JENDL-5 (Neutron sublibrary (up to 20 MeV)) Cm-248 0 0 0 0 9.624800+4 2.459410+2 1 1 6 19649 1451 1 0.000000+0 1.000000+0 0 0 0 69649 1451 2 1.000000+0 2.000000+7 0 0 10 59649 1451 3 0.000000+0 0.000000+0 3 0 440 929649 1451 4 96-Cm-248 JAEA+ EVAL-JAN10 O.Iwamoto,T.Nakagawa,T.Ohsawa+ 9649 1451 5 DIST-DEC21 20100319 9649 1451 6 ----JENDL-5 MATERIAL 9649 9649 1451 7 -----INCIDENT NEUTRON DATA 9649 1451 8 ------ENDF-6 FORMAT 9649 1451 9 9649 1451 10 History 9649 1451 11 06-01 Fission cross section was evaluated with GMA code. 9649 1451 12 06-05 Resolved resonance parameters were modified. 9649 1451 13 07-03 Fission spectra were evaluated. 9649 1451 14 07-05 New calculation was made with CCONE code. 9649 1451 15 08-03 Interpolation of (5,18) was changed. 9649 1451 16 Recalculation with CCONE code was performed. 9649 1451 17 Data were compiled as JENDL/AC-2008/1/. 9649 1451 18 09-08 (MF1,MT458) was evaluated. 9649 1451 19 10-01 Data of prompt gamma rays due to fission were given. 9649 1451 20 10-03 Covariance data were given. 9649 1451 21 21-08 QI of MT57 was slightly shifted to avoid duplication with 9649 1451 22 MT56 by S. Nakayama. 9649 1451 23 9649 1451 24 21-11 revised by O.Iwamoto 9649 1451 25 (MF3/MT19-21,38) deleted 9649 1451 26 (MF8/MT16-18,37,102) JENDL/AD-2017 adopted 9649 1451 27 (MF8/MT4) added 9649 1451 28 9649 1451 29 MF= 1 General information 9649 1451 30 MT=452 Number of Neutrons per fission 9649 1451 31 Sum of MT's=455 and 456. 9649 1451 32 9649 1451 33 MT=455 Delayed neutron data 9649 1451 34 (same as JENDL-3.3) 9649 1451 35 Semi-empirical formula by Tuttle/2/. 9649 1451 36 9649 1451 37 MT=456 Number of prompt neutrons per fission 9649 1451 38 (same as JENDL-3.3) 9649 1451 39 At the 0 eV, the experimental data of Zhuravlev et al./3/ 9649 1451 40 was adopted. An energy-dependent term was based on the semi- 9649 1451 41 empirical formula by Howerton/4/. 9649 1451 42 9649 1451 43 MT=458 Components of energy release due to fission 9649 1451 44 Total energy and prompt energy were calculated from mass 9649 1451 45 balance using JENDL-4 fission yields data and mass excess 9649 1451 46 evaluation. Mass excess values were from Audi's 2009 9649 1451 47 evaluation/5/. Delayed energy values were calculated from 9649 1451 48 the energy release for infinite irradiation using JENDL FP 9649 1451 49 Decay Data File 2000 and JENDL-4 yields data. For delayed 9649 1451 50 neutron energy, as the JENDL FP Decay Data File 2000/6/ does 9649 1451 51 not include average neutron energy values, the average values 9649 1451 52 were calculated using the formula shown in the report by 9649 1451 53 T.R. England/7/. The fractions of prompt energy were 9649 1451 54 calculated using the fractions of Sher's evaluation/8/ when 9649 1451 55 they were provided. When the fractions were not given by Sher,9649 1451 56 averaged fractions were used. 9649 1451 57 9649 1451 58 9649 1451 59 MF= 2 Resonance parameters 9649 1451 60 MT=151 9649 1451 61 Resolved resonance parameters (MLBW: 1.0E-5 - 1500 eV) 9649 1451 62 Resonance parameters for JENDL-3.3 were evaluated on the basis9649 1451 63 of the data of Benjamin et al./9/, Moore and Keyworth/10/ 9649 1451 64 and Maguire et al./11/. Comment for JENDL-3.3 is as follows: 9649 1451 65 9649 1451 66 * RESONANCE ENERGIES, NEUTRON AND RADIATIVE WIDTHS WERE 9649 1451 67 TAKEN FROM THE EXPERIMENTAL DATA OF BENJAMIN ET AL./9/. 9649 1451 68 FOR RESONANCES WHOSE RADIATIVE WIDTH WAS UNKNOWN, THE 9649 1451 69 AVERAGE VALUE OF 0.026 EV/9/ WAS ADOPTED. THE FISSION 9649 1451 70 WIDTHS were adopted from Moore and Keyworth /10/ and 9649 1451 71 Maguire et al./11/ THE AVERAGE FISSION WIDTH OF 0.0013 9649 1451 72 EV/10/ WAS USED FOR ALL RESONANCES OF WHICH FISSION 9649 1451 73 WIDTH HAD NOT BEEN MEASURED. Then the fission widths were 9649 1451 74 roughly adjusted to the fission cross section measured by 9649 1451 75 Maguire et al. R=9.1 FM WAS ASSUMED TO REPRODUCE THE 9649 1451 76 POTENTIAL SCATTERING CROSS SECTION OF 10.4 BARNS ASSUMED 9649 1451 77 BY BENJAMIN ET AL./9/. THE NEUTRON WIDTH OF THE FIRST 9649 1451 78 RESONANCE WAS SLIGHTLY ADJUSTED TO REPRODUCE THE CAPTURE 9649 1451 79 CROSS SECTION OF 2.57 BARNS AT 0.0253 EV. BACKGROUND 9649 1451 80 CROSS SECTIONS WERE GIVEN ONLY FOR THE FISSION AND TOTAL 9649 1451 81 CROSS SECTIONS BY ASSUMING THE FORM OF 1/V. THE THERMAL 9649 1451 82 CROSS SECTIONS TO BE REPRODUCED WERE ESTIMATED FROM 9649 1451 83 AVAILABLE EXPERIMENTAL DATA. 9649 1451 84 9649 1451 85 For the present file, a negative resonance was added at -30 eV9649 1451 86 to reproduce the thermal cross sections, and background cross 9649 1451 87 sections were removed. 