JENDL-5 (Neutron sublibrary (up to 20 MeV)) Pa-231 0 0 0 0 9.123100+4 2.290510+2 1 1 6 19131 1451 1 0.000000+0 1.000000+0 0 0 0 69131 1451 2 1.000000+0 2.000000+7 0 0 10 59131 1451 3 0.000000+0 0.000000+0 3 0 472 1349131 1451 4 91-Pa-231 JAEA+ EVAL-JAN10 O.Iwamoto, T.Nakagawa, et al. 9131 1451 5 DIST-DEC21 20100323 9131 1451 6 ----JENDL-5 MATERIAL 9131 9131 1451 7 -----INCIDENT NEUTRON DATA 9131 1451 8 ------ENDF-6 FORMAT 9131 1451 9 9131 1451 10 History 9131 1451 11 05-11 Fission cross section was evaluated with GMA code. 9131 1451 12 06-08 Resonance parameters were revised. 9131 1451 13 07-10 Theoretical calculation was performed with CCONE code. 9131 1451 14 Data were compiled as JENDL/AC-2008/1/. 9131 1451 15 09-04 MF01 was revised. 9131 1451 16 09-08 (MF1,MT458) was evaluated. 9131 1451 17 10-01 Data of prompt gamma rays due to fission were given. 9131 1451 18 10-03 Covariance data were given. 9131 1451 19 9131 1451 20 21-11 revised by O.Iwamoto 9131 1451 21 (MF3/MT19-21,38) deleted 9131 1451 22 (MF8/MT16-18,102) JENDL/AD-2017 adopted 9131 1451 23 (MF8/MT4) added 9131 1451 24 9131 1451 25 MF=1 General information 9131 1451 26 MT=452 Number of Neutrons per fission 9131 1451 27 Sum of MT's=455 and 456. 9131 1451 28 9131 1451 29 MT=455 Delayed neutron data 9131 1451 30 Determined from nu-d of the following three fissioning 9131 1451 31 nuclides and partial fission cross sections calculated with 9131 1451 32 CCONE code/2/. 9131 1451 33 Pa-232 = 0.01083 9131 1451 34 Pa-231 = 0.007461 9131 1451 35 Pa-230 = 0.005154 9131 1451 36 They are averages of systematics by Tuttle/3/, 9131 1451 37 Benedetti et al./4/ and Waldo et al./5/ 9131 1451 38 9131 1451 39 Decay constants were evaluated by Brady and England/6/. 9131 1451 40 9131 1451 41 MT=456 Number of prompt neutrons per fission 9131 1451 42 Estimated from Ohsawa's systematics/7/. 9131 1451 43 9131 1451 44 MT=458 Components of energy release due to fission 9131 1451 45 Total energy and prompt energy were calculated from mass 9131 1451 46 balance using JENDL-4 fission yields data and mass excess 9131 1451 47 evaluation. Mass excess values were from Audi's 2009 9131 1451 48 evaluation/8/. Delayed energy values were calculated from 9131 1451 49 the energy release for infinite irradiation using JENDL FP 9131 1451 50 Decay Data File 2000 and JENDL-4 yields data. For delayed 9131 1451 51 neutron energy, as the JENDL FP Decay Data File 2000/9/ does 9131 1451 52 not include average neutron energy values, the average values 9131 1451 53 were calculated using the formula shown in the report by 9131 1451 54 T.R. England/10/. The fractions of prompt energy were 9131 1451 55 calculated using the fractions of Sher's evaluation/11/ when 9131 1451 56 they were provided. When the fractions were not given by Sher,9131 1451 57 averaged fractions were used. 9131 1451 58 9131 1451 59 9131 1451 60 MF= 2 Resonance parameters 9131 1451 61 MT=151 9131 1451 62 Resolved resonance parameters (MLBW; below 115 eV) 9131 1451 63 The resonance parameters of JENDL-3.3 were based on the 9131 1451 64 following data: 9131 1451 65 Resonance energies, neutron and gamma widths: 9131 1451 66 Hussein et al./12/ 9131 1451 67 Fission area: Plattard et al./13/ 9131 1451 68 Parameters of resonances below 1.24 eV: Mughabghab/14/ 9131 1451 69 9131 1451 70 Those data were revised by comparing with the total cross 9131 1451 71 section of Simpson et al./15/ and the fission cross section 9131 1451 72 of Kobayashi et al./16/ 9131 1451 73 9131 1451 74 The resonance formula was changed to MLBW. Total spin of each 9131 1451 75 level was assumed with JCONV code/17/. 9131 1451 76 9131 1451 77 Thermal cross section and resonance integral calculated from 9131 1451 78 the present resonance parameters are given in the following 9131 1451 79 table. The thermal cross sections to be reproduced were 9131 1451 80 determined from experimental data: 9131 1451 81 Total = 211.0+-3.1 b 9131 1451 82 Simpson et al./15/ 9131 1451 83 9131 1451 84 Fission = 0.0239+-0.0007 b 9131 1451 85 Wagemans et al./18,19/, Kobayashi et al./20/ 9131 1451 86 9131 1451 87 Capture = 202.2+-5.3 b 9131 1451 88 Smith et al./21/, Aleksandrov et al./22/, 9131 1451 89 Gryntakis et al./23/, Kobayashi/24/ 9131 1451 90 9131 1451 91 The capture resonance integrals reported by Jurova et al./25/ 9131 1451 92 and Aleksandrov et al./22/ were 1044b and 1180b, respectively.9131 1451 93 9131 1451 94 Unresolved resonance parameters (115 eV - 10 keV) 9131 1451 95 Cross sections were reproduced with average resonance 9131 1451 96 parameters determined by ASREP code/26/. These parameters 9131 1451 97 are used only for self-shielding effects. 