JENDL-5 (Neutron sublibrary (up to 20 MeV)) Cf-249 0 0 0 0 9.824900+4 2.469350+2 1 1 6 19852 1451 1 0.000000+0 1.000000+0 0 0 0 69852 1451 2 1.000000+0 2.000000+7 0 0 10 59852 1451 3 0.000000+0 0.000000+0 3 0 425 999852 1451 4 98-Cf-249 JAEA+ EVAL-JAN10 O.Iwamoto,T.Nakagawa,+ 9852 1451 5 DIST-DEC21 20100318 9852 1451 6 ----JENDL-5 MATERIAL 9852 9852 1451 7 -----INCIDENT NEUTRON DATA 9852 1451 8 ------ENDF-6 FORMAT 9852 1451 9 9852 1451 10 History 9852 1451 11 05-12 Fission cross section above 70 eV was revised. 9852 1451 12 07-09 Theoretical calculation was made with CCONE code. 9852 1451 13 Data were compiled as JENDL/AC-2008/1/. 9852 1451 14 09-08 (MF1,MT458) was evaluated. 9852 1451 15 09-12 New theoretical calculation was made with CCONE code. 9852 1451 16 10-01 Data of prompt gamma rays due to fission were given. 9852 1451 17 10-03 Covariance data were given. 9852 1451 18 21-08 QI of MT58 was slightly shifted to avoid duplication with 9852 1451 19 MT57 by S. Nakayama. 9852 1451 20 9852 1451 21 21-11 revised by O.Iwamoto 9852 1451 22 (MF3/MT19-21,38) deleted 9852 1451 23 (MF8/MT16-18,37,102) JENDL/AD-2017 adopted 9852 1451 24 (MF8/MT4) added 9852 1451 25 9852 1451 26 MF= 1 General information 9852 1451 27 MT=452 Number of Neutrons per fission 9852 1451 28 Sum of MT's = 455 and 456. 9852 1451 29 9852 1451 30 MT=455 Delayed neutron data 9852 1451 31 (Same as JENDL-3.3) 9852 1451 32 Semi-empirical formula by Tuttle/2/. 9852 1451 33 Decay constants were evaluated by Brady and England/3/. 9852 1451 34 9852 1451 35 MT=456 Number of prompt neutrons per fission 9852 1451 36 (same as JENDL-3.3) 9852 1451 37 At the thermal energy, the data of Volodin et al./4/ was 9852 1451 38 adopted. An energy dependent term was based on the semi- 9852 1451 39 empirical formula by Howerton/5/. 9852 1451 40 9852 1451 41 MT=458 Components of energy release due to fission 9852 1451 42 Total energy and prompt energy were calculated from mass 9852 1451 43 balance using JENDL-4 fission yields data and mass excess 9852 1451 44 evaluation. Mass excess values were from Audi's 2009 9852 1451 45 evaluation/6/. Delayed energy values were calculated from 9852 1451 46 the energy release for infinite irradiation using JENDL FP 9852 1451 47 Decay Data File 2000 and JENDL-4 yields data. For delayed 9852 1451 48 neutron energy, as the JENDL FP Decay Data File 2000/7/ does 9852 1451 49 not include average neutron energy values, the average values 9852 1451 50 were calculated using the formula shown in the report by 9852 1451 51 T.R. England/8/. The fractions of prompt energy were 9852 1451 52 calculated using the fractions of Sher's evaluation/9/ when 9852 1451 53 they were provided. When the fractions were not given by Sher,9852 1451 54 averaged fractions were used. 9852 1451 55 9852 1451 56 9852 1451 57 MF= 2 Resonance parameters 9852 1451 58 MT=151 9852 1451 59 Resolved resonance parameters (MLBW: 1.0e-5 - 70.0 eV) 9852 1451 60 Resonance energies, neutron and fission widths were taken 9852 1451 61 from the experimental data of Benjamin et al./10/ Radiative 9852 1451 62 widths were assumed to be 0.04 eV according to Dabbs et 9852 1451 63 al./11/ A negative resonance was added so as to reproduce 9852 1451 64 thermal cross sections. 9852 1451 65 9852 1451 66 capture = 507+-20 /12,13/ 9852 1451 67 fission = 1671+-28 /14,15,16,17/ 9852 1451 68 9852 1451 69 Unresolved resonance parameters (70 eV - 30 keV) 9852 1451 70 Parameters (URP) were determined with ASREP code/18/ so as to 9852 1451 71 reproduce the cross sections in this energy region. URP are 9852 1451 72 used only for self-shielding calculations. 