9649 1451 88 9649 1451 89 The thermal cross sections to be reproduced: 9649 1451 90 Fission = 0.337 +- 0.032 b 9649 1451 91 Benjamin et al./12/, Zhuravlev et al./13/, 9649 1451 92 Serot et al./14/ 9649 1451 93 Capture = 2.87 +- 0.26 b 9649 1451 94 Druschel et al./15/, Gavrilov et al./16/ 9649 1451 95 9649 1451 96 Unresolved resonance parameters (1.5 - 200 keV) 9649 1451 97 Parameters were determined with ASREP code/17/ so as to 9649 1451 98 reproduce the cross sections. They are used only for self- 9649 1451 99 shielding calculations. 9649 1451 100 9649 1451 101 Thermal cross sections and resonance integrals (at 300K) 9649 1451 102 ------------------------------------------------------- 9649 1451 103 0.0253 eV reson. integ.(*) 9649 1451 104 (barns) (barns) 9649 1451 105 ------------------------------------------------------- 9649 1451 106 total 10.198 9649 1451 107 elastic 6.989 9649 1451 108 fission 0.337 7.84 9649 1451 109 capture 2.872 267 9649 1451 110 ------------------------------------------------------- 9649 1451 111 (*) In the energy range from 0.5 eV to 10 MeV. 9649 1451 112 9649 1451 113 9649 1451 114 MF= 3 Neutron cross sections 9649 1451 115 Cross sections above the resolved resonance region except for 9649 1451 116 the elastic scattering (MT=2) and fission cross sections (MT=18,9649 1451 117 19, 20, 21, 38) were calculated with CCONE code/18/. 9649 1451 118 9649 1451 119 MT= 1 Total cross section 9649 1451 120 The cross section was calculated with CC OMP of Soukhovitskii 9649 1451 121 et al./19/ 9649 1451 122 9649 1451 123 MT= 2 Elastic scattering cross section 9649 1451 124 Calculated as total - non-elastic scattering cross sections. 9649 1451 125 9649 1451 126 MT=18 Fission cross section 9649 1451 127 The following experimental data were analyzed in the energy 9649 1451 128 range from 1.5 keV to 7 MeV with the GMA code/20/: 9649 1451 129 9649 1451 130 Authors Energy range Data points Reference 9649 1451 131 Moore+ 1.4 keV - 2.8 MeV 413 /10/ 9649 1451 132 Fomushkin+ 0.3 - 5.5 MeV 20 /21/ 9649 1451 133 Maguire+ 1.4 keV - 80 keV 44 /11/ 9649 1451 134 Fomushkin+ 14.1MeV 1 /22/ 9649 1451 135 Fursov+ 510 keV - 6.8 MeV 37 /23/*1) 9649 1451 136 *1) Ratio to Pu-239 fission, converted to cross section 9649 1451 137 by using JENDL-3.3 data. 9649 1451 138 9649 1451 139 The results of GMA were used to determine the parameters in 9649 1451 140 the CCONE calculation. 9649 1451 141 9649 1451 142 Above 8 MeV, JENDL-3.3 was adopted. 9649 1451 143 9649 1451 144 MT=19, 20, 21, 38 Multi-chance fission cross sections 9649 1451 145 Calculated with CCONE code, and renormalized to the total 9649 1451 146 fission cross section (MT=18). 9649 1451 147 9649 1451 148 9649 1451 149 MF= 4 Angular distributions of secondary neutrons 9649 1451 150 MT=2 Elastic scattering 9649 1451 151 Calculated with CCONE code. 9649 1451 152 9649 1451 153 MT=18 Fission 9649 1451 154 Isotropic distributions in the laboratory system were assumed.9649 1451 155 9649 1451 156 9649 1451 157 MF= 5 Energy distributions of secondary neutrons 9649 1451 158 MT=18 Fission neutron spectra 9649 1451 159 Below 6 MeV, calculated by Ohsawa /24/ with modified 9649 1451 160 Madland-Nix formula considering multi-mode fission processes 9649 1451 161 (standard-1, standard-2, superlong). 9649 1451 162 Above 7 MeV, calculated with CCONE code. 9649 1451 163 9649 1451 164 9649 1451 165 MF= 6 Energy-angle distributions 9649 1451 166 Calculated with CCONE code. 9649 1451 167 Distributions from fission (MT=18) are not included. 9649 1451 168 9649 1451 169 9649 1451 170 MF=12 Photon production multiplicities 9649 1451 171 MT=18 Fission 9649 1451 172 Calculated from the total energy released by the prompt 9649 1451 173 gamma-rays due to fission given in MF=1/MT=458 and the 9649 1451 174 average energy of gamma-rays. 9649 1451 175 9649 1451 176 9649 1451 177 MF=14 Photon angular distributions 9649 1451 178 MT=18 Fission 9649 1451 179 Isotoropic distributions were assumed. 9649 1451 180 9649 1451 181 9649 1451 182 MF=15 Continuous photon energy spectra 9649 1451 183 MT=18 Fission 9649 1451 184 Experimental data measured by Verbinski et al./25/ for 9649 1451 185 Pu-239 thermal fission were adopted. 