9437 1451 871 CR0SS-SECTIONS(BARN) 9437 1451 872 ------------------------------------------ 9437 1451 873 TOTAL FISSION CAPTURE 9437 1451 874 ENERGY -------------- -------------- ------- 9437 1451 875 (KEV) CALC(A) EXP(B) CALC(A) EXP(C) CALC(A) 9437 1451 876 ************************************************************** 9437 1451 877 2.0-2.1 17.34 17.30 2.034 2.062 3.223 9437 1451 878 2.1-2.2 20.27 19.80 2.949 2.999 4.051 9437 1451 879 2.2-2.3 19.34 19.10 2.357 2.393 3.324 9437 1451 880 2.3-2.4 21.28 21.20 3.646 3.679 3.640 9437 1451 881 2.4-2.5 20.03 20.60 3.956 4.024 3.128 9437 1451 882 ************************************************************** 9437 1451 883 2.0-2.5 19.65 19.60 2.989 3.031 3.473 9437 1451 884 ************************************************************** 9437 1451 885 (A) TOTAL, FISSION AND CAPTURE CROSS SECTIONS CALCULATED BY 9437 1451 886 RESENDD, 1% ACCURACY, AT 300 K,FROM THE RESONANCE PARAME- 9437 1451 887 TERS. 9437 1451 888 (B) AVERAGE TOTAL CROSS SECTIONS OBTAINED FROM THE AVERAGE 9437 1451 889 EXPERIMENTAL EFFECTIVE CROSS SECTIONS IN REFERENCE/19/. 9437 1451 890 (C) 1988 HIGH RESOLUTION DATA OF WESTON AND TODD NORMALIZED 9437 1451 891 TO ENDF/B-VI STANDARD IN THE ENERGY RANGE FROM 1 KEV TO 9437 1451 892 2 KEV. 9437 1451 893 ***************************************************************** 9437 1451 894 9437 1451 895 9437 1451 896 ***************************************************************** 9437 1451 897 FISSION AND CAPTURE RESONANCE INTEGRALS 9437 1451 898 ***************************************************************** 9437 1451 899 9437 1451 900 THE FISSION AND CAPTURE RESONANCE INTEGRALS ARE COMPARED TO 9437 1451 901 JENDL-3 DATA IN THE FOLLOWING TABLE: 9437 1451 902 9437 1451 903 ********************************************************** 9437 1451 904 ENERGY RANGE(EV) FISSION(BARN) CAPTURE(BARN) 9437 1451 905 ********************************************************** 9437 1451 906 JENDL-3 PRESENT JENDL-3 PRESENT 9437 1451 907 0.5 - 5.0 85.725 84.879 28.651 28.723 9437 1451 908 5.0 - 10.0 25.081 25.147 19.059 18.950 9437 1451 909 10.0 - 50.0 96.856 99.715 77.181 74.686 9437 1451 910 50.0 - 100.0 40.479 41.552 25.930 25.376 9437 1451 911 100.0 - 301.0 19.677 20.252 17.952 17.729 9437 1451 912 301.0 -1000.0 10.047 10.317 8.348 8.418 9437 1451 913 1000.0 -2000.0 3.484 3.206 2.840 2.634 9437 1451 914 2000.0 -2.E+07 17.783 (17.783) 5.224 (5.224) 9437 1451 915 ********************************************************** 9437 1451 916 TOTAL 299.132 302.851 185.185 181.739 9437 1451 917 ********************************************************** 9437 1451 918 9437 1451 919 THE JENDL-3 RESONANCE PARAMETERS ARE THOSE OBTAINED IN 1987 IN 9437 1451 920 THE ENERGY RANGE 0 KEV TO 1 KEV. THEY ARE SLIGTHLY DIFFERENT FROM 9437 1451 921 THOSE PUBLISHED IN 1989. THAT EXPLAINS THE SMALL DIFFERENCES OB- 9437 1451 922 SERVED BETWEEN JENDL-3 AND THE PRESENT RESULTS IN THIS ENERGY RAN-9437 1451 923 GE. IN THE ENERGY RANGE 1 KEV TO 2 KEV JENDL-3 IS UNRESOLVED 9437 1451 924 RANGE. THE FISSION AND CAPTURE RESONANCE INTEGRALS CALCULATED 9437 1451 925 FROM ENDF/B-V AND THOSE FOUND IN BNL-325 ARE THE FOLLOWING: 9437 1451 926 9437 1451 927 ENDF/B-V FISSION: 302.13 B CAPTURE: 194.10 B 9437 1451 928 BNL-325 FISSION: 310+-10 B CAPTURE: 200+-20 B 9437 1451 929 9437 1451 930 THE CONSEQUENCE OF CHANGING FROM THE OLD SETS OF RESONANCE 9437 1451 931 PARAMETERS(ENDF/B-V AND PREVIOUS SETS) TO THE NEW SET IS THAT 9437 1451 932 THE CAPTURE RESONANCE INTEGRAL WILL DECREASE BY 6.7% COMPARED 9437 1451 933 WITH ENDF/B-V VALUE. 