9852 1451 73 9852 1451 74 9852 1451 75 Thermal cross sections and resonance integrals (at 300K) 9852 1451 76 ------------------------------------------------------- 9852 1451 77 0.0253 eV reson. integ.(*) 9852 1451 78 (barns) (barns) 9852 1451 79 ------------------------------------------------------- 9852 1451 80 total 2185.5 9852 1451 81 elastic 6.25 9852 1451 82 fission 1672.7 2220 9852 1451 83 capture 506.5 696 9852 1451 84 ------------------------------------------------------- 9852 1451 85 (*) In the energy range from 0.5 eV to 10 MeV. 9852 1451 86 9852 1451 87 9852 1451 88 MF= 3 Neutron cross sections 9852 1451 89 Cross sections above the resolved resonance region except for 9852 1451 90 the elastic scattering (MT=2) and fission cross sections (MT=18,9852 1451 91 19, 20, 21, 38) were calculated with CCONE code/19/. 9852 1451 92 9852 1451 93 MT= 1 Total cross section 9852 1451 94 The cross section was calculated with CC OMP of Soukhovitskii 9852 1451 95 et al./20/ 9852 1451 96 9852 1451 97 MT= 2 Elastic scattering cross section 9852 1451 98 Calculated as total - non-elastic scattering cross sections. 9852 1451 99 9852 1451 100 MT=18 Fission cross section 9852 1451 101 In the energy range from 70 to 300 eV, the fission cross 9852 1451 102 section was determined from the data measured by Dabbs et 9852 1451 103 al./21/ Resonance structure was kept in the present file. 9852 1451 104 9852 1451 105 Above 300 eV, the following experimental data were analyzed 9852 1451 106 with the GMA code/22/: 9852 1451 107 9852 1451 108 Authors Energy range Data points Reference 9852 1451 109 Silbert 280 eV - 2.9 MeV 2083 /23/ 9852 1451 110 Fursov+ 0.5 - 7 MeV 13 /24/ (*1) 9852 1451 111 Dabbs+ 280 eV - 17 MeV 956 /21/ 9852 1451 112 Kuprijanov+ 0.13 - 7.4 MeV 43 /25/ (*1) 9852 1451 113 9852 1451 114 (*1) Relative to Pu-239 fission. Data were converted 9852 1451 115 to cross sections using JENDL-3.3 data. 9852 1451 116 9852 1451 117 The results of GMA were used to determine the parameters in 9852 1451 118 the CCONE calculation. 9852 1451 119 9852 1451 120 In the energy region from 10 to 20 MeV, the data of JENDL-3.3 9852 1451 121 were adopted. 9852 1451 122 9852 1451 123 9852 1451 124 MT=19, 20, 21, 38 Multi-chance fission cross sections 9852 1451 125 Calculated with CCONE code, and renormalized to the total 9852 1451 126 fission cross section (MT=18). 9852 1451 127 9852 1451 128 9852 1451 129 MF= 4 Angular distributions of secondary neutrons 9852 1451 130 MT=2 Elastic scattering 9852 1451 131 Calculated with CCONE code/19/. 9852 1451 132 9852 1451 133 MT=18 Fission 9852 1451 134 Isotropic distributions in the laboratory system were assumed.9852 1451 135 9852 1451 136 9852 1451 137 MF= 5 Energy distributions of secondary neutrons 9852 1451 138 MT=18 Prompt neutrons 9852 1451 139 Calculated with CCONE code/19/. 9852 1451 140 9852 1451 141 MT=455 Delayed neutrons 9852 1451 142 Calculated by Brady and England/3/. 9852 1451 143 9852 1451 144 9852 1451 145 MF= 6 Energy-angle distributions 9852 1451 146 Calculated with CCONE code/19/. 9852 1451 147 Distributions from fission (MT=18) are not included. 9852 1451 148 9852 1451 149 9852 1451 150 MF=12 Photon production multiplicities 9852 1451 151 MT=18 Fission 9852 1451 152 Calculated from the total energy released by the prompt 9852 1451 153 gamma-rays due to fission given in MF=1/MT=458 and the 9852 1451 154 average energy of gamma-rays. 9852 1451 155 9852 1451 156 9852 1451 157 MF=14 Photon angular distributions 9852 1451 158 MT=18 Fission 9852 1451 159 Isotoropic distributions were assumed. 