JENDL-5 (Neutron sublibrary (up to 20 MeV)) Pa-233 0 0 0 0 9.123300+4 2.310380+2 1 1 6 19137 1451 1 0.000000+0 1.000000+0 0 0 0 69137 1451 2 1.000000+0 2.000000+7 0 0 10 59137 1451 3 0.000000+0 0.000000+0 3 0 388 1219137 1451 4 91-Pa-233 JAEA+ EVAL-FEB10 O.Iwamoto, T.Nakagawa, et al. 9137 1451 5 DIST-DEC21 20100318 9137 1451 6 ----JENDL-5 MATERIAL 9137 9137 1451 7 -----INCIDENT NEUTRON DATA 9137 1451 8 ------ENDF-6 FORMAT 9137 1451 9 9137 1451 10 History 9137 1451 11 06-07 Resonance parameters were modified. 9137 1451 12 07-10 Theoretical calculation was done with CCONE code. 9137 1451 13 Data were compiled as JENDL/AC-2008/1/. 9137 1451 14 08-12 (1,455) was modified. 9137 1451 15 09-04 (1,452), (1,455) and (1,456) were revised. 9137 1451 16 10-02 Data of prompt gamma rays due to fission were given. 9137 1451 17 10-03 Covariance data were given. 9137 1451 18 21-08 QI of MT75 was slightly shifted to avoid duplication with 9137 1451 19 MT74 by S. Nakayama. 9137 1451 20 9137 1451 21 21-11 revised by O.Iwamoto 9137 1451 22 (MF3/MT19-21,38) deleted 9137 1451 23 (MF8/MT4,16-18,37,102) added 9137 1451 24 9137 1451 25 MF=1 General information 9137 1451 26 MT=452 Number of Neutrons per fission 9137 1451 27 Sum of MT's=455 and 456. 9137 1451 28 9137 1451 29 MT=455 Delayed neutron data 9137 1451 30 Determined from nu-d of the following three fissioning 9137 1451 31 nuclides and partial fission cross sections calculated with 9137 1451 32 CCONE code/2/. 9137 1451 33 Pa-234 = 0.02301 9137 1451 34 Pa-233 = 0.01577 9137 1451 35 Pa-232 = 0.01083 9137 1451 36 They are averages of systematics by Tuttle/3/, 9137 1451 37 Benedetti et al./4/ and Waldo et al./5/ 9137 1451 38 9137 1451 39 MT=456 Number of prompt neutrons per fission 9137 1451 40 Estimated from Ohsawa's systematics/6/. 9137 1451 41 9137 1451 42 9137 1451 43 MF= 2 Resonance parameters 9137 1451 44 MT=151 9137 1451 45 Resolved resonance parameters (MLBW: 1.0E-5 - 100 eV) 9137 1451 46 Resonance parameters evaluated by Morogovskii and Bakhanovich 9137 1451 47 /7/ were adopted. Total spin of each resonance was 9137 1451 48 assigned at random. Parameters of a negative resonance were 9137 1451 49 adjusted to the thermal cross sections. 9137 1451 50 9137 1451 51 9137 1451 52 The thermal cross sections to be reproduced: 9137 1451 53 Total = 55.0 +- 4.2 b 9137 1451 54 Simpson et al./8/ 9137 1451 55 9137 1451 56 Capture = 39.4 +- 1.2 b 9137 1451 57 Smith et al./9/, Eastwood et al./10/, Halperin et 9137 1451 58 al./11/, Connor/12/, Bringer et al./13/ 9137 1451 59 9137 1451 60 Unresolved resonance parameters (100 eV - 10 keV) 9137 1451 61 Cross sections were reproduced with average resonance 9137 1451 62 parameters determined by ASREP code/14/. These parameters 9137 1451 63 are used only for self-shielding effects. 9137 1451 64 9137 1451 65 9137 1451 66 Thermal cross sections and resonance integrals (at 300K) 9137 1451 67 ------------------------------------------------------- 9137 1451 68 0.0253 eV reson. integ.(*) 9137 1451 69 (barns) (barns) 9137 1451 70 ------------------------------------------------------- 9137 1451 71 total 53.56 9137 1451 72 elastic 14.14 9137 1451 73 fission 2.5E-6 0.977 9137 1451 74 capture 39.42 835 9137 1451 75 ------------------------------------------------------- 9137 1451 76 (*) In the energy range from 0.5 eV to 10 MeV. 9137 1451 77 9137 1451 78 9137 1451 79 MF= 3 Neutron cross sections 9137 1451 80 Cross sections above the resolved resonance region were 9137 1451 81 calculated with CCONE code/2/. 9137 1451 82 9137 1451 83 MT= 1 Total cross section 9137 1451 84 The cross section was calculated with CC OMP of Soukhovitskii 9137 1451 85 et al./15/ with modification of the quadrupole deformation 9137 1451 86 parameter. 9137 1451 87 9137 1451 88 MT=18, 19 Fission cross section 9137 1451 89 Above 30 keV, calculated with CCONE code. 9137 1451 90 From 1 eV to 10 keV, a constant cross section of 4.0E-7 b 9137 1451 91 was assumed. 9137 1451 92 Below 1 eV, 1/v shape cross section was assumed. 9137 1451 93 9137 1451 94 The experimental data of Petit et al./16/ and Tovesson et 9137 1451 95 al./17/ were used to determine the parameters in the CCONE 9137 1451 96 calculation. 9137 1451 97 9137 1451 98 9137 1451 99 MF= 4 Angular distributions of secondary neutrons 9137 1451 100 MT=2 Elastic scattering 9137 1451 101 Calculated with CCONE code/2/. 