JENDL-5 (Neutron sublibrary (up to 20 MeV)) Pu-242 0 0 0 0 9.424200+4 2.399790+2 1 1 6 19446 1451 1 0.000000+0 1.000000+0 0 0 0 69446 1451 2 1.000000+0 2.000000+7 0 0 10 59446 1451 3 0.000000+0 0.000000+0 3 0 490 1089446 1451 4 94-Pu-242 JAEA+ EVAL-JAN10 O.Iwamoto, T.Nakagawa, Murata, + 9446 1451 5 DIST-DEC21 20130704 9446 1451 6 ----JENDL-5 MATERIAL 9446 9446 1451 7 -----INCIDENT NEUTRON DATA 9446 1451 8 ------ENDF-6 FORMAT 9446 1451 9 9446 1451 10 History 9446 1451 11 06-08 Nu-p was revised. 9446 1451 12 06-09 Resonance parameters were revised. 9446 1451 13 06-12 Fission cross section was revised. 9446 1451 14 07-05 Data were calculated with CCONE code. 9446 1451 15 Data were compiled as JENDL/AC-2008/1/. 9446 1451 16 09-03 (1,452), (1,455) and (1,456) were revised. 9446 1451 17 09-08 (MF1,MT458) was evaluated. 9446 1451 18 10-01 Data of prompt gamma rays due to fission were given. 9446 1451 19 10-03 Covariance data were given. 9446 1451 20 13-07 (32,151) were corrected. 9446 1451 21 19-12 JENDL-5a2 9446 1451 22 21-07 Resonance parameters of 2.676 eV resonace were revised 9446 1451 23 by S. Nakayama. 9446 1451 24 21-08 Uncertainties of 2.676 eV resonace parameters were 9446 1451 25 revised by S. Nakayama. 9446 1451 26 21-11 JENDL-5b3 9446 1451 27 (MF2/MT151) RP below 1 keV, Lerendegui-Marco(2018) adopted 9446 1451 28 21-11 revised by O.Iwamoto 9446 1451 29 (MF3/MT19-21,38) deleted 9446 1451 30 (MF8/MT16-18,37,102) JENDL/AD-2017 adopted 9446 1451 31 (MF8/MT4) added 9446 1451 32 21-11 above 20 MeV, JENDL-4.0/HE merged by O.Iwamoto 9446 1451 33 21-11 (MF6/MT5) recoil spectrum added by O.Iwamoto 9446 1451 34 21-12 (MF32/MT151) modified by O.Iwamoto 9446 1451 35 RP unc. of Lerendegui-Marco et al.,PRC97,024605(2018) 9446 1451 36 21-12 (MF1/MT452,456) by O.Iwamoto 9446 1451 37 revise nu-p (En > 20 MeV) by a systematics 9446 1451 38 (MF6/MT5) by O.Iwamoto 9446 1451 39 modify multiplicity of ZAP=1 to compensate 9446 1451 40 the revision of nu-p 9446 1451 41 9446 1451 42 9446 1451 43 MF= 1 General information 9446 1451 44 MT=452 Number of Neutrons per fission 9446 1451 45 Sum of MT=455 and 456 9446 1451 46 9446 1451 47 MT=455 Delayed neutrons 9446 1451 48 Determined from nu-d of the following three nuclides and 9446 1451 49 partial fission cross sections calculated with CCONE code/2/. 9446 1451 50 9446 1451 51 Pu-243 = 0.0153 an average of experimental data of Krick 9446 1451 52 and Evans /3, 4/ 9446 1451 53 Pu-242 = 0.011 0.00160 /5/ was multiplied by 0.7. 9446 1451 54 Pu-241 = 0.0064 0.00911 /5/ was multiplied by 0.7. 9446 1451 55 9446 1451 56 Values for Pu-242 and 241 were multiplied by 0.7 to 9446 1451 57 reproduce the nu-d of 0.0113+-0.0009 at 14.7MeV/6/ 9446 1451 58 9446 1451 59 Decay constants were evaluated by Brady and England/7/. 9446 1451 60 9446 1451 61 MT=456 Number of prompt neutrons per fission 9446 1451 62 Least-squares fitting of a straight line to the experimental 9446 1451 63 data of Khokhlov et al./8/ Since their data were total 9446 1451 64 numbers of neutrons per fission, numbers of delayed neutrons 9446 1451 65 (MT=455) were subtracted. 9446 1451 66 9446 1451 67 nu-p = 2.8779 + 0.13755*E(MeV) 9446 1451 68 9446 1451 69 MT=458 Components of energy release due to fission 9446 1451 70 Total energy and prompt energy were calculated from mass 9446 1451 71 balance using JENDL-4 fission yields data and mass excess 9446 1451 72 evaluation. Mass excess values were from Audi's 2009 9446 1451 73 evaluation/9/. Delayed energy values were calculated from 9446 1451 74 the energy release for infinite irradiation using JENDL FP 9446 1451 75 Decay Data File 2000 and JENDL-4 yields data. For delayed 9446 1451 76 neutron energy, as the JENDL FP Decay Data File 2000/10/ does 9446 1451 77 not include average neutron energy values, the average values 9446 1451 78 were calculated using the formula shown in the report by 9446 1451 79 T.R. England/11/. The fractions of prompt energy were 9446 1451 80 calculated using the fractions of Sher's evaluation/12/ when 9446 1451 81 they were provided. When the fractions were not given by Sher,9446 1451 82 averaged fractions were used. 9446 1451 83 9446 1451 84 9446 1451 85 MF= 2 Resonance parameters 9446 1451 86 MT=151 9446 1451 87 Resolved resonance parameters (below 1 keV) 9446 1451 88 Resonance parameters of JENDL-3.3 were modified: 9446 1451 89 * Upper boundary was decreased from 1.9 keV to 1 keV. 9446 1451 90 * Capture width of 2.67-eV resonances was changed from 22 9446 1451 91 meV to 26.8 meV. 9446 1451 92 * Fission width of 53.46-eV resonance was increased from 9446 1451 93 1.825 micro-eV to 36 micro-eV. 9446 1451 94 9446 1451 95 Thermal capture cross section of 19.98+-0.66 b to be 9446 1451 96 reproduced was determined from Butler et al./13/, Durham 9446 1451 97 and Molson/14/ and Marie et al./15/. 