9852 1451 160 9852 1451 161 9852 1451 162 MF=15 Continuous photon energy spectra 9852 1451 163 MT=18 Fission 9852 1451 164 Experimental data measured by Verbinski et al./26/ for 9852 1451 165 Pu-239 thermal fission were adopted. 9852 1451 166 9852 1451 167 9852 1451 168 MF=31 Covariances of average number of neutrons per fission 9852 1451 169 MT=452 Number of neutrons per fission 9852 1451 170 Sum of covariances for MT=455 and MT=456. 9852 1451 171 9852 1451 172 MT=455 9852 1451 173 Error of 15% was assumed. 9852 1451 174 9852 1451 175 MT=456 9852 1451 176 Covariance was obtained by fitting a linear function to the 9852 1451 177 data at 0.0 and 5.0 MeV with an uncertainty of 1% and 5%, 9852 1451 178 respectively. The uncertainty of 1% was based on the data of 9852 1451 179 Volodin et al./4/ 9852 1451 180 9852 1451 181 9852 1451 182 MF=32 Covariances of resonance parameters 9852 1451 183 MT=151 Resolved resonance parameterss 9852 1451 184 Format of LCOMP=0 was adopted. 9852 1451 185 9852 1451 186 Uncertainties of parameters were taken from Mughabghab /27/. 9852 1451 187 For the parameters without any information on uncertainty, 9852 1451 188 the following uncertainties were assumed: 9852 1451 189 Resonance energy 0.1 % 9852 1451 190 Neutron width 10 % 9852 1451 191 Capture width 20 % 9852 1451 192 Fission width 10 % 9852 1451 193 9852 1451 194 They were further modified by considering experimental data 9852 1451 195 of the fission and capture cross sections at the thermal 9852 1451 196 neutron energy. 9852 1451 197 9852 1451 198 9852 1451 199 MF=33 Covariances of neutron cross sections 9852 1451 200 Covariances were given to all the cross sections by using 9852 1451 201 KALMAN code/28/ and the covariances of model parameters 9852 1451 202 used in the cross-section calculations. 9852 1451 203 9852 1451 204 For the fission cross section, covariances obtained with the 9852 1451 205 GMA analysis were adopted. Standard deviations (SD) were 9852 1451 206 multiplied by a factor of 1.5. SD of 6% were assumed in the 9852 1451 207 energy region above 6 MeV. 9852 1451 208 9852 1451 209 In the resolved resonance region, the following standard 9852 1451 210 deviations were added to the contributions from resonance 9852 1451 211 parameters: 9852 1451 212 Elastic scattering 20 % 9852 1451 213 9852 1451 214 9852 1451 215 MF=34 Covariances for Angular Distributions 9852 1451 216 MT=2 Elastic scattering 9852 1451 217 Covariances were given only to P1 components. 9852 1451 218 9852 1451 219 9852 1451 220 MF=35 Covariances for Energy Distributions 9852 1451 221 MT=18 Fission spectra 9852 1451 222 Estimated with CCONE and KALMAN codes. 9852 1451 223 9852 1451 224 9852 1451 225 ***************************************************************** 9852 1451 226 Calculation with CCONE code 9852 1451 227 ***************************************************************** 9852 1451 228 9852 1451 229 Models and parameters used in the CCONE/19/ calculation 9852 1451 230 1) Coupled channel optical model 9852 1451 231 Levels in the rotational band were included. Optical model 9852 1451 232 potential and coupled levels are shown in Table 1. 9852 1451 233 9852 1451 234 2) Two-component exciton model/29/ 9852 1451 235 * Global parametrization of Koning-Duijvestijn/30/ 9852 1451 236 was used. 9852 1451 237 * Gamma emission channel/31/ was added to simulate direct 9852 1451 238 and semi-direct capture reaction. 