9137 1451 102 9137 1451 103 MT=18 Fission 9137 1451 104 Isotropic distributions in the laboratory system were assumed.9137 1451 105 9137 1451 106 9137 1451 107 MF= 5 Energy distributions of secondary neutrons 9137 1451 108 MT=18 Prompt neutrons 9137 1451 109 Calculated with CCONE code/2/. 9137 1451 110 9137 1451 111 9137 1451 112 MF= 6 Energy-angle distributions 9137 1451 113 Calculated with CCONE code/2/. 9137 1451 114 Distributions from fission (MT=18) are not included. 9137 1451 115 9137 1451 116 9137 1451 117 MF=12 Photon production multiplicities 9137 1451 118 MT=18 Fission 9137 1451 119 Calculated from the total energy released by the prompt 9137 1451 120 gamma-rays due to fission which was estimated from its 9137 1451 121 systematics, and the average energy of gamma-rays. 9137 1451 122 9137 1451 123 9137 1451 124 MF=14 Photon angular distributions 9137 1451 125 MT=18 Fission 9137 1451 126 Isotoropic distributions were assumed. 9137 1451 127 9137 1451 128 9137 1451 129 MF=15 Continuous photon energy spectra 9137 1451 130 MT=18 Fission 9137 1451 131 Experimental data measured by Verbinski et al./18/ for 9137 1451 132 U-235 thermal fission were adopted. 9137 1451 133 9137 1451 134 9137 1451 135 MF=31 Covariances of average number of neutrons per fission 9137 1451 136 MT=452 Number of neutrons per fission 9137 1451 137 Sum of covariances for MT=455 and MT=456. 9137 1451 138 9137 1451 139 MT=455 9137 1451 140 Error of 15% was assumed. 9137 1451 141 9137 1451 142 MT=456 9137 1451 143 Covariance was obtained by fitting a linear function to the 9137 1451 144 data at 0.0 and 5.0 MeV with an uncertainty of 5%. 9137 1451 145 9137 1451 146 9137 1451 147 MF=32 Covariances of resonance parameters 9137 1451 148 MT=151 Resolved resonance parameterss 9137 1451 149 Format of LCOMP=0 was adopted. 9137 1451 150 9137 1451 151 Uncertainties of parameters were taken from Mughabghab /19/. 9137 1451 152 For the parameters without any information on uncertainty, 9137 1451 153 the following uncertainties were assumed: 9137 1451 154 Resonance energy 0.1 % 9137 1451 155 Neutron width 10 % 9137 1451 156 Capture width 50 % 9137 1451 157 Fission width 20 % 9137 1451 158 They were further modified by considering experimental data 9137 1451 159 of the capture cross section at the thermal neutron energy. 9137 1451 160 9137 1451 161 9137 1451 162 MF=33 Covariances of neutron cross sections 9137 1451 163 Covariances were given to all the cross sections by using 9137 1451 164 KALMAN code/20/ and the covariances of model parameters 9137 1451 165 used in the cross-section calculations. 9137 1451 166 9137 1451 167 Covariances of the fission cross section were determined by 9137 1451 168 considering the experimental data (see MF=3). 9137 1451 169 9137 1451 170 In the resolved resonance region, the following standard 9137 1451 171 deviations were added to the contributions from resonance 9137 1451 172 parameters: 9137 1451 173 Total 0 - 10 % 9137 1451 174 Elastic scattering 20 % 9137 1451 175 Fission 90 % 9137 1451 176 Capture 0 - 10 % 9137 1451 177 9137 1451 178 9137 1451 179 MF=34 Covariances for Angular Distributions 9137 1451 180 MT=2 Elastic scattering 9137 1451 181 Covariances were given only to P1 components. 9137 1451 182 9137 1451 183 9137 1451 184 MF=35 Covariances for Energy Distributions 9137 1451 185 MT=18 Fission spectra 9137 1451 186 Estimated with CCONE and KALMAN codes. 9137 1451 187 9137 1451 188 9137 1451 189 ***************************************************************** 9137 1451 190 Calculation with CCONE code 9137 1451 191 ***************************************************************** 9137 1451 192 9137 1451 193 Models and parameters used in the CCONE/2/ calculation 9137 1451 194 1) Coupled channel optical model 9137 1451 195 Levels in the rotational band were included. Optical model 9137 1451 196 potential and coupled levels are shown in Table 1. 9137 1451 197 9137 1451 198 2) Two-component exciton model/21/ 9137 1451 199 * Global parametrization of Koning-Duijvestijn/22/ 9137 1451 200 was used. 9137 1451 201 * Gamma emission channel/23/ was added to simulate direct 9137 1451 202 and semi-direct capture reaction. 9137 1451 203 9137 1451 204 3) Hauser-Feshbach statistical model 9137 1451 205 * Moldauer width fluctuation correction/24/ was included. 