9446 1451 98 9446 1451 99 Unresolved resonance parameters (1 keV - 100 keV) 9446 1451 100 Parameters were estimated with ASREP code/16/ so as to 9446 1451 101 total, fission and capture cross sections in this energy 9446 1451 102 region. They are used only for self-shielding calculations. 9446 1451 103 9446 1451 104 9446 1451 105 Thermal cross sections and resonance integrals (at 300K) 9446 1451 106 ------------------------------------------------------- 9446 1451 107 0.0253 eV reson. integ.(*) 9446 1451 108 (barns) (barns) 9446 1451 109 ------------------------------------------------------- 9446 1451 110 total 28.213 9446 1451 111 elastic 8.326 9446 1451 112 fission 0.00244 4.36 9446 1451 113 capture 19.885 1130 9446 1451 114 ------------------------------------------------------- 9446 1451 115 (*) In the energy range from 0.5 eV to 10 MeV. 9446 1451 116 9446 1451 117 9446 1451 118 MF= 3 Neutron cross sections 9446 1451 119 Cross sections above the resolved resonance region except for 9446 1451 120 the elastic scattering (MT=2) and fission cross sections (MT=18,9446 1451 121 19, 20, 21, 38) were calculated with CCONE code/2/. 9446 1451 122 9446 1451 123 MT= 1 Total cross section 9446 1451 124 Calculated with CCONE code and modified below 500 keV by 9446 1451 125 multiplying an energy-dependent factor so as to reproduce 9446 1451 126 average total cross sections obtained from the data of Young 9446 1451 127 et al. /17/ The calculation was made with CC OMP of 9446 1451 128 Soukhovitskii et al./18/ 9446 1451 129 9446 1451 130 MT= 2 Elastic scattering cross section 9446 1451 131 Calculated as total cross section - sum of partial cross 9446 1451 132 sections. 9446 1451 133 9446 1451 134 MT=18 Fission cross section 9446 1451 135 The following experimental data were analyzed in the energy 9446 1451 136 range from 1 keV to 20 MeV with the GMA code/19/: 9446 1451 137 9446 1451 138 Authors Energy range Data points Reference 9446 1451 139 Bulter 141 keV - 1.66 MeV 65 /20/ 9446 1451 140 Fomushkin+ 14.5 MeV 1 /21/ 9446 1451 141 Bergen+ 0.1 - 2.96 MeV 141 /22/(*1) 9446 1451 142 Auchampaugh+ 0.95 keV - 3.99 MeV 3102 /23/ 9446 1451 143 Meadows 0.397 - 9.92 MeV 49 /24/(*2) 9446 1451 144 Behrens 97.2 keV - 20.0 MeV 133 /25/(*2) 9446 1451 145 Kuprijanov+ 0.127 - 7.4 MeV 71 /26/(*2) 9446 1451 146 Cance+ 2.47 MeV 2 /27/ 9446 1451 147 Alkhazov+ 14.7 MeV 1 /28/ 9446 1451 148 Weigmann+ 0.3 - 9.7 MeV 222 /29/ 9446 1451 149 Arlt+ 14.7 MeV 1 /30/ 9446 1451 150 Meadows 14.7 MeV 1 /31/(*2) 9446 1451 151 Iwasaki+ 0.597 - 6.76 MeV 17 /32/(*2) 9446 1451 152 Staples 0.514 - 19.5 MeV 124 /33/(*2) 9446 1451 153 9446 1451 154 *1) only the data above 100 keV were used. 9446 1451 155 *2) ratio to U-235 fission cross section 9446 1451 156 9446 1451 157 The results of GMA were used to determine the parameters in 9446 1451 158 the CCONE calculation. 9446 1451 159 9446 1451 160 MT=19, 20, 21, 38 Multi-chance fission cross sections 9446 1451 161 Calculated with CCONE code, and renormalized to the total 9446 1451 162 fission cross section (MT=18). 9446 1451 163 9446 1451 164 MT=102 Capture cross section 9446 1451 165 Calculated with CCONE code. The experimental data of Wisshak 9446 1451 166 and Kaeppeler /34,35/ and Hockenbury et al./36/ were used to 9446 1451 167 determine the parameters in the CCONE calculation. 9446 1451 168 9446 1451 169 9446 1451 170 MF= 4 Angular distributions of secondary neutrons 9446 1451 171 MT=2 Elastic scattering 9446 1451 172 Calculated with CCONE code. 9446 1451 173 9446 1451 174 MT=18 Fission 9446 1451 175 Isotropic distributions in the laboratory system were assumed.9446 1451 176 9446 1451 177 9446 1451 178 MF= 5 Energy distributions of secondary neutrons 9446 1451 179 MT=18 Fission spectra 9446 1451 180 Calculated with CCONE code. 9446 1451 181 9446 1451 182 MT=455 Delayed neutron spectra 9446 1451 183 (Same as JENDL-3.3) 9446 1451 184 Results of summation calculation made by Brady and England/7/ 9446 1451 185 were adopted. 9446 1451 186 9446 1451 187 MF= 6 Energy-angle distributions 9446 1451 188 Calculated with CCONE code. 9446 1451 189 Distributions from fission (MT=18) are not included. 