JENDL-5 (Neutron sublibrary (activation cs)) Cm-246 0 0 0 0 9.624600+4 2.439530+2 0 0 6 19643 1451 1 0.000000+0 1.000000+0 0 0 0 69643 1451 2 1.000000+0 2.000000+7 0 0 10 59643 1451 3 2.936000+2 0.000000+0 4 0 497 129643 1451 4 96-Cm-246 JAEA+ EVAL-JAN10 O.Iwamoto,T.Nakagawa,T.Ohsawa,+ 9643 1451 5 DIST-DEC21 20100318 9643 1451 6 ----JENDL-5 MATERIAL 9643 9643 1451 7 -----INCIDENT NEUTRON DATA 9643 1451 8 ------ENDF-6 FORMAT 9643 1451 9 9643 1451 10 History 9643 1451 11 06-01 Fission cross section was evaluated with GMA. 9643 1451 12 06-05 Resonance parameters were modified. 9643 1451 13 06-11 New calculation was made with CCONE code. 9643 1451 14 07-03 Fission spectra were evaluated. 9643 1451 15 07-05 Re-calculation with CCONE code. 9643 1451 16 08-03 Interpolation of (5,18) was changed. 9643 1451 17 Data were compiled as JENDL/AC-2008/1/. 9643 1451 18 09-08 (MF1,MT458) was evaluated. 9643 1451 19 09-11 New calculation was made with CCONE code. 9643 1451 20 10-01 Data of prompt gamma rays due to fission were given. 9643 1451 21 10-03 Covariance data were given. 9643 1451 22 21-04 JENDL-5b1 9643 1451 23 (MF3,MT2) recalculated 9643 1451 24 (MF3,MT102) modified from 400 eV to 2 MeV 9643 1451 25 21-10 JENDL-5b3 9643 1451 26 (MF2,MT151) revised 9643 1451 27 21-10 Nu-p was revised. 9643 1451 28 21-11 revised by O.Iwamoto 9643 1451 29 (MF3/MT19-21,38) deleted 9643 1451 30 (MF8/MT16-18,102) JENDL/AD-2017 adopted 9643 1451 31 (MF8/MT4) added 9643 1451 32 21-12 revised by S.Nakayama 9643 1451 33 (MF32/MT151) revised 9643 1451 34 9643 1451 35 ==================================================================9643 1451 36 JENDL-5 revised part 9643 1451 37 ==================================================================9643 1451 38 9643 1451 39 MF= 1 General information 9643 1451 40 MT=452 Number of Neutrons per fission 9643 1451 41 Recalculated by sum of MT's=455 and 456. 9643 1451 42 9643 1451 43 MT=456 Number of prompt neutrons per fission 9643 1451 44 Reevaluated with reference to the value measured using a 9643 1451 45 surrogate reaction method by Hirose et al. /1/. 9643 1451 46 9643 1451 47 MF= 2 Resonance parameters 9643 1451 48 MT=151 9643 1451 49 Resolved resonance parameters (MLBW: 1.0E-5 - 400eV) 9643 1451 50 Resonance energies, neutron widths, and radiation widths up 9643 1451 51 to 400 eV reported by Kawase et al. /2/ were adopted. The 9643 1451 52 parameters from 400 to 1000 eV in /2/ were not adopted since 9643 1451 53 it appears to be missing. 9643 1451 54 Fission widths were modified so as to reproduce the fission 9643 1451 55 cross sections of JENDL-4.0. 9643 1451 56 9643 1451 57 MF=32 Covariances of resonance parameters 9643 1451 58 Format of LCOMP=0 was adopted. 9643 1451 59 9643 1451 60 Standard deviations were adopted from the data reported by 9643 1451 61 Kawase et al. /2/. 9643 1451 62 For the parameters not reported in Ref. /2/, the errors of 9643 1451 63 JENDL-4.0 were adopted. 9643 1451 64 9643 1451 65 References 9643 1451 66 1) K.Hirose: private communication (2021). 9643 1451 67 2) S.Kawase et al.: J. Nucl. Sci. Technol., 58, 764 (2021). 9643 1451 68 9643 1451 69 9643 1451 70 ==================================================================9643 1451 71 JENDL-4.0 9643 1451 72 ==================================================================9643 1451 73 9643 1451 74 MF= 1 General information 9643 1451 75 MT=452 Number of Neutrons per fission 9643 1451 76 Sum of MT's = 455 and 456. 9643 1451 77 9643 1451 78 MT=455 Delayed neutron data 9643 1451 79 (same as JENDL-3.3) 9643 1451 80 Evaluated by Maslov et al./2/ 9643 1451 81 * NUMBER OF NEUTRONS PER FISSION FROM TUTTLE'S SYSTEMATICS/3/.9643 1451 82 9643 1451 83 MT=456 Number of prompt neutrons per fission 9643 1451 84 The experimental data of Zhuravlev et al./4/ was adopted. 9643 1451 85 An energy dependent term was based on the systematics derived 9643 1451 86 by Ohsawa/5/. 