9649 1451 186 9649 1451 187 9649 1451 188 MF=31 Covariances of average number of neutrons per fission 9649 1451 189 MT=452 Number of neutrons per fission 9649 1451 190 Sum of covariances for MT=455 and MT=456. 9649 1451 191 9649 1451 192 MT=455 9649 1451 193 Error of 15% was assumed. 9649 1451 194 9649 1451 195 MT=456 9649 1451 196 Covariance was obtained by fitting a linear function to the 9649 1451 197 data at 0.0 and 5.0 MeV with an uncertainty of 4% and 5%, 9649 1451 198 respevtively. The uncertainty at 0 eV was estimated from the 9649 1451 199 experimental data of Zhuravlev et al./3/ 9649 1451 200 9649 1451 201 9649 1451 202 MF=32 Covariances of resonance parameters 9649 1451 203 MT=151 Resolved resonance parameterss 9649 1451 204 Format of LCOMP=0 was adopted. 9649 1451 205 9649 1451 206 Uncertainties of parameters were taken from Mughabghab /26/. 9649 1451 207 For the parameters without any information on uncertainty, 9649 1451 208 the following uncertainties were assumed: 9649 1451 209 Resonance energy 0.1 % 9649 1451 210 Neutron width 10 % 9649 1451 211 Capture width 20 % 9649 1451 212 Fission width 10 % 9649 1451 213 9649 1451 214 9649 1451 215 MF=33 Covariances of neutron cross sections 9649 1451 216 Covariances were given to all the cross sections by using 9649 1451 217 KALMAN code/27/ and the covariances of model parameters 9649 1451 218 used in the cross-section calculations. 9649 1451 219 9649 1451 220 For the fission cross section, covariances obtained with the 9649 1451 221 GMA analysis were adopted. Standard deviations (SD) were 9649 1451 222 multiplied by a factor of 2. SD of 10% were assumed in the 9649 1451 223 energy region above 8 MeV. 9649 1451 224 9649 1451 225 In the resolved resonance region, the following standard 9649 1451 226 deviations were added to the contributions from resonance 9649 1451 227 parameters: 9649 1451 228 Total 10 - 20 % 9649 1451 229 Elastic scattering 10 - 20 % 9649 1451 230 9649 1451 231 9649 1451 232 MF=34 Covariances for Angular Distributions 9649 1451 233 MT=2 Elastic scattering 9649 1451 234 Covariances were given only to P1 components. 9649 1451 235 9649 1451 236 9649 1451 237 MF=35 Covariances for Energy Distributions 9649 1451 238 MT=18 Fission spectra 9649 1451 239 Below 6 MeV, covarinaces of Pu239 fission spectra given in 9649 1451 240 JENDL-3.3 were adopted after multiplying a factor of 9. 9649 1451 241 Above 6 MeV, estimated with CCONE and KALMAN codes. 9649 1451 242 9649 1451 243 9649 1451 244 ***************************************************************** 9649 1451 245 Calculation with CCONE code 9649 1451 246 ***************************************************************** 9649 1451 247 9649 1451 248 Models and parameters used in the CCONE/18/ calculation 9649 1451 249 1) Coupled channel optical model 9649 1451 250 Levels in the rotational band were included. Optical model 9649 1451 251 potential and coupled levels are shown in Table 1. 9649 1451 252 9649 1451 253 2) Two-component exciton model/28/ 9649 1451 254 * Global parametrization of Koning-Duijvestijn/29/ 9649 1451 255 was used. 9649 1451 256 * Gamma emission channel/30/ was added to simulate direct 9649 1451 257 and semi-direct capture reaction. 9649 1451 258 9649 1451 259 3) Hauser-Feshbach statistical model 9649 1451 260 * Moldauer width fluctuation correction/31/ was included. 9649 1451 261 * Neutron, gamma and fission decay channel were included. 9649 1451 262 * Transmission coefficients of neutrons were taken from 9649 1451 263 coupled channel calculation in Table 1. 9649 1451 264 * The level scheme of the target is shown in Table 2. 9649 1451 265 * Level density formula of constant temperature and Fermi-gas 9649 1451 266 model were used with shell energy correction and collective 9649 1451 267 enhancement factor. Parameters are shown in Table 3. 9649 1451 268 * Fission channel: 9649 1451 269 Double humped fission barriers were assumed. 9649 1451 270 Fission barrier penetrabilities were calculated with 9649 1451 271 Hill-Wheler formula/32/. Fission barrier parameters were 9649 1451 272 shown in Table 4. Transition state model was used and 9649 1451 273 continuum levels are assumed above the saddles. The level 9649 1451 274 density parameters for inner and outer saddles are shown in 9649 1451 275 Tables 5 and 6, respectively. 