9446 1451 190 9446 1451 191 9446 1451 192 MF=12 Photon production multiplicities 9446 1451 193 MT=18 Fission 9446 1451 194 Calculated from the total energy released by the prompt 9446 1451 195 gamma-rays due to fission given in MF=1/MT=458 and the 9446 1451 196 average energy of gamma-rays. 9446 1451 197 9446 1451 198 9446 1451 199 MF=14 Photon angular distributions 9446 1451 200 MT=18 Fission 9446 1451 201 Isotoropic distributions were assumed. 9446 1451 202 9446 1451 203 9446 1451 204 MF=15 Continuous photon energy spectra 9446 1451 205 MT=18 Fission 9446 1451 206 Experimental data measured by Verbinski et al./37/ for 9446 1451 207 Pu-239 thermal fission were adopted. 9446 1451 208 9446 1451 209 9446 1451 210 MF=31 Covariances of average number of neutrons per fission 9446 1451 211 MT=452 Number of neutrons per fission 9446 1451 212 Combination of covariances for MT=455 and MT=456. 9446 1451 213 9446 1451 214 MT=455 9446 1451 215 Error of 10% was assumed below 5 MeV and above 5 MeV, 9446 1451 216 respectively by comparing with experimental data/4, 6/ 9446 1451 217 9446 1451 218 MT=456 9446 1451 219 Covariance was obtained by fitting a linear function to the 9446 1451 220 experimental data of Khokhlov et al./8/(see MF1,MT456). 9446 1451 221 Variances were multiplied by a factor of 2. 9446 1451 222 9446 1451 223 9446 1451 224 MF=32 Covariances of resonance parameters 9446 1451 225 Format of LCOMP=0 was adopted. 9446 1451 226 9446 1451 227 Standard deviations of resonance energy, neutron and capture 9446 1451 228 widths were taken from Mughabghab /38/ Those of fission 9446 1451 229 width were based on the data of fission area reported by 9446 1451 230 Weigmann et al./29/ and Auchampaugh et al./23/. 9446 1451 231 9446 1451 232 If no information was available, uncertainties were assumed. 9446 1451 233 9446 1451 234 9446 1451 235 MF=33 Covariances of neutron cross sections 9446 1451 236 Covariances were given to all the cross sections by using 9446 1451 237 KALMAN code/39/ and the covariances of model parameters 9446 1451 238 used in the theoretical calculations. 9446 1451 239 9446 1451 240 For the following cross sections, covariances were determined 9446 1451 241 by different methods. 9446 1451 242 9446 1451 243 MT=1, 2 Total and elastic scattering cross sections 9446 1451 244 In the resonance region (below 1 keV), uncertainty of 8 % 9446 1451 245 was added. 9446 1451 246 9446 1451 247 Above 1 keV, covariance matrix was obtained with CCONE and 9446 1451 248 KALMAN codes/39/. 9446 1451 249 9446 1451 250 MT=18 Fission cross section 9446 1451 251 In the resonance region from 10 to 1000 eV, addtional error 9446 1451 252 of 50% was given. 9446 1451 253 9446 1451 254 Above the resonance region, cross section was evaluated with 9446 1451 255 GMA code/19/. Standard deviation obatianed was multiplied 9446 1451 256 by a factor of 2.0. 9446 1451 257 9446 1451 258 MT=102 Capture cross section 9446 1451 259 In the resonance region from 10 to 1000 eV, addtional error 9446 1451 260 of 10% was given. 9446 1451 261 9446 1451 262 Above 1 keV, covariance matrix was obtained with CCONE and 9446 1451 263 KALMAN codes/39/. 9446 1451 264 9446 1451 265 9446 1451 266 MF=34 Covariances for Angular Distributions 9446 1451 267 MT=2 Elastic scattering 9446 1451 268 Covariances were given only to P1 components. 9446 1451 269 9446 1451 270 9446 1451 271 MF=35 Covariances for Energy Distributions 9446 1451 272 MT=18 Fission spectra 9446 1451 273 Estimated with CCONE and KALMAN codes. 9446 1451 274 9446 1451 275 9446 1451 276 ***************************************************************** 9446 1451 277 Calculation with CCONE code 9446 1451 278 ***************************************************************** 9446 1451 279 9446 1451 280 Models and parameters used in the CCONE/2/ calculation 9446 1451 281 1) Coupled channel optical model 9446 1451 282 Levels in the rotational band were included. Optical model 9446 1451 283 potential and coupled levels are shown in Table 1. 9446 1451 284 9446 1451 285 2) Two-component exciton model/40/ 9446 1451 286 * Global parametrization of Koning-Duijvestijn/41/ 9446 1451 287 was used. 9446 1451 288 * Gamma emission channel/42/ was added to simulate direct 9446 1451 289 and semi-direct capture reaction. 9446 1451 290 9446 1451 291 3) Hauser-Feshbach statistical model 9446 1451 292 * Moldauer width fluctuation correction/43/ was included. 9446 1451 293 * Neutron, gamma and fission decay channel were included. 9446 1451 294 * Transmission coefficients of neutrons were taken from 9446 1451 295 coupled channel calculation in Table 1. 9446 1451 296 * The level scheme of the target is shown in Table 2. 