9137 1451 206 * Neutron, gamma and fission decay channel were included. 9137 1451 207 * Transmission coefficients of neutrons were taken from 9137 1451 208 coupled channel calculation in Table 1. 9137 1451 209 * The level scheme of the target is shown in Table 2. 9137 1451 210 * Level density formula of constant temperature and Fermi-gas 9137 1451 211 model were used with shell energy correction and collective 9137 1451 212 enhancement factor. Parameters are shown in Table 3. 9137 1451 213 * Fission channel: 9137 1451 214 Double humped fission barriers were assumed. 9137 1451 215 Fission barrier penetrabilities were calculated with 9137 1451 216 Hill-Wheler formula/25/. Fission barrier parameters were 9137 1451 217 shown in Table 4. Transition state model was used and 9137 1451 218 continuum levels are assumed above the saddles. The level 9137 1451 219 density parameters for inner and outer saddles are shown in 9137 1451 220 Tables 5 and 6, respectively. 9137 1451 221 * Gamma-ray strength function of Kopecky et al/26/,/27/ 9137 1451 222 was used. The prameters are shown in Table 7. 9137 1451 223 9137 1451 224 9137 1451 225 ------------------------------------------------------------------9137 1451 226 Tables 9137 1451 227 ------------------------------------------------------------------9137 1451 228 9137 1451 229 Table 1. Coupled channel calculation 9137 1451 230 -------------------------------------------------- 9137 1451 231 * rigid rotor model was applied 9137 1451 232 * coupled levels = 0,1,2,3,9,12 (see Table 2) 9137 1451 233 * optical potential parameters /15/ 9137 1451 234 Volume: 9137 1451 235 V_0 = 49.97 MeV 9137 1451 236 lambda_HF = 0.01004 1/MeV 9137 1451 237 C_viso = 15.9 MeV 9137 1451 238 A_v = 12.04 MeV 9137 1451 239 B_v = 81.36 MeV 9137 1451 240 E_a = 385 MeV 9137 1451 241 r_v = 1.2568 fm 9137 1451 242 a_v = 0.633 fm 9137 1451 243 Surface: 9137 1451 244 W_0 = 17.2 MeV 9137 1451 245 B_s = 11.19 MeV 9137 1451 246 C_s = 0.01361 1/MeV 9137 1451 247 C_wiso = 23.5 MeV 9137 1451 248 r_s = 1.1803 fm 9137 1451 249 a_s = 0.601 fm 9137 1451 250 Spin-orbit: 9137 1451 251 V_so = 5.75 MeV 9137 1451 252 lambda_so = 0.005 1/MeV 9137 1451 253 W_so = -3.1 MeV 9137 1451 254 B_so = 160 MeV 9137 1451 255 r_so = 1.1214 fm 9137 1451 256 a_so = 0.59 fm 9137 1451 257 Coulomb: 9137 1451 258 C_coul = 1.3 9137 1451 259 r_c = 1.2452 fm 9137 1451 260 a_c = 0.545 fm 9137 1451 261 Deformation: 9137 1451 262 beta_2 = 0.19 9137 1451 263 beta_4 = 0.066 9137 1451 264 beta_6 = 0.0015 9137 1451 265 9137 1451 266 * Calculated strength function 9137 1451 267 S0= 0.73e-4 S1= 2.68e-4 R'= 9.58 fm (En=1 keV) 9137 1451 268 -------------------------------------------------- 9137 1451 269 9137 1451 270 Table 2. Level Scheme of Pa-233 9137 1451 271 ------------------- 9137 1451 272 No. Ex(MeV) J PI 9137 1451 273 ------------------- 9137 1451 274 0 0.00000 3/2 - * 9137 1451 275 1 0.00667 1/2 - * 9137 1451 276 2 0.05710 7/2 - * 9137 1451 277 3 0.07054 5/2 - * 9137 1451 278 4 0.08647 5/2 + 9137 1451 279 5 0.09465 3/2 + 9137 1451 280 6 0.10364 7/2 + 9137 1451 281 7 0.10907 9/2 + 9137 1451 282 8 0.13320 11/2 + 9137 1451 283 9 0.16351 11/2 - * 9137 1451 284 10 0.16917 1/2 + 9137 1451 285 11 0.17300 13/2 + 9137 1451 286 12 0.17900 9/2 - * 9137 1451 287 13 0.20163 3/2 + 9137 1451 288 14 0.21234 5/2 + 9137 1451 289 15 0.23789 5/2 + 9137 1451 290 16 0.25718 5/2 - 9137 1451 291 17 0.27972 7/2 + 9137 1451 292 18 0.29600 5/2 + 9137 1451 293 19 0.30050 7/2 + 9137 1451 294 20 0.30359 9/2 + 9137 1451 295 21 0.30610 7/2 - 9137 1451 296 22 0.32380 15/2 - 9137 1451 297 23 0.33080 13/2 - 9137 1451 298 24 0.35500 3/2 + 9137 1451 299 25 0.35500 9/2 - 9137 1451 300 ------------------- 9137 1451 301 *) Coupled levels in CC calculation 9137 1451 302 9137 1451 303 Table 3. Level density parameters 9137 1451 304 -------------------------------------------------------- 9137 1451 305 Nuclide a* Pair Eshell T E0 Ematch 9137 1451 306 1/MeV MeV MeV MeV MeV MeV 9137 1451 307 -------------------------------------------------------- 9137 1451 308 Pa-234 18.1029 0.0000 3.1132 0.2754 -0.6749 1.0000 9137 1451 309 Pa-233 18.0364 0.7861 3.1759 0.4099 -1.1882 3.4195 9137 1451 310 Pa-232 17.9699 0.0000 2.9784 0.2779 -0.6740 1.0000 9137 1451 311 Pa-231 17.9034 0.7895 3.1164 0.4176 -1.2470 3.5007 9137 1451 312 Pa-230 17.8368 0.0000 2.9470 0.2794 -0.6728 1.0000 9137 1451 313 -------------------------------------------------------- 9137 1451 314 9137 1451 315 Table 4. Fission barrier parameters 9137 1451 316 ---------------------------------------- 9137 1451 317 Nuclide V_A hw_A V_B hw_B 9137 1451 318 MeV MeV MeV MeV 9137 1451 319 ---------------------------------------- 9137 1451 320 Pa-234 5.800 0.800 6.300 0.400 9137 1451 321 Pa-233 5.900 0.800 6.100 0.520 9137 1451 322 Pa-232 5.800 0.800 6.180 0.400 9137 1451 323 Pa-231 6.000 0.800 5.750 0.520 9137 1451 324 Pa-230 5.800 0.800 6.180 0.400 9137 1451 325 ---------------------------------------- 9137 1451 326 9137 1451 327 Table 5. Level density above inner saddle 9137 1451 328 -------------------------------------------------------- 9137 1451 329 Nuclide a* Pair Eshell T E0 Ematch 9137 1451 330 1/MeV MeV MeV MeV MeV MeV 9137 1451 331 -------------------------------------------------------- 9137 1451 332 Pa-234 20.8184 0.0000 2.6000 0.3401 -2.6082 2.2000 9137 1451 333 Pa-233 19.8401 0.9172 2.6000 0.3346 -1.5060 2.9172 9137 1451 334 Pa-232 20.6654 0.0000 2.6000 0.3415 -2.6081 2.2000 9137 1451 335 Pa-231 20.5889 0.9211 2.6000 0.3276 -1.4734 2.9211 9137 1451 336 Pa-230 20.5123 0.0000 2.6000 0.3428 -2.6080 2.2000 9137 1451 337 -------------------------------------------------------- 9137 1451 338 9137 1451 339 Table 6. Level density above outer saddle 9137 1451 340 -------------------------------------------------------- 9137 1451 341 Nuclide a* Pair Eshell T E0 Ematch 9137 1451 342 1/MeV MeV MeV MeV MeV MeV 9137 1451 343 -------------------------------------------------------- 9137 1451 344 Pa-234 20.2753 0.0000 -0.0000 0.3874 -1.8655 2.2000 9137 1451 345 Pa-233 19.8401 0.9172 -0.0400 0.3622 -0.6209 2.7172 9137 1451 346 Pa-232 20.6654 0.0000 -0.0800 0.4050 -2.1087 2.5000 9137 1451 347 Pa-231 20.5889 0.9211 -0.1200 0.3706 -0.7702 2.9211 9137 1451 348 Pa-230 20.5123 0.0000 -0.1600 0.3867 -1.8562 2.2000 9137 1451 349 -------------------------------------------------------- 9137 1451 350 9137 1451 351 Table 7. Gamma-ray strength function for Pa-234 9137 1451 352 -------------------------------------------------------- 9137 1451 353 K0 = 1.501 E0 = 4.500 (MeV) 9137 1451 354 * E1: ER = 11.03 (MeV) EG = 2.71 (MeV) SIG = 302.00 (mb) 9137 1451 355 ER = 13.87 (MeV) EG = 4.77 (MeV) SIG = 449.00 (mb) 9137 1451 356 * M1: ER = 6.65 (MeV) EG = 4.00 (MeV) SIG = 2.77 (mb) 9137 1451 357 * E2: ER = 10.22 (MeV) EG = 3.30 (MeV) SIG = 6.38 (mb) 9137 1451 358 -------------------------------------------------------- 9137 1451 359 9137 1451 360 9137 1451 361 References 9137 1451 362 1) O.Iwamoto et al.: J. Nucl. Sci. Technol., 46, 510 (2009). 9137 1451 363 2) O.Iwamoto: J. Nucl. Sci. Technol., 44, 687 (2007). 9137 1451 364 3) R.J.Tuttle: INDC(NDS)-107/G+Special, p.29 (1979). 9137 1451 365 4) G.Benedetti et al.: Nucl. Sci. Eng., 80, 379 (1982). 9137 1451 366 5) R.Waldo et al.: Phys. Rev., C23, 1113 (1981). 9137 1451 367 6) T.Ohsawa: J. Nucl. Radiochem. Sci., 9, 19 (2008). 9137 1451 368 7) G.B.Morogovskii, L.A.Bakhanovich: INDC(CCP)-440, p.7 (2004). 9137 1451 369 8) F.B.Simpson, J.W.Codding Jr.: Nucl. Sci. Eng., 28, 133 (1967).9137 1451 370 9) R.R.Smith et al.: IDO-16226 (1955). 9137 1451 371 10) T.A.Eastwood, R.D.Werner: Canadian J. Phys., 38, 751 (1960). 9137 1451 372 11) J.Halperin et al.: ORNL-3320, p.1 (1962). 9137 1451 373 12) J.C.Connor: WAPD-TM-837 (1970). 9137 1451 374 13) O.Bringer et al.: 2006 Vancouver (PHYSOR-2006), C034(2006). 9137 1451 375 14) Y.Kikuchi et al.: JAERI-Data/Code 99-025 (1999) in Japanese. 9137 1451 376 15) E.Sh.Soukhovitskii et al.: Phys. Rev. C72, 024604 (2005). 9137 1451 377 16) M.Petit et al.: Nucl. Phys., A735, 345 (2004). 9137 1451 378 17) F.Tovesson et al.: Nucl. Phys., A735, 3 (2004). 9137 1451 379 18) V.V.Verbinski et al.: Phys. Rev., C7, 1173 (1973). 9137 1451 380 19) S.F.Mughabghab: "Atlas of Neutron Resonances," Elsevier 9137 1451 381 (2006). 9137 1451 382 20) T.Kawano, K.Shibata, JAERI-Data/Code 97-037 (1997) in 9137 1451 383 Japanese. 9137 1451 384 21) C.Kalbach: Phys. Rev. C33, 818 (1986). 9137 1451 385 22) A.J.Koning, M.C.Duijvestijn: Nucl. Phys. A744, 15 (2004). 9137 1451 386 23) J.M.Akkermans, H.Gruppelaar: Phys. Lett. 157B, 95 (1985). 