9649 1451 276 * Gamma-ray strength function of Kopecky et al/33/,/34/ 9649 1451 277 was used. The prameters are shown in Table 7. 9649 1451 278 9649 1451 279 9649 1451 280 ------------------------------------------------------------------9649 1451 281 Tables 9649 1451 282 ------------------------------------------------------------------9649 1451 283 9649 1451 284 Table 1. Coupled channel calculation 9649 1451 285 -------------------------------------------------- 9649 1451 286 * rigid rotor model was applied 9649 1451 287 * coupled levels = 0,1,2,3,4 (see Table 2) 9649 1451 288 * optical potential parameters /19/ 9649 1451 289 Volume: 9649 1451 290 V_0 = 49.97 MeV 9649 1451 291 lambda_HF = 0.01004 1/MeV 9649 1451 292 C_viso = 15.9 MeV 9649 1451 293 A_v = 12.04 MeV 9649 1451 294 B_v = 81.36 MeV 9649 1451 295 E_a = 385 MeV 9649 1451 296 r_v = 1.2568 fm 9649 1451 297 a_v = 0.633 fm 9649 1451 298 Surface: 9649 1451 299 W_0 = 17.2 MeV 9649 1451 300 B_s = 11.19 MeV 9649 1451 301 C_s = 0.01361 1/MeV 9649 1451 302 C_wiso = 23.5 MeV 9649 1451 303 r_s = 1.1803 fm 9649 1451 304 a_s = 0.601 fm 9649 1451 305 Spin-orbit: 9649 1451 306 V_so = 5.75 MeV 9649 1451 307 lambda_so = 0.005 1/MeV 9649 1451 308 W_so = -3.1 MeV 9649 1451 309 B_so = 160 MeV 9649 1451 310 r_so = 1.1214 fm 9649 1451 311 a_so = 0.59 fm 9649 1451 312 Coulomb: 9649 1451 313 C_coul = 1.3 9649 1451 314 r_c = 1.2452 fm 9649 1451 315 a_c = 0.545 fm 9649 1451 316 Deformation: 9649 1451 317 beta_2 = 0.213 9649 1451 318 beta_4 = 0.066 9649 1451 319 beta_6 = 0.0015 9649 1451 320 9649 1451 321 * Calculated strength function 9649 1451 322 S0= 1.21e-4 S1= 3.23e-4 R'= 9.08 fm (En=1 keV) 9649 1451 323 -------------------------------------------------- 9649 1451 324 9649 1451 325 Table 2. Level Scheme of Cm-248 9649 1451 326 ------------------- 9649 1451 327 No. Ex(MeV) J PI 9649 1451 328 ------------------- 9649 1451 329 0 0.00000 0 + * 9649 1451 330 1 0.04340 2 + * 9649 1451 331 2 0.14360 4 + * 9649 1451 332 3 0.29810 6 + * 9649 1451 333 4 0.50500 8 + * 9649 1451 334 5 0.76070 10 + 9649 1451 335 6 1.04900 2 + 9649 1451 336 7 1.04900 1 - 9649 1451 337 8 1.06130 12 + 9649 1451 338 9 1.08400 0 + 9649 1451 339 10 1.09400 3 - 9649 1451 340 11 1.12600 2 + 9649 1451 341 12 1.14300 4 + 9649 1451 342 13 1.17200 5 - 9649 1451 343 14 1.22200 4 + 9649 1451 344 15 1.23500 3 - 9649 1451 345 ------------------- 9649 1451 346 *) Coupled levels in CC calculation 9649 1451 347 9649 1451 348 Table 3. Level density parameters 9649 1451 349 -------------------------------------------------------- 9649 1451 350 Nuclide a* Pair Eshell T E0 Ematch 9649 1451 351 1/MeV MeV MeV MeV MeV MeV 9649 1451 352 -------------------------------------------------------- 9649 1451 353 Cm-249 19.0966 0.7605 2.3053 0.3737 -0.8387 2.9359 9649 1451 354 Cm-248 18.5357 1.5240 2.0504 0.3482 0.2818 3.2555 9649 1451 355 Cm-247 18.3955 0.7635 1.7794 0.3734 -0.6804 2.7533 9649 1451 356 Cm-246 18.8984 1.5302 1.7310 0.3608 0.1621 3.4286 9649 1451 357 Cm-245 18.8322 0.7667 1.4601 0.3623 -0.5771 2.6382 9649 1451 358 -------------------------------------------------------- 9649 1451 359 9649 1451 360 Table 4. Fission barrier parameters 9649 1451 361 ---------------------------------------- 9649 1451 362 Nuclide V_A hw_A V_B hw_B 9649 1451 363 MeV MeV MeV MeV 9649 1451 364 ---------------------------------------- 9649 1451 365 Cm-249 5.500 0.750 5.100 0.430 9649 1451 366 Cm-248 6.100 1.040 4.950 0.600 9649 1451 367 Cm-247 5.400 0.800 5.650 0.650 9649 1451 368 Cm-246 6.300 1.040 5.100 0.600 9649 1451 369 Cm-245 6.050 0.500 5.700 0.420 9649 1451 370 ---------------------------------------- 9649 1451 371 9649 1451 372 Table 5. Level density above inner saddle 9649 1451 373 -------------------------------------------------------- 9649 1451 374 Nuclide a* Pair Eshell T E0 Ematch 9649 1451 375 1/MeV MeV MeV MeV MeV MeV 9649 1451 376 -------------------------------------------------------- 9649 1451 377 Cm-249 21.0062 0.8872 2.6000 0.3388 -1.7502 3.0872 9649 1451 378 Cm-248 20.9336 1.5000 2.6000 0.3323 -1.0300 3.6000 9649 1451 379 Cm-247 20.8609 0.8908 2.6000 0.3256 -1.5320 2.8908 9649 1451 380 Cm-246 20.7882 1.6500 2.6000 0.3263 -0.7728 3.6500 9649 1451 381 Cm-245 20.7155 0.8944 2.6000 0.3342 -1.6357 2.9944 9649 1451 382 -------------------------------------------------------- 9649 1451 383 9649 1451 384 Table 6. Level density above outer saddle 9649 1451 385 -------------------------------------------------------- 9649 1451 386 Nuclide a* Pair Eshell T E0 Ematch 9649 1451 387 1/MeV MeV MeV MeV MeV MeV 9649 1451 388 -------------------------------------------------------- 9649 1451 389 Cm-249 19.0966 0.8872 0.9000 0.3432 -0.5123 2.4872 9649 1451 390 Cm-248 20.9336 1.7780 0.8600 0.3706 -0.1043 3.9780 9649 1451 391 Cm-247 20.8609 0.8908 0.8200 0.3573 -0.8210 2.8908 9649 1451 392 Cm-246 20.7882 1.7852 0.7800 0.3658 -0.0107 3.8852 9649 1451 393 Cm-245 20.7155 0.8944 0.7400 0.3596 -0.8163 2.8944 9649 1451 394 -------------------------------------------------------- 9649 1451 395 9649 1451 396 Table 7. Gamma-ray strength function for Cm-249 9649 1451 397 -------------------------------------------------------- 9649 1451 398 * E1: ER = 11.38 (MeV) EG = 2.71 (MeV) SIG = 332.90 (mb) 9649 1451 399 ER = 14.28 (MeV) EG = 4.18 (MeV) SIG = 431.66 (mb) 9649 1451 400 * M1: ER = 6.52 (MeV) EG = 4.00 (MeV) SIG = 1.49 (mb) 9649 1451 401 * E2: ER = 10.01 (MeV) EG = 3.12 (MeV) SIG = 7.06 (mb) 9649 1451 402 -------------------------------------------------------- 9649 1451 403 9649 1451 404 9649 1451 405 References 9649 1451 406 1) O.Iwamoto et al.: J. Nucl. Sci. Technol., 46, 510 (2009). 9649 1451 407 2) R.J.Tuttle: INDC(NDS)-107/G+Special, p.29 (1979). 9649 1451 408 3) K.D.Zhuravlev et al.: 1973 Kiev, vol. 4, p.57 (1973). 9649 1451 409 4) R.J.Howerton: Nucl. Sci. Eng., 62, 438 (1977). 9649 1451 410 5) G.Audi: Private communication (April 2009). 9649 1451 411 6) J.Katakura et al.: JAERI 1343 (2001). 9649 1451 412 7) T.R.England et al.: LA-11151-MS (1988). 9649 1451 413 8) R.Sher, C.Beck: EPRI NP-1771 (1981). 9649 1451 414 9) R.W.Benjamin et al.: Nucl. Sci. Eng., 55, 440 (1974). 9649 1451 415 10) M.S.Moore, G.A.Keyworth: Phys. Rev., C3, 1656 (1971). 9649 1451 416 11) H.T.Maguire, Jr. et al.: Nucl. Sci. Eng., 89, 293 (1985). 9649 1451 417 12) R.W.Benjamin et al.: Nucl. Sci. Eng., 47, 203 (1972). 9649 1451 418 13) K.D.Zhuravlev et al.: Sov. At. Energy, 39, 907 (1975). 9649 1451 419 14) O.Serot et al.: 2005 Cadarache, p.182 (2005). 9649 1451 420 15) R.E.Druscell et al.: ORNL-4891, p.23 (1973). 9649 1451 421 16) V.D.Gavrilov, V.A.Goncharov: Sov. At. Energy, 44, 274 (1978). 9649 1451 422 17) Y.Kikuchi et al.: JAERI-Data/Code 99-025 (1999) in Japanese. 9649 1451 423 18) O.Iwamoto: J. Nucl. Sci. Technol., 44, 687 (2007). 9649 1451 424 19) E.Sh.Soukhovitskii et al.: Phys. Rev. C72, 024604 (2005). 9649 1451 425 20) W.P.Poenitz: BNL-NCS-51363, Vol.I, p.249 (1981). 9649 1451 426 S.Chiba, D.L.Smith: ANL/NDM-121 (1991). 9649 1451 427 21) E.F.Fomushkin et al.: 1980 Kiev, Vol.3, p.25 (1980). 9649 1451 428 22) E.F.Fomushkin et al.: 1991 Juelich, p.439 (1991). 9649 1451 429 23) B.I.Fursov et al.: 1997 Trieste, Vol.1, p.488 (1997). 9649 1451 430 24) T.Ohsawa: Private communication (2007). 9649 1451 431 25) V.V.Verbinski et al.: Phys. Rev., C7, 1173 (1973). 9649 1451 432 26) S.F.Mughabghab: "Atlas of Neutron Resonances," Elsevier 9649 1451 433 (2006). 9649 1451 434 27) T.Kawano, K.Shibata, JAERI-Data/Code 97-037 (1997) in 9649 1451 435 Japanese. 9649 1451 436 28) C.Kalbach: Phys. Rev. C33, 818 (1986). 9649 1451 437 29) A.J.Koning, M.C.Duijvestijn: Nucl. Phys. A744, 15 (2004). 9649 1451 438 30) J.M.Akkermans, H.Gruppelaar: Phys. Lett. 157B, 95 (1985). 9649 1451 439 31) P.A.Moldauer: Nucl. Phys. A344, 185 (1980). 9649 1451 440 32) D.L.Hill, J.A.Wheeler: Phys. Rev. 89, 1102 (1953). 9649 1451 441 33) J.Kopecky, M.Uhl: Phys. Rev. C41, 1941 (1990). 9649 1451 442 34) J.Kopecky, M.Uhl, R.E.Chrien: Phys. Rev. C47, 312 (1990). 9649 1451 443 9649 1451 444 1 451 536 09649 1451 445 1 452 5 09649 1451 446 1 455 7 09649 1451 447 1 456 4 09649 1451 448 1 458 5 19649 1451 449 2 151 158 19649 1451 450 3 1 43 19649 1451 451 3 2 43 19649 1451 452 3 4 27 19649 1451 453 3 16 13 19649 1451 454 3 17 9 19649 1451 455 3 18 41 19649 1451 456 3 37 4 19649 1451 457 3 51 26 19649 1451 458 3 52 25 19649 1451 459 3 53 24 19649 1451 460 3 54 22 19649 1451 461 3 55 21 19649 1451 462 3 56 20 19649 1451 463 3 57 20 19649 1451 464 3 58 20 19649 1451 465 3 59 19 19649 1451 466 3 60 19 19649 1451 467 3 61 19 19649 1451 468 3 62 18 19649 1451 469 3 63 18 19649 1451 470 3 64 18 19649 1451 471 3 65 17 19649 1451 472 3 91 25 19649 1451 473 3 102 30 19649 1451 474 4 2 368 19649 1451 475 4 18 2 19649 1451 476 5 18 2150 19649 1451 477 6 16 1391 19649 1451 478 6 17 683 19649 