9437 1451 934 9437 1451 935 REFERENCES OF APPENDIX 9437 1451 936 1) R.GWIN ET AL.,NUCL.SCI.ENG.,45,25(1971) 9437 1451 937 2) R.GWIN ET AL.,NUCL.SCI.ENG.,59,79(1976) 9437 1451 938 3) R.GWIN ET AL.,NUCL.SCI.ENG.,61,116(1976) 9437 1451 939 4) R.GWIN ET AL.,NUCL.SCI.ENG.,88,37(1984) 9437 1451 940 5) J.BLONS, NUCL.SCI.ENG.,51,130(1973) 9437 1451 941 6) L.W.WESTON ET AL.,NUCL.SCI.ENG.88,567(1984) 9437 1451 942 7) L.W.WESTON ET AL.,TO BE PUBLISHED(HIGH RESOLUTION 1988 DATA) 9437 1451 943 8) R.R.SPENCER ET AL.,NUCL.SCI.ENG.,96,318(1987) 9437 1451 944 9) J.A.HARVEY ,MITO 1988,PAGE 115 9437 1451 945 10) A.CARLSON ET AL.,PRELIMINARY RESULTS OF THE ENDF/B-6 STANDARD 9437 1451 946 EVALUATION(SEPT 8 1987) 9437 1451 947 11) H.DERRIEN AND G. DE SAUSSURE,ORNL-TM-10986(1988) 9437 1451 948 12) H.DERRIEN ET AL.,NUCL.SCI.ENG.,106,434(1990) 9437 1451 949 13) H.DERRIEN, J.NUCL>SCI.TECHNOL.,30,845(1993). 9437 1451 950 14) N.M.LARSON ET AL.,ORNL/TM-7485,ORNL/TM-9179,ORNL/TM-9719/R1 9437 1451 951 15) L.LEAL AND R.N.HWANG,TRANS.AM.NUC.SOC.,55,340(1987) 9437 1451 952 16) T.NAKAGAWA,RESENDD A JAERI VERSION OF RESEND,JAER=-M 84-192 9437 1451 953 (1984). 9437 1451 954 17) C.WAGEMANS ET AL.,MITO 1988,PAGE 91 9437 1451 955 18) L.W.WESTON,PRIVATE COMMUNICATION(1992) 9437 1451 956 19) H.DERRIEN,J.NUCL.SCI.TECHNOL.,29,794(1992). 9437 1451 957 1 451 1085 09437 1451 958 1 452 36 09437 1451 959 1 455 9 09437 1451 960 1 456 34 09437 1451 961 2 151 1220 09437 1451 962 3 1 105 09437 1451 963 3 2 110 09437 1451 964 3 4 27 09437 1451 965 3 5 21 09437 1451 966 3 16 9 09437 1451 967 3 17 7 09437 1451 968 3 18 68 09437 1451 969 3 37 5 09437 1451 970 3 51 21 09437 1451 971 3 52 19 09437 1451 972 3 53 19 09437 1451 973 3 54 17 09437 1451 974 3 55 17 09437 1451 975 3 56 17 09437 1451 976 3 57 16 09437 1451 977 3 58 16 09437 1451 978 3 59 16 09437 1451 979 3 60 16 09437 1451 980 3 61 16 09437 1451 981 3 62 16 09437 1451 982 3 63 16 09437 1451 983 3 64 16 09437 1451 984 3 65 16 09437 1451 985 3 66 16 09437 1451 986 3 67 16 09437 1451 987 3 68 16 09437 1451 988 3 91 16 09437 1451 989 3 102 37 09437 1451 990 3 203 11 09437 1451 991 3 204 9 09437 1451 992 3 205 10 09437 1451 993 3 206 7 09437 1451 994 3 207 11 09437 1451 995 3 208 8 09437 1451 996 3 209 8 09437 1451 997 3 210 8 09437 1451 998 4 2 2973 09437 1451 999 4 16 16 09437 1451 1000 4 17 16 09437 1451 1001 4 37 16 09437 1451 1002 4 51 67 09437 1451 1003 4 52 67 09437 1451 1004 4 53 67 09437 1451 1005 4 54 67 09437 1451 1006 4 55 67 09437 1451 1007 4 56 40 09437 1451 1008 4 57 67 09437 1451 1009 4 58 40 09437 1451 1010 4 59 67 09437 1451 1011 4 60 40 09437 1451 1012 4 61 40 09437 1451 1013 4 62 40 09437 1451 1014 4 63 40 09437 1451 1015 4 64 40 09437 1451 1016 4 65 40 09437 1451 1017 4 66 40 09437 1451 1018 4 67 38 09437 1451 1019 4 68 38 09437 1451 1020 4 91 38 09437 1451 1021 5 16 189 09437 1451 1022 5 17 69 09437 1451 1023 5 37 21 09437 1451 1024 5 91 332 09437 1451 1025 5 455 585 09437 1451 1026 6 5 203554 09437 1451 1027 6 18 79920 09437 1451 1028 6 208 2994 09437 1451 1029 6 209 2994 09437 1451 1030 6 210 2994 09437 1451 1031 12 16 9 09437 1451 1032 12 17 7 09437 1451 1033 12 18 11 09437 1451 1034 12 37 5 09437 1451 1035 12 51 3 09437 1451 1036 12 52 3 09437 1451 1037 12 53 3 09437 1451 1038 12 54 3 09437 1451 1039 12 55 3 09437 1451 1040 12 56 4 09437 1451 1041 12 57 3 09437 1451 1042 12 58 5 09437 1451 1043 12 59 3 09437 1451 1044 12 60 4 09437 1451 1045 12 61 4 09437 1451 1046 12 62 3 09437 1451 1047 12 63 3 09437 1451 1048 12 64 3 09437 1451 1049 12 65 3 09437 