9131 1451 98 9131 1451 99 Thermal cross sections and resonance integrals (at 300K) 9131 1451 100 ------------------------------------------------------- 9131 1451 101 0.0253 eV reson. integ.(*) 9131 1451 102 (barns) (barns) 9131 1451 103 ------------------------------------------------------- 9131 1451 104 total 212.32 9131 1451 105 elastic 10.59 9131 1451 106 fission 0.0236 3.24 9131 1451 107 capture 201.71 542 9131 1451 108 ------------------------------------------------------- 9131 1451 109 (*) In the energy range from 0.5 eV to 10 MeV. 9131 1451 110 9131 1451 111 9131 1451 112 MF= 3 Neutron cross sections 9131 1451 113 Cross sections above the resolved resonance region except for 9131 1451 114 elastic scattering and fission cross sections (MT's =2, 18-21, 9131 1451 115 38) were calculated with CCONE code/2/. 9131 1451 116 9131 1451 117 MT= 1 Total cross section 9131 1451 118 The cross section was calculated with CC OMP of Soukhovitskii 9131 1451 119 et al./27/ with modification of the quadrupole deformation 9131 1451 120 parameter. 9131 1451 121 9131 1451 122 MT=2 Elastic scattering cross section 9131 1451 123 Calculated as total - non-elstic scattering cross sections 9131 1451 124 9131 1451 125 MT=18 Fission cross section (Above 115 eV) 9131 1451 126 The following experimental data were analyzed in the energy 9131 1451 127 ranges from 115 eV to 12 keV, and from 110 keV to 12 MeV with 9131 1451 128 the GMA code/28/: 9131 1451 129 9131 1451 130 Authors Energy range Data points Reference 9131 1451 131 Plattard+ 0.112 - 16.9 MeV 4120 /29/ 9131 1451 132 Fursov+ 0.135 - 7.4 MeV 69 /30/(*1) 9131 1451 133 Kobayashi+ 0.089 - 12.6 keV 44 /16/ 9131 1451 134 Oberstedt+ 0.76 - 3.46 MeV 15 /31/ 9131 1451 135 (*1) The data were measured relatively to Pu-239 fission. 9131 1451 136 They were converted to Pa-231 fission by using JENDL-9131 1451 137 3.3 data. 9131 1451 138 The results of the analysis were adopted in the energy ranges 9131 1451 139 from 115 eV to 10 keV and from 120 keV to 9.5 MeV. 9131 1451 140 9131 1451 141 CCONE calculation was adopted in the energy ranges from 10 to 9131 1451 142 120 keV and above 9.5 MeV. 9131 1451 143 9131 1451 144 The results of GMA below 10 MeV, the preliminary experimental 9131 1451 145 data of IRMM/32/ above 15 MeV, and the experimental data of 9131 1451 146 Birgul and Lyle/33/ at 15 MeV were used to determine the 9131 1451 147 parameters in the CCONE calculation. 9131 1451 148 9131 1451 149 MT=19, 20, 21, 38 Multi-chance fission cross sections 9131 1451 150 Calculated with CCONE code, and renormalized to the total 9131 1451 151 fission cross section (MT=18). 9131 1451 152 9131 1451 153 9131 1451 154 MF= 4 Angular distributions of secondary neutrons 9131 1451 155 MT=2 Elastic scattering 9131 1451 156 Calculated with CCONE code/2/. 9131 1451 157 9131 1451 158 MT=18 Fission 9131 1451 159 Isotropic distributions in the laboratory system were assumed.9131 1451 160 9131 1451 161 MF= 5 Energy distributions of secondary neutrons 9131 1451 162 MT=18 Prompt neutrons 9131 1451 163 Calculated with CCONE code/2/. 9131 1451 164 9131 1451 165 MT=455 Delayed neutrons 9131 1451 166 Calculated by Brady and England/6/. 9131 1451 167 9131 1451 168 MF= 6 Energy-angle distributions 9131 1451 169 Calculated with CCONE code/2/. 9131 1451 170 Distributions from fission (MT=18) are not included. 9131 1451 171 9131 1451 172 9131 1451 173 MF=12 Photon production multiplicities 9131 1451 174 MT=18 Fission 9131 1451 175 Calculated from the total energy released by the prompt 9131 1451 176 gamma-rays due to fission given in MF=1/MT=458 and the 9131 1451 177 average energy of gamma-rays. 9131 1451 178 9131 1451 179 9131 1451 180 MF=14 Photon angular distributions 9131 1451 181 MT=18 Fission 9131 1451 182 Isotoropic distributions were assumed. 