9852 1451 239 9852 1451 240 3) Hauser-Feshbach statistical model 9852 1451 241 * Moldauer width fluctuation correction/32/ was included. 9852 1451 242 * Neutron, gamma and fission decay channel were included. 9852 1451 243 * Transmission coefficients of neutrons were taken from 9852 1451 244 coupled channel calculation in Table 1. 9852 1451 245 * The level scheme of the target is shown in Table 2. 9852 1451 246 * Level density formula of constant temperature and Fermi-gas 9852 1451 247 model were used with shell energy correction and collective 9852 1451 248 enhancement factor. Parameters are shown in Table 3. 9852 1451 249 * Fission channel: 9852 1451 250 Double humped fission barriers were assumed. 9852 1451 251 Fission barrier penetrabilities were calculated with 9852 1451 252 Hill-Wheler formula/33/. Fission barrier parameters were 9852 1451 253 shown in Table 4. Transition state model was used and 9852 1451 254 continuum levels are assumed above the saddles. The level 9852 1451 255 density parameters for inner and outer saddles are shown in 9852 1451 256 Tables 5 and 6, respectively. 9852 1451 257 * Gamma-ray strength function of Kopecky et al/34/,/35/ 9852 1451 258 was used. The prameters are shown in Table 7. 9852 1451 259 9852 1451 260 9852 1451 261 ------------------------------------------------------------------9852 1451 262 Tables 9852 1451 263 ------------------------------------------------------------------9852 1451 264 9852 1451 265 Table 1. Coupled channel calculation 9852 1451 266 -------------------------------------------------- 9852 1451 267 * rigid rotor model was applied 9852 1451 268 * coupled levels = 0,1,2,5,7 (see Table 2) 9852 1451 269 * optical potential parameters /20/ 9852 1451 270 Volume: 9852 1451 271 V_0 = 49.97 MeV 9852 1451 272 lambda_HF = 0.01004 1/MeV 9852 1451 273 C_viso = 15.9 MeV 9852 1451 274 A_v = 12.04 MeV 9852 1451 275 B_v = 81.36 MeV 9852 1451 276 E_a = 385 MeV 9852 1451 277 r_v = 1.2568 fm 9852 1451 278 a_v = 0.633 fm 9852 1451 279 Surface: 9852 1451 280 W_0 = 17.2 MeV 9852 1451 281 B_s = 11.19 MeV 9852 1451 282 C_s = 0.01361 1/MeV 9852 1451 283 C_wiso = 23.5 MeV 9852 1451 284 r_s = 1.1803 fm 9852 1451 285 a_s = 0.601 fm 9852 1451 286 Spin-orbit: 9852 1451 287 V_so = 5.75 MeV 9852 1451 288 lambda_so = 0.005 1/MeV 9852 1451 289 W_so = -3.1 MeV 9852 1451 290 B_so = 160 MeV 9852 1451 291 r_so = 1.1214 fm 9852 1451 292 a_so = 0.59 fm 9852 1451 293 Coulomb: 9852 1451 294 C_coul = 1.3 9852 1451 295 r_c = 1.2452 fm 9852 1451 296 a_c = 0.545 fm 9852 1451 297 Deformation: 9852 1451 298 beta_2 = 0.213 9852 1451 299 beta_4 = 0.05 9852 1451 300 beta_6 = 0.0015 9852 1451 301 9852 1451 302 * Calculated strength function 9852 1451 303 S0= 1.13e-4 S1= 3.05e-4 R'= 8.98 fm (En=1 keV) 9852 1451 304 -------------------------------------------------- 9852 1451 305 9852 1451 306 Table 2. Level Scheme of Cf-249 9852 1451 307 ------------------- 9852 1451 308 No. Ex(MeV) J PI 9852 1451 309 ------------------- 9852 1451 310 0 0.00000 9/2 - * 9852 1451 311 1 0.06249 11/2 - * 9852 1451 312 2 0.13620 13/2 - * 9852 1451 313 3 0.14496 5/2 + 9852 1451 314 4 0.18794 7/2 + 9852 1451 315 5 0.22000 15/2 - * 9852 1451 316 6 0.24307 9/2 + 9852 1451 317 7 0.31500 17/2 - * 9852 1451 318 8 0.31500 11/2 + 9852 1451 319 9 0.37952 7/2 + 9852 1451 320 10 0.38400 13/2 + 9852 1451 321 11 0.41680 1/2 + 9852 1451 322 12 0.42500 19/2 - 9852 1451 323 13 0.43756 9/2 + 9852 1451 324 14 0.44000 3/2 + 9852 1451 325 15 0.44298 7/2 + 9852 1451 326 16 0.46000 5/2 + 9852 1451 327 17 0.50070 9/2 + 