1451 1050 12 66 4 09437 1451 1051 12 67 4 09437 1451 1052 12 68 5 09437 1451 1053 12 91 11 09437 1451 1054 12 102 12 09437 1451 1055 14 16 1 09437 1451 1056 14 17 1 09437 1451 1057 14 18 1 09437 1451 1058 14 37 1 09437 1451 1059 14 51 1 09437 1451 1060 14 52 1 09437 1451 1061 14 53 1 09437 1451 1062 14 54 1 09437 1451 1063 14 55 1 09437 1451 1064 14 56 1 09437 1451 1065 14 57 1 09437 1451 1066 14 58 1 09437 1451 1067 14 59 1 09437 1451 1068 14 60 1 09437 1451 1069 14 61 1 09437 1451 1070 14 62 1 09437 1451 1071 14 63 1 09437 1451 1072 14 64 1 09437 1451 1073 14 65 1 09437 1451 1074 14 66 1 09437 1451 1075 14 67 1 09437 1451 1076 14 68 1 09437 1451 1077 14 91 1 09437 1451 1078 14 102 1 09437 1451 1079 15 16 136 09437 1451 1080 15 17 60 09437 1451 1081 15 18 222 09437 1451 1082 15 37 20 09437 1451 1083 15 91 218 09437 1451 1084 15 102 327 09437 1451 1085 9437 1 099999 9.423900+4 2.369990+2 0 2 0 09437 1452 1 0.0 0.0 0 0 1 979437 1452 2 97 2 9437 1452 3 1.000000-5 2.884320+0 2.530000-2 2.884320+0 5.000000-2 2.884320+09437 1452 4 7.500000-2 2.880120+0 1.500000-1 2.868120+0 2.000000-1 2.864420+09437 1452 5 2.500000-1 2.863720+0 3.500000-1 2.864420+0 4.500000-1 2.866120+09437 1452 6 6.000000-1 2.870220+0 7.000000-1 2.872120+0 2.000000+1 2.872120+09437 1452 7 4.000000+1 2.835520+0 4.800000+1 2.838020+0 5.800000+1 2.890220+09437 1452 8 9.600000+1 2.872120+0 1.050000+2 2.826320+0 1.250000+2 2.887220+09437 1452 9 2.000000+2 2.887220+0 3.200000+2 2.858120+0 4.500000+2 2.888220+09437 1452 10 5.000000+2 2.888220+0 5.000000+2 2.915220+0 1.000000+5 2.915230+09437 1452 11 1.000000+5 2.887230+0 1.000000+6 3.008840+0 1.500000+6 3.076400+09437 1452 12 3.000000+6 3.306720+0 5.300000+6 3.658560+0 7.000000+6 3.916380+09437 1452 13 1.000000+7 4.372700+0 1.100000+7 4.524770+0 1.150000+7 4.600710+09437 1452 14 1.450000+7 4.991710+0 1.500000+7 5.056970+0 1.960000+7 5.657170+09437 1452 15 2.000000+7 5.693170+0 2.000000+7 4.551810+0 2.200000+7 4.644500+09437 1452 16 2.400000+7 4.773670+0 2.600000+7 4.780570+0 2.780000+7 4.786780+09437 1452 17 2.800000+7 4.787470+0 2.860000+7 4.789540+0 2.950000+7 4.792650+09437 1452 18 3.000000+7 4.794370+0 3.040000+7 4.801510+0 3.130000+7 4.817560+09437 1452 19 3.220000+7 4.833620+0 3.320000+7 4.851460+0 3.420000+7 4.869300+09437 1452 20 3.500000+7 4.883570+0 3.520000+7 4.887140+0 3.630000+7 4.906760+09437 1452 21 3.740000+7 4.926390+0 3.850000+7 4.946010+0 3.970000+7 4.967420+09437 1452 22 4.000000+7 4.972770+0 4.080000+7 4.984610+0 4.500000+7 5.046770+09437 1452 23 5.000000+7 5.120770+0 5.500000+7 5.228920+0 6.000000+7 5.337070+09437 1452 24 6.500000+7 5.448350+0 7.000000+7 5.559620+0 7.500000+7 5.670900+09437 1452 25 8.000000+7 5.782170+0 8.500000+7 5.903150+0 9.000000+7 6.024120+09437 1452 26 9.500000+7 6.145140+0 1.000000+8 6.266030+0 1.100000+8 6.476710+09437 1452 27 1.200000+8 6.687360+0 1.250000+8 6.792660+0 1.300000+8 6.886660+09437 1452 28 1.400000+8 7.074650+0 1.500000+8 7.262720+0 1.600000+8 7.442250+09437 1452 29 1.700000+8 7.621790+0 1.750000+8 7.711620+0 1.800000+8 7.812240+09437 1452 30 1.900000+8 8.013580+0 2.000000+8 8.214920+0 2.100000+8 8.428310+09437 1452 31 2.200000+8 8.641880+0 2.300000+8 8.855280+0 2.400000+8 9.068770+09437 1452 32 2.500000+8 9.282270+0 3.500000+8 1.319766+1 5.000000+8 1.451502+19437 1452 33 6.000000+8 1.510966+1 7.000000+8 1.544308+1 8.000000+8 1.567346+19437 1452 34 1.000000+9 1.599544+1 1.500000+9 1.636077+1 2.000000+9 1.650329+19437 1452 35 3.000000+9 1.658583+1 9437 1452 36 9437 1 099999 9.423900+4 2.369990+2 0 2 0 09437 1455 1 0.0 0.0 0 0 6 