9131 1451 183 9131 1451 184 9131 1451 185 MF=15 Continuous photon energy spectra 9131 1451 186 MT=18 Fission 9131 1451 187 Experimental data measured by Verbinski et al./34/ for 9131 1451 188 U-235 thermal fission were adopted. 9131 1451 189 9131 1451 190 9131 1451 191 MF=31 Covariances of average number of neutrons per fission 9131 1451 192 MT=452 Number of neutrons per fission 9131 1451 193 Sum of covariances for MT=455 and MT=456. 9131 1451 194 9131 1451 195 MT=455 9131 1451 196 Error of 15% was assumed. 9131 1451 197 9131 1451 198 MT=456 9131 1451 199 Covariance was obtained by fitting a linear function to the 9131 1451 200 data at 0.0 and 5.0 MeV with an uncertainty of 5%. 9131 1451 201 9131 1451 202 9131 1451 203 MF=32 Covariances of resonance parameters 9131 1451 204 MT=151 Resolved resonance parameterss 9131 1451 205 Format of LCOMP=0 was adopted. 9131 1451 206 9131 1451 207 Uncertainties of parameters were taken from Mughabghab /35/. 9131 1451 208 For the parameters without any information on uncertainty, 9131 1451 209 the following uncertainties were assumed: 9131 1451 210 Resonance energy 0.1 % 9131 1451 211 Neutron width 10 % 9131 1451 212 Capture width 20 % 9131 1451 213 Fission width 20 % 9131 1451 214 They were further modified by considering experimental data 9131 1451 215 of the fission and capture cross sections at the thermal 9131 1451 216 neutron energy. 9131 1451 217 9131 1451 218 9131 1451 219 MF=33 Covariances of neutron cross sections 9131 1451 220 Covariances were given to all the cross sections by using 9131 1451 221 KALMAN code/36/ and the covariances of model parameters 9131 1451 222 used in the cross-section calculations. 9131 1451 223 9131 1451 224 Covariances of the total, elastic-scattering and capture cross 9131 1451 225 sections were determined by considering the experimental data 9131 1451 226 (see MF=3). 9131 1451 227 9131 1451 228 For the fission cross section, covariances obtained with the 9131 1451 229 GMA analysis were adopted. Standard deviations (SD) were 9131 1451 230 multiplied by a factor of 1.5. SD of 18% was assumed in the 9131 1451 231 energy region above 13 MeV. 9131 1451 232 9131 1451 233 In the resolved resonance region, the following standard 9131 1451 234 deviations were added to the contributions from resonance 9131 1451 235 parameters: 9131 1451 236 Total 2 b 9131 1451 237 Elastic scattering 10 % 9131 1451 238 9131 1451 239 9131 1451 240 MF=34 Covariances for Angular Distributions 9131 1451 241 MT=2 Elastic scattering 9131 1451 242 Covariances were given only to P1 components. 9131 1451 243 9131 1451 244 9131 1451 245 MF=35 Covariances for Energy Distributions 9131 1451 246 MT=18 Fission spectra 9131 1451 247 Estimated with CCONE and KALMAN codes. 9131 1451 248 9131 1451 249 9131 1451 250 ***************************************************************** 9131 1451 251 Calculation with CCONE code 9131 1451 252 ***************************************************************** 9131 1451 253 9131 1451 254 Models and parameters used in the CCONE/2/ calculation 9131 1451 255 1) Coupled channel optical model 9131 1451 256 Levels in the rotational band were included. Optical model 9131 1451 257 potential and coupled levels are shown in Table 1. 9131 1451 258 9131 1451 259 2) Two-component exciton model/37/ 9131 1451 260 * Global parametrization of Koning-Duijvestijn/38/ 9131 1451 261 was used. 9131 1451 262 * Gamma emission channel/39/ was added to simulate direct 9131 1451 263 and semi-direct capture reaction. 9131 1451 264 9131 1451 265 3) Hauser-Feshbach statistical model 9131 1451 266 * Moldauer width fluctuation correction/40/ was included. 9131 1451 267 * Neutron, gamma and fission decay channel were included. 9131 1451 268 * Transmission coefficients of neutrons were taken from 9131 1451 269 coupled channel calculation in Table 1. 9131 1451 270 * The level scheme of the target is shown in Table 2. 9131 1451 271 * Level density formula of constant temperature and Fermi-gas 9131 1451 272 model were used with shell energy correction and collective 9131 1451 273 enhancement factor. Parameters are shown in Table 3. 9131 1451 274 * Fission channel: 9131 1451 275 Double humped fission barriers were assumed. 