9852 1451 328 ------------------- 9852 1451 329 *) Coupled levels in CC calculation 9852 1451 330 9852 1451 331 Table 3. Level density parameters 9852 1451 332 -------------------------------------------------------- 9852 1451 333 Nuclide a* Pair Eshell T E0 Ematch 9852 1451 334 1/MeV MeV MeV MeV MeV MeV 9852 1451 335 -------------------------------------------------------- 9852 1451 336 Cf-250 19.3542 1.5179 1.0208 0.3946 -0.1776 3.8329 9852 1451 337 Cf-249 19.0966 0.7605 0.7689 0.3773 -0.6847 2.7641 9852 1451 338 Cf-248 19.0305 1.5240 0.7495 0.3921 -0.0631 3.7096 9852 1451 339 Cf-247 18.9645 0.7635 0.5924 0.3748 -0.6176 2.6898 9852 1451 340 Cf-246 18.8984 1.5302 0.7686 0.4030 -0.1574 3.8448 9852 1451 341 -------------------------------------------------------- 9852 1451 342 9852 1451 343 Table 4. Fission barrier parameters 9852 1451 344 ---------------------------------------- 9852 1451 345 Nuclide V_A hw_A V_B hw_B 9852 1451 346 MeV MeV MeV MeV 9852 1451 347 ---------------------------------------- 9852 1451 348 Cf-250 6.200 1.150 5.450 0.600 9852 1451 349 Cf-249 6.000 1.200 6.000 0.800 9852 1451 350 Cf-248 6.200 1.040 5.400 0.600 9852 1451 351 Cf-247 6.700 1.000 5.900 0.800 9852 1451 352 Cf-246 6.200 1.040 5.400 0.600 9852 1451 353 ---------------------------------------- 9852 1451 354 9852 1451 355 Table 5. Level density above inner saddle 9852 1451 356 -------------------------------------------------------- 9852 1451 357 Nuclide a* Pair Eshell T E0 Ematch 9852 1451 358 1/MeV MeV MeV MeV MeV MeV 9852 1451 359 -------------------------------------------------------- 9852 1451 360 Cf-250 21.4621 1.7709 2.5000 0.2827 -0.1068 3.2709 9852 1451 361 Cf-249 20.0514 0.8872 2.5000 0.3486 -1.7837 3.0872 9852 1451 362 Cf-248 21.3142 1.7780 2.5000 0.3226 -0.6352 3.7780 9852 1451 363 Cf-247 21.2402 0.8908 2.5000 0.3232 -1.5224 2.8908 9852 1451 364 Cf-246 21.1662 1.7852 2.5000 0.3238 -0.6280 3.7852 9852 1451 365 -------------------------------------------------------- 9852 1451 366 9852 1451 367 Table 6. Level density above outer saddle 9852 1451 368 -------------------------------------------------------- 9852 1451 369 Nuclide a* Pair Eshell T E0 Ematch 9852 1451 370 1/MeV MeV MeV MeV MeV MeV 9852 1451 371 -------------------------------------------------------- 9852 1451 372 Cf-250 21.4621 1.7709 0.9600 0.3499 0.0610 3.7709 9852 1451 373 Cf-249 20.0514 0.8872 0.9200 0.3794 -1.0059 3.0872 9852 1451 374 Cf-248 21.3142 1.7780 0.8800 0.3522 0.0693 3.7780 9852 1451 375 Cf-247 21.2402 0.8908 0.8400 0.3533 -0.8173 2.8908 9852 1451 376 Cf-246 21.1662 1.7852 0.8000 0.3544 0.0777 3.7852 9852 1451 377 -------------------------------------------------------- 9852 1451 378 9852 1451 379 Table 7. Gamma-ray strength function for Cf-250 9852 1451 380 -------------------------------------------------------- 9852 1451 381 K0 = 1.500 E0 = 4.500 (MeV) 9852 1451 382 * E1: ER = 11.31 (MeV) EG = 2.67 (MeV) SIG = 255.17 (mb) 9852 1451 383 ER = 14.32 (MeV) EG = 4.20 (MeV) SIG = 510.34 (mb) 9852 1451 384 * M1: ER = 6.51 (MeV) EG = 4.00 (MeV) SIG = 1.84 (mb) 9852 1451 385 * E2: ER = 10.00 (MeV) EG = 3.11 (MeV) SIG = 7.35 (mb) 9852 1451 386 -------------------------------------------------------- 9852 1451 387 9852 1451 388 9852 1451 389 References 9852 1451 390 1) O.Iwamoto et al.: J. Nucl. Sci. Technol., 46, 510 (2009). 9852 1451 391 2) R.J.Tuttld: INDC(NDS)-107/G+Special, p.29 (1979). 9852 1451 392 3) M.C.Brady, T.R.England: Nucl. Sci. Eng., 103, 129 (1989). 9852 1451 393 4) K.E.Volodin et al.: Sov. J. Nucl. Phys., 15, 17 (1972). 