1451 479 6 37 58 19649 1451 480 6 51 273 19649 1451 481 6 52 260 19649 1451 482 6 53 245 19649 1451 483 6 54 235 19649 1451 484 6 55 151 19649 1451 485 6 56 126 19649 1451 486 6 57 125 19649 1451 487 6 58 127 19649 1451 488 6 59 124 19649 1451 489 6 60 120 19649 1451 490 6 61 120 19649 1451 491 6 62 117 19649 1451 492 6 63 115 19649 1451 493 6 64 115 19649 1451 494 6 65 114 19649 1451 495 6 91 3005 19649 1451 496 6 102 3590 19649 1451 497 8 4 2 09649 1451 498 8 16 2 09649 1451 499 8 17 2 09649 1451 500 8 18 2 09649 1451 501 8 37 2 09649 1451 502 8 102 2 09649 1451 503 12 18 4 19649 1451 504 14 18 1 19649 1451 505 15 18 20 19649 1451 506 31 452 5 19649 1451 507 31 455 4 19649 1451 508 31 456 32 19649 1451 509 32 151 149 19649 1451 510 33 1 124 19649 1451 511 33 2 124 19649 1451 512 33 4 10 19649 1451 513 33 16 13 19649 1451 514 33 17 7 19649 1451 515 33 18 168 19649 1451 516 33 37 4 19649 1451 517 33 51 71 19649 1451 518 33 52 58 19649 1451 519 33 53 53 19649 1451 520 33 54 46 19649 1451 521 33 55 42 19649 1451 522 33 56 35 19649 1451 523 33 57 35 19649 1451 524 33 58 35 19649 1451 525 33 59 35 19649 1451 526 33 60 35 19649 1451 527 33 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18 1866 1.487500+7 1.09928-10 1.496000+7 1.04290-10 1.504500+7 9.89393-119649 5 18 1867 1.513000+7 9.38617-11 1.521500+7 8.90430-11 1.530000+7 8.44702-119649 5 18 1868 1.538500+7 8.01307-11 1.547000+7 7.60129-11 1.555500+7 7.21054-119649 5 18 1869 1.564000+7 6.83976-11 1.572500+7 6.48793-11 1.581000+7 6.15410-119649 5 18 1870 1.589500+7 5.83735-11 1.598000+7 5.53680-11 1.606500+7 5.25164-119649 5 18 1871 1.615000+7 4.98109-11 1.623500+7 4.72440-11 1.632000+7 4.48087-119649 5 18 1872 1.640500+7 4.24982-11 1.649000+7 4.03062-11 1.657500+7 3.82266-119649 5 18 1873 1.666000+7 3.62538-11 1.674500+7 3.43823-11 1.683000+7 3.26069-119649 5 18 1874 1.691500+7 3.09227-11 1.700000+7 2.93251-11 1.708500+7 2.78096-119649 5 18 1875 1.717000+7 2.63720-11 1.725500+7 2.50084-11 1.734000+7 2.37149-119649 5 18 1876 1.742500+7 2.24880-11 1.751000+7 2.13243-11 1.759500+7 2.02205-119649 5 18 1877 1.768000+7 1.91736-11 1.776500+7 1.81807-11 1.785000+7 1.72389-119649 5 18 1878 1.793500+7 1.63457-11 1.802000+7 1.54985-11 1.810500+7 1.46951-119649 5 18 1879 1.819000+7 1.39331-11 1.827500+7 1.32105-11 1.836000+7 1.25252-119649 5 18 1880 1.844500+7 1.18753-11 1.853000+7 1.12590-11 1.861500+7 1.06745-119649 5 18 1881 1.870000+7 1.01202-11 1.878500+7 9.59461-12 1.887000+7 9.09619-129649 5 18 1882 1.895500+7 8.62356-12 1.904000+7 8.17538-12 1.912500+7 7.75041-129649 5 18 1883 1.921000+7 7.34744-12 1.929500+7 6.96533-12 1.938000+7 6.60303-129649 5 18 1884 1.946500+7 6.25949-12 1.955000+7 5.93376-12 1.963500+7 5.62492-129649 5 18 1885 1.972000+7 5.33209-12 1.980500+7 5.05445-12 1.989000+7 4.79121-129649 5 18 1886 1.997500+7 4.54163-12 2.017500+7 0.000000+0 9649 5 18 1887 0.000000+0 1.800000+7 0 0 1 3749649 5 18 1888 374 2 9649 5 18 1889 0.000000+0 0.000000+0 1.000000-5 1.53138-12 1.200000-5 1.67754-129649 5 18 1890 1.400000-5 1.81195-12 1.600000-5 1.93706-12 1.800000-5 2.05456-129649 5 18 1891 2.200000-5 2.27140-12 2.500000-5 2.42132-12 2.900000-5 2.60785-129649 5 18 1892 3.400000-5 2.82372-12 4.000000-5 3.06276-12 4.600000-5 3.28444-129649 5 18 1893 5.400000-5 3.55861-12 6.300000-5 3.84373-12 7.400000-5 4.16580-129649 5 18 1894 8.600000-5 4.49089-12 1.000000-4 4.84265-12 1.200000-4 5.30486-129649 5 18 1895 1.400000-4 5.72990-12 1.600000-4 6.12552-12 1.800000-4 6.49710-129649 5 18 1896 2.200000-4 7.18281-12 2.500000-4 7.65691-12 2.900000-4 8.24674-129649 5 18 1897 3.400000-4 8.92941-12 4.000000-4 9.68531-12 4.600000-4 1.03863-119649 5 18 1898 5.400000-4 1.12533-11 6.300000-4 1.21550-11 7.400000-4 1.31735-119649 5 18 1899 8.600000-4 1.42015-11 1.000000-3 1.53138-11 1.200000-3 1.67755-119649 5 18 1900 1.400000-3 1.81196-11 1.600000-3 1.93707-11 1.800000-3 2.05457-119649 5 18 1901 2.200000-3 2.27141-11 2.500000-3 2.42134-11 2.900000-3 2.60786-119649 5 18 1902 3.400000-3 2.82374-11 4.000000-3 3.06278-11 4.600000-3 3.28447-119649 5 18 1903 5.400000-3 3.55863-11 6.300000-3 3.84377-11 7.400000-3 4.16584-119649 5 18 1904 8.600000-3 4.49093-11 1.000000-2 4.84270-11 1.200000-2 5.30492-119649 5 18 1905 1.400000-2 5.72997-11 1.600000-2 6.12561-11 1.800000-2 6.49719-119649 5 18 1906 2.200000-2 7.18293-11 2.500000-2 7.65704-11 2.900000-2 8.24689-119649 5 18 1907 3.400000-2 8.92959-11 