9446 1451 297 * Level density formula of constant temperature and Fermi-gas 9446 1451 298 model were used with shell energy correction and collective 9446 1451 299 enhancement factor. Parameters are shown in Table 3. 9446 1451 300 * Fission channel: 9446 1451 301 Double humped fission barriers were assumed. 9446 1451 302 Fission barrier penetrabilities were calculated with 9446 1451 303 Hill-Wheler formula/44/. Fission barrier parameters were 9446 1451 304 shown in Table 4. Transition state model was used and 9446 1451 305 continuum levels are assumed above the saddles. The level 9446 1451 306 density parameters for inner and outer saddles are shown in 9446 1451 307 Tables 5 and 6, respectively. 9446 1451 308 * Gamma-ray strength function of Kopecky et al/45/,/46/ 9446 1451 309 was used. The prameters are shown in Table 7. 9446 1451 310 9446 1451 311 9446 1451 312 ------------------------------------------------------------------9446 1451 313 Tables 9446 1451 314 ------------------------------------------------------------------9446 1451 315 9446 1451 316 Table 1. Coupled channel calculation 9446 1451 317 -------------------------------------------------- 9446 1451 318 * rigid rotor model was applied 9446 1451 319 * coupled levels = 0,1,2,3,4 (see Table 2) 9446 1451 320 * optical potential parameters /18/ 9446 1451 321 Volume: 9446 1451 322 V_0 = 49.97 MeV 9446 1451 323 lambda_HF = 0.01004 1/MeV 9446 1451 324 C_viso = 15.9 MeV 9446 1451 325 A_v = 12.04 MeV 9446 1451 326 B_v = 81.36 MeV 9446 1451 327 E_a = 385 MeV 9446 1451 328 r_v = 1.2568 fm 9446 1451 329 a_v = 0.633 fm 9446 1451 330 Surface: 9446 1451 331 W_0 = 17.2 MeV 9446 1451 332 B_s = 11.19 MeV 9446 1451 333 C_s = 0.01361 1/MeV 9446 1451 334 C_wiso = 23.5 MeV 9446 1451 335 r_s = 1.1803 fm 9446 1451 336 a_s = 0.601 fm 9446 1451 337 Spin-orbit: 9446 1451 338 V_so = 5.75 MeV 9446 1451 339 lambda_so = 0.005 1/MeV 9446 1451 340 W_so = -3.1 MeV 9446 1451 341 B_so = 160 MeV 9446 1451 342 r_so = 1.1214 fm 9446 1451 343 a_so = 0.59 fm 9446 1451 344 Coulomb: 9446 1451 345 C_coul = 1.3 9446 1451 346 r_c = 1.2452 fm 9446 1451 347 a_c = 0.545 fm 9446 1451 348 Deformation: 9446 1451 349 beta_2 = 0.23892 9446 1451 350 beta_4 = 0.04807 9446 1451 351 beta_6 = -0.02376 9446 1451 352 9446 1451 353 * Calculated strength function 9446 1451 354 S0= 0.98e-4 S1= 2.93e-4 R'= 9.32 fm (En=1 keV) 9446 1451 355 -------------------------------------------------- 9446 1451 356 9446 1451 357 Table 2. Level Scheme of Pu-242 9446 1451 358 ------------------- 9446 1451 359 No. Ex(MeV) J PI 9446 1451 360 ------------------- 9446 1451 361 0 0.00000 0 + * 9446 1451 362 1 0.04454 2 + * 9446 1451 363 2 0.14730 4 + * 9446 1451 364 3 0.30640 6 + * 9446 1451 365 4 0.51810 8 + * 9446 1451 366 5 0.77860 10 + 9446 1451 367 6 0.78045 1 - 9446 1451 368 7 0.83230 3 - 9446 1451 369 8 0.86500 3 + 9446 1451 370 9 0.92700 5 - 9446 1451 371 10 0.95600 0 + 9446 1451 372 11 0.99250 2 + 9446 1451 373 12 1.01950 3 - 9446 1451 374 13 1.03920 1 + 9446 1451 375 14 1.06400 4 - 9446 1451 376 15 1.08440 12 + 9446 1451 377 16 1.09210 6 + 9446 1451 378 17 1.10200 2 + 9446 1451 379 18 1.12200 5 - 9446 1451 380 19 1.15100 2 - 9446 1451 381 20 1.15450 3 - 9446 1451 382 ------------------- 9446 1451 383 *) Coupled levels in CC calculation 9446 1451 384 9446 1451 385 Table 3. Level density parameters 9446 1451 386 -------------------------------------------------------- 9446 1451 387 Nuclide a* Pair Eshell T E0 Ematch 9446 1451 388 1/MeV MeV MeV MeV MeV MeV 9446 1451 389 -------------------------------------------------------- 9446 1451 390 Pu-243 18.6999 0.7698 2.4578 0.3280 -0.3352 2.3315 9446 1451 391 Pu-242 18.6337 1.5428 2.4520 0.3701 0.0291 3.6198 9446 1451 392 Pu-241 18.5675 0.7730 2.1853 0.3473 -0.4715 2.5167 9446 1451 393 Pu-240 18.5012 1.5492 2.1440 0.3871 -0.0917 3.7899 9446 1451 394 Pu-239 18.4349 0.7762 1.8503 0.3560 -0.5001 2.5655 9446 1451 395 -------------------------------------------------------- 9446 1451 396 9446 1451 397 Table 4. Fission barrier parameters 9446 1451 398 ---------------------------------------- 9446 1451 399 Nuclide V_A hw_A V_B hw_B 9446 1451 400 MeV MeV MeV MeV 9446 1451 401 ---------------------------------------- 9446 1451 402 Pu-243 5.750 0.680 5.520 0.520 9446 1451 403 Pu-242 6.100 1.000 4.850 0.600 9446 1451 404 Pu-241 5.950 0.580 5.480 0.520 9446 1451 405 Pu-240 6.250 1.040 4.920 0.600 9446 1451 406 Pu-239 6.050 0.700 5.700 0.600 9446 1451 407 ---------------------------------------- 9446 1451 408 9446 1451 409 Table 5. Level density above inner saddle 9446 1451 410 -------------------------------------------------------- 9446 1451 411 Nuclide