9643 1451 87 9643 1451 88 MT=458 Components of energy release due to fission 9643 1451 89 Total energy and prompt energy were calculated from mass 9643 1451 90 balance using JENDL-4 fission yields data and mass excess 9643 1451 91 evaluation. Mass excess values were from Audi's 2009 9643 1451 92 evaluation/6/. Delayed energy values were calculated from 9643 1451 93 the energy release for infinite irradiation using JENDL FP 9643 1451 94 Decay Data File 2000 and JENDL-4 yields data. For delayed 9643 1451 95 neutron energy, as the JENDL FP Decay Data File 2000/7/ does 9643 1451 96 not include average neutron energy values, the average values 9643 1451 97 were calculated using the formula shown in the report by 9643 1451 98 T.R. England/8/. The fractions of prompt energy were 9643 1451 99 calculated using the fractions of Sher's evaluation/9/ when 9643 1451 100 they were provided. When the fractions were not given by Sher,9643 1451 101 averaged fractions were used. 9643 1451 102 9643 1451 103 9643 1451 104 MF= 2 Resonance parameters 9643 1451 105 MT=151 9643 1451 106 Resolved resonance parameters (MLBW: 1.0E-5 - 400 eV) 9643 1451 107 The resonance parameters adopted in JENDL-3.3 were evaluated 9643 1451 108 by Maslov et al./2/ They took the data of Berreth et al./10/, 9643 1451 109 Benjamin et ak./11/, Belanova et al./12/, Cote et al./13/ 9643 1451 110 into account, and adjusted the parameters to the fission cross9643 1451 111 section of Moore and Keyworth/14/ and Maguire et al./15,16/ 9643 1451 112 and gave background data to the fission. 9643 1451 113 9643 1451 114 In the present work, the parameters of 4.3-eV resonance and 9643 1451 115 background cross sections were modified. 9643 1451 116 9643 1451 117 The thermal cross sections to be reproduced: 9643 1451 118 Fission = 0.044 +- 0.022 b 9643 1451 119 Benjamin et al./10/, Zhuravlev et al./17/, 9643 1451 120 Serot et al./18/ 9643 1451 121 Capture = 1.15 +- 0.27 b 9643 1451 122 Halperin et al./19/, Gavrilov et al./20/ 9643 1451 123 9643 1451 124 Unresolved resonance parameters (400 eV - 140 keV) 9643 1451 125 Parameters were determined with ASREP code/21/ so as to 9643 1451 126 reproduce the cross sections. They are used only for self- 9643 1451 127 shielding calculations. 9643 1451 128 9643 1451 129 Thermal cross sections and resonance integrals (at 300K) 9643 1451 130 ------------------------------------------------------- 9643 1451 131 0.0253 eV reson. integ.(*) 9643 1451 132 (barns) (barns) 9643 1451 133 ------------------------------------------------------- 9643 1451 134 total 10.445 9643 1451 135 elastic 9.222 9643 1451 136 fission 0.044 7.60 9643 1451 137 capture 1.179 113 9643 1451 138 ------------------------------------------------------- 9643 1451 139 (*) In the energy range from 0.5 eV to 10 MeV. 9643 1451 140 9643 1451 141 9643 1451 142 MF= 3 Neutron cross sections 9643 1451 143 Cross sections above the resolved resonance region except for 9643 1451 144 the elastic scattering (MT=2) and fission cross sections (MT=18,9643 1451 145 19, 20, 21, 38) were calculated with CCONE code/22/. 9643 1451 146 9643 1451 147 MT= 1 Total cross section 9643 1451 148 The cross section was calculated with CC OMP of Soukhovitskii 9643 1451 149 et al./23/ 9643 1451 150 9643 1451 151 MT= 2 Elastic scattering cross section 9643 1451 152 Calculated as total - non-elastic scattering cross sections. 9643 1451 153 9643 1451 154 MT=18 Fission cross section 9643 1451 155 The following experimental data were analyzed with the GMA 9643 1451 156 code/24/: 9643 1451 157 9643 1451 158 Authors Energy range Data points Reference 9643 1451 159 Moore+ 400eV - 2.83MeV 753 /14/ 9643 1451 160 Fomushkin+ 0.3 - 4.5MeV 18 /25/ 9643 1451 161 Maguire+ 0.13eV - 80keV 58 /15/ 9643 1451 162 Fomushkin+ 14.1MeV 1 /26/ 9643 1451 163 Fursov+ 0.164 - 6.8MeV 45 /27/(*1) 9643 1451 164 Ivanin+ 0.637 - 11.37MeV 25 /28/ 9643 1451 165 9643 1451 166 (*1) Ratio to Pu-239 fission. JENDL-3.3 data was used to 9643 1451 167 convert them into the cross section. 9643 1451 168 9643 1451 169 Above 7 MeV, an eye-guided cross section curve was adopted. 9643 1451 170 9643 1451 171 The results of GMA were used to determine the parameters in 9643 1451 172 the CCONE calculation. 9643 1451 173 9643 1451 174 MT=19, 20, 21, 38 Multi-chance fission cross sections 9643 1451 175 Calculated with CCONE code, and renormalized to the total 9643 1451 176 fission cross section (MT=18). 9643 1451 177 9643 1451 178 9643 1451 179 MF= 4 Angular distributions of secondary neutrons 9643 1451 180 MT=2 Elastic scattering 9643 1451 181 Calculated with CCONE code. 9643 1451 182 9643 1451 183 MT=18 Fission 9643 1451 184 Isotropic distributions in the laboratory system were assumed.9643 1451 185 9643 1451 186 9643 1451 187 MF= 5 Energy distributions of secondary neutrons 9643 1451 188 MT=18 Fission neutron spectra 9643 1451 189 Below 6 MeV, calculated by Ohsawa /29/ with modified 9643 1451 190 Madland-Nix formula considering multi-mode fission processes 9643 1451 191 (standard-1, standard-2, superlong). 