9131 1451 276 Fission barrier penetrabilities were calculated with 9131 1451 277 Hill-Wheler formula/41/. Fission barrier parameters were 9131 1451 278 shown in Table 4. Transition state model was used and 9131 1451 279 continuum levels are assumed above the saddles. The level 9131 1451 280 density parameters for inner and outer saddles are shown in 9131 1451 281 Tables 5 and 6, respectively. 9131 1451 282 * Gamma-ray strength function of Kopecky et al/42/,/43/ 9131 1451 283 was used. The prameters are shown in Table 7. 9131 1451 284 9131 1451 285 9131 1451 286 ------------------------------------------------------------------9131 1451 287 Tables 9131 1451 288 ------------------------------------------------------------------9131 1451 289 9131 1451 290 Table 1. Coupled channel calculation 9131 1451 291 -------------------------------------------------- 9131 1451 292 * rigid rotor model was applied 9131 1451 293 * coupled levels = 0,1,2,3,9,14 (see Table 2) 9131 1451 294 * optical potential parameters /27/ 9131 1451 295 Volume: 9131 1451 296 V_0 = 49.97 MeV 9131 1451 297 lambda_HF = 0.01004 1/MeV 9131 1451 298 C_viso = 15.9 MeV 9131 1451 299 A_v = 12.04 MeV 9131 1451 300 B_v = 81.36 MeV 9131 1451 301 E_a = 385 MeV 9131 1451 302 r_v = 1.2568 fm 9131 1451 303 a_v = 0.633 fm 9131 1451 304 Surface: 9131 1451 305 W_0 = 17.2 MeV 9131 1451 306 B_s = 11.19 MeV 9131 1451 307 C_s = 0.01361 1/MeV 9131 1451 308 C_wiso = 23.5 MeV 9131 1451 309 r_s = 1.1803 fm 9131 1451 310 a_s = 0.601 fm 9131 1451 311 Spin-orbit: 9131 1451 312 V_so = 5.75 MeV 9131 1451 313 lambda_so = 0.005 1/MeV 9131 1451 314 W_so = -3.1 MeV 9131 1451 315 B_so = 160 MeV 9131 1451 316 r_so = 1.1214 fm 9131 1451 317 a_so = 0.59 fm 9131 1451 318 Coulomb: 9131 1451 319 C_coul = 1.3 9131 1451 320 r_c = 1.2452 fm 9131 1451 321 a_c = 0.545 fm 9131 1451 322 Deformation: 9131 1451 323 beta_2 = 0.19 9131 1451 324 beta_4 = 0.066 9131 1451 325 beta_6 = 0.0015 9131 1451 326 9131 1451 327 * Calculated strength function 9131 1451 328 S0= 0.81e-4 S1= 2.50e-4 R'= 9.64 fm (En=1 keV) 9131 1451 329 -------------------------------------------------- 9131 1451 330 9131 1451 331 Table 2. Level Scheme of Pa-231 9131 1451 332 ------------------- 9131 1451 333 No. Ex(MeV) J PI 9131 1451 334 ------------------- 9131 1451 335 0 0.00000 3/2 - * 9131 1451 336 1 0.00921 1/2 - * 9131 1451 337 2 0.05857 7/2 - * 9131 1451 338 3 0.07769 5/2 - * 9131 1451 339 4 0.08421 5/2 + 9131 1451 340 5 0.10141 7/2 + 9131 1451 341 6 0.10227 3/2 + 9131 1451 342 7 0.11165 9/2 + 9131 1451 343 8 0.13400 11/2 + 9131 1451 344 9 0.16860 11/2 - * 9131 1451 345 10 0.17150 11/2 + 9131 1451 346 11 0.17416 5/2 - 9131 1451 347 12 0.18350 5/2 + 9131 1451 348 13 0.18890 13/2 + 9131 1451 349 14 0.19350 9/2 - * 9131 1451 350 15 0.21824 7/2 - 9131 1451 351 16 0.24732 7/2 + 9131 1451 352 17 0.27200 9/2 - 9131 1451 353 18 0.27380 1/2 + 9131 1451 354 19 0.29660 17/2 + 9131 1451 355 20 0.30070 15/2 + 9131 1451 356 21 0.30400 9/2 + 9131 1451 357 22 0.31150 5/2 + 9131 1451 358 23 0.31680 17/2 + 9131 1451 359 24 0.31795 3/2 + 9131 1451 360 25 0.32021 3/2 - 9131 1451 361 26 0.32870 15/2 - 9131 1451 362 27 0.34000 11/2 - 9131 1451 363 28 0.35150 13/2 - 9131 1451 364 29 0.35184 5/2 - 9131 1451 365 30 0.38500 23/2 + 9131 1451 366 ------------------- 9131 1451 367 *) Coupled levels in CC calculation 9131 1451 368 9131 1451 369 Table 3. Level density parameters 9131 1451 370 -------------------------------------------------------- 9131 1451 371 Nuclide a* Pair Eshell T E0 Ematch 9131 1451 372 1/MeV MeV MeV MeV MeV MeV 9131 1451 373 -------------------------------------------------------- 9131 1451 374 Pa-232 17.9699 0.0000 2.9784 0.2779 -0.6740 1.0000 9131 1451 375 Pa-231 17.9034 0.7895 3.1164 0.4176 -1.2470 3.5007 9131 1451 376 Pa-230 17.8368 0.0000 2.9470 0.2794 -0.6728 1.0000 9131 1451 377 Pa-229 17.7702 0.7930 3.0707 0.3881 -0.8689 3.0597 9131 1451 378 Pa-228 17.7035 0.0000 2.9095 0.2810 -0.6716 1.0000 9131 1451 379 -------------------------------------------------------- 9131 1451 380 9131 1451 381 Table 4. Fission barrier parameters 9131 1451 382 ---------------------------------------- 9131 1451 383 Nuclide V_A hw_A V_B hw_B 9131 1451 384 MeV MeV