09437 1455 2 1.277000-2 3.014000-2 1.238000-1 3.254000-1 1.122000+0 2.697000+09437 1455 3 0.0 0.0 0 0 1 109437 1455 4 10 2 9437 1455 5 1.000000-5 6.220000-3 2.530000-2 6.220000-3 3.000000+6 6.590000-39437 1455 6 7.000000+6 4.800000-3 1.100000+7 4.800000-3 1.450000+7 4.170000-39437 1455 7 2.000000+7 4.170000-3 2.500000+8 4.170000-3 2.500000+8 0.0 9437 1455 8 3.000000+9 0.0 9437 1455 9 9437 1 099999 9.423900+4 2.369990+2 0 2 0 09437 1456 1 0.0 0.0 0 0 1 939437 1456 2 93 2 9437 1456 3 1.000000-5 2.878100+0 2.530000-2 2.878100+0 5.000000-2 2.878100+09437 1456 4 7.500000-2 2.873900+0 1.500000-1 2.861900+0 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8.881304-7-6.018150-1 8.828964-79437 4 2 1859 -5.877850-1 7.971407-7-5.735760-1 6.422304-7-5.591930-1 4.555191-79437 4 2 1860 -5.446390-1 2.996228-7-5.299190-1 2.536300-7-5.150380-1 3.953974-79437 4 2 1861 -5.000000-1 7.757738-7-4.848100-1 1.390864-6-4.694710-1 2.161761-69437 4 2 1862 -4.539900-1 2.935138-6-4.383710-1 3.513266-6-4.226180-1 3.713415-69437 4 2 1863 -4.067370-1 3.442566-6-3.907310-1 2.756559-6-3.746070-1 1.879402-69437 4 2 1864 -3.583680-1 1.159625-6-3.420200-1 9.724870-7-3.255680-1 1.595073-69437 4 2 1865 -3.090170-1 3.095027-6-2.923720-1 5.270058-6-2.756370-1 7.662739-69437 4 2 1866 -2.588190-1 9.660700-6-2.419220-1 1.067706-5-2.249510-1 1.038236-59437 4 2 1867 -2.079120-1 8.920023-6-1.908090-1 7.004521-6-1.736480-1 5.792406-69437 4 2 1868 -1.564340-1 6.492213-6-1.391730-1 9.817010-6-1.218690-1 1.551084-59437 4 2 1869 -1.045280-1 2.222101-5-8.715570-2 2.787499-5-6.975640-2 3.049357-59437 4 2 1870 -5.233590-2 2.914738-5-3.489940-2 2.465670-5-1.745230-2 1.967812-59437 4 2 1871 7.549790-8 1.800283-5 1.745250-2 2.315990-5 3.489960-2 3.670045-59437 4 2 1872 5.233600-2 5.683417-5 6.975650-2 7.819408-5 8.715580-2 9.326212-59437 4 2 1873 1.045290-1 9.544541-5 1.218690-1 8.273996-5 1.391730-1 6.039055-59437 4 2 1874 1.564350-1 4.073723-5 1.736480-1 3.944294-5 1.908090-1 6.884772-59437 4 2 1875 2.079120-1 1.308405-4 2.249510-1 2.125591-4 2.419220-1 2.879858-49437 4 2 1876 2.588190-1 3.264927-4 2.756370-1 3.067027-4 2.923720-1 2.306031-49437 4 2 1877 3.090170-1 1.309235-4 3.255680-1 6.546703-5 3.420200-1 9.649230-59437 4 2 1878 3.583680-1 2.605519-4 3.746070-1 5.412748-4 3.907310-1 8.603815-49437 4 2 1879 4.067370-1 1.097535-3 4.226180-1 1.138945-3 4.383710-1 9.388591-49437 4 2 1880 4.539910-1 5.670507-4 4.694720-1 2.134911-4 4.848100-1 1.318265-49437 4 2 1881 5.000000-1 5.295868-4 5.150380-1 1.443274-3 5.299190-1 2.659909-39437 4 2 1882 5.446390-1 3.746045-3 5.591930-1 4.207083-3 5.735760-1 3.739595-39437 4 2 1883 5.877850-1 2.467280-3 6.018150-1 1.029236-3 6.156610-1 4.129283-49437 4 2 1884 6.293200-1 1.535344-3 6.427880-1 4.711501-3 6.560590-1 9.268132-39437 4 2 1885 6.691310-1 1.357954-2 6.819980-1 1.566574-2 6.946580-1 1.422194-29437 4 2 1886 7.071070-1 9.644560-3 7.193400-1 4.432582-3 7.313540-1 2.500230-39437 4 2 1887 7.431450-1 7.387760-3 7.547100-1 2.003802-2 7.660440-1 3.732425-29437 4 2 1888 7.771460-1 5.251058-2 7.880110-1 5.810326-2 7.986360-1 5.021969-29437 4 2 1889 8.090170-1 3.241017-2 8.191520-1 1.620923-2 8.290380-1 1.694733-29437 4 2 1890 8.386710-1 4.558421-2 8.480480-1 1.002996-1 8.571670-1 1.631383-19437 4 2 1891 8.660250-1 2.057652-1 8.746200-1 2.041232-1 8.829480-1 1.558644-19437 4 2 1892 8.910060-1 9.041553-2 8.987940-1 6.218314-2 9.063080-1 1.249575-19437 4 2 1893 9.135460-1 2.967398-1 9.205050-1 5.343908-1 9.271840-1 7.385610-19437 4 2 1894 9.335800-1 7.982887-1 9.396930-1 6.623423-1 9.455180-1 4.027113-19437 4 2 1895 