9643 1451 192 Above 7 MeV, calculated with CCONE code/22/. 9643 1451 193 9643 1451 194 9643 1451 195 MF= 6 Energy-angle distributions 9643 1451 196 Calculated with CCONE code. 9643 1451 197 Distributions from fission (MT=18) are not included. 9643 1451 198 9643 1451 199 9643 1451 200 MF=12 Photon production multiplicities 9643 1451 201 MT=18 Fission 9643 1451 202 Calculated from the total energy released by the prompt 9643 1451 203 gamma-rays due to fission given in MF=1/MT=458 and the 9643 1451 204 average energy of gamma-rays. 9643 1451 205 9643 1451 206 9643 1451 207 MF=14 Photon angular distributions 9643 1451 208 MT=18 Fission 9643 1451 209 Isotoropic distributions were assumed. 9643 1451 210 9643 1451 211 9643 1451 212 MF=15 Continuous photon energy spectra 9643 1451 213 MT=18 Fission 9643 1451 214 Experimental data measured by Verbinski et al./30/ for 9643 1451 215 Pu-239 thermal fission were adopted. 9643 1451 216 9643 1451 217 9643 1451 218 MF=31 Covariances of average number of neutrons per fission 9643 1451 219 MT=452 Number of neutrons per fission 9643 1451 220 Combination of covariances for MT=455 and MT=456. 9643 1451 221 9643 1451 222 MT=455 9643 1451 223 Error of 15% was assumed below 5 MeV and above 5 MeV, 9643 1451 224 respectively. 9643 1451 225 9643 1451 226 MT=456 9643 1451 227 Covariance was obtained by fitting a linear function to the 9643 1451 228 data at the thermal energy /4/ and 5 MeV (derived from 9643 1451 229 systematics) with uncertainties of about 4% and 5%, 9643 1451 230 respectively. 9643 1451 231 9643 1451 232 9643 1451 233 MF=32 Covariances of resonance parameters 9643 1451 234 Format of LCOMP=0 was adopted. 9643 1451 235 9643 1451 236 Standard deviations were adopted from the data of Moore and 9643 1451 237 Keyworth/14/, Belanova et al./12/, and others. 9643 1451 238 For the parameters having no information on uncertainties, 9643 1451 239 the following errors were assumed: 9643 1451 240 0.1% to resonance energies 9643 1451 241 10% to neutron and fission widths 9643 1451 242 20% to capture widths 9643 1451 243 9643 1451 244 MF=33 Covariances of neutron cross sections 9643 1451 245 Covariances were given to all the cross sections by using 9643 1451 246 KALMAN code/31/ and the covariances of model parameters 9643 1451 247 used in the theoretical calculations. 9643 1451 248 9643 1451 249 For the following cross sections, covariances were determined 9643 1451 250 by different methods. 9643 1451 251 9643 1451 252 MT=1, 2 Total and elastic scattering cross sections 9643 1451 253 In the resonance region (below 400 eV), uncertainty of 10 % 9643 1451 254 was added. 9643 1451 255 9643 1451 256 MT=18 Fission cross section 9643 1451 257 In the resonance region, standard deviation of 50 % was 9643 1451 258 added. 9643 1451 259 9643 1451 260 Above the resonance region, cross section was evaluated with 9643 1451 261 GMA code/24/. Standard deviations obtained were multiplied 9643 1451 262 by a factor of 1.5. Above 7 MeV, they were assumed to be 20%. 9643 1451 263 9643 1451 264 MT=102 Capture cross section 9643 1451 265 In the resonance region, addtional error of 15 % was given. 9643 1451 266 9643 1451 267 Above 400 eV, covariance matrix was obtained with CCONE and 9643 1451 268 KALMAN codes/31/. 9643 1451 269 9643 1451 270 9643 1451 271 MF=34 Covariances for Angular Distributions 9643 1451 272 MT=2 Elastic scattering 9643 1451 273 Covariances were given only to P1 components. 9643 1451 274 9643 1451 275 9643 1451 276 MF=35 Covariances for Energy Distributions 9643 1451 277 MT=18 Fission spectra 9643 1451 278 Below 6 MeV, covarinaces of Pu239 fission spectra given in 9643 1451 279 JENDL-3.3 were adopted after multiplying a factor of 9. 9643 1451 280 Above 6 MeV, estimated with CCONE and KALMAN codes. 9643 1451 281 9643 1451 282 9643 1451 283 ***************************************************************** 9643 1451 284 Calculation with CCONE code 9643 1451 285 ***************************************************************** 9643 1451 286 9643 1451 287 Models and parameters used in the CCONE/22/ calculation 9643 1451 288 1) Coupled channel optical model 9643 1451 289 Levels in the rotational band were included. Optical model 9643 1451 290 potential and coupled levels are shown in Table 1. 9643 1451 291 9643 1451 292 2) Two-component exciton model/32/ 9643 1451 293 * Global parametrization of Koning-Duijvestijn/33/ 9643 1451 294 was used. 9643 1451 295 * Gamma emission channel/34/ was added to simulate direct 9643 1451 296 and semi-direct capture reaction. 