a* Pair Eshell T E0 Ematch 9446 1451 412 1/MeV MeV MeV MeV MeV MeV 9446 1451 413 -------------------------------------------------------- 9446 1451 414 Pu-243 20.5699 0.8981 2.6000 0.3633 -2.0616 3.3981 9446 1451 415 Pu-242 20.4971 1.7999 2.6000 0.3503 -0.9450 4.0999 9446 1451 416 Pu-241 20.4242 0.9018 2.6000 0.3647 -2.0579 3.4018 9446 1451 417 Pu-240 20.3513 1.8074 2.6000 0.3300 -0.6156 3.8074 9446 1451 418 Pu-239 20.2784 0.9056 2.6000 0.3523 -1.8394 3.2056 9446 1451 419 -------------------------------------------------------- 9446 1451 420 9446 1451 421 Table 6. Level density above outer saddle 9446 1451 422 -------------------------------------------------------- 9446 1451 423 Nuclide a* Pair Eshell T E0 Ematch 9446 1451 424 1/MeV MeV MeV MeV MeV MeV 9446 1451 425 -------------------------------------------------------- 9446 1451 426 Pu-243 20.9439 0.8981 0.5400 0.3740 -0.9758 3.0981 9446 1451 427 Pu-242 20.4971 1.7999 0.5000 0.3933 -0.2466 4.1999 9446 1451 428 Pu-241 20.4242 0.9018 0.4600 0.3804 -0.9744 3.1018 9446 1451 429 Pu-240 20.5363 1.8074 0.4200 0.3796 -0.0661 4.0074 9446 1451 430 Pu-239 20.2784 0.9056 0.3800 0.3901 -1.0534 3.2056 9446 1451 431 -------------------------------------------------------- 9446 1451 432 9446 1451 433 Table 7. Gamma-ray strength function for Pu-243 9446 1451 434 -------------------------------------------------------- 9446 1451 435 K0 = 2.100 E0 = 4.500 (MeV) 9446 1451 436 * E1: ER = 10.90 (MeV) EG = 2.50 (MeV) SIG = 300.00 (mb) 9446 1451 437 ER = 13.80 (MeV) EG = 4.70 (MeV) SIG = 450.00 (mb) 9446 1451 438 * M1: ER = 6.57 (MeV) EG = 4.00 (MeV) SIG = 3.39 (mb) 9446 1451 439 * E2: ER = 10.10 (MeV) EG = 3.19 (MeV) SIG = 6.78 (mb) 9446 1451 440 -------------------------------------------------------- 9446 1451 441 9446 1451 442 9446 1451 443 References 9446 1451 444 1) O.Iwamoto et al.: J. Nucl. Sci. Technol., 46, 510 (2009). 9446 1451 445 2) O.Iwamoto: J. Nucl. Sci. Technol., 44, 687 (2007). 9446 1451 446 3) M.S.Krick, A.E.Evans: Nucl. Sci. Eng., 47, 311 (1972). 9446 1451 447 4) A.E.Evans et al.: Nucl. Sci. Eng., 50, 80 (1973). 9446 1451 448 5) G.Benedetti et al.: Nucl. Sci. Eng., 80, 379 (1982). 9446 1451 449 6) E.Yu.Bobkov et al.: At. 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2.16473-10 1.314500+7 2.08509-109446 5 18 1817 1.320000+7 2.00836-10 1.325500+7 1.93442-10 1.331000+7 1.86318-109446 5 18 1818 1.336500+7 1.79453-10 1.342000+7 1.72839-10 1.347500+7 1.66467-109446 5 18 1819 1.353000+7 1.60328-10 1.358500+7 1.54413-10 1.364000+7 1.48714-109446 5 18 1820 1.369500+7 1.43223-10 1.375000+7 1.37934-10 1.380500+7 1.32838-109446 5 18 1821 1.386000+7 1.27929-10 1.391500+7 1.23199-10 1.397000+7 1.18643-109446 5 18 1822 1.402500+7 1.14254-10 1.408000+7 1.10026-10 1.413500+7 1.05953-109446 5 18 1823 1.419000+7 1.02029-10 1.424500+7 9.82496-11 1.430000+7 9.46089-119446 5 18 1824 1.435500+7 9.11021-11 1.441000+7 8.77241-11 1.446500+7 8.44703-119446 5 18 1825 1.452000+7 8.13362-11 1.457500+7 7.83175-11 1.463000+7 7.54099-119446 5 18 1826 1.468500+7 7.26093-11 1.474000+7 6.99119-11 1.479500+7 6.73139-119446 5 18 1827 1.485000+7 6.48117-11 1.490500+7 6.24018-11 1.496000+7 6.00807-119446 5 18 1828 1.501500+7 5.78453-11 1.507000+7 5.56925-11 1.512500+7 5.36191-119446 5 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1.25794-11 1.727000+7 1.21060-119446 5 18 1842 1.732500+7 1.16503-11 1.738000+7 1.12117-11 1.743500+7 1.07895-119446 5 18 1843 1.749000+7 1.03831-11 1.754500+7 9.99189-12 1.760000+7 9.61533-129446 5 18 1844 1.765500+7 9.25287-12 1.771000+7 8.90400-12 1.776500+7 8.56819-129446 5 18 1845 1.782000+7 8.24497-12 1.787500+7 7.93387-12 1.793000+7 7.63444-129446 5 18 1846 1.798500+7 7.34623-12 1.804000+7 7.06885-12 1.809500+7 6.80187-129446 5 18 1847 1.815000+7 6.54491-12 1.820500+7 6.29760-12 1.826000+7 6.05959-129446 5 18 1848 1.831500+7 5.83051-12 1.837000+7 5.61004-12 1.842500+7 5.39786-129446 5 18 1849 1.848000+7 5.19366-12 1.853500+7 4.99714-12 1.859000+7 4.80801-129446 5 18 1850 1.864500+7 4.62600-12 1.870000+7 4.45083-12 1.875500+7 4.28226-129446 5 18 1851 1.881000+7 4.12004-12 1.886500+7 3.96393-12 1.892000+7 3.81370-129446 5 18 1852 1.897500+7 3.66914-12 1.903000+7 3.53002-12 1.908500+7 3.39614-129446 5 18 1853 1.914000+7 3.26732-12 1.919500+7 3.14335-12 1.925000+7 3.02407-129446 5 18 1854 1.930500+7 2.90928-12 1.936000+7 2.79883-12 1.941500+7 2.69254-129446 5 18 1855 1.947000+7 2.59027-12 1.952500+7 2.49187-12 1.958000+7 2.39718-129446 5 18 1856 1.963500+7 2.30607-12 1.969000+7 2.21841-12 1.974500+7 2.13406-129446 5 18 1857 1.980000+7 2.05290-12 