MeV MeV 9131 1451 385 ---------------------------------------- 9131 1451 386 Pa-232 5.800 0.800 6.180 0.400 9131 1451 387 Pa-231 6.000 0.800 5.750 0.520 9131 1451 388 Pa-230 5.800 0.800 6.180 0.400 9131 1451 389 Pa-229 6.000 0.800 5.800 0.520 9131 1451 390 Pa-228 5.800 0.800 6.180 0.400 9131 1451 391 ---------------------------------------- 9131 1451 392 9131 1451 393 Table 5. Level density above inner saddle 9131 1451 394 -------------------------------------------------------- 9131 1451 395 Nuclide a* Pair Eshell T E0 Ematch 9131 1451 396 1/MeV MeV MeV MeV MeV MeV 9131 1451 397 -------------------------------------------------------- 9131 1451 398 Pa-232 20.6654 0.0000 2.6000 0.3415 -2.6081 2.2000 9131 1451 399 Pa-231 20.5889 0.9211 2.6000 0.3276 -1.4734 2.9211 9131 1451 400 Pa-230 20.5123 0.0000 2.6000 0.3428 -2.6080 2.2000 9131 1451 401 Pa-229 20.4357 0.9251 2.6000 0.3435 -1.6829 3.1251 9131 1451 402 Pa-228 20.3591 0.0000 2.6000 0.3442 -2.6080 2.2000 9131 1451 403 -------------------------------------------------------- 9131 1451 404 9131 1451 405 Table 6. Level density above outer saddle 9131 1451 406 -------------------------------------------------------- 9131 1451 407 Nuclide a* Pair Eshell T E0 Ematch 9131 1451 408 1/MeV MeV MeV MeV MeV MeV 9131 1451 409 -------------------------------------------------------- 9131 1451 410 Pa-232 20.6654 0.0000 -0.0800 0.4050 -2.1087 2.5000 9131 1451 411 Pa-231 20.5889 0.9211 -0.1200 0.3706 -0.7702 2.9211 9131 1451 412 Pa-230 20.5123 0.0000 -0.1600 0.3867 -1.8562 2.2000 9131 1451 413 Pa-229 20.4357 0.9251 -0.2000 0.3880 -0.9302 3.1251 9131 1451 414 Pa-228 20.3591 0.0000 -0.2400 0.3894 -1.8544 2.2000 9131 1451 415 -------------------------------------------------------- 9131 1451 416 9131 1451 417 Table 7. Gamma-ray strength function for Pa-232 9131 1451 418 -------------------------------------------------------- 9131 1451 419 K0 = 1.502 E0 = 4.500 (MeV) 9131 1451 420 * E1: ER = 11.03 (MeV) EG = 2.71 (MeV) SIG = 302.00 (mb) 9131 1451 421 ER = 13.87 (MeV) EG = 4.77 (MeV) SIG = 449.00 (mb) 9131 1451 422 * M1: ER = 6.67 (MeV) EG = 4.00 (MeV) SIG = 2.79 (mb) 9131 1451 423 * E2: ER = 10.25 (MeV) EG = 3.33 (MeV) SIG = 6.39 (mb) 9131 1451 424 -------------------------------------------------------- 9131 1451 425 9131 1451 426 9131 1451 427 References 9131 1451 428 1) O.Iwamoto et al.: J. Nucl. Sci. Technol., 46, 510 (2009). 9131 1451 429 2) O.Iwamoto: J. Nucl. Sci. Technol., 44, 687 (2007). 9131 1451 430 3) R.J.Tuttle: INDC(NDS)-107/G+Special, p.29 (1979). 9131 1451 431 4) G.Benedetti et al.: Nucl. Sci. Eng., 80, 379 (1982). 9131 1451 432 5) R.Waldo et al.: Phys. Rev., C23, 1113 (1981). 9131 1451 433 6) M.C.Brady, T.R.England: Nucl. Sci. Eng., 103, 129 (1989). 9131 1451 434 7) T.Ohsawa: J. 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C47, 312 (1990). 9131 1451 475 9131 1451 476 1 451 610 09131 1451 477 1 452 9 19131 1451 478 1 455 11 19131 1451 479 1 456 4 19131 1451 480 1 458 5 19131 1451 481 2 151 231 19131 1451 482 3 1 63 19131 1451 483 3 2 63 19131 1451 484 3 4 36 19131 1451 485 3 16 13 19131 1451 486 3 17 9 19131 1451 487 3 18 60 19131 1451 488 3 51 36 19131 1451 489 3 52 34 19131 1451 490 3 53 33 19131 1451 491 3 54 33 19131 1451 492 3 55 32 19131 1451 493 3 56 32 19131 1451 494 3 57 32 19131 1451 495 3 58 31 19131 1451 496 3 59 30 19131 1451 497 3 60 30 19131 1451 498 3 61 29 19131 1451 499 3 62 29 19131 1451 500 3 63 29 19131 1451 501 3 64 28 19131 1451 502 3 65 28 19131 1451 503 3 66 27 19131 1451 504 3 67 27 19131 1451 505 3 68 26 19131 1451 506 3 69 26 19131 1451 507 3 70 25 19131 1451 508 3 71 25 19131 1451 509 3 72 25 19131 1451 510 3 73 24 19131 1451 511 3 74 24 19131 1451 512 3 75 24 19131 1451 513 3 76 23 19131 1451 514 3 77 23 19131 1451 515 3 78 23 19131 1451 516 3 79 22 19131 1451 517 3 80 22 19131 1451 518 3 91 33 19131 1451 519 3 102 40 19131 1451 520 4 2 524 19131 1451 521 4 18 2 19131 1451 522 5 18 3974 19131 1451 523 5 455 579 19131 1451 524 6 16 1748 19131 1451 525 6 17 580 19131 1451 526 6 51 209 19131 1451 527 6 52 313 19131 1451 528 6 53 308 19131 1451 529 6 54 205 19131 1451 530 6 55 204 19131 1451 531 6 56 207 19131 1451 532 6 57 202 19131 1451 533 6 58 199 19131 1451 534 6 59 