9643 1451 297 9643 1451 298 3) Hauser-Feshbach statistical model 9643 1451 299 * Moldauer width fluctuation correction/35/ was included. 9643 1451 300 * Neutron, gamma and fission decay channel were included. 9643 1451 301 * Transmission coefficients of neutrons were taken from 9643 1451 302 coupled channel calculation in Table 1. 9643 1451 303 * The level scheme of the target is shown in Table 2. 9643 1451 304 * Level density formula of constant temperature and Fermi-gas 9643 1451 305 model were used with shell energy correction and collective 9643 1451 306 enhancement factor. Parameters are shown in Table 3. 9643 1451 307 * Fission channel: 9643 1451 308 Double humped fission barriers were assumed. 9643 1451 309 Fission barrier penetrabilities were calculated with 9643 1451 310 Hill-Wheler formula/36/. Fission barrier parameters were 9643 1451 311 shown in Table 4. Transition state model was used and 9643 1451 312 continuum levels are assumed above the saddles. The level 9643 1451 313 density parameters for inner and outer saddles are shown in 9643 1451 314 Tables 5 and 6, respectively. 9643 1451 315 * Gamma-ray strength function of Kopecky et al/37/,/38/ 9643 1451 316 was used. The prameters are shown in Table 7. 9643 1451 317 9643 1451 318 9643 1451 319 ------------------------------------------------------------------9643 1451 320 Tables 9643 1451 321 ------------------------------------------------------------------9643 1451 322 9643 1451 323 Table 1. Coupled channel calculation 9643 1451 324 -------------------------------------------------- 9643 1451 325 * rigid rotor model was applied 9643 1451 326 * coupled levels = 0,1,2,3,4 (see Table 2) 9643 1451 327 * optical potential parameters /23/ 9643 1451 328 Volume: 9643 1451 329 V_0 = 49.97 MeV 9643 1451 330 lambda_HF = 0.01004 1/MeV 9643 1451 331 C_viso = 15.9 MeV 9643 1451 332 A_v = 12.04 MeV 9643 1451 333 B_v = 81.36 MeV 9643 1451 334 E_a = 385 MeV 9643 1451 335 r_v = 1.2568 fm 9643 1451 336 a_v = 0.633 fm 9643 1451 337 Surface: 9643 1451 338 W_0 = 17.2 MeV 9643 1451 339 B_s = 11.19 MeV 9643 1451 340 C_s = 0.01361 1/MeV 9643 1451 341 C_wiso = 23.5 MeV 9643 1451 342 r_s = 1.1803 fm 9643 1451 343 a_s = 0.601 fm 9643 1451 344 Spin-orbit: 9643 1451 345 V_so = 5.75 MeV 9643 1451 346 lambda_so = 0.005 1/MeV 9643 1451 347 W_so = -3.1 MeV 9643 1451 348 B_so = 160 MeV 9643 1451 349 r_so = 1.1214 fm 9643 1451 350 a_so = 0.59 fm 9643 1451 351 Coulomb: 9643 1451 352 C_coul = 1.3 9643 1451 353 r_c = 1.2452 fm 9643 1451 354 a_c = 0.545 fm 9643 1451 355 Deformation: 9643 1451 356 beta_2 = 0.2 9643 1451 357 beta_4 = 0.055 9643 1451 358 beta_6 = 0.0015 9643 1451 359 9643 1451 360 * Calculated strength function 9643 1451 361 S0= 0.81e-4 S1= 3.33e-4 R'= 9.06 fm (En=1 keV) 9643 1451 362 -------------------------------------------------- 9643 1451 363 9643 1451 364 Table 2. Level Scheme of Cm-246 9643 1451 365 ------------------- 9643 1451 366 No. Ex(MeV) J PI 9643 1451 367 ------------------- 9643 1451 368 0 0.00000 0 + * 9643 1451 369 1 0.04285 2 + * 9643 1451 370 2 0.14201 4 + * 9643 1451 371 3 0.29490 6 + * 9643 1451 372 4 0.49980 8 + * 9643 1451 373 5 0.84168 2 - 9643 1451 374 6 0.87645 3 - 9643 1451 375 7 0.92331 4 - 9643 1451 376 8 0.98100 5 - 9643 1451 377 9 1.05110 6 - 9643 1451 378 10 1.05900 5 + 9643 1451 379 11 1.07885 1 - 9643 1451 380 12 1.10486 2 - 9643 1451 381 13 1.12428 2 + 9643 1451 382 14 1.12802 3 - 9643 1451 383 15 1.12880 7 - 9643 1451 384 16 1.16549 3 + 9643 1451 385 17 1.17474 0 + 9643 1451 386 18 1.17860 8 - 9643 1451 387 19 1.21053 2 + 9643 1451 388 20 1.21998 4 + 9643 1451 389 21 1.22100 3 + 9643 1451 390 22 1.24977 1 - 9643 1451 391 23 1.28930 0 + 9643 1451 392 24 1.30045 3 - 9643 1451 393 25 1.31757 2 + 9643 1451 394 26 1.34020 3 - 9643 1451 395 27 1.34886 1 - 9643 1451 396 28 1.36663 2 - 9643 1451 397 29 1.37923 4 + 9643 1451 398 30 1.39700 5 - 9643 1451 399 ------------------- 9643 1451 400 *) Coupled levels in CC calculation 9643 1451 401 9643 1451 402 Table 3. Level density parameters 9643 1451 403 -------------------------------------------------------- 9643 1451 404 Nuclide a* Pair Eshell T E0 Ematch 9643 1451 405 1/MeV MeV MeV MeV MeV MeV 9643 1451 406 -------------------------------------------------------- 9643 1451 407 Cm-247 18.3955 0.7635 1.7794 0.3734 -0.6804 2.7533 9643 1451 408 Cm-246 