9.510560-1 2.250031-1 9.563050-1 3.958634-1 9.612620-1 1.095955+09437 4 2 1896 9.659260-1 2.257561+0 9.702960-1 3.484446+0 9.743700-1 4.150443+09437 4 2 1897 9.781480-1 3.718435+0 9.816270-1 2.220671+0 9.848080-1 7.289890-19437 4 2 1898 9.876880-1 1.574274+0 9.902680-1 8.091517+0 9.925460-1 2.380630+19437 4 2 1899 9.945220-1 5.119839+1 9.961950-1 9.041553+1 9.975640-1 1.384194+29437 4 2 1900 9.986290-1 1.890442+2 9.993910-1 2.340870+2 9.998480-1 2.652559+29437 4 2 1901 1.000000+0 2.764059+2 9437 4 2 1902 0.0 1.800000+8 0 0 1 1819437 4 2 1903 181 2 9437 4 2 1904 -1.000000+0 3.663172-8-9.998480-1 3.766172-8-9.993910-1 4.018500-89437 4 2 1905 -9.986290-1 4.274589-8-9.975640-1 4.358079-8-9.961950-1 4.138460-89437 4 2 1906 -9.945220-1 3.590212-8-9.925460-1 2.814906-8-9.902680-1 2.017490-89437 4 2 1907 -9.876880-1 1.440813-8-9.848080-1 1.283314-8-9.816270-1 1.629512-89437 4 2 1908 -9.781480-1 2.417758-8-9.743700-1 3.457243-8-9.702960-1 4.488568-89437 4 2 1909 -9.659260-1 5.266244-8-9.612620-1 5.637412-8-9.563050-1 5.589653-89437 4 2 1910 -9.510560-1 5.259854-8-9.455180-1 4.896206-8-9.396920-1 4.792797-89437 4 2 1911 -9.335800-1 5.208705-8-9.271840-1 6.294369-8-9.205050-1 8.040011-89437 4 2 1912 -9.135450-1 1.026285-7-9.063080-1 1.263614-7-8.987940-1 1.475973-79437 4 2 1913 -8.910060-1 1.625452-7-8.829470-1 1.685962-7-8.746200-1 1.649932-79437 4 2 1914 -8.660250-1 1.530763-7-8.571670-1 1.359133-7-8.480480-1 1.175424-79437 4 2 1915 -8.386700-1 1.020195-7-8.290370-1 9.260305-8-8.191520-1 9.129435-89437 4 2 1916 -8.090170-1 9.871392-8-7.986350-1 1.142524-7-7.880110-1 1.362743-79437 4 2 1917 -7.771460-1 1.623342-7-7.660440-1 1.893611-7-7.547090-1 2.139100-79437 4 2 1918 -7.431450-1 2.325169-7-7.313540-1 2.421588-7-7.193400-1 2.407528-79437 4 2 1919 -7.071070-1 2.276999-7-6.946580-1 2.046860-7-6.819980-1 1.767221-79437 4 2 1920 -6.691310-1 1.531663-7-6.560590-1 1.479313-7-6.427880-1 1.777491-79437 4 2 1921 -6.293200-1 2.578297-7-6.156610-1 3.955321-7-6.018150-1 5.840481-79437 4 2 1922 -5.877850-1 7.988871-7-5.735760-1 1.000075-6-5.591930-1 1.139814-69437 4 2 1923 -5.446390-1 1.175274-6-5.299190-1 1.082765-6-5.150380-1 8.710887-79437 4 2 1924 -5.000000-1 5.902901-7-4.848100-1 3.327314-7-4.694710-1 2.208069-79437 4 2 1925 -4.539900-1 3.779332-7-4.383710-1 8.837617-7-4.226180-1 1.725592-69437 4 2 1926 -4.067370-1 2.767446-6-3.907310-1 3.760902-6-3.746070-1 4.409968-69437 4 2 1927 -3.583680-1 4.479168-6-3.420200-1 3.905311-6-3.255680-1 2.866616-69437 4 2 1928 -3.090170-1 1.766691-6-2.923720-1 1.126694-6-2.756370-1 1.412833-69437 4 2 1929 -2.588190-1 2.855746-6-2.419220-1 5.321904-6-2.249510-1 8.287079-69437 4 2 1930 -2.079120-1 1.094465-5-1.908090-1 1.245034-5-1.736480-1 1.226344-59437 4 2 1931 -1.564340-1 1.048205-5-1.391730-1 8.009551-6-1.218690-1 6.378609-69437 4 2 1932 -1.045280-1 7.198025-6-8.715570-2 1.137524-5-6.975640-2 1.847661-59437 4 2 1933 -5.233590-2 2.660917-5-3.489940-2 3.302494-5-1.745230-2 3.528953-59437 4 2 1934 7.549790-8 3.256584-5 1.745250-2 2.643877-5 3.489960-2 2.080890-59437 4 2 1935 5.233600-2 2.066640-5 6.975650-2 2.997295-5 8.715580-2 4.934946-59437 4 2 1936 1.045290-1 7.465024-5 1.218690-1 9.754432-5 1.391730-1 1.085365-49437 4 2 1937 1.564350-1 1.017225-4 1.736480-1 7.926821-5 1.908090-1 5.303094-59437 4 2 1938 2.079120-1 4.150500-5 2.249510-1 6.230070-5 2.419220-1 1.226494-49437 4 2 1939 2.588190-1 2.122740-4 2.756370-1 3.029935-4 2.923720-1 3.576003-49437 4 2 1940 3.090170-1 3.466413-4 3.255680-1 2.672267-4 3.420200-1 1.544072-49437 4 2 1941 3.583680-1 7.603033-5 3.746070-1 