9852 1451 394 5) R.J.Howerton: Nucl. Sci. Eng., 62, 438 (1977). 9852 1451 395 6) G.Audi: Private communication (April 2009). 9852 1451 396 7) J.Katakura et al.: JAERI 1343 (2001). 9852 1451 397 8) T.R.England et al.: LA-11151-MS (1988). 9852 1451 398 9) R.Sher, C.Beck: EPRI NP-1771 (1981). 9852 1451 399 10) R.W.Benjamin et al.: Nucl. Sci. Eng., 85, 261 (1983). 9852 1451 400 11) J.W.T.Dabbs et al.: ORNL-4973, p.181 (1974). 9852 1451 401 12) J.Halperin et al.: ORNL-4706, p.47 (1971). 9852 1451 402 13) V.D.Gavrilov et al.: Sov. At. Energy, 41, 808 (1976). 9852 1451 403 14) E.F.Fomushkin et al.: Sov. J. Nucl. Phys., 14, 41 (1972). 9852 1451 404 15) B.I.Fursov et al.: Sov. At. Energy, 32, 205 (1972). 9852 1451 405 16) R.W.Benjamin et al.: Nucl. Sci. Eng., 47, 203 (1972). 9852 1451 406 17) K.D.Zhuravlev et al.: Sov. At. Energy, 39, 907 (1975). 9852 1451 407 18) Y.Kikuchi et al.: JAERI-Data/Code 99-025 (1999) in Japanese. 9852 1451 408 19) O.Iwamoto: J. Nucl. Sci. 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Lett. 157B, 95 (1985). 9852 1451 424 32) P.A.Moldauer: Nucl. Phys. A344, 185 (1980). 9852 1451 425 33) D.L.Hill, J.A.Wheeler: Phys. Rev. 89, 1102 (1953). 9852 1451 426 34) J.Kopecky, M.Uhl: Phys. Rev. C41, 1941 (1990). 9852 1451 427 35) J.Kopecky, M.Uhl, R.E.Chrien: Phys. Rev. C47, 312 (1990). 9852 1451 428 9852 1451 429 1 451 528 09852 1451 430 1 452 5 19852 1451 431 1 455 7 19852 1451 432 1 456 5 09852 1451 433 1 458 5 19852 1451 434 2 151 239 19852 1451 435 3 1 454 19852 1451 436 3 2 55 19852 1451 437 3 4 30 19852 1451 438 3 16 13 19852 1451 439 3 17 9 19852 1451 440 3 18 452 19852 1451 441 3 37 4 19852 1451 442 3 51 30 19852 1451 443 3 52 29 19852 1451 444 3 53 28 19852 1451 445 3 54 27 19852 1451 446 3 55 27 19852 1451 447 3 56 26 19852 1451 448 3 57 25 19852 1451 449 3 58 25 19852 1451 450 3 59 25 19852 1451 451 3 60 25 19852 1451 452 3 61 24 19852 1451 453 3 62 24 19852 1451 454 3 63 23 19852 1451 455 3 64 23 19852 1451 456 3 65 23 19852 1451 457 3 66 22 19852 1451 458 3 67 22 19852 1451 459 3 91 29 19852 1451 460 3 102 36 19852 1451 461 4 2 490 19852 1451 462 4 18 2 19852 1451 463 5 18 3974 19852 1451 464 5 455 577 19852 1451 465 6 16 2439 19852 1451 466 6 17 601 19852 1451 467 6 37 40 19852 1451 468 6 51 289 19852 1451 469 6 52 280 19852 1451 470 6 53 183 19852 1451 471 6 54 174 19852 1451 472 6 55 267 19852 1451 473 6 56 172 19852 1451 474 6 57 260 19852 1451 475 6 58 161 19852 1451 476 6 59 162 19852 1451 477 6 60 160 19852 1451 478 6 61 155 19852 1451 479 6 62 159 19852 1451 480 6 63 161 19852 1451 481 6 64 153 19852 1451 482 6 65 152 19852 1451 483 6 66 145 19852 1451 484 6 67 142 19852 1451 485 6 91 5817 19852 1451 486 6 102 4182 19852 1451 487 8 4 2 09852 1451 488 8 16 2 09852 1451 489 8 17 2 09852 1451 490 8 18 2 09852 1451 491 8 37 2 09852 1451 492 8 102 2 09852 1451 493 12 18 4 19852 1451 494 14 18 1 19852 1451 495 15 18 20 19852 1451 496 31 452 5 19852 1451 497 31 455 4 19852 1451 498 31 456 32 19852 1451 499 32 151 173 19852 1451 500 33 1 121 19852 1451 501 33 2 124 19852 1451 502 33 4 10 19852 1451 503 33 16 14 19852 1451 504 33 17 6 19852 1451 505 33 18 150 19852 1451 506 33 37 4 19852 1451 507 33 51 66 19852 1451 508 33 52 58 19852 1451 509 33 53 58 19852 1451 510 33 54 58 19852 1451 511 33 55 53 19852 1451 512 33 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18 1857 5.400000+4 1.322110-7 6.300000+4 1.426900-7 7.400000+4 1.544470-79852 5 18 1858 8.600000+4 1.662140-7 1.000000+5 1.788200-7 2.000000+5 2.390710-79852 5 18 1859 3.000000+5 