18.8984 1.5302 1.7310 0.3608 0.1621 3.4286 9643 1451 409 Cm-245 18.8322 0.7667 1.4601 0.3623 -0.5771 2.6382 9643 1451 410 Cm-244 19.1414 1.5364 1.5347 0.3530 0.2436 3.3454 9643 1451 411 Cm-243 18.3259 0.7698 1.3577 0.3635 -0.5169 2.5698 9643 1451 412 -------------------------------------------------------- 9643 1451 413 9643 1451 414 Table 4. Fission barrier parameters 9643 1451 415 ---------------------------------------- 9643 1451 416 Nuclide V_A hw_A V_B hw_B 9643 1451 417 MeV MeV MeV MeV 9643 1451 418 ---------------------------------------- 9643 1451 419 Cm-247 5.400 0.800 5.650 0.650 9643 1451 420 Cm-246 6.300 1.040 5.100 0.600 9643 1451 421 Cm-245 6.050 0.500 5.700 0.420 9643 1451 422 Cm-244 6.100 0.900 5.100 0.600 9643 1451 423 Cm-243 6.150 0.600 5.800 0.400 9643 1451 424 ---------------------------------------- 9643 1451 425 9643 1451 426 Table 5. Level density above inner saddle 9643 1451 427 -------------------------------------------------------- 9643 1451 428 Nuclide a* Pair Eshell T E0 Ematch 9643 1451 429 1/MeV MeV MeV MeV MeV MeV 9643 1451 430 -------------------------------------------------------- 9643 1451 431 Cm-247 20.8609 0.8908 2.6000 0.3256 -1.5320 2.8908 9643 1451 432 Cm-246 20.7882 1.6500 2.6000 0.3263 -0.7728 3.6500 9643 1451 433 Cm-245 20.7155 0.8944 2.6000 0.3342 -1.6357 2.9944 9643 1451 434 Cm-244 20.6427 1.7925 2.6000 0.3275 -0.6303 3.7925 9643 1451 435 Cm-243 20.5699 0.8981 2.6000 0.3281 -1.5248 2.8981 9643 1451 436 -------------------------------------------------------- 9643 1451 437 9643 1451 438 Table 6. Level density above outer saddle 9643 1451 439 -------------------------------------------------------- 9643 1451 440 Nuclide a* Pair Eshell T E0 Ematch 9643 1451 441 1/MeV MeV MeV MeV MeV MeV 9643 1451 442 -------------------------------------------------------- 9643 1451 443 Cm-247 20.8609 0.8908 0.8200 0.3573 -0.8210 2.8908 9643 1451 444 Cm-246 20.7882 1.7852 0.7800 0.3658 -0.0107 3.8852 9643 1451 445 Cm-245 20.7155 0.8944 0.7400 0.3596 -0.8163 2.8944 9643 1451 446 Cm-244 20.6427 1.7925 0.7000 0.3455 0.2502 3.5925 9643 1451 447 Cm-243 20.5699 0.8981 0.6600 0.3619 -0.8115 2.8981 9643 1451 448 -------------------------------------------------------- 9643 1451 449 9643 1451 450 Table 7. Gamma-ray strength function for Cm-247 9643 1451 451 -------------------------------------------------------- 9643 1451 452 * E1: ER = 11.41 (MeV) EG = 2.72 (MeV) SIG = 330.04 (mb) 9643 1451 453 ER = 14.31 (MeV) EG = 4.19 (MeV) SIG = 427.95 (mb) 9643 1451 454 * M1: ER = 6.53 (MeV) EG = 4.00 (MeV) SIG = 1.47 (mb) 9643 1451 455 * E2: ER = 10.04 (MeV) EG = 3.15 (MeV) SIG = 7.06 (mb) 9643 1451 456 -------------------------------------------------------- 9643 1451 457 9643 1451 458 9643 1451 459 References 9643 1451 460 1) O.Iwamoto et al.: J. Nucl. Sci. 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C47, 312 (1990). 9643 1451 500 9643 1451 501 1 451 513 19643 1451 502 2 151 4 19643 1451 503 3 4 33 19643 1451 504 3 16 12 19643 1451 505 3 17 8 19643 1451 506 3 18 808 19643 1451 507 3 102 2125 19643 1451 508 8 4 2 19643 1451 509 8 16 2 19643 1451 510 8 17 2 19643 1451 511 8 18 2 19643 1451 512 8 102 2 19643 1451 513 9643 1 099999 9643 0 0 0 9.624600+4 2.439530+2 0 0 1 09643 2151 1 9.624600+4 1.000000+0 0 0 1 09643 2151 2 1.000000-5 4.000000+2 0 0 0 09643 2151 3 0.000000+0 9.040000-1 0 0 0 09643 2151 4 9643 2 099999 9643 0 0 0 9.624600+4 2.439530+2 0 0 0 09643 3 4 1 0.000000+0-4.285100+4 0 0 1 889643 3 4 2 88 2 9643 3 4 3 4.302670+4 0.000000+0 5.000000+4 1.228910-1 7.000000+4 4.497660-19643 3 4 4 1.000000+5 7.503120-1 1.150000+5 8.534100-1 1.300000+5 9.565169-19643 3 4 5 1.425920+5 1.020869+0 1.700000+5 1.135219+0 2.000000+5 1.232539+09643 3 4 6 2.961090+5 1.461735+0 3.000000+5 1.467882+0 4.000000+5 1.643570+09643 3 4 7 5.000000+5 1.727473+0 5.018490+5 1.729875+0 6.000000+5 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3.602269+2 6.546807+09643 3102 1855 3.602462+2 6.874549+0 3.602654+2 7.236541+0 3.602856+2 7.658415+09643 3102 1856 3.603067+2 8.153336+0 3.603239+2 8.605293+0 3.603441+2 9.194368+09643 3102 1857 3.603633+2 9.825166+0 3.603778+2 1.035214+1 3.603922+2 1.092646+19643 3102 1858 3.604066+2 1.155399+1 3.604210+2 1.224132+1 3.604383+2 1.315226+19643 3102 1859 3.604536+2 1.405198+1 3.604680+2 1.498069+1 3.604824+2 1.599946+19643 3102 1860 3.604968+2 1.712026+1 3.605113+2 1.834964+1 3.605270+2 1.982773+19643 3102 1861 3.605393+2 2.108558+1 3.605516+2 2.244441+1 