293 19131 1451 535 6 60 191 19131 1451 536 6 61 193 19131 1451 537 6 62 191 19131 1451 538 6 63 185 19131 1451 539 6 64 278 19131 1451 540 6 65 181 19131 1451 541 6 66 188 19131 1451 542 6 67 182 19131 1451 543 6 68 177 19131 1451 544 6 69 180 19131 1451 545 6 70 171 19131 1451 546 6 71 177 19131 1451 547 6 72 158 19131 1451 548 6 73 168 19131 1451 549 6 74 156 19131 1451 550 6 75 168 19131 1451 551 6 76 158 19131 1451 552 6 77 162 19131 1451 553 6 78 154 19131 1451 554 6 79 152 19131 1451 555 6 80 148 19131 1451 556 6 91 6369 19131 1451 557 6 102 3690 19131 1451 558 8 4 2 09131 1451 559 8 16 2 09131 1451 560 8 17 2 09131 1451 561 8 18 2 09131 1451 562 8 102 2 09131 1451 563 12 18 4 19131 1451 564 14 18 1 19131 1451 565 15 18 20 19131 1451 566 31 452 5 19131 1451 567 31 455 4 19131 1451 568 31 456 32 19131 1451 569 32 151 419 19131 1451 570 33 1 124 19131 1451 571 33 2 124 19131 1451 572 33 4 15 19131 1451 573 33 16 13 19131 1451 574 33 17 6 19131 1451 575 33 18 350 19131 1451 576 33 51 91 19131 1451 577 33 52 71 19131 1451 578 33 53 66 19131 1451 579 33 54 62 19131 1451 580 33 55 58 19131 1451 581 33 56 58 19131 1451 582 33 57 58 19131 1451 583 33 58 58 19131 1451 584 33 59 58 19131 1451 585 33 60 58 19131 1451 586 33 61 58 19131 1451 587 33 62 58 19131 1451 588 33 63 58 19131 1451 589 33 64 58 19131 1451 590 33 65 53 19131 1451 591 33 66 53 19131 1451 592 33 67 53 19131 1451 593 33 68 53 19131 1451 594 33 69 53 19131 1451 595 33 70 49 19131 1451 596 33 71 49 19131 1451 597 33 72 49 19131 1451 598 33 73 49 19131 1451 599 33 74 49 19131 1451 600 33 75 49 19131 1451 601 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18 1868 3.000000+6 1.359580-7 3.100000+6 1.286590-7 3.200000+6 1.216830-79131 5 18 1869 3.300000+6 1.150240-7 3.400000+6 1.086770-7 3.500000+6 1.026320-79131 5 18 1870 3.600000+6 9.688140-8 3.700000+6 9.141500-8 3.800000+6 8.622320-89131 5 18 1871 3.900000+6 8.129600-8 4.000000+6 7.662340-8 4.100000+6 7.219510-89131 5 18 1872 4.200000+6 6.800080-8 4.300000+6 6.403070-8 4.400000+6 6.027470-89131 5 18 1873 4.500000+6 5.672310-8 4.600000+6 5.336650-8 4.700000+6 5.019560-89131 5 18 1874 4.800000+6 4.720130-8 4.900000+6 4.437510-8 5.000000+6 4.170860-89131 5 18 1875 5.100000+6 3.919360-8 5.200000+6 3.682240-8 5.300000+6 3.458760-89131 5 18 1876 5.400000+6 3.248190-8 5.500000+6 3.049850-8 5.600000+6 2.863080-89131 5 18 1877 5.700000+6 2.687270-8 5.800000+6 2.521810-8 5.900000+6 2.366130-89131 5 18 1878 6.000000+6 2.219700-8 6.100000+6 2.081990-8 6.200000+6 1.952530-89131 5 18 1879 6.300000+6 1.830830-8 6.400000+6 1.716460-8 6.500000+6 1.609010-89131 5 18 1880 6.600000+6 1.508070-8 6.700000+6 1.413260-8 6.800000+6 1.324240-89131 5 18 1881 6.900000+6 1.240670-8 7.000000+6 1.162220-8 7.100000+6 1.088590-89131 5 18 1882 7.200000+6 1.019500-8 7.300000+6 9.546870-9 7.400000+6 8.938860-99131 5 18 1883 7.500000+6 8.368610-9 7.600000+6 7.833860-9 7.700000+6 7.332470-99131 5 18 1884 7.800000+6 6.862430-9 7.900000+6 6.421840-9 8.000000+6 6.008910-99131 5 18 1885 8.100000+6 5.621950-9 8.200000+6 5.259390-9 8.300000+6 4.919730-99131 5 18 1886 8.400000+6 4.601550-9 8.500000+6 4.303550-9 8.600000+6 4.024470-99131 5 18 1887 8.700000+6 3.763140-9 8.800000+6 3.518460-9 8.900000+6 3.289390-99131 5 18 1888 9.000000+6 3.074970-9 9.100000+6 2.874280-9 9.200000+6 2.686460-99131 5 18 1889 9.300000+6 2.510710-9 9.400000+6 2.346260-9 9.500000+6 2.192400-99131 5 18 1890 9.600000+6 2.048470-9 9.700000+6 1.913830-9 9.800000+6 1.787910-99131 5 18 1891 9.900000+6 1.670140-9 1.000000+7 1.560010-9 1.010000+7 1.457040-99131 5 18 1892 1.020000+7 1.360760-9 1.030000+7 1.270750-9 1.040000+7 1.186620-99131 5 18 1893 1.050000+7 1.107970-9 1.060000+7 1.034460-9 1.070000+7 9.65766-109131 5 18 1894 1.080000+7 9.01570-10 1.090000+7 8.41585-10 1.100000+7 7.85538-109131 5 18 1895 1.110000+7 7.33176-10 1.120000+7 6.84260-10 1.130000+7 6.38566-109131 5 18 1896 1.140000+7 5.95886-10 1.150000+7 5.56024-10 1.160000+7 5.18796-109131 5 18 1897 1.170000+7 4.84030-10 1.180000+7 4.51567-10 1.190000+7 4.21256-109131 5 18 1898 1.200000+7 3.92957-10 1.210000+7 3.66537-10 1.220000+7 3.41873-109131 5 18 1899 1.230000+7 3.18850-10 1.240000+7 2.97361-10 1.250000+7 2.77305-109131 5 18 1900 1.260000+7 