9137 1451 387 24) P.A.Moldauer: Nucl. Phys. A344, 185 (1980). 9137 1451 388 25) D.L.Hill, J.A.Wheeler: Phys. Rev. 89, 1102 (1953). 9137 1451 389 26) J.Kopecky, M.Uhl: Phys. Rev. C41, 1941 (1990). 9137 1451 390 27) J.Kopecky, M.Uhl, R.E.Chrien: Phys. Rev. C47, 312 (1990). 9137 1451 391 9137 1451 392 1 451 513 09137 1451 393 1 452 9 19137 1451 394 1 455 11 19137 1451 395 1 456 4 19137 1451 396 2 151 192 19137 1451 397 3 1 43 19137 1451 398 3 2 42 19137 1451 399 3 4 36 19137 1451 400 3 16 13 19137 1451 401 3 17 9 19137 1451 402 3 18 34 19137 1451 403 3 37 4 19137 1451 404 3 51 34 19137 1451 405 3 52 32 19137 1451 406 3 53 31 19137 1451 407 3 54 31 19137 1451 408 3 55 31 19137 1451 409 3 56 30 19137 1451 410 3 57 30 19137 1451 411 3 58 29 19137 1451 412 3 59 28 19137 1451 413 3 60 28 19137 1451 414 3 61 27 19137 1451 415 3 62 27 19137 1451 416 3 63 26 19137 1451 417 3 64 26 19137 1451 418 3 65 26 19137 1451 419 3 66 25 19137 1451 420 3 67 25 19137 1451 421 3 68 24 19137 1451 422 3 69 24 19137 1451 423 3 70 23 19137 1451 424 3 71 23 19137 1451 425 3 72 23 19137 1451 426 3 73 22 19137 1451 427 3 74 22 19137 1451 428 3 75 22 19137 1451 429 3 91 30 19137 1451 430 3 102 38 19137 1451 431 4 2 514 19137 1451 432 4 18 2 19137 1451 433 5 18 3974 19137 1451 434 6 16 1825 19137 1451 435 6 17 987 19137 1451 436 6 37 33 19137 1451 437 6 51 313 19137 1451 438 6 52 303 19137 1451 439 6 53 297 19137 1451 440 6 54 196 19137 1451 441 6 55 197 19137 1451 442 6 56 195 19137 1451 443 6 57 194 19137 1451 444 6 58 191 19137 1451 445 6 59 288 19137 1451 446 6 60 184 19137 1451 447 6 61 181 19137 1451 448 6 62 270 19137 1451 449 6 63 176 19137 1451 450 6 64 170 19137 1451 451 6 65 170 19137 1451 452 6 66 170 19137 1451 453 6 67 167 19137 1451 454 6 68 161 19137 1451 455 6 69 164 19137 1451 456 6 70 158 19137 1451 457 6 71 154 19137 1451 458 6 72 155 19137 1451 459 6 73 150 19137 1451 460 6 74 151 19137 1451 461 6 75 149 19137 1451 462 6 91 5951 19137 1451 463 6 102 3482 19137 1451 464 8 4 2 09137 1451 465 8 16 2 09137 1451 466 8 17 2 09137 1451 467 8 18 2 09137 1451 468 8 37 2 09137 1451 469 8 102 2 09137 1451 470 12 18 4 19137 1451 471 14 18 1 19137 1451 472 15 18 20 19137 1451 473 31 452 5 19137 1451 474 31 455 4 19137 1451 475 31 456 32 19137 1451 476 32 151 284 19137 1451 477 33 1 124 19137 1451 478 33 2 124 19137 1451 479 33 4 13 19137 1451 480 33 16 13 19137 1451 481 33 17 6 19137 1451 482 33 18 124 19137 1451 483 33 37 4 19137 1451 484 33 51 97 19137 1451 485 33 52 71 19137 1451 486 33 53 66 19137 1451 487 33 54 62 19137 1451 488 33 55 62 19137 1451 489 33 56 58 19137 1451 490 33 57 58 19137 1451 491 33 58 58 19137 1451 492 33 59 58 19137 1451 493 33 60 58 19137 1451 494 33 61 58 19137 1451 495 33 62 58 19137 1451 496 33 63 53 19137 1451 497 33 64 53 19137 1451 498 33 65 53 19137 1451 499 33 66 53 19137 1451 500 33 67 53 19137 1451 501 33 68 53 19137 1451 502 33 69 49 19137 1451 503 33 70 49 19137 1451 504 33 71 49 19137 1451 505 33 72 49 19137 1451 506 33 73 49 19137 1451 507 33 74 49 19137 1451 508 33 75 49 19137 1451 509 33 91 58 19137 1451 510 33 102 124 19137 1451 511 34 2 122 19137 1451 512 35 18 5089 19137 1451 513 9137 1 099999 9.123300+4 2.310380+2 0 2 0 09137 1452 1 0.000000+0 0.000000+0 0 0 1 179137 1452 2 17 2 9137 1452 3 1.000000-5 2.109010+0 5.000000+5 2.178310+0 1.000000+6 2.247620+09137 1452 4 2.000000+6 2.386230+0 3.000000+6 2.524840+0 4.000000+6 2.663450+09137 1452 5 5.000000+6 2.802060+0 6.000000+6 2.940590+0 7.000000+6 3.075370+09137 1452 6 8.000000+6 3.213190+0 9.000000+6 3.352060+0 1.000000+7 3.491050+09137 1452 7 1.200000+7 3.768610+0 1.400000+7 4.045020+0 1.600000+7 4.319400+09137 1452 8 1.800000+7 4.595720+0 2.000000+7 4.872780+0 9137 1452 9 9137 1 099999 9.123300+4 2.310380+2 0 2 0 09137 1455 1 0.000000+0 0.000000+0 0 0 1 09137 1455 2 1.000000+0 9137 1455 3 0.000000+0 0.000000+0 0 0 1 179137 1455 4 17 2 9137 1455 5 1.000000-5 2.301000-2 5.000000+5 2.301000-2 1.000000+6 2.301000-29137 1455 6 2.000000+6 2.301000-2 3.000000+6 2.301000-2 4.000000+6 2.301000-29137 1455 7 5.000000+6 2.301000-2 6.000000+6 2.293320-2 7.000000+6 1.910480-29137 1455 8 8.000000+6 1.830840-2 9.000000+6 1.857210-2 1.000000+7 1.895010-29137 1455 9 1.200000+7 1.928920-2 1.400000+7 1.847600-2 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1.013850-7 2.900000+4 1.093010-79137 5 18 1856 3.400000+4 