3.605639+2 2.391139+19643 3102 1862 3.605777+2 2.570247+1 3.605931+2 2.788016+1 3.606084+2 3.026866+19643 3102 1863 3.606238+2 3.288417+1 3.606392+2 3.574334+1 3.606546+2 3.886297+19643 3102 1864 3.606699+2 4.225976+1 3.606853+2 4.595035+1 3.607007+2 4.995111+19643 3102 1865 3.607161+2 5.427773+1 3.607314+2 5.894482+1 3.607468+2 6.396597+19643 3102 1866 3.607622+2 6.934893+1 3.607775+2 7.510313+1 3.607929+2 8.124080+19643 3102 1867 3.608082+2 8.776766+1 3.608236+2 9.469273+1 3.608467+2 1.058252+29643 3102 1868 3.608697+2 1.178275+2 3.608928+2 1.306645+2 3.609158+2 1.442808+29643 3102 1869 3.609466+2 1.635001+2 3.609850+2 1.888492+2 3.610778+2 2.522548+29643 3102 1870 3.611147+2 2.761288+2 3.611479+2 2.958782+2 3.611774+2 3.114516+29643 3102 1871 3.612032+2 3.232354+2 3.612315+2 3.338323+2 3.612573+2 3.411468+29643 3102 1872 3.612785+2 3.453571+2 3.613016+2 3.480120+2 3.613197+2 3.486517+29643 3102 1873 3.613415+2 3.477300+2 3.613618+2 3.452267+2 3.613839+2 3.407292+29643 3102 1874 3.614060+2 3.344638+2 3.614282+2 3.265374+2 3.614515+2 3.165049+29643 3102 1875 3.614774+2 3.036309+2 3.615106+2 2.848564+2 3.615475+2 2.616731+29643 3102 1876 3.615982+2 2.274782+2 3.616612+2 1.844038+2 3.616935+2 1.631994+29643 3102 1877 3.617257+2 1.430887+2 3.617503+2 1.286622+2 3.617749+2 1.151320+29643 3102 1878 3.617934+2 1.056103+2 3.618118+2 9.664540+1 3.618318+2 8.757292+19643 3102 1879 3.618471+2 8.104863+1 3.618625+2 7.491355+1 3.618779+2 6.916187+19643 3102 1880 3.618932+2 6.378519+1 3.619086+2 5.877322+1 3.619240+2 5.411397+19643 3102 1881 3.619393+2 4.979388+1 3.619518+2 4.652270+1 3.619662+2 4.300261+19643 3102 1882 3.619806+2 3.974340+1 3.619950+2 3.673183+1 3.620094+2 3.395387+19643 3102 1883 3.620239+2 3.139607+1 3.620383+2 2.904406+1 3.620527+2 2.688504+19643 3102 1884 3.620671+2 2.490555+1 3.620815+2 2.309296+1 3.620959+2 2.143479+19643 3102 1885 3.621070+2 2.025089+1 3.621197+2 1.900081+1 3.621324+2 1.784715+19643 3102 1886 3.621451+2 1.678290+1 3.621578+2 1.580138+1 3.621704+2 1.489631+19643 3102 1887 3.621831+2 1.406179+1 3.621958+2 1.329227+1 3.622085+2 1.258252+19643 3102 1888 3.622212+2 1.192769+1 3.622339+2 1.132329+1 3.622529+2 1.050220+19643 3102 1889 3.622719+2 9.772248+0 3.622909+2 9.122172+0 3.623113+2 8.503312+09643 3102 1890 3.623266+2 8.082688+0 3.623420+2 7.697302+0 3.623651+2 7.177390+09643 3102 1891 3.623881+2 6.717776+0 3.624111+2 6.309456+0 3.624342+2 5.944781+09643 3102 1892 3.624572+2 5.617391+0 3.624803+2 5.321946+0 3.625033+2 5.054014+09643 3102 1893 3.625340+2 4.733220+0 3.625590+2 4.498712+0 3.625878+2 4.252861+09643 3102 1894 3.626166+2 4.029886+0 3.626455+2 3.826626+0 3.626839+2 3.581862+09643 3102 1895 3.627223+2 3.362657+0 3.627607+2 3.165153+0 3.627992+2 2.986273+09643 3102 1896 3.628376+2 2.823528+0 3.628799+2 2.660732+0 3.629260+2 2.499973+09643 3102 1897 3.629721+2 2.354448+0 3.630182+2 2.222185+0 3.630643+2 2.101539+09643 3102 1898 3.631104+2 1.991124+0 3.631565+2 1.889766+0 3.632026+2 1.796462+09643 3102 1899 3.632563+2 1.696630+0 3.633178+2 1.593023+0 3.633793+2 1.499207+09643 3102 1900 3.634408+2 1.413950+0 3.635022+2 1.336212+0 3.635637+2 1.265111+09643 3102 1901 3.636252+2 1.199893+0 3.636867+2 1.139913+0 3.637558+2 1.078005+09643 3102 1902 3.638327+2 1.015335+0 3.639095+2 9.583331-1 3.639863+2 9.063224-19643 3102 1903 3.640632+2 8.587252-1 3.641400+2 8.150470-1 3.642168+2 7.748619-19643 3102 1904 3.643321+2 7.203399-1 3.644320+2 6.779577-1 3.645319+2 6.395016-19643 3102 1905 3.646318+2 6.044877-1 3.647317+2 5.725059-1 3.648316+2 5.432064-19643 3102 1906 3.649315+2 5.162921-1 3.650814+2 4.798440-1 3.652005+2 4.538140-19643 3102 1907 3.653388+2 4.264221-1 3.654771+2 4.016981-1 3.656154+2 3.793051-19643 3102 1908 3.657537+2 3.589577-1 3.658920+2 3.404134-1 3.660303+2 3.234653-19643 3102 1909 3.661686+2 3.079357-1 3.663300+2 2.914083-1 3.665144+2 2.743661-19643 3102 1910 3.666988+2 2.590462-1 3.668832+2 2.452343-1 3.670677+2 2.327506-19643 3102 1911 3.672521+2 2.214364-1 3.674365+2 2.111484-1 3.676209+2 2.017655-19643 3102 1912 3.678360+2 1.918373-1 3.680819+2 1.816858-1 3.683278+2 1.726585-19643 3102 1913 3.685737+2 1.646205-1 3.688196+2 1.574584-1 3.690655+2 1.510766-19643 3102 1914 3.693114+2 1.453947-1 3.695573+2 1.403453-1 3.699261+2 1.338354-19643 3102 1915 3.702949+2 1.284695-1 3.706638+2 1.241365-1 3.710326+2 1.207507-19643 3102 1916 3.714014+2 1.182266-1 3.716473+2 1.170217-1 3.719826+2 1.159830-19643 3102 1917 3.723180+2 1.156196-1 3.726904+2 