4.000000-2 9.68552-11 4.600000-2 1.03866-109649 5 18 1908 5.400000-2 1.12536-10 6.300000-2 1.21553-10 7.400000-2 1.31738-109649 5 18 1909 8.600000-2 1.42019-10 1.000000-1 1.53144-10 1.200000-1 1.67761-109649 5 18 1910 1.400000-1 1.81203-10 1.600000-1 1.93715-10 1.800000-1 2.05467-109649 5 18 1911 2.200000-1 2.27153-10 2.500000-1 2.42147-10 2.900000-1 2.60801-109649 5 18 1912 3.400000-1 2.82392-10 4.000000-1 3.06299-10 4.600000-1 3.28471-109649 5 18 1913 5.400000-1 3.55892-10 6.300000-1 3.84410-10 7.400000-1 4.16624-109649 5 18 1914 8.600000-1 4.49140-10 1.000000+0 4.84324-10 1.200000+0 5.30557-109649 5 18 1915 1.400000+0 5.73074-10 1.600000+0 6.12648-10 1.800000+0 6.49818-109649 5 18 1916 2.200000+0 7.18414-10 2.500000+0 7.65842-10 2.900000+0 8.24851-109649 5 18 1917 3.400000+0 8.93149-10 4.000000+0 9.68777-10 4.600000+0 1.038920-99649 5 18 1918 5.400000+0 1.125670-9 6.300000+0 1.215890-9 7.400000+0 1.317810-99649 5 18 1919 8.600000+0 1.420690-9 1.000000+1 1.532020-9 1.200000+1 1.678310-99649 5 18 1920 1.400000+1 1.812860-9 1.600000+1 1.938100-9 1.800000+1 2.055730-99649 5 18 1921 2.200000+1 2.272850-9 2.500000+1 2.422980-9 2.900000+1 2.609780-99649 5 18 1922 3.400000+1 2.826010-9 4.000000+1 3.065460-9 4.600000+1 3.287580-99649 5 18 1923 5.400000+1 3.562310-9 6.300000+1 3.848090-9 7.400000+1 4.170970-99649 5 18 1924 8.600000+1 4.496939-9 1.000000+2 4.849739-9 1.200000+2 5.313459-99649 5 18 1925 1.400000+2 5.740019-9 1.600000+2 6.137179-9 1.800000+2 6.510299-99649 5 18 1926 2.200000+2 7.199129-9 2.500000+2 7.675589-9 2.900000+2 8.268599-99649 5 18 1927 3.400000+2 8.955269-9 4.000000+2 9.716009-9 4.600000+2 1.042190-89649 5 18 1928 5.400000+2 1.129540-8 6.300000+2 1.220450-8 7.400000+2 1.323210-89649 5 18 1929 8.600000+2 1.427020-8 1.000000+3 1.539430-8 1.200000+3 1.687270-89649 5 18 1930 1.400000+3 1.823370-8 1.600000+3 1.950170-8 1.800000+3 2.069370-89649 5 18 1931 2.200000+3 2.289600-8 2.500000+3 2.442050-8 2.900000+3 2.631940-89649 5 18 1932 3.400000+3 2.852000-8 4.000000+3 3.096020-8 4.600000+3 3.322650-89649 5 18 1933 5.400000+3 3.603320-8 6.300000+3 3.895660-8 7.400000+3 4.226390-89649 5 18 1934 8.600000+3 4.560719-8 1.000000+4 4.923009-8 1.200000+4 5.399779-89649 5 18 1935 1.400000+4 5.838839-8 1.600000+4 6.247959-8 1.800000+4 6.632529-89649 5 18 1936 2.200000+4 7.342799-8 2.500000+4 7.834119-8 2.900000+4 8.445419-89649 5 18 1937 3.400000+4 9.152679-8 4.000000+4 9.935009-8 4.600000+4 1.065930-79649 5 18 1938 5.400000+4 1.155290-7 6.300000+4 1.247880-7 7.400000+4 1.351950-79649 5 18 1939 8.600000+4 1.456320-7 9.000000+4 1.489310-7 1.800000+5 2.079010-79649 5 18 1940 2.700000+5 2.500580-7 3.600000+5 2.829910-7 4.500000+5 2.980430-79649 5 18 1941 5.400000+5 3.086740-7 6.300000+5 3.159570-7 7.200000+5 3.206480-79649 5 18 1942 8.100000+5 3.208570-7 9.000000+5 3.194210-7 9.900000+5 3.166530-79649 5 18 1943 1.080000+6 3.128030-7 1.170000+6 3.069330-7 1.260000+6 3.004050-79649 5 18 1944 1.350000+6 2.933700-7 1.440000+6 2.859560-7 1.530000+6 2.772810-79649 5 18 1945 1.620000+6 2.684150-7 1.710000+6 2.594310-7 1.800000+6 2.503880-79649 5 18 1946 1.890000+6 2.410520-7 1.980000+6 2.317460-7 2.070000+6 2.225030-79649 5 18 1947 2.160000+6 2.133500-7 2.250000+6 2.045580-7 2.340000+6 1.958970-79649 5 18 1948 2.430000+6 1.873800-7 2.520000+6 1.790170-7 2.610000+6 1.712260-79649 5 18 1949 2.700000+6 1.636040-7 2.790000+6 1.561560-7 2.880000+6 1.488860-79649 5 18 1950 2.970000+6 1.422130-7 3.060000+6 1.357190-7 3.150000+6 1.294020-79649 5 18 1951 3.240000+6 1.232630-7 3.330000+6 1.176260-7 3.420000+6 1.121610-79649 5 18 1952 3.510000+6 1.068640-7 3.600000+6 1.017320-7 3.690000+6 9.701189-89649 5 18 1953 3.780000+6 9.244919-8 3.870000+6 8.803909-8 3.960000+6 8.377729-89649 5 18 1954 4.050000+6 7.985499-8 4.140000+6 7.607199-8 4.230000+6 7.242359-89649 5 18 1955 4.320000+6 6.890539-8 4.410000+6 6.564189-8 4.500000+6 6.249959-89649 5 18 1956 4.590000+6 5.947389-8 4.680000+6 5.656059-8 4.770000+6 5.387089-89649 5 18 1957 4.860000+6 5.128519-8 4.950000+6 4.879919-8 5.040000+6 4.640899-89649 5 18 1958 5.130000+6 4.421009-8 5.220000+6 4.209950-8 5.310000+6 4.007330-89649 5 18 1959 5.400000+6 3.812810-8 5.490000+6 3.635180-8 5.580000+6 3.464970-89649 5 18 1960 5.670000+6 3.301860-8 5.760000+6 3.145550-8 5.850000+6 3.003340-89649 5 18 1961 5.940000+6 2.867330-8 6.030000+6 2.737270-8 6.120000+6 2.612870-89649 5 18 1962 6.210000+6 2.498100-8 6.300000+6 