1.184610-7 4.000000+4 1.285950-7 4.600000+4 1.379780-79137 5 18 1857 5.400000+4 1.495540-7 6.300000+4 1.615500-7 7.400000+4 1.750320-79137 5 18 1858 8.600000+4 1.885500-7 1.000000+5 2.030550-7 2.000000+5 2.600030-79137 5 18 1859 3.000000+5 2.929760-7 4.000000+5 3.151330-7 5.000000+5 3.298150-79137 5 18 1860 6.000000+5 3.386320-7 7.000000+5 3.428480-7 8.000000+5 3.434060-79137 5 18 1861 9.000000+5 3.410510-7 1.000000+6 3.363620-7 1.100000+6 3.297860-79137 5 18 1862 1.200000+6 3.216810-7 1.300000+6 3.124270-7 1.400000+6 3.023500-79137 5 18 1863 1.500000+6 2.917030-7 1.600000+6 2.806910-7 1.700000+6 2.694770-79137 5 18 1864 1.800000+6 2.581910-7 1.900000+6 2.469380-7 2.000000+6 2.358020-79137 5 18 1865 2.100000+6 2.248480-7 2.200000+6 2.141290-7 2.300000+6 2.036840-79137 5 18 1866 2.400000+6 1.935450-7 2.500000+6 1.837330-7 2.600000+6 1.742650-79137 5 18 1867 2.700000+6 1.651490-7 2.800000+6 1.563930-7 2.900000+6 1.479970-79137 5 18 1868 3.000000+6 1.399610-7 3.100000+6 1.322800-7 3.200000+6 1.249510-79137 5 18 1869 3.300000+6 1.179650-7 3.400000+6 1.113130-7 3.500000+6 1.049870-79137 5 18 1870 3.600000+6 9.897720-8 3.700000+6 9.327170-8 3.800000+6 8.786010-89137 5 18 1871 3.900000+6 8.273110-8 4.000000+6 7.787350-8 4.100000+6 7.327610-89137 5 18 1872 4.200000+6 6.892750-8 4.300000+6 6.481670-8 4.400000+6 6.093290-89137 5 18 1873 4.500000+6 5.726540-8 4.600000+6 5.380390-8 4.700000+6 5.053830-89137 5 18 1874 4.800000+6 4.745890-8 4.900000+6 4.455620-8 5.000000+6 4.182130-89137 5 18 1875 5.100000+6 3.924530-8 5.200000+6 3.681990-8 5.300000+6 3.453720-89137 5 18 1876 5.400000+6 3.238930-8 5.500000+6 3.036900-8 5.600000+6 2.846920-89137 5 18 1877 5.700000+6 2.668330-8 5.800000+6 2.500500-8 5.900000+6 2.342810-89137 5 18 1878 6.000000+6 2.194690-8 6.100000+6 2.055590-8 6.200000+6 1.925000-89137 5 18 1879 6.300000+6 1.802420-8 6.400000+6 1.687390-8 6.500000+6 1.579470-89137 5 18 1880 6.600000+6 1.478240-8 6.700000+6 1.383290-8 6.800000+6 1.294270-89137 5 18 1881 6.900000+6 1.210810-8 7.000000+6 1.132580-8 7.100000+6 1.059270-89137 5 18 1882 7.200000+6 9.905810-9 7.300000+6 9.262300-9 7.400000+6 8.659550-99137 5 18 1883 7.500000+6 8.095060-9 7.600000+6 7.566490-9 7.700000+6 7.071630-99137 5 18 1884 7.800000+6 6.608390-9 7.900000+6 6.174810-9 8.000000+6 5.769070-99137 5 18 1885 8.100000+6 5.389410-9 8.200000+6 5.034220-9 8.300000+6 4.701950-99137 5 18 1886 8.400000+6 4.391180-9 8.500000+6 4.100540-9 8.600000+6 3.828770-99137 5 18 1887 8.700000+6 3.574670-9 8.800000+6 3.337120-9 8.900000+6 3.115070-99137 5 18 1888 9.000000+6 2.907520-9 9.100000+6 2.713570-9 9.200000+6 2.532330-99137 5 18 1889 9.300000+6 2.362990-9 9.400000+6 2.204780-9 9.500000+6 2.057000-99137 5 18 1890 9.600000+6 1.918960-9 9.700000+6 1.790040-9 9.800000+6 1.669640-99137 5 18 1891 9.900000+6 1.557220-9 1.000000+7 1.452250-9 1.010000+7 1.354250-99137 5 18 1892 1.020000+7 1.262770-9 1.030000+7 1.177390-9 1.040000+7 1.097690-99137 5 18 1893 1.050000+7 1.023310-9 1.060000+7 9.53903-10 1.070000+7 8.89140-109137 5 18 1894 1.080000+7 8.28714-10 1.090000+7 7.72341-10 1.100000+7 7.19753-109137 5 18 1895 1.110000+7 6.70700-10 1.120000+7 6.24947-10 1.130000+7 5.82277-109137 5 18 1896 1.140000+7 5.42484-10 1.150000+7 5.05378-10 1.160000+7 4.70779-109137 5 18 1897 1.170000+7 4.38521-10 1.180000+7 4.08447-10 1.190000+7 3.80412-109137 5 18 1898 1.200000+7 3.54280-10 1.210000+7 3.29922-10 1.220000+7 3.07220-109137 5 18 1899 1.230000+7 2.86064-10 1.240000+7 2.66348-10 1.250000+7 2.47976-109137 5 18 1900 1.260000+7 2.30859-10 1.270000+7 2.14910-10 1.280000+7 2.00052-109137 5 18 1901 1.290000+7 1.86211-10 1.300000+7 1.73317-10 1.310000+7 1.61307-109137 5 18 1902 1.320000+7 1.50122-10 1.330000+7 1.39704-10 1.340000+7 1.30002-109137 5 18 1903 1.350000+7 1.20968-10 1.360000+7 1.12555-10 1.370000+7 1.04722-109137 5 18 1904 1.380000+7 9.74288-11 1.390000+7 9.06390-11 1.400000+7 8.43180-119137 5 18 1905 1.410000+7 7.84338-11 1.420000+7 7.29567-11 1.430000+7 6.78586-119137 5 18 1906 1.440000+7 6.31136-11 1.450000+7 5.86975-11 1.460000+7 5.45878-119137 5 18 1907 1.470000+7 5.07634-11 1.480000+7 4.72046-11 1.490000+7 4.38932-119137 5 18 1908 1.500000+7 4.08122-11 1.510000+7 3.79457-11 1.520000+7 3.52789-119137 5 18 1909 1.530000+7 3.27980-11 1.540000+7 3.04902-11 1.550000+7 2.83434-119137 5 18 1910 1.560000+7 