1.985500+7 1.97481-12 1.991000+7 1.89967-129446 5 18 1858 1.996500+7 1.82738-12 2.016500+7 0.000000+0 9446 5 18 1859 0.000000+0 6.000000+6 0 0 1 4829446 5 18 1860 482 2 9446 5 18 1861 0.000000+0 0.000000+0 1.000000-5 1.94464-12 1.200000-5 2.13025-129446 5 18 1862 1.400000-5 2.30093-12 1.600000-5 2.45980-12 1.800000-5 2.60901-129446 5 18 1863 2.200000-5 2.88437-12 2.500000-5 3.07475-12 2.900000-5 3.31161-129446 5 18 1864 3.400000-5 3.58574-12 4.000000-5 3.88929-12 4.600000-5 4.17080-129446 5 18 1865 5.400000-5 4.51895-12 6.300000-5 4.88102-12 7.400000-5 5.29001-129446 5 18 1866 8.600000-5 5.70283-12 1.000000-4 6.14952-12 1.200000-4 6.73647-129446 5 18 1867 1.400000-4 7.27623-12 1.600000-4 7.77862-12 1.800000-4 8.25048-129446 5 18 1868 2.200000-4 9.12126-12 2.500000-4 9.72330-12 2.900000-4 1.04723-119446 5 18 1869 3.400000-4 1.13392-11 4.000000-4 1.22992-11 4.600000-4 1.31894-119446 5 18 1870 5.400000-4 1.42904-11 6.300000-4 1.54354-11 7.400000-4 1.67288-119446 5 18 1871 8.600000-4 1.80343-11 1.000000-3 1.94469-11 1.200000-3 2.13030-119446 5 18 1872 1.400000-3 2.30100-11 1.600000-3 2.45988-11 1.800000-3 2.60910-119446 5 18 1873 2.200000-3 2.88448-11 2.500000-3 3.07487-11 2.900000-3 3.31175-119446 5 18 1874 3.400000-3 3.58591-11 4.000000-3 3.88949-11 4.600000-3 4.17103-119446 5 18 1875 5.400000-3 4.51922-11 6.300000-3 4.88134-11 7.400000-3 5.29038-119446 5 18 1876 8.600000-3 5.70326-11 1.000000-2 6.15002-11 1.200000-2 6.73706-119446 5 18 1877 1.400000-2 7.27692-11 1.600000-2 7.77941-11 1.800000-2 8.25137-119446 5 18 1878 2.200000-2 9.12234-11 2.500000-2 9.72454-11 2.900000-2 1.04738-109446 5 18 1879 3.400000-2 1.13409-10 4.000000-2 1.23011-10 4.600000-2 1.31917-109446 5 18 1880 5.400000-2 1.42930-10 6.300000-2 1.54385-10 7.400000-2 1.67324-109446 5 18 1881 8.600000-2 1.80385-10 1.000000-1 1.94518-10 1.200000-1 2.13090-109446 5 18 1882 1.400000-1 2.30169-10 1.600000-1 2.46067-10 1.800000-1 2.60999-109446 5 18 1883 2.200000-1 2.88557-10 2.500000-1 3.07611-10 2.900000-1 3.31318-109446 5 18 1884 3.400000-1 3.58760-10 4.000000-1 3.89147-10 4.600000-1 4.17330-109446 5 18 1885 5.400000-1 4.52189-10 6.300000-1 4.88446-10 7.400000-1 5.29405-109446 5 18 1886 8.600000-1 5.70752-10 1.000000+0 6.15498-10 1.200000+0 6.74302-109446 5 18 1887 1.400000+0 7.28387-10 1.600000+0 7.78735-10 1.800000+0 8.26031-109446 5 18 1888 2.200000+0 9.13328-10 2.500000+0 9.73696-10 2.900000+0 1.048820-99446 5 18 1889 3.400000+0 1.135780-9 4.000000+0 1.232100-9 4.600000+0 1.321460-99446 5 18 1890 5.400000+0 1.432000-9 6.300000+0 1.546990-9 7.400000+0 1.676940-99446 5 18 1891 8.600000+0 1.808140-9 1.000000+1 1.950180-9 1.200000+1 2.136900-99446 5 18 1892 1.400000+1 2.308700-9 1.600000+1 2.468680-9 1.800000+1 2.619010-99446 5 18 1893 2.200000+1 2.896600-9 2.500000+1 3.088660-9 2.900000+1 3.327760-99446 5 18 1894 3.400000+1 3.604690-9 4.000000+1 3.911600-9 4.600000+1 4.196480-99446 5 18 1895 5.400000+1 4.549130-9 6.300000+1 4.916270-9 7.400000+1 5.331450-99446 5 18 1896 8.600000+1 5.751040-9 1.000000+2 6.205640-9 1.200000+2 6.803890-99446 5 18 1897 1.400000+2 7.354970-9 1.600000+2 7.868690-9 1.800000+2 8.351900-99446 5 18 1898 2.200000+2 9.245390-9 2.500000+2 9.864490-9 2.900000+2 1.063630-89446 5 18 1899 3.400000+2 1.153170-8 4.000000+2 1.252580-8 4.600000+2 1.345030-89446 5 18 1900 5.400000+2 1.459700-8 6.300000+2 1.579350-8 7.400000+2 1.714980-89446 5 18 1901 8.600000+2 1.852400-8 1.000000+3 2.001680-8 1.200000+3 2.198750-89446 5 18 1902 1.400000+3 2.380900-8 1.600000+3 2.551240-8 1.800000+3 2.711910-89446 5 18 1903 2.200000+3 3.010190-8 2.500000+3 3.217740-8 2.900000+3 3.477470-89446 5 18 1904 3.400000+3 3.780170-8 4.000000+3 4.117920-8 4.600000+3 4.433560-89446 5 18 1905 5.400000+3 4.827120-8 6.300000+3 5.240120-8 7.400000+3 5.711150-89446 5 18 1906 8.600000+3 6.191360-8 1.000000+4 6.716350-8 1.200000+4 7.414530-89446 5 18 1907 1.400000+4 8.064810-8 1.600000+4 8.677050-8 1.800000+4 9.258130-89446 5 18 1908 2.200000+4 1.034550-7 2.500000+4 1.110850-7 2.900000+4 1.207030-79446 5 18 1909 3.400000+4 1.320020-7 4.000000+4 1.447200-7 4.600000+4 1.567010-79446 5 18 1910 5.400000+4 1.717600-7 6.000000+4 1.824870-7 1.200000+5 2.733300-79446 5 18 1911 1.800000+5 3.192190-7 2.400000+5 3.559870-7 3.000000+5 3.713790-79446 5 18 1912 3.600000+5 3.822990-7 4.200000+5 3.844190-7 4.800000+5 3.837330-79446 5 18 1913 5.400000+5 3.792380-7 6.000000+5 3.728280-7 6.600000+5 3.664020-79446 5 18 1914 7.200000+5 3.586100-7 7.800000+5 3.515850-7 8.400000+5 3.435540-79446 5 18 1915 9.000000+5 3.369610-7 9.600000+5 3.296140-7 1.020000+6 3.231600-79446 5 18 