1.076605-4 3.907310-1 2.942576-49437 4 2 1942 4.067370-1 6.152600-4 4.226180-1 9.736762-4 4.383710-1 1.223564-39437 4 2 1943 4.539910-1 1.233674-3 4.694720-1 9.655153-4 4.848100-1 5.282414-49437 4 2 1944 5.000000-1 1.724802-4 5.150380-1 2.030910-4 5.299190-1 8.294599-49437 4 2 1945 5.446390-1 2.013760-3 5.591930-1 3.404103-3 5.735760-1 4.424638-39437 4 2 1946 5.877850-1 4.529558-3 6.018150-1 3.536473-3 6.156610-1 1.869511-39437 4 2 1947 6.293200-1 5.405004-4 6.427880-1 7.766242-4 6.560590-1 3.380903-39437 4 2 1948 6.691310-1 8.103560-3 6.819980-1 1.340853-2 6.946580-1 1.693362-29437 4 2 1949 7.071070-1 1.664332-2 7.193400-1 1.222924-2 7.313540-1 5.981121-39437 4 2 1950 7.431450-1 2.362058-3 7.547100-1 6.051070-3 7.660440-1 1.909561-29437 4 2 1951 7.771460-1 3.865821-2 7.880110-1 5.704342-2 7.986360-1 6.490668-29437 4 2 1952 8.090170-1 5.679152-2 8.191520-1 3.625902-2 8.290380-1 1.709352-29437 4 2 1953 8.386710-1 1.812871-2 8.480480-1 5.274144-2 8.571670-1 1.179564-19437 4 2 1954 8.660250-1 1.904781-1 8.746200-1 2.350029-1 8.829480-1 2.240859-19437 4 2 1955 8.910060-1 1.604092-1 8.987940-1 8.712017-2 9.063080-1 7.434564-29437 4 2 1956 9.135460-1 1.816561-1 9.205050-1 4.128310-1 9.271840-1 6.913356-19437 4 2 1957 9.335800-1 8.824077-1 9.396930-1 8.657868-1 9.455180-1 6.309789-19437 4 2 1958 9.510560-1 3.380343-1 9.563050-1 2.870716-1 9.612620-1 7.749322-19437 4 2 1959 9.659260-1 1.884291+0 9.702960-1 3.316784+0 9.743700-1 4.408838+09437 4 2 1960 9.781480-1 4.422378+0 9.816270-1 3.087285+0 9.848080-1 1.214614+09437 4 2 1961 9.876880-1 1.081755+0 9.902680-1 6.287599+0 9.925460-1 2.091530+19437 4 2 1962 9.945220-1 4.812346+1 9.961950-1 8.857177+1 9.975640-1 1.393273+29437 4 2 1963 9.986290-1 1.937541+2 9.993910-1 2.427268+2 9.998480-1 2.768576+29437 4 2 1964 1.000000+0 2.891016+2 9437 4 2 1965 0.0 1.900000+8 0 0 1 1819437 4 2 1966 181 2 9437 4 2 1967 -1.000000+0 3.690710-8-9.998480-1 3.638871-8-9.993910-1 3.481801-89437 4 2 1968 -9.986290-1 3.218163-8-9.975640-1 2.856085-8-9.961950-1 2.423327-89437 4 2 1969 -9.945220-1 1.972760-8-9.925460-1 1.577272-8-9.902680-1 1.311683-89437 4 2 1970 -9.876880-1 1.225613-8-9.848080-1 1.317693-8-9.816270-1 1.524532-89437 4 2 1971 -9.781480-1 1.734181-8-9.743700-1 1.824550-8-9.702960-1 1.713961-89437 4 2 1972 -9.659260-1 1.403533-8-9.612620-1 9.892287-9-9.563050-1 6.342966-99437 4 2 1973 -9.510560-1 5.073593-9-9.455180-1 7.100212-9-9.396920-1 1.225113-89437 4 2 1974 -9.335800-1 1.912140-8-9.271840-1 2.557636-8-9.205050-1 2.964334-89437 4 2 1975 -9.135450-1 3.045634-8-9.063080-1 2.884425-8-8.987940-1 2.726455-89437 4 2 1976 -8.910060-1 2.904065-8-8.829470-1 3.713660-8-8.746200-1 5.292962-89437 4 2 1977 -8.660250-1 7.546370-8-8.571670-1 1.015035-7-8.480480-1 1.263753-79437 4 2 1978 -8.386700-1 1.453492-7-8.290370-1 1.549912-7-8.191520-1 1.540932-79437 4 2 1979 -8.090170-1 1.439282-7-7.986350-1 1.278663-7-7.880110-1 1.105824-79437 4 2 1980 -7.771460-1 9.716638-8-7.660440-1 9.216621-8-7.547090-1 9.874727-89437 4 2 1981 -7.431450-1 1.179364-7-7.313540-1 1.482032-7-7.193400-1 1.856670-79437 4 2 1982 -7.071070-1 2.249778-7-6.946580-1 2.605576-7-6.819980-1 2.875955-79437 4 2 1983 -6.691310-1 3.022524-7-6.560590-1 3.013594-7-6.427880-1 2.826695-79437 4 2 1984 -6.293200-1 2.469267-7-6.156610-1 2.017139-7-6.018150-1 1.650931-79437 4 2 1985 -5.877850-1 1.654011-7-5.735760-1 2.343738-7-5.591930-1 3.941219-79437 4 2 1986 -5.446390-1 6.428056-7-5.299190-1 9.462530-7-5.150380-1 1.240913-69437 4 2 1987 -5.000000-1 1.448932-6-4.848100-1 1.501232-6-4.694710-1 1.361803-69437 4 2 1988 -4.539900-1 