2.388510-8 6.390000+6 2.283850-89649 5 18 1963 6.480000+6 2.183900-8 6.570000+6 2.091300-8 6.660000+6 2.003000-89649 5 18 1964 6.750000+6 1.918780-8 6.840000+6 1.838460-8 6.930000+6 1.762780-89649 5 18 1965 7.020000+6 1.690640-8 7.110000+6 1.621870-8 7.200000+6 1.556320-89649 5 18 1966 7.290000+6 1.494340-8 7.380000+6 1.435280-8 7.470000+6 1.378990-89649 5 18 1967 7.560000+6 1.325350-8 7.650000+6 1.274520-8 7.740000+6 1.226080-89649 5 18 1968 7.830000+6 1.179920-8 7.920000+6 1.135930-8 8.010000+6 1.093790-89649 5 18 1969 8.100000+6 1.053620-8 8.190000+6 1.015310-8 8.280000+6 9.787829-99649 5 18 1970 8.370000+6 9.437279-9 8.460000+6 9.102799-9 8.550000+6 8.783599-99649 5 18 1971 8.640000+6 8.478919-9 8.730000+6 8.184269-9 8.820000+6 7.902739-99649 5 18 1972 8.910000+6 7.633679-9 9.000000+6 7.376469-9 9.090000+6 7.132549-99649 5 18 1973 9.180000+6 6.899329-9 9.270000+6 6.676259-9 9.360000+6 6.462849-99649 5 18 1974 9.450000+6 6.270759-9 9.540000+6 6.087379-9 9.630000+6 5.912269-99649 5 18 1975 9.720000+6 5.745009-9 9.810000+6 5.604999-9 9.900000+6 5.472079-99649 5 18 1976 9.990000+6 5.345869-9 1.008000+7 5.226049-9 1.017000+7 5.139799-99649 5 18 1977 1.026000+7 5.059309-9 1.035000+7 4.984269-9 1.044000+7 4.914409-99649 5 18 1978 1.053000+7 4.753759-9 1.062000+7 4.597769-9 1.071000+7 4.446199-99649 5 18 1979 1.080000+7 4.298840-9 1.089000+7 4.119360-9 1.098000+7 3.943650-99649 5 18 1980 1.107000+7 3.771540-9 1.116000+7 3.602820-9 1.125000+7 3.700340-99649 5 18 1981 1.134000+7 3.800920-9 1.143000+7 3.904400-9 1.152000+7 4.010630-99649 5 18 1982 1.161000+7 3.949320-9 1.170000+7 3.890490-9 1.179000+7 3.834000-99649 5 18 1983 1.188000+7 3.779740-9 1.197000+7 3.493880-9 1.206000+7 3.210010-99649 5 18 1984 1.215000+7 2.928050-9 1.224000+7 2.647880-9 1.233000+7 2.384790-99649 5 18 1985 1.242000+7 2.123310-9 1.251000+7 1.863360-9 1.260000+7 1.604870-99649 5 18 1986 1.269000+7 1.423350-9 1.278000+7 1.243140-9 1.287000+7 1.064160-99649 5 18 1987 1.296000+7 8.86352-10 1.305000+7 7.81735-10 1.314000+7 6.78169-109649 5 18 1988 1.323000+7 5.75600-10 1.332000+7 4.73975-10 1.341000+7 4.27873-109649 5 18 1989 1.350000+7 3.82618-10 1.359000+7 3.38166-10 1.368000+7 2.94475-109649 5 18 1990 1.377000+7 2.71363-10 1.386000+7 2.48933-10 1.395000+7 2.27150-109649 5 18 1991 1.404000+7 2.05980-10 1.413000+7 1.92777-10 1.422000+7 1.80124-109649 5 18 1992 1.431000+7 1.67991-10 1.440000+7 1.56352-10 1.449000+7 1.47541-109649 5 18 1993 1.458000+7 1.39173-10 1.467000+7 1.31223-10 1.476000+7 1.23671-109649 5 18 1994 1.485000+7 1.16971-10 1.494000+7 1.10627-10 1.503000+7 1.04620-109649 5 18 1995 1.512000+7 9.89320-11 1.521000+7 9.35944-11 1.530000+7 8.85427-119649 5 18 1996 1.539000+7 8.37616-11 1.548000+7 7.92369-11 1.557000+7 7.49579-119649 5 18 1997 1.566000+7 7.09087-11 1.575000+7 6.70769-11 1.584000+7 6.34510-119649 5 18 1998 1.593000+7 6.00201-11 1.602000+7 5.67737-11 1.611000+7 5.37019-119649 5 18 1999 1.620000+7 5.07954-11 1.629000+7 4.80453-11 1.638000+7 4.54434-119649 5 18 2000 1.647000+7 4.29815-11 1.656000+7 4.06524-11 1.665000+7 3.84488-119649 5 18 2001 1.674000+7 3.63640-11 1.683000+7 3.43917-11 1.692000+7 3.25258-119649 5 18 2002 1.701000+7 3.07607-11 1.710000+7 2.90908-11 1.719000+7 2.75112-119649 5 18 2003 1.728000+7 2.60169-11 1.737000+7 2.46034-11 1.746000+7 2.32663-119649 5 18 2004 1.755000+7 2.20016-11 1.764000+7 2.08052-11 1.773000+7 1.96737-119649 5 18 2005 1.782000+7 1.86033-11 1.791000+7 1.75910-11 1.800000+7 1.66335-119649 5 18 2006 1.809000+7 1.57279-11 1.818000+7 1.48713-11 1.827000+7 1.40612-119649 5 18 2007 1.836000+7 1.32951-11 1.845000+7 1.25705-11 1.854000+7 1.18852-119649 5 18 2008 1.863000+7 1.12372-11 1.872000+7 1.06243-11 1.881000+7 1.00447-119649 5 18 2009 1.890000+7 9.49661-12 1.899000+7 8.97830-12 1.908000+7 8.48817-129649 5 18 2010 1.917000+7 8.02469-12 1.926000+7 7.58641-12 1.935000+7 7.17198-129649 5 18 2011 1.944000+7 6.78010-12 1.953000+7 6.40956-12 1.962000+7 6.05918-129649 5 18 2012 1.971000+7 5.72789-12 1.980000+7 5.41465-12 1.989000+7 5.11847-129649 5 18 2013 1.998000+7 4.83843-12 2.018000+7 0.000000+0 9649 5 18 2014 0.000000+0 2.000000+7 0 0 1 4019649 5 18 2015 401 2 9649 5 18 2016 0.000000+0 0.000000+0 1.000000-5 1.50230-12 1.200000-5 1.64568-129649 5 18 2017 1.400000-5 1.77754-12 1.600000-5 1.90027-12 1.800000-5 2.01554-129649 5 18 2018 2.200000-5 2.22827-12 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