1916 1.080000+6 3.161320-7 1.140000+6 3.098030-7 1.200000+6 3.030720-79446 5 18 1917 1.260000+6 2.967620-7 1.320000+6 2.901780-7 1.380000+6 2.836790-79446 5 18 1918 1.440000+6 2.770050-7 1.500000+6 2.707410-7 1.560000+6 2.643770-79446 5 18 1919 1.620000+6 2.580810-7 1.680000+6 2.517420-7 1.740000+6 2.454630-79446 5 18 1920 1.800000+6 2.391860-7 1.860000+6 2.329720-7 1.920000+6 2.267930-79446 5 18 1921 1.980000+6 2.206880-7 2.040000+6 2.146430-7 2.100000+6 2.086820-79446 5 18 1922 2.160000+6 2.028010-7 2.220000+6 1.970130-7 2.280000+6 1.913190-79446 5 18 1923 2.340000+6 1.857260-7 2.400000+6 1.802370-7 2.460000+6 1.748560-79446 5 18 1924 2.520000+6 1.695850-7 2.580000+6 1.644260-7 2.640000+6 1.593800-79446 5 18 1925 2.700000+6 1.544500-7 2.760000+6 1.496350-7 2.820000+6 1.449370-79446 5 18 1926 2.880000+6 1.403540-7 2.940000+6 1.358860-7 3.000000+6 1.315340-79446 5 18 1927 3.060000+6 1.272960-7 3.120000+6 1.231710-7 3.180000+6 1.191580-79446 5 18 1928 3.240000+6 1.152550-7 3.300000+6 1.114610-7 3.360000+6 1.077750-79446 5 18 1929 3.420000+6 1.041940-7 3.480000+6 1.007170-7 3.540000+6 9.734180-89446 5 18 1930 3.600000+6 9.406640-8 3.660000+6 9.088870-8 3.720000+6 8.780680-89446 5 18 1931 3.780000+6 8.481860-8 3.840000+6 8.192190-8 3.900000+6 7.911470-89446 5 18 1932 3.960000+6 7.639470-8 4.020000+6 7.376000-8 4.080000+6 7.120830-89446 5 18 1933 4.140000+6 6.873760-8 4.200000+6 6.634570-8 4.260000+6 6.403070-89446 5 18 1934 4.320000+6 6.179040-8 4.380000+6 5.962270-8 4.440000+6 5.752580-89446 5 18 1935 4.500000+6 5.549770-8 4.560000+6 5.353630-8 4.620000+6 5.163980-89446 5 18 1936 4.680000+6 4.980630-8 4.740000+6 4.803400-8 4.800000+6 4.632110-89446 5 18 1937 4.860000+6 4.466580-8 4.920000+6 4.306630-8 4.980000+6 4.152110-89446 5 18 1938 5.040000+6 4.002830-8 5.100000+6 3.858650-8 5.160000+6 3.719410-89446 5 18 1939 5.220000+6 3.584940-8 5.280000+6 3.455110-8 5.340000+6 3.329760-89446 5 18 1940 5.400000+6 3.208750-8 5.460000+6 3.091940-8 5.520000+6 2.979210-89446 5 18 1941 5.580000+6 2.870410-8 5.640000+6 2.765420-8 5.700000+6 2.664120-89446 5 18 1942 5.760000+6 2.566380-8 5.820000+6 2.472090-8 5.880000+6 2.381140-89446 5 18 1943 5.940000+6 2.293400-8 6.000000+6 2.208780-8 6.060000+6 2.127180-89446 5 18 1944 6.120000+6 2.048480-8 6.180000+6 1.972600-8 6.240000+6 1.899430-89446 5 18 1945 6.300000+6 1.828890-8 6.360000+6 1.760880-8 6.420000+6 1.695320-89446 5 18 1946 6.480000+6 1.632130-8 6.540000+6 1.571220-8 6.600000+6 1.512520-89446 5 18 1947 6.660000+6 1.455940-8 6.720000+6 1.401420-8 6.780000+6 1.348890-89446 5 18 1948 6.840000+6 1.298270-8 6.900000+6 1.249490-8 6.960000+6 1.202500-89446 5 18 1949 7.020000+6 1.157230-8 7.080000+6 1.113620-8 7.140000+6 1.071610-89446 5 18 1950 7.200000+6 1.031150-8 7.260000+6 9.921730-9 7.320000+6 9.546360-99446 5 18 1951 7.380000+6 9.184840-9 7.440000+6 8.836690-9 7.500000+6 8.501430-99446 5 18 1952 7.560000+6 8.178590-9 7.620000+6 7.867740-9 7.680000+6 7.568430-99446 5 18 1953 7.740000+6 7.280260-9 7.800000+6 7.002820-9 7.860000+6 6.735730-99446 5 18 1954 7.920000+6 6.478610-9 7.980000+6 6.231100-9 8.040000+6 5.992850-99446 5 18 1955 8.100000+6 5.763530-9 8.160000+6 5.542800-9 8.220000+6 5.330370-99446 5 18 1956 8.280000+6 5.125910-9 8.340000+6 4.929140-9 8.400000+6 4.739790-99446 5 18 1957 8.460000+6 4.557570-9 8.520000+6 4.382220-9 8.580000+6 4.213500-99446 5 18 1958 8.640000+6 4.051160-9 8.700000+6 3.894960-9 8.760000+6 3.744670-99446 5 18 1959 8.820000+6 3.600090-9 8.880000+6 3.460990-9 8.940000+6 3.327170-99446 5 18 1960 9.000000+6 3.198440-9 9.060000+6 3.074600-9 9.120000+6 2.955480-99446 5 18 1961 9.180000+6 2.840910-9 9.240000+6 2.730700-9 9.300000+6 2.624700-99446 5 18 1962 9.360000+6 2.522740-9 9.420000+6 2.424690-9 9.480000+6 2.330390-99446 5 18 1963 9.540000+6 2.239700-9 9.600000+6 2.152490-9 9.660000+6 2.068620-99446 5 18 1964 9.720000+6 1.987970-9 9.780000+6 1.910420-9 9.840000+6 1.835850-99446 5 18 1965 9.900000+6 1.764150-9 9.960000+6 1.695210-9 1.002000+7 1.628920-99446 5 18 1966 1.008000+7 1.565190-9 1.014000+7 1.503920-9 1.020000+7 1.445020-99446 5 18 1967 1.026000+7 1.388390-9 1.032000+7 1.333950-9 1.038000+7 1.281620-99446 5 18 1968 1.044000+7 1.231310-9 1.050000+7 1.182950-9 1.056000+7 1.136470-99446 5 18 1969 1.062000+7 1.091790-9 1.068000+7 1.048850-9 1.074000+7 1.007570-99446 5 18 1970 1.080000+7 9.67895-10 1.086000+7 9.29764-10 1.092000+7 8.93118-109446 5 18 1971 1.098000+7 8.57898-10 1.104000+7 8.24050-10 1.110000+7 7.91522-109446 5 18 1972 1.116000+7 7.60262-10 1.122000+7 7.30223-10 1.128000+7 7.01357-109446 5 18 1973 1.134000+7 6.73619-10 