2.58587-10 1.270000+7 2.41119-10 1.280000+7 2.24819-109131 5 18 1901 1.290000+7 2.09609-10 1.300000+7 1.95418-10 1.310000+7 1.82177-109131 5 18 1902 1.320000+7 1.69825-10 1.330000+7 1.58303-10 1.340000+7 1.47554-109131 5 18 1903 1.350000+7 1.37528-10 1.360000+7 1.28177-10 1.370000+7 1.19456-109131 5 18 1904 1.380000+7 1.11322-10 1.390000+7 1.03737-10 1.400000+7 9.66647-119131 5 18 1905 1.410000+7 9.00698-11 1.420000+7 8.39207-11 1.430000+7 7.81878-119131 5 18 1906 1.440000+7 7.28430-11 1.450000+7 6.78604-11 1.460000+7 6.32156-119131 5 18 1907 1.470000+7 5.88861-11 1.480000+7 5.48506-11 1.490000+7 5.10893-119131 5 18 1908 1.500000+7 4.75837-11 1.510000+7 4.43168-11 1.520000+7 4.12723-119131 5 18 1909 1.530000+7 3.84352-11 1.540000+7 3.57916-11 1.550000+7 3.33284-119131 5 18 1910 1.560000+7 3.10334-11 1.570000+7 2.88952-11 1.580000+7 2.69032-119131 5 18 1911 1.590000+7 2.50474-11 1.600000+7 2.33187-11 1.610000+7 2.17084-119131 5 18 1912 1.620000+7 2.02084-11 1.630000+7 1.88114-11 1.640000+7 1.75102-119131 5 18 1913 1.650000+7 1.62983-11 1.660000+7 1.51697-11 1.670000+7 1.41187-119131 5 18 1914 1.680000+7 1.31400-11 1.690000+7 1.22287-11 1.700000+7 1.13801-119131 5 18 1915 1.710000+7 1.05901-11 1.720000+7 9.85443-12 1.730000+7 9.16956-129131 5 18 1916 1.740000+7 8.53197-12 1.750000+7 7.93841-12 1.760000+7 7.38587-129131 5 18 1917 1.770000+7 6.87153-12 1.780000+7 6.39278-12 1.790000+7 5.94716-129131 5 18 1918 1.800000+7 5.53241-12 1.810000+7 5.14639-12 1.820000+7 4.78714-129131 5 18 1919 1.830000+7 4.45280-12 1.840000+7 4.14167-12 1.850000+7 3.85214-129131 5 18 1920 1.860000+7 3.58273-12 1.870000+7 3.33205-12 1.880000+7 3.09879-129131 5 18 1921 1.890000+7 2.88177-12 1.900000+7 2.67985-12 1.910000+7 2.49200-129131 5 18 1922 1.920000+7 2.31724-12 1.930000+7 2.15466-12 1.940000+7 2.00342-129131 5 18 1923 1.950000+7 1.86274-12 1.960000+7 1.73187-12 1.970000+7 1.61015-129131 5 18 1924 1.980000+7 1.49694-12 1.990000+7 1.39164-12 2.000000+7 1.29370-129131 5 18 1925 2.020000+7 0.000000+0 9131 5 18 1926 0.000000+0 6.500000+6 0 0 1 3529131 5 18 1927 352 2 9131 5 18 1928 0.000000+0 0.000000+0 1.000000-5 1.73805-12 1.200000-5 1.90393-129131 5 18 1929 1.400000-5 2.05649-12 1.600000-5 2.19848-12 1.800000-5 2.33184-129131 5 18 1930 2.200000-5 2.57795-12 2.500000-5 2.74810-12 2.900000-5 2.95980-129131 5 18 1931 3.400000-5 3.20481-12 4.000000-5 3.47611-12 4.600000-5 3.72772-129131 5 18 1932 5.400000-5 4.03888-12 6.300000-5 4.36250-12 7.400000-5 4.72804-129131 5 18 1933 8.600000-5 5.09701-12 1.000000-4 5.49625-12 1.200000-4 6.02085-129131 5 18 1934 1.400000-4 6.50327-12 1.600000-4 6.95230-12 1.800000-4 7.37404-129131 5 18 1935 2.200000-4 8.15233-12 2.500000-4 8.69043-12 2.900000-4 9.35990-129131 5 18 1936 3.400000-4 1.01347-11 4.000000-4 1.09927-11 4.600000-4 1.17884-119131 5 18 1937 5.400000-4 1.27724-11 6.300000-4 1.37959-11 7.400000-4 1.49519-119131 5 18 1938 8.600000-4 1.61187-11 1.000000-3 1.73813-11 1.200000-3 1.90404-119131 5 18 1939 1.400000-3 2.05661-11 1.600000-3 2.19862-11 1.800000-3 2.33200-119131 5 18 1940 2.200000-3 2.57814-11 2.500000-3 2.74832-11 2.900000-3 2.96006-119131 5 18 1941 3.400000-3 3.20512-11 4.000000-3 3.47647-11 4.600000-3 3.72813-119131 5 18 1942 5.400000-3 4.03937-11 6.300000-3 4.36306-11 7.400000-3 4.72870-119131 5 18 1943 8.600000-3 5.09778-11 1.000000-2 5.49715-11 1.200000-2 6.02193-119131 5 18 1944 1.400000-2 6.50453-11 1.600000-2 6.95373-11 1.800000-2 7.37565-119131 5 18 1945 2.200000-2 8.15430-11 2.500000-2 8.69267-11 2.900000-2 9.36249-119131 5 18 1946 3.400000-2 1.01378-10 4.000000-2 1.09963-10 4.600000-2 1.17925-109131 5 18 1947 5.400000-2 1.27773-10 6.300000-2 1.38015-10 7.400000-2 1.49585-109131 5 18 1948 8.600000-2 1.61264-10 1.000000-1 1.73903-10 1.200000-1 1.90512-109131 5 18 1949 1.400000-1 2.05787-10 1.600000-1 2.20005-10 1.800000-1 2.33361-109131 5 18 1950 2.200000-1 2.58011-10 2.500000-1 2.75057-10 2.900000-1 2.96266-109131 5 18 1951 3.400000-1 3.20817-10 4.000000-1 3.48005-10 4.600000-1 3.73225-109131 5 18 1952 5.400000-1 4.04421-10 6.300000-1 4.36871-10 7.400000-1 4.73534-109131 5 18 1953 8.600000-1 5.10549-10 1.000000+0 5.50611-10 1.200000+0 6.03269-109131 5 18 1954 1.400000+0 6.51708-10 1.600000+0 6.96808-10 1.800000+0 