2.63467-11 1.570000+7 2.44895-11 1.580000+7 2.27622-119137 5 18 1911 1.590000+7 2.11558-11 1.600000+7 1.96619-11 1.610000+7 1.82727-119137 5 18 1912 1.620000+7 1.69810-11 1.630000+7 1.57799-11 1.640000+7 1.46631-119137 5 18 1913 1.650000+7 1.36247-11 1.660000+7 1.26594-11 1.670000+7 1.17620-119137 5 18 1914 1.680000+7 1.09277-11 1.690000+7 1.01523-11 1.700000+7 9.43140-129137 5 18 1915 1.710000+7 8.76139-12 1.720000+7 8.13864-12 1.730000+7 7.55986-129137 5 18 1916 1.740000+7 7.02196-12 1.750000+7 6.52207-12 1.760000+7 6.05754-129137 5 18 1917 1.770000+7 5.62587-12 1.780000+7 5.22476-12 1.790000+7 4.85207-129137 5 18 1918 1.800000+7 4.50578-12 1.810000+7 4.18406-12 1.820000+7 3.88516-129137 5 18 1919 1.830000+7 3.60747-12 1.840000+7 3.34951-12 1.850000+7 3.10989-129137 5 18 1920 1.860000+7 2.88729-12 1.870000+7 2.68054-12 1.880000+7 2.48850-129137 5 18 1921 1.890000+7 2.31013-12 1.900000+7 2.14447-12 1.910000+7 1.99062-129137 5 18 1922 1.920000+7 1.84775-12 1.930000+7 1.71507-12 1.940000+7 1.59185-129137 5 18 1923 1.950000+7 1.47744-12 1.960000+7 1.37121-12 1.970000+7 1.27257-129137 5 18 1924 1.980000+7 1.18099-12 1.990000+7 1.09596-12 2.000000+7 1.01702-129137 5 18 1925 2.020000+7 0.000000+0 9137 5 18 1926 0.000000+0 6.500000+6 0 0 1 3529137 5 18 1927 352 2 9137 5 18 1928 0.000000+0 0.000000+0 1.000000-5 1.83275-12 1.200000-5 2.00768-129137 5 18 1929 1.400000-5 2.16854-12 1.600000-5 2.31827-12 1.800000-5 2.45890-129137 5 18 1930 2.200000-5 2.71842-12 2.500000-5 2.89785-12 2.900000-5 3.12108-129137 5 18 1931 3.400000-5 3.37945-12 4.000000-5 3.66553-12 4.600000-5 3.93085-129137 5 18 1932 5.400000-5 4.25898-12 6.300000-5 4.60023-12 7.400000-5 4.98570-129137 5 18 1933 8.600000-5 5.37477-12 1.000000-4 5.79578-12 1.200000-4 6.34897-129137 5 18 1934 1.400000-4 6.85769-12 1.600000-4 7.33120-12 1.800000-4 7.77592-129137 5 18 1935 2.200000-4 8.59664-12 2.500000-4 9.16408-12 2.900000-4 9.87005-129137 5 18 1936 3.400000-4 1.06871-11 4.000000-4 1.15919-11 4.600000-4 1.24310-119137 5 18 1937 5.400000-4 1.34687-11 6.300000-4 1.45479-11 7.400000-4 1.57670-119137 5 18 1938 8.600000-4 1.69975-11 1.000000-3 1.83290-11 1.200000-3 2.00785-119137 5 18 1939 1.400000-3 2.16875-11 1.600000-3 2.31851-11 1.800000-3 2.45916-119137 5 18 1940 2.200000-3 2.71874-11 2.500000-3 2.89821-11 2.900000-3 3.12151-119137 5 18 1941 3.400000-3 3.37995-11 4.000000-3 3.66612-11 4.600000-3 3.93153-119137 5 18 1942 5.400000-3 4.25977-11 6.300000-3 4.60115-11 7.400000-3 4.98678-119137 5 18 1943 8.600000-3 5.37603-11 1.000000-2 5.79724-11 1.200000-2 6.35073-119137 5 18 1944 1.400000-2 6.85974-11 1.600000-2 7.33354-11 1.800000-2 7.77857-119137 5 18 1945 2.200000-2 8.59987-11 2.500000-2 9.16774-11 2.900000-2 9.87430-119137 5 18 1946 3.400000-2 1.06921-10 4.000000-2 1.15977-10 4.600000-2 1.24377-109137 5 18 1947 5.400000-2 1.34766-10 6.300000-2 1.45571-10 7.400000-2 1.57778-109137 5 18 1948 8.600000-2 1.70101-10 1.000000-1 1.83436-10 1.200000-1 2.00962-109137 5 18 1949 1.400000-1 2.17080-10 1.600000-1 2.32085-10 1.800000-1 2.46181-109137 5 18 1950 2.200000-1 2.72197-10 2.500000-1 2.90188-10 2.900000-1 3.12576-109137 5 18 1951 3.400000-1 3.38494-10 4.000000-1 3.67199-10 4.600000-1 3.93828-109137 5 18 1952 5.400000-1 4.26769-10 6.300000-1 4.61040-10 7.400000-1 4.99764-109137 5 18 1953 8.600000-1 5.38865-10 1.000000+0 5.81192-10 1.200000+0 6.36834-109137 5 18 1954 1.400000+0 6.88029-10 1.600000+0 7.35702-10 1.800000+0 7.80498-109137 5 18 1955 2.200000+0 8.63216-10 2.500000+0 9.20443-10 2.900000+0 9.91686-109137 5 18 1956 3.400000+0 1.074200-9 4.000000+0 1.165640-9 4.600000+0 1.250520-99137 5 18 1957 5.400000+0 1.355580-9 6.300000+0 1.464960-9 7.400000+0 1.588640-99137 5 18 1958 8.600000+0 1.713630-9 1.000000+1 1.849040-9 1.200000+1 2.027230-99137 5 18 1959 1.400000+1 2.191350-9 1.600000+1 2.344330-9 1.800000+1 2.488220-99137 5 18 1960 2.200000+1 2.754260-9 2.500000+1 2.938570-9 2.900000+1 3.168320-99137 5 18 1961 3.400000+1 3.434830-9 4.000000+1 3.730680-9 4.600000+1 4.005770-99137 5 18 1962 5.400000+1 4.346930-9 6.300000+1 4.702830-9 7.400000+1 5.106210-99137 5 18 1963 8.600000+1 5.514820-9 1.000000+2 5.958620-9 1.200000+2 6.544370-99137 5 18 1964 1.400000+2 7.085640-9 1.600000+2 7.591690-9 1.800000+2 8.068960-99137 5 18 1965 2.200000+2 8.954740-9 2.500000+2 9.570970-9 2.900000+2 1.034200-89137 5 18 1966 