2.740410-7 4.000000+5 2.915000-7 5.000000+5 2.990790-79852 5 18 1860 6.000000+5 3.026530-7 7.000000+5 3.040860-7 8.000000+5 3.036310-79852 5 18 1861 9.000000+5 3.016030-7 1.000000+6 2.981290-7 1.100000+6 2.933750-79852 5 18 1862 1.200000+6 2.875740-7 1.300000+6 2.809360-7 1.400000+6 2.736480-79852 5 18 1863 1.500000+6 2.658690-7 1.600000+6 2.577330-7 1.700000+6 2.493570-79852 5 18 1864 1.800000+6 2.408350-7 1.900000+6 2.322480-7 2.000000+6 2.236590-79852 5 18 1865 2.100000+6 2.151240-7 2.200000+6 2.066850-7 2.300000+6 1.983780-79852 5 18 1866 2.400000+6 1.902320-7 2.500000+6 1.822690-7 2.600000+6 1.745070-79852 5 18 1867 2.700000+6 1.669590-7 2.800000+6 1.596340-7 2.900000+6 1.525400-79852 5 18 1868 3.000000+6 1.456800-7 3.100000+6 1.390570-7 3.200000+6 1.326720-79852 5 18 1869 3.300000+6 1.265240-7 3.400000+6 1.206100-7 3.500000+6 1.149270-79852 5 18 1870 3.600000+6 1.094710-7 3.700000+6 1.042380-7 3.800000+6 9.922240-89852 5 18 1871 3.900000+6 9.441880-8 4.000000+6 8.982120-8 4.100000+6 8.542350-89852 5 18 1872 4.200000+6 8.121950-8 4.300000+6 7.720290-8 4.400000+6 7.336720-89852 5 18 1873 4.500000+6 6.970600-8 4.600000+6 6.621290-8 4.700000+6 6.288160-89852 5 18 1874 4.800000+6 5.970590-8 4.900000+6 5.667960-8 5.000000+6 5.379670-89852 5 18 1875 5.100000+6 5.105130-8 5.200000+6 4.843770-8 5.300000+6 4.595030-89852 5 18 1876 5.400000+6 4.358370-8 5.500000+6 4.133260-8 5.600000+6 3.919200-89852 5 18 1877 5.700000+6 3.715700-8 5.800000+6 3.522270-8 5.900000+6 3.338460-89852 5 18 1878 6.000000+6 3.163830-8 6.100000+6 2.997960-8 6.200000+6 2.840440-89852 5 18 1879 6.300000+6 2.690880-8 6.400000+6 2.548890-8 6.500000+6 2.414130-89852 5 18 1880 6.600000+6 2.286250-8 6.700000+6 2.164910-8 6.800000+6 2.049800-89852 5 18 1881 6.900000+6 1.940610-8 7.000000+6 1.837070-8 7.100000+6 1.738880-89852 5 18 1882 7.200000+6 1.645780-8 7.300000+6 1.557530-8 7.400000+6 1.473880-89852 5 18 1883 7.500000+6 1.394600-8 7.600000+6 1.319470-8 7.700000+6 1.248290-89852 5 18 1884 7.800000+6 1.180850-8 7.900000+6 1.116970-8 8.000000+6 1.056460-89852 5 18 1885 8.100000+6 9.991530-9 8.200000+6 9.448830-9 8.300000+6 8.934970-99852 5 18 1886 8.400000+6 8.448440-9 8.500000+6 7.987850-9 8.600000+6 7.551840-99852 5 18 1887 8.700000+6 7.139160-9 8.800000+6 6.748570-9 8.900000+6 6.378940-99852 5 18 1888 9.000000+6 6.029170-9 9.100000+6 5.698220-9 9.200000+6 5.385110-99852 5 18 1889 9.300000+6 5.088890-9 9.400000+6 4.808680-9 9.500000+6 4.543630-99852 5 18 1890 9.600000+6 4.292940-9 9.700000+6 4.055850-9 9.800000+6 3.831640-99852 5 18 1891 9.900000+6 3.619620-9 1.000000+7 3.419160-9 1.010000+7 3.229620-99852 5 18 1892 1.020000+7 3.050420-9 1.030000+7 2.881020-9 1.040000+7 2.720890-99852 5 18 1893 1.050000+7 2.569530-9 1.060000+7 2.426470-9 1.070000+7 2.291260-99852 5 18 1894 1.080000+7 2.163480-9 1.090000+7 2.042730-9 1.100000+7 1.928630-99852 5 18 1895 1.110000+7 1.820820-9 1.120000+7 1.718950-9 1.130000+7 1.622710-99852 5 18 1896 1.140000+7 1.531790-9 1.150000+7 1.445900-9 1.160000+7 1.364770-99852 5 18 1897 1.170000+7 1.288130-9 1.180000+7 1.215750-9 1.190000+7 1.147380-99852 5 18 1898 1.200000+7 1.082820-9 1.210000+7 1.021840-9 1.220000+7 9.64263-109852 5 18 1899 1.230000+7 9.09891-10 1.240000+7 8.58551-10 1.250000+7 8.10076-109852 5 18 1900 1.260000+7 7.64308-10 1.270000+7 7.21099-10 1.280000+7 6.80306-109852 5 18 1901 1.290000+7 6.41797-10 1.300000+7 6.05445-10 1.310000+7 5.71131-109852 5 18 1902 1.320000+7 5.38743-10 1.330000+7 5.08172-10 1.340000+7 4.79320-109852 5 18 1903 1.350000+7 4.52089-10 1.360000+7 4.26391-10 