7.39179-109131 5 18 1955 2.200000+0 8.17403-10 2.500000+0 8.71508-10 2.900000+0 9.38850-109131 5 18 1956 3.400000+0 1.016830-9 4.000000+0 1.103220-9 4.600000+0 1.183380-99131 5 18 1957 5.400000+0 1.282570-9 6.300000+0 1.385800-9 7.400000+0 1.502490-99131 5 18 1958 8.600000+0 1.620360-9 1.000000+1 1.748000-9 1.200000+1 1.915880-99131 5 18 1959 1.400000+1 2.070420-9 1.600000+1 2.214410-9 1.800000+1 2.349760-99131 5 18 1960 2.200000+1 2.599850-9 2.500000+1 2.772990-9 2.900000+1 2.988670-99131 5 18 1961 3.400000+1 3.238670-9 4.000000+1 3.515940-9 4.600000+1 3.773520-99131 5 18 1962 5.400000+1 4.092650-9 6.300000+1 4.425230-9 7.400000+1 4.801720-99131 5 18 1963 8.600000+1 5.182630-9 1.000000+2 5.595810-9 1.200000+2 6.140320-99131 5 18 1964 1.400000+2 6.642650-9 1.600000+2 7.111570-9 1.800000+2 7.553210-99131 5 18 1965 2.200000+2 8.371290-9 2.500000+2 8.939220-9 2.900000+2 9.648460-99131 5 18 1966 3.400000+2 1.047300-8 4.000000+2 1.139060-8 4.600000+2 1.224590-89131 5 18 1967 5.400000+2 1.330940-8 6.300000+2 1.442210-8 7.400000+2 1.568720-89131 5 18 1968 8.600000+2 1.697300-8 1.000000+3 1.837430-8 1.200000+3 2.023130-89131 5 18 1969 1.400000+3 2.195480-8 1.600000+3 2.357250-8 1.800000+3 2.510370-89131 5 18 1970 2.200000+3 2.795960-8 2.500000+3 2.995690-8 2.900000+3 3.246760-89131 5 18 1971 3.400000+3 3.540920-8 4.000000+3 3.871090-8 4.600000+3 4.181470-89131 5 18 1972 5.400000+3 4.570840-8 6.300000+3 4.982240-8 7.400000+3 5.454810-89131 5 18 1973 8.600000+3 5.940210-8 1.000000+4 6.474920-8 1.200000+4 7.192370-89131 5 18 1974 1.400000+4 7.866910-8 1.600000+4 8.507380-8 1.800000+4 9.119910-89131 5 18 1975 2.200000+4 1.027800-7 2.500000+4 1.109950-7 2.900000+4 1.214500-79131 5 18 1976 3.400000+4 1.338720-7 4.000000+4 1.480230-7 4.600000+4 1.615150-79131 5 18 1977 5.400000+4 1.786810-7 6.300000+4 1.970900-7 7.400000+4 2.185530-79131 5 18 1978 8.600000+4 2.409200-7 1.000000+5 2.659040-7 2.000000+5 3.847880-79131 5 18 1979 3.000000+5 4.488450-7 4.000000+5 4.736590-7 5.000000+5 4.751520-79131 5 18 1980 6.000000+5 4.512130-7 7.000000+5 4.110710-7 8.000000+5 3.639450-79131 5 18 1981 9.000000+5 3.277800-7 1.000000+6 3.058540-7 1.100000+6 2.925060-79131 5 18 1982 1.200000+6 2.826250-7 1.300000+6 2.736120-7 1.400000+6 2.645690-79131 5 18 1983 1.500000+6 2.552670-7 1.600000+6 2.457240-7 1.700000+6 2.360240-79131 5 18 1984 1.800000+6 2.262620-7 1.900000+6 2.165220-7 2.000000+6 2.068760-79131 5 18 1985 2.100000+6 1.973800-7 2.200000+6 1.880810-7 2.300000+6 1.790130-79131 5 18 1986 2.400000+6 1.702040-7 2.500000+6 1.616740-7 2.600000+6 1.534360-79131 5 18 1987 2.700000+6 1.455000-7 2.800000+6 1.378720-7 2.900000+6 1.305540-79131 5 18 1988 3.000000+6 1.235440-7 3.100000+6 1.168410-7 3.200000+6 1.104390-79131 5 18 1989 3.300000+6 1.043340-7 3.400000+6 9.851700-8 3.500000+6 9.298160-89131 5 18 1990 3.600000+6 8.771890-8 3.700000+6 8.271990-8 3.800000+6 7.797520-89131 5 18 1991 3.900000+6 7.347540-8 4.000000+6 6.921100-8 4.100000+6 6.517210-89131 5 18 1992 4.200000+6 6.134940-8 4.300000+6 5.773320-8 4.400000+6 5.431440-89131 5 18 1993 4.500000+6 5.108380-8 4.600000+6 4.803250-8 4.700000+6 4.515190-89131 5 18 1994 4.800000+6 4.243360-8 4.900000+6 3.986960-8 5.000000+6 3.745190-89131 5 18 1995 5.100000+6 3.517310-8 5.200000+6 3.302600-8 5.300000+6 3.100360-89131 5 18 1996 5.400000+6 2.909930-8 5.500000+6 2.730680-8 5.600000+6 2.561990-89131 5 18 1997 5.700000+6 2.403300-8 5.800000+6 2.254050-8 5.900000+6 2.113700-89131 5 18 1998 6.000000+6 1.981780-8 6.100000+6 1.857790-8 6.200000+6 1.741290-89131 5 18 1999 6.300000+6 1.631860-8 6.400000+6 1.529070-8 6.500000+6 1.432560-89131 5 18 2000 6.600000+6 1.341950-8 6.700000+6 1.256910-8 6.800000+6 1.177100-89131 5 18 2001 6.900000+6 1.102220-8 7.000000+6 1.031970-8 7.100000+6 9.660770-99131 5 18 2002 7.200000+6 9.042860-9 7.300000+6 8.463480-9 7.400000+6 7.920320-99131 5 18 2003 7.500000+6 7.411180-9 7.600000+6 6.934020-9 7.700000+6 6.486880-99131 5 18 2004 7.800000+6 6.067940-9 7.900000+6 5.675470-9 8.000000+6 5.307860-99131 5 18 2005 8.100000+6 4.963560-9 8.200000+6 4.641140-9 8.300000+6 4.339260-99131 5 18 2006 8.400000+6 4.056630-9 8.500000+6 3.792070-9 8.600000+6 3.544440-99131 5 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