3.400000+2 1.124040-8 4.000000+2 1.224260-8 4.600000+2 1.317920-89137 5 18 1967 5.400000+2 1.434680-8 6.300000+2 1.557220-8 7.400000+2 1.696980-89137 5 18 1968 8.600000+2 1.839500-8 1.000000+3 1.995350-8 1.200000+3 2.202720-89137 5 18 1969 1.400000+3 2.396000-8 1.600000+3 2.578130-8 1.800000+3 2.751140-89137 5 18 1970 2.200000+3 3.075370-8 2.500000+3 3.303290-8 2.900000+3 3.591120-89137 5 18 1971 3.400000+3 3.930160-8 4.000000+3 4.312930-8 4.600000+3 4.674820-89137 5 18 1972 5.400000+3 5.131540-8 6.300000+3 5.617250-8 7.400000+3 6.178990-89137 5 18 1973 8.600000+3 6.760030-8 1.000000+4 7.404580-8 1.200000+4 8.276400-89137 5 18 1974 1.400000+4 9.102980-8 1.600000+4 9.893610-8 1.800000+4 1.065480-79137 5 18 1975 2.200000+4 1.210650-7 2.500000+4 1.314570-7 2.900000+4 1.447870-79137 5 18 1976 3.400000+4 1.607670-7 4.000000+4 1.791470-7 4.600000+4 1.968310-79137 5 18 1977 5.400000+4 2.195440-7 6.300000+4 2.441420-7 7.400000+4 2.731120-79137 5 18 1978 8.600000+4 3.036130-7 1.000000+5 3.380230-7 2.000000+5 4.577830-79137 5 18 1979 3.000000+5 4.675080-7 4.000000+5 4.170860-7 5.000000+5 3.675360-79137 5 18 1980 6.000000+5 3.390090-7 7.000000+5 3.270730-7 8.000000+5 3.213200-79137 5 18 1981 9.000000+5 3.168010-7 1.000000+6 3.115620-7 1.100000+6 3.050970-79137 5 18 1982 1.200000+6 2.974060-7 1.300000+6 2.887180-7 1.400000+6 2.792940-79137 5 18 1983 1.500000+6 2.693550-7 1.600000+6 2.590870-7 1.700000+6 2.486380-79137 5 18 1984 1.800000+6 2.381300-7 1.900000+6 2.276600-7 2.000000+6 2.173050-79137 5 18 1985 2.100000+6 2.071250-7 2.200000+6 1.971690-7 2.300000+6 1.874740-79137 5 18 1986 2.400000+6 1.780680-7 2.500000+6 1.689700-7 2.600000+6 1.601940-79137 5 18 1987 2.700000+6 1.517510-7 2.800000+6 1.436440-7 2.900000+6 1.358750-79137 5 18 1988 3.000000+6 1.284430-7 3.100000+6 1.213440-7 3.200000+6 1.145720-79137 5 18 1989 3.300000+6 1.081200-7 3.400000+6 1.019810-7 3.500000+6 9.614550-89137 5 18 1990 3.600000+6 9.060350-8 3.700000+6 8.534520-8 3.800000+6 8.036010-89137 5 18 1991 3.900000+6 7.563770-8 4.000000+6 7.116720-8 4.100000+6 6.693820-89137 5 18 1992 4.200000+6 6.294000-8 4.300000+6 5.916230-8 4.400000+6 5.559480-89137 5 18 1993 4.500000+6 5.222750-8 4.600000+6 4.905090-8 4.700000+6 4.605540-89137 5 18 1994 4.800000+6 4.323200-8 4.900000+6 4.057190-8 5.000000+6 3.806660-89137 5 18 1995 5.100000+6 3.570790-8 5.200000+6 3.348820-8 5.300000+6 3.139990-89137 5 18 1996 5.400000+6 2.943590-8 5.500000+6 2.758940-8 5.600000+6 2.585370-89137 5 18 1997 5.700000+6 2.422290-8 5.800000+6 2.269090-8 5.900000+6 2.125210-89137 5 18 1998 6.000000+6 1.990120-8 6.100000+6 1.863310-8 6.200000+6 1.744310-89137 5 18 1999 6.300000+6 1.632660-8 6.400000+6 1.527920-8 6.500000+6 1.429700-89137 5 18 2000 6.600000+6 1.337600-8 6.700000+6 1.251260-8 6.800000+6 1.170330-89137 5 18 2001 6.900000+6 1.094490-8 7.000000+6 1.023440-8 7.100000+6 9.568760-99137 5 18 2002 7.200000+6 8.945320-9 7.300000+6 8.361500-9 7.400000+6 7.814860-99137 5 18 2003 7.500000+6 7.303110-9 7.600000+6 6.824100-9 7.700000+6 6.375810-99137 5 18 2004 7.800000+6 5.956320-9 7.900000+6 5.563830-9 8.000000+6 5.196670-99137 5 18 2005 8.100000+6 4.853240-9 8.200000+6 4.532060-9 8.300000+6 4.231710-99137 5 18 2006 8.400000+6 3.950880-9 8.500000+6 3.688340-9 8.600000+6 3.442930-99137 5 18 2007 8.700000+6 3.213550-9 8.800000+6 2.999180-9 8.900000+6 2.798860-99137 5 18 2008 9.000000+6 2.611700-9 9.100000+6 2.436840-9 9.200000+6 2.273500-99137 5 18 2009 9.300000+6 2.120930-9 9.400000+6 1.978430-9 9.500000+6 1.845370-99137 5 18 2010 9.600000+6 1.721110-9 9.700000+6 1.605100-9 9.800000+6 1.496790-99137 5 18 2011 9.900000+6 1.395680-9 1.000000+7 1.301310-9 1.010000+7 1.213230-99137 5 18 2012 1.020000+7 1.131030-9 1.030000+7 1.054320-9 1.040000+7 9.82744-109137 5 18 2013 1.050000+7 9.15964-10 1.060000+7 8.53664-10 1.070000+7 7.95546-109137 5 18 2014 1.080000+7 7.41336-10 1.090000+7 6.90774-10 1.100000+7 6.43618-109137 5 18 2015 1.110000+7 5.99643-10 1.120000+7 5.58637-10 1.130000+7 5.20402-109137 5 18 2016 1.140000+7 4.84754-10 1.150000+7 4.51520-10 1.160000+7 4.20539-109137 5 18 2017 1.170000+7 3.91660-10 1.180000+7 3.64743-10 1.190000+7 3.39656-109137 5 18 2018 1.200000+7 3.16276-10 1.210000+7 2.94488-10 1.220000+7 2.74186-109137 5 18 2019 1.230000+7 2.55269-10 1.240000+7 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