1.160395-1 3.730628+2 1.173768-19643 3102 1918 3.734352+2 1.196840-1 3.736834+2 1.218122-1 3.739317+2 1.244675-19643 3102 1919 3.741800+2 1.276998-1 3.744253+2 1.315178-1 3.746678+2 1.359693-19643 3102 1920 3.749102+2 1.411805-1 3.751527+2 1.472546-1 3.753951+2 1.543172-19643 3102 1921 3.756376+2 1.625205-1 3.758194+2 1.695303-1 3.760013+2 1.773769-19643 3102 1922 3.761831+2 1.861757-1 3.763713+2 1.964391-1 3.765627+2 2.082735-19643 3102 1923 3.767542+2 2.217455-1 3.768818+2 2.317718-1 3.770094+2 2.427468-19643 3102 1924 3.771370+2 2.547847-1 3.772646+2 2.680180-1 3.773794+2 2.810761-19643 3102 1925 3.774943+2 2.953579-1 3.776091+2 3.110148-1 3.777240+2 3.282225-19643 3102 1926 3.778388+2 3.471865-1 3.779536+2 3.681473-1 3.780685+2 3.913884-19643 3102 1927 3.781833+2 4.172446-1 3.783077+2 4.486778-1 3.783907+2 4.718995-19643 3102 1928 3.784736+2 4.971836-1 3.785566+2 5.247821-1 3.786395+2 5.549880-19643 3102 1929 3.787225+2 5.881438-1 3.788054+2 6.246507-1 3.788788+2 6.601138-19643 3102 1930 3.789426+2 6.936759-1 3.790064+2 7.300772-1 3.790702+2 7.696504-19643 3102 1931 3.791340+2 8.127792-1 3.791978+2 8.599084-1 3.792616+2 9.115559-19643 3102 1932 3.793254+2 9.683286-1 3.793828+2 1.024394+0 3.794339+2 1.078693+09643 3102 1933 3.794849+2 1.137712+0 3.795359+2 1.202030+0 3.795870+2 1.272323+09643 3102 1934 3.796380+2 1.349382+0 3.796890+2 1.434140+0 3.797401+2 1.527709+09643 3102 1935 3.797863+2 1.621237+0 3.798278+2 1.713158+0 3.798693+2 1.813761+09643 3102 1936 3.799108+2 1.924271+0 3.799522+2 2.046175+0 3.799937+2 2.181296+09643 3102 1937 3.800352+2 2.331909+0 3.800663+2 2.456751+0 3.800974+2 2.593441+09643 3102 1938 3.801293+2 2.747916+0 3.801612+2 2.919363+0 3.801931+2 3.110989+09643 3102 1939 3.802170+2 3.270364+0 3.802410+2 3.445493+0 3.802649+2 3.638964+09643 3102 1940 3.802888+2 3.853891+0 3.803127+2 4.094105+0 3.803367+2 4.364179+09643 3102 1941 3.803526+2 4.563531+0 3.803749+2 4.872743+0 3.803917+2 5.131068+09643 3102 1942 3.804084+2 5.415345+0 3.804252+2 5.729024+0 3.804419+2 6.075951+09643 3102 1943 3.804586+2 6.460600+0 3.804754+2 6.887828+0 3.804921+2 7.363228+09643 3102 1944 3.805089+2 7.892974+0 3.805256+2 8.484033+0 3.805384+2 8.980686+09643 3102 1945 3.805528+2 9.592464+0 3.805671+2 1.026552+1 3.805815+2 1.100609+19643 3102 1946 3.805967+2 1.186782+1 3.806086+2 1.261156+1 3.806206+2 1.341635+19643 3102 1947 3.806337+2 1.437541+1 3.806461+2 1.535809+1 3.806585+2 1.642062+19643 3102 1948 3.806708+2 1.757084+1 3.806844+2 1.894656+1 3.806963+2 2.025362+19643 3102 1949 3.807083+2 2.166713+1 3.807203+2 2.318999+1 3.807323+2 2.482358+19643 3102 1950 3.807442+2 2.657776+1 3.807562+2 2.845905+1 3.807681+2 3.047436+19643 3102 1951 3.807801+2 3.263011+1 3.807940+2 3.531611+1 3.808079+2 3.821058+19643 3102 1952 3.808235+2 4.173281+1 3.808362+2 4.482239+1 3.808490+2 4.811320+19643 3102 1953 3.808617+2 5.161192+1 3.808745+2 5.532860+1 3.808937+2 6.132370+19643 3102 1954 3.809128+2 6.783016+1 3.809320+2 7.484858+1 3.809511+2 8.238732+19643 3102 1955 3.809702+2 9.044860+1 3.809893+2 9.902565+1 3.810085+2 1.081007+29643 3102 1956 3.810340+2 1.209460+2 3.810595+2 1.345658+2 3.810914+2 1.524674+29643 3102 1957 3.811489+2 1.862943+2 3.812081+2 2.212992+2 3.812407+2 2.396107+29643 3102 1958 3.812724+2 2.560312+2 3.813030+2 2.702180+2 3.813275+2 2.801110+29643 3102 1959 3.813490+2 2.875140+2 3.813724+2 2.941548+2 3.813938+2 2.987911+29643 3102 1960 3.814169+2 3.021513+2 3.814388+2 3.037494+2 3.814500+2 3.039496+29643 3102 1961 3.814755+2 3.028502+2 3.814990+2 2.999446+2 3.815235+2 2.950434+29643 3102 1962 3.815480+2 2.883296+2 3.815766+2 2.783807+2 3.816011+2 2.682285+29643 3102 1963 3.816297+2 2.547837+2 3.816626+2 2.375677+2 3.817001+2 2.163412+29643 3102 1964 3.817971+2 1.589171+2 3.818277+2 1.414644+2 3.818596+2 1.241703+29643 3102 1965 3.818826+2 1.124092+2 3.819055+2 1.013109+2 3.819285+2 9.092292+19643 3102 1966 3.819477+2 8.283169+1 3.819630+2 7.673595+1 3.819783+2 7.097625+19643 3102 1967 3.819936+2 6.555112+1 3.820089+2 6.045655+1 3.820242+2 5.568655+19643 3102 1968 3.820395+2 5.123335+1 3.820548+2 4.708748+1 3.820673+2 4.393787+19643 3102 1969 3.820816+2 4.053893+1 3.820960+2 3.738148+1 3.821103+2 3.445493+19643 3102 1970 3.821247+2 3.174774+1 3.821390+2 2.924872+1 3.821534+2 2.694556+19643 3102 1971 3.821678+2 2.482726+1 3.821821+2 2.288199+1 3.821965+2 2.109856+19643 3102 1972 3.822108+2 1.946573+1 3.822212+2 1.837385+1 3.822324+2 1.727488+19643 3102 1973 3.822435+2 1.625139+1 