1.048714-6-4.383710-1 6.469826-7-4.226180-1 3.060314-79437 4 2 1989 -4.067370-1 2.134399-7-3.907310-1 5.382341-7-3.746070-1 1.353413-69437 4 2 1990 -3.583680-1 2.566846-6-3.420200-1 3.902659-6-3.255680-1 4.964294-69437 4 2 1991 -3.090170-1 5.374541-6-2.923720-1 4.945554-6-2.756370-1 3.804920-69437 4 2 1992 -2.588190-1 2.409977-6-2.419220-1 1.430622-6-2.249510-1 1.524612-69437 4 2 1993 -2.079120-1 3.075884-6-1.908090-1 5.984638-6-1.736480-1 9.594849-69437 4 2 1994 -1.564340-1 1.283073-5-1.391730-1 1.455332-5-1.218690-1 1.407473-59437 4 2 1995 -1.045280-1 1.163674-5-8.715570-2 8.580364-6-6.975640-2 6.995603-69437 4 2 1996 -5.233590-2 8.848143-6-3.489940-2 1.491942-5-1.745230-2 2.409777-59437 4 2 1997 7.549790-8 3.351032-5 1.745250-2 3.961129-5 3.489960-2 3.986499-59437 4 2 1998 5.233600-2 3.434252-5 6.975650-2 2.639136-5 8.715580-2 2.188268-59437 4 2 1999 1.045290-1 2.690436-5 1.218690-1 4.457636-5 1.391730-1 7.236831-59437 4 2 2000 1.564350-1 1.016085-4 1.736480-1 1.203444-4 1.908090-1 1.191034-49437 4 2 2001 2.079120-1 9.720928-5 2.249510-1 6.618935-5 2.419220-1 4.740245-59437 4 2 2002 2.588190-1 6.339446-5 2.756370-1 1.258323-4 2.923720-1 2.254428-49437 4 2 2003 3.090170-1 3.301192-4 3.255680-1 3.951369-4 3.420200-1 3.841530-49437 4 2 2004 3.583680-1 2.934504-4 3.746070-1 1.663491-4 3.907310-1 8.571394-59437 4 2 2005 4.067370-1 1.405213-4 4.226180-1 3.767410-4 4.383710-1 7.558470-49437 4 2 2006 4.539910-1 1.148014-3 4.694720-1 1.375893-3 4.848100-1 1.301813-39437 4 2 2007 5.000000-1 9.233791-4 5.150380-1 4.260517-4 5.299190-1 1.452172-49437 4 2 2008 5.446390-1 4.251927-4 5.591930-1 1.418482-3 5.735760-1 2.923854-39437 4 2 2009 5.877850-1 4.377617-3 6.018150-1 5.065003-3 6.156610-1 4.506816-39437 4 2 2010 6.293200-1 2.850855-3 6.427880-1 1.024475-3 6.560590-1 4.649685-49437 4 2 2011 6.691310-1 2.423247-3 6.819980-1 7.113092-3 6.946580-1 1.318403-29437 4 2 2012 7.071070-1 1.799210-2 7.193400-1 1.882710-2 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1.836138+7 5.82740-109437 6 5 1914 1.854318+7 5.39268-10 1.872497+7 5.02623-10 1.890677+7 4.66651-109437 6 5 1915 1.908856+7 4.31391-10 1.927036+7 3.96789-10 1.945215+7 3.62792-109437 6 5 1916 1.963395+7 3.29442-10 1.981575+7 2.96781-10 1.999754+7 2.64764-109437 6 5 1917 2.017934+7 2.33368-10 2.036113+7 2.02637-10 2.054293+7 1.72582-109437 6 5 1918 2.072472+7 1.43111-10 2.090652+7 1.44972-10 2.108832+7 1.027432-99437 6 5 1919 2.127011+7 5.424033-9 2.145191+7 7.968832-9 2.163370+7 0.0 9437 6 5 1920 2.181550+7 0.0 2.200000+7 0.0 9437 6 5 1921 0.0 -9.396926-1 0 0 1 1229437 6 5 1922 122 1 9437 6 5 1923 0.0 5.460662-8 1.817958+5 1.374436-7 3.635917+5 1.626787-79437 6 5 1924 5.453875+5 1.679055-7 7.271833+5 1.689461-7 9.089792+5 1.787847-79437 6 5 1925 1.090775+6 1.570809-7 1.272571+6 1.456958-7 1.454367+6 1.308210-79437 6 5 1926 1.636162+6 1.148140-7 1.817958+6 9.917796-8 1.999754+6 8.962506-89437 6 5 1927 2.181550+6 7.481576-8 2.363346+6 6.144323-8 2.545142+6 5.274525-89437 6 5 1928 2.726938+6 4.558181-8 2.908733+6 3.957711-8 3.090529+6 3.444583-89437 6 5 1929 3.272325+6 3.013611-8 3.454121+6 2.652539-8 3.635917+6 2.430630-89437 6 5 1930 3.817712+6 2.146359-8 3.999508+6 1.873811-8 4.181304+6 1.648674-89437 6 5 1931 4.363100+6 1.487301-8 4.544896+6 1.349358-8 4.726692+6 1.233950-89437 6 5 1932 4.908488+6 1.135839-8 5.090283+6 1.050627-8 5.272079+6 9.769656-99437 6 5 1933 5.453875+6 9.131039-9 5.635671+6 8.733284-9 5.817467+6 8.294178-99437 6 5 1934 5.999262+6 7.762716-9 6.181058+6 7.371154-9 6.362854+6 6.954086-99437 6 5 1935 6.544650+6 6.581411-9 