1.140000+7 6.46965-10 1.146000+7 6.21354-109446 5 18 1974 1.152000+7 5.96745-10 1.158000+7 5.73100-10 1.164000+7 5.50382-109446 5 18 1975 1.170000+7 5.28554-10 1.176000+7 5.07583-10 1.182000+7 4.87434-109446 5 18 1976 1.188000+7 4.68077-10 1.194000+7 4.49481-10 1.200000+7 4.31615-109446 5 18 1977 1.206000+7 4.14452-10 1.212000+7 3.97965-10 1.218000+7 3.82127-109446 5 18 1978 1.224000+7 3.66912-10 1.230000+7 3.52297-10 1.236000+7 3.38259-109446 5 18 1979 1.242000+7 3.24774-10 1.248000+7 3.11822-10 1.254000+7 2.99381-109446 5 18 1980 1.260000+7 2.87431-10 1.266000+7 2.75954-10 1.272000+7 2.64931-109446 5 18 1981 1.278000+7 2.54344-10 1.284000+7 2.44176-10 1.290000+7 2.34410-109446 5 18 1982 1.296000+7 2.25032-10 1.302000+7 2.16025-10 1.308000+7 2.07375-109446 5 18 1983 1.314000+7 1.99069-10 1.320000+7 1.91092-10 1.326000+7 1.83432-109446 5 18 1984 1.332000+7 1.76076-10 1.338000+7 1.69013-10 1.344000+7 1.62230-109446 5 18 1985 1.350000+7 1.55718-10 1.356000+7 1.49464-10 1.362000+7 1.43460-109446 5 18 1986 1.368000+7 1.37694-10 1.374000+7 1.32158-10 1.380000+7 1.26843-109446 5 18 1987 1.386000+7 1.21740-10 1.392000+7 1.16841-10 1.398000+7 1.12137-109446 5 18 1988 1.404000+7 1.07620-10 1.410000+7 1.03285-10 1.416000+7 9.91220-119446 5 18 1989 1.422000+7 9.51259-11 1.428000+7 9.12895-11 1.434000+7 8.76067-119446 5 18 1990 1.440000+7 8.40712-11 1.446000+7 8.06772-11 1.452000+7 7.74192-119446 5 18 1991 1.458000+7 7.42918-11 1.464000+7 7.12897-11 1.470000+7 6.84079-119446 5 18 1992 1.476000+7 6.56418-11 1.482000+7 6.29866-11 1.488000+7 6.04381-119446 5 18 1993 1.494000+7 5.79919-11 1.500000+7 5.56439-11 1.506000+7 5.33903-119446 5 18 1994 1.512000+7 5.12273-11 1.518000+7 4.91513-11 1.524000+7 4.71588-119446 5 18 1995 1.530000+7 4.52464-11 1.536000+7 4.34111-11 1.542000+7 4.16497-119446 5 18 1996 1.548000+7 3.99592-11 1.554000+7 3.83369-11 1.560000+7 3.67799-119446 5 18 1997 1.566000+7 3.52857-11 1.572000+7 3.38519-11 1.578000+7 3.24758-119446 5 18 1998 1.584000+7 3.11554-11 1.590000+7 2.98882-11 1.596000+7 2.86722-119446 5 18 1999 1.602000+7 2.75054-11 1.608000+7 2.63857-11 1.614000+7 2.53113-119446 5 18 2000 1.620000+7 2.42804-11 1.626000+7 2.32911-11 1.632000+7 2.23419-119446 5 18 2001 1.638000+7 2.14312-11 1.644000+7 2.05573-11 1.650000+7 1.97188-119446 5 18 2002 1.656000+7 1.89143-11 1.662000+7 1.81424-11 1.668000+7 1.74018-119446 5 18 2003 1.674000+7 1.66912-11 1.680000+7 1.60095-11 1.686000+7 1.53554-119446 5 18 2004 1.692000+7 1.47279-11 1.698000+7 1.41259-11 1.704000+7 1.35483-119446 5 18 2005 1.710000+7 1.29942-11 1.716000+7 1.24626-11 1.722000+7 1.19527-119446 5 18 2006 1.728000+7 1.14634-11 1.734000+7 1.09941-11 1.740000+7 1.05439-119446 5 18 2007 1.746000+7 1.01120-11 1.752000+7 9.69769-12 1.758000+7 9.30025-129446 5 18 2008 1.764000+7 8.91900-12 1.770000+7 8.55329-12 1.776000+7 8.20249-129446 5 18 2009 1.782000+7 7.86599-12 1.788000+7 7.54321-12 1.794000+7 7.23361-129446 5 18 2010 1.800000+7 6.93663-12 1.806000+7 6.65178-12 1.812000+7 6.37856-129446 5 18 2011 1.818000+7 6.11650-12 1.824000+7 5.86515-12 1.830000+7 5.62406-129446 5 18 2012 1.836000+7 5.39283-12 1.842000+7 5.17106-12 1.848000+7 4.95835-129446 5 18 2013 1.854000+7 4.75435-12 1.860000+7 4.55869-12 1.866000+7 4.37104-129446 5 18 2014 1.872000+7 4.19107-12 1.878000+7 4.01848-12 1.884000+7 3.85295-129446 5 18 2015 1.890000+7 3.69420-12 1.896000+7 3.54196-12 1.902000+7 3.39596-129446 5 18 2016 1.908000+7 3.25595-12 1.914000+7 3.12168-12 1.920000+7 2.99291-129446 5 18 2017 1.926000+7 2.86943-12 1.932000+7 2.75102-12 1.938000+7 2.63747-129446 5 18 2018 1.944000+7 2.52858-12 1.950000+7 2.42417-12 1.956000+7 2.32404-129446 5 18 2019 1.962000+7 2.22803-12 1.968000+7 2.13596-12 1.974000+7 2.04768-129446 5 18 2020 1.980000+7 1.96303-12 1.986000+7 1.88187-12 1.992000+7 1.80404-129446 5 18 2021 1.998000+7 1.72941-12 2.018000+7 0.000000+0 9446 5 18 2022 0.000000+0 6.500000+6 0 0 1 4579446 5 18 2023 457 2 9446 5 18 2024 0.000000+0 0.000000+0 1.000000-5 1.86744-12 1.200000-5 2.04568-129446 5 18 2025 1.400000-5 2.20958-12 1.600000-5 2.36215-12 1.800000-5 2.50544-129446 5 18 2026 2.200000-5 2.76986-12 2.500000-5 2.95269-12 2.900000-5 3.18014-129446 5 18 2027 3.400000-5 3.44340-12 4.000000-5 3.73489-12 4.600000-5 4.00522-129446 5 18 2028 5.400000-5 4.33955-12 6.300000-5 4.68726-12 7.400000-5 5.08001-129446 5 18 2029 8.600000-5 5.47644-12 1.000000-4 5.90540-12 1.200000-4 6.46905-129446 5 18 2030 1.400000-4 6.98737-12 1.600000-4 7.46982-12 1.800000-4 7.92295-129446 5 18 2031 2.200000-4 8.75916-12 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