3.822547+2 1.529878+1 3.822659+2 1.441260+19643 3102 1974 3.822770+2 1.358863+1 3.822882+2 1.282284+1 3.822994+2 1.211138+19643 3102 1975 3.823105+2 1.145054+1 3.823217+2 1.083683+1 3.823329+2 1.026698+19643 3102 1976 3.823496+2 9.487703+0 3.823664+2 8.790263+0 3.823831+2 8.165907+09643 3102 1977 3.823943+2 7.786238+0 3.824087+2 7.337014+0 3.824230+2 6.927587+09643 3102 1978 3.824374+2 6.553995+0 3.824517+2 6.212714+0 3.824661+2 5.900465+09643 3102 1979 3.824804+2 5.614379+0 3.824948+2 5.351792+0 3.825163+2 4.996875+09643 3102 1980 3.825379+2 4.682574+0 3.825594+2 4.402924+0 3.825809+2 4.152914+09643 3102 1981 3.826025+2 3.928284+0 3.826240+2 3.725476+0 3.826527+2 3.483884+09643 3102 1982 3.826814+2 3.269939+0 3.827101+2 3.078992+0 3.827388+2 2.907368+09643 3102 1983 3.827675+2 2.752112+0 3.827962+2 2.610867+0 3.828345+2 2.441073+09643 3102 1984 3.828728+2 2.289225+0 3.829111+2 2.152533+0 3.829525+2 2.019001+09643 3102 1985 3.829972+2 1.889664+0 3.830419+2 1.773196+0 3.830865+2 1.667817+09643 3102 1986 3.831312+2 1.572073+0 3.831758+2 1.484760+0 3.832205+2 1.404871+09643 3102 1987 3.832652+2 1.331552+0 3.833162+2 1.254871+0 3.833736+2 1.176581+09643 3102 1988 3.834311+2 1.105679+0 3.834885+2 1.041241+0 3.835459+2 9.824830-19643 3102 1989 3.836033+2 9.287429-1 3.836608+2 8.794536-1 3.837182+2 8.341273-19643 3102 1990 3.837820+2 7.879059-1 3.838522+2 7.415240-1 3.839223+2 6.992664-19643 3102 1991 3.839925+2 6.606513-1 3.840627+2 6.252655-1 3.841329+2 5.927534-19643 3102 1992 3.842030+2 5.628070-1 3.843083+2 5.221218-1 3.843976+2 4.910834-19643 3102 1993 3.844870+2 4.628328-1 3.845763+2 4.370402-1 3.846656+2 4.134256-19643 3102 1994 3.847549+2 3.917478-1 3.848443+2 3.718001-1 3.849336+2 3.534017-19643 3102 1995 3.850229+2 3.363957-1 3.851378+2 3.163555-1 3.852526+2 2.981368-19643 3102 1996 3.853675+2 2.815230-1 3.854823+2 2.663294-1 3.855972+2 2.523968-19643 3102 1997 3.857120+2 2.395884-1 3.858269+2 2.277851-1 3.859417+2 2.168834-19643 3102 1998 3.860693+2 2.057188-1 3.861969+2 1.954477-1 3.863883+2 1.815149-19643 3102 1999 3.865797+2 1.691191-1 3.867711+2 1.580429-1 3.869625+2 1.481042-19643 3102 2000 3.871412+2 1.397146-1 3.873198+2 1.320705-1 3.874985+2 1.250837-19643 3102 2001 3.876771+2 1.186819-1 3.878558+2 1.128021-1 3.881237+2 1.048418-19643 3102 2002 3.883917+2 9.777366-2 3.886469+2 9.175206-2 3.889021+2 8.632867-29643 3102 2003 3.891573+2 8.142768-2 3.894126+2 7.698452-2 3.896678+2 7.293789-29643 3102 2004 3.899230+2 6.923463-2 3.901782+2 6.583821-2 3.904334+2 6.272085-29643 3102 2005 3.908162+2 5.850440-2 3.911990+2 5.475991-2 3.915818+2 5.141752-29643 3102 2006 3.919646+2 4.842449-2 3.923474+2 4.572841-2 3.927436+2 4.319926-29643 3102 2007 3.931465+2 4.087813-2 3.935494+2 3.877952-2 3.940867+2 3.626884-29643 3102 2008 3.946239+2 3.403757-2 3.951356+2 3.214221-2 3.956473+2 3.044303-29643 3102 2009 3.961590+2 2.890530-2 3.966707+2 2.750745-2 3.972041+2 2.618427-29643 3102 2010 3.977375+2 2.498080-2 3.984042+2 2.362389-2 3.987375+2 2.303110-29643 3102 2011 3.988229+2 2.296146-2 3.988789+2 2.300846-2 3.989163+2 2.312476-29643 3102 2012 3.989537+2 2.335639-2 3.989817+2 2.364341-2 3.990097+2 2.406881-29643 3102 2013 3.990284+2 2.445358-2 3.990471+2 2.494070-2 3.990658+2 2.555241-29643 3102 2014 3.990845+2 2.631524-2 3.991032+2 2.726039-2 3.991172+2 2.811095-29643 3102 2015 3.991312+2 2.910229-2 3.991452+2 3.025441-2 3.991592+2 3.158942-29643 3102 2016 3.991732+2 3.313219-2 3.991872+2 3.491004-2 3.992012+2 3.695346-29643 3102 2017 3.992153+2 3.929561-2 3.992293+2 4.197386-2 3.992386+2 4.396552-29643 3102 2018 3.992480+2 4.613705-2 3.992573+2 4.850222-2 3.992666+2 5.107543-29643 3102 2019 3.992760+2 5.387172-2 3.992853+2 5.690706-2 3.992947+2 6.019841-29643 3102 2020 3.993040+2 6.376349-2 3.993134+2 6.762070-2 3.993227+2 7.178944-29643 3102 2021 3.993320+2 7.629029-2 3.993414+2 8.114447-2 3.993507+2 8.637378-29643 3102 2022 3.993601+2 9.200114-2 3.993694+2 9.805060-2 3.993787+2 1.045469-19643 3102 2023 3.993881+2 1.115152-1 3.993974+2 1.189819-1 3.994068+2 1.269748-19643 3102 2024 3.994161+2 1.355218-1 3.994255+2 1.446509-1 3.994348+2 1.543915-19643 3102 2025 3.994441+2 1.647737-1 3.994535+2 1.758281-1 3.994675+2 1.937370-19643 3102 2026 3.994815+2 2.133353-1 3.994955+2 2.347297-1 3.995095+2 2.580312-19643 3102 2027 3.995236+2 2.833468-1 3.995376+2 3.107875-1 3.995516+2 3.404568-19643 3102 2028 3.995656+2 3.724693-1 3.995796+2 4.069180-1 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