6.726446+6 6.308640-9 6.908242+6 6.057602-99437 6 5 1936 7.090038+6 5.824506-9 7.271833+6 5.609121-9 7.453629+6 5.409449-99437 6 5 1937 7.635425+6 5.221794-9 7.817221+6 5.045103-9 7.999017+6 4.879881-99437 6 5 1938 8.180812+6 4.818162-9 8.362608+6 4.665601-9 8.544404+6 4.477287-99437 6 5 1939 8.726200+6 4.385843-9 8.907996+6 4.214597-9 9.089792+6 4.133092-99437 6 5 1940 9.271588+6 3.936745-9 9.453383+6 3.827683-9 9.635179+6 3.722116-99437 6 5 1941 9.816975+6 3.620139-9 9.998771+6 3.522238-9 1.018057+7 3.427952-99437 6 5 1942 1.036236+7 3.336342-9 1.054416+7 3.246641-9 1.072595+7 3.158128-99437 6 5 1943 1.090775+7 3.070447-9 1.108955+7 3.013219-9 1.127134+7 2.925908-99437 6 5 1944 1.145314+7 2.868104-9 1.163493+7 2.755431-9 1.181673+7 2.673282-99437 6 5 1945 1.199852+7 2.592999-9 1.218032+7 2.514504-9 1.236212+7 2.437657-99437 6 5 1946 1.254391+7 2.362315-9 1.272571+7 2.265928-9 1.290750+7 2.194959-99437 6 5 1947 1.308930+7 2.125388-9 1.327110+7 2.057388-9 1.345289+7 1.990984-99437 6 5 1948 1.363469+7 1.925939-9 1.381648+7 1.862185-9 1.399828+7 1.799792-99437 6 5 1949 1.418008+7 1.738768-9 1.436187+7 1.679017-9 1.454367+7 1.636610-99437 6 5 1950 1.472546+7 1.578269-9 1.490726+7 1.521192-9 1.508905+7 1.465227-99437 6 5 1951 1.527085+7 1.410281-9 1.545265+7 1.356296-9 1.563444+7 1.303258-99437 6 5 1952 1.581624+7 1.238855-9 1.599803+7 1.200579-9 1.617983+7 1.150435-99437 6 5 1953 1.636162+7 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9.089792+5 1.685596-79437 6 5 1968 1.090775+6 1.676187-7 1.272571+6 1.451204-7 1.454367+6 1.303145-79437 6 5 1969 1.636162+6 1.143836-7 1.817958+6 9.882355-8 1.999754+6 8.477236-89437 6 5 1970 2.181550+6 7.329680-8 2.363346+6 6.435086-8 2.545142+6 5.445900-89437 6 5 1971 2.726938+6 4.647431-8 2.908733+6 3.954520-8 3.090529+6 3.444560-89437 6 5 1972 3.272325+6 3.016368-8 3.454121+6 2.657749-8 3.635917+6 2.351021-89437 6 5 1973 3.817712+6 2.087732-8 3.999508+6 1.883481-8 4.181304+6 1.708100-89437 6 5 1974 4.363100+6 1.540007-8 4.544896+6 1.396501-8 4.726692+6 1.276899-89437 6 5 1975 4.908488+6 1.164590-8 5.090283+6 1.068195-8 5.272079+6 9.952271-99437 6 5 1976 5.453875+6 9.319586-9 5.635671+6 8.760805-9 5.817467+6 8.266175-99437 6 5 1977 5.999262+6 7.835460-9 6.181058+6 7.458776-9 6.362854+6 7.191689-99437 6 5 1978 6.544650+6 6.882542-9 6.726446+6 6.667427-9 6.908242+6 6.344027-99437 6 5 1979 7.090038+6 6.105424-9 7.271833+6 5.884604-9 7.453629+6 5.735085-99437 6 5 1980 7.635425+6 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1.752705-99437 6 5 1993 1.472546+7 1.674885-9 1.490726+7 1.632158-9 1.508905+7 1.557876-99437 6 5 1994 1.527085+7 1.516090-9 1.545265+7 1.444887-9 1.563444+7 1.390053-99437 6 5 1995 1.581624+7 1.336141-9 1.599803+7 1.283178-9 1.617983+7 1.231149-99437 6 5 1996 1.636162+7 1.179999-9 1.654342+7 1.140890-9 1.672522+7 1.079683-99437 6 5 1997 1.690701+7 1.041171-9 1.708881+7 9.82556-10 1.727060+7 9.44695-109437 6 5 1998 1.745240+7 8.88581-10 1.763420+7 8.51313-10 1.781599+7 7.97647-109437 6 5 1999 1.799779+7 7.60952-10 1.817958+7 7.09576-10 1.836138+7 6.73434-109437 6 5 2000 1.854318+7 6.24400-10 1.872497+7 5.88849-10 1.890677+7 5.42011-109437 6 5 2001 1.908856+7 5.07032-10 1.927036+7 4.62381-10 1.945215+7 4.27888-109437 6 5 2002 1.963395+7 3.85268-10 1.981575+7 3.51348-10 1.999754+7 3.10833-109437 6 5 2003 2.017934+7 2.74747-10 2.036113+7 2.39325-10 2.054293+7 2.04586-109437 6 5 2004 2.072472+7 1.70435-10 2.090652+7 1.70935-10 2.108832+7 1.110622-99437 6 5 2005 2.127011+7 5.899201-9 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