1.370000+7 4.02139-109852 5 18 1904 1.380000+7 3.79254-10 1.390000+7 3.57659-10 1.400000+7 3.37283-109852 5 18 1905 1.410000+7 3.18057-10 1.420000+7 2.99916-10 1.430000+7 2.82801-109852 5 18 1906 1.440000+7 2.66655-10 1.450000+7 2.51422-10 1.460000+7 2.37051-109852 5 18 1907 1.470000+7 2.23496-10 1.480000+7 2.10708-10 1.490000+7 1.98646-109852 5 18 1908 1.500000+7 1.87269-10 1.510000+7 1.76538-10 1.520000+7 1.66417-109852 5 18 1909 1.530000+7 1.56872-10 1.540000+7 1.47870-10 1.550000+7 1.39380-109852 5 18 1910 1.560000+7 1.31374-10 1.570000+7 1.23824-10 1.580000+7 1.16704-109852 5 18 1911 1.590000+7 1.09991-10 1.600000+7 1.03661-10 1.610000+7 9.76931-119852 5 18 1912 1.620000+7 9.20658-11 1.630000+7 8.67603-11 1.640000+7 8.17583-119852 5 18 1913 1.650000+7 7.70426-11 1.660000+7 7.25970-11 1.670000+7 6.84060-119852 5 18 1914 1.680000+7 6.44553-11 1.690000+7 6.07311-11 1.700000+7 5.72207-119852 5 18 1915 1.710000+7 5.39117-11 1.720000+7 5.07928-11 1.730000+7 4.78532-119852 5 18 1916 1.740000+7 4.50825-11 1.750000+7 4.24712-11 1.760000+7 4.00101-119852 5 18 1917 1.770000+7 3.76907-11 1.780000+7 3.55049-11 1.790000+7 3.34450-119852 5 18 1918 1.800000+7 3.15039-11 1.810000+7 2.96747-11 1.820000+7 2.79511-119852 5 18 1919 1.830000+7 2.63270-11 1.840000+7 2.47966-11 1.850000+7 2.33547-119852 5 18 1920 1.860000+7 2.19960-11 1.870000+7 2.07160-11 1.880000+7 1.95100-119852 5 18 1921 1.890000+7 1.83738-11 1.900000+7 1.73033-11 1.910000+7 1.62949-119852 5 18 1922 1.920000+7 1.53449-11 1.930000+7 1.44499-11 1.940000+7 1.36069-119852 5 18 1923 1.950000+7 1.28127-11 1.960000+7 1.20647-11 1.970000+7 1.13601-119852 5 18 1924 1.980000+7 1.06964-11 1.990000+7 1.00712-11 2.000000+7 9.48240-129852 5 18 1925 2.020000+7 0.000000+0 9852 5 18 1926 0.000000+0 6.500000+6 0 0 1 3529852 5 18 1927 352 2 9852 5 18 1928 0.000000+0 0.000000+0 1.000000-5 1.74429-12 1.200000-5 1.91078-129852 5 18 1929 1.400000-5 2.06387-12 1.600000-5 2.20637-12 1.800000-5 2.34021-129852 5 18 1930 2.200000-5 2.58720-12 2.500000-5 2.75797-12 2.900000-5 2.97042-129852 5 18 1931 3.400000-5 3.21632-12 4.000000-5 3.48859-12 4.600000-5 3.74109-129852 5 18 1932 5.400000-5 4.05337-12 6.300000-5 4.37814-12 7.400000-5 4.74499-129852 5 18 1933 8.600000-5 5.11527-12 1.000000-4 5.51594-12 1.200000-4 6.04241-129852 5 18 1934 1.400000-4 6.52655-12 1.600000-4 6.97718-12 1.800000-4 7.40041-129852 5 18 1935 2.200000-4 8.18147-12 2.500000-4 8.72148-12 2.900000-4 9.39332-129852 5 18 1936 3.400000-4 1.01709-11 4.000000-4 1.10319-11 4.600000-4 1.18304-119852 5 18 1937 5.400000-4 1.28179-11 6.300000-4 1.38449-11 7.400000-4 1.50050-119852 5 18 1938 8.600000-4 1.61760-11 1.000000-3 1.74430-11 1.200000-3 1.91079-119852 5 18 1939 1.400000-3 2.06388-11 1.600000-3 2.20639-11 1.800000-3 2.34023-119852 5 18 1940 2.200000-3 2.58722-11 2.500000-3 2.75799-11 2.900000-3 2.97045-119852 5 18 1941 3.400000-3 3.21634-11 4.000000-3 3.48862-11 4.600000-3 3.74113-119852 5 18 1942 5.400000-3 4.05341-11 6.300000-3 4.37819-11 7.400000-3 4.74505-119852 5 18 1943 8.600000-3 5.11534-11 1.000000-2 5.51602-11 1.200000-2 6.04250-119852 5 18 1944 1.400000-2 6.52666-11 1.600000-2 6.97730-11 1.800000-2 7.40056-119852 5 18 1945 2.200000-2 8.18164-11 2.500000-2 8.72167-11 2.900000-2 9.39355-119852 5 18 1946 3.400000-2 1.01712-10 4.000000-2 1.10322-10 4.600000-2 1.18308-109852 5 18 1947 5.400000-2 1.28183-10 6.300000-2 1.38454-10 7.400000-2 1.50056-109852 5 18 1948 8.600000-2 1.61766-10 1.000000-1 1.74438-10 1.200000-1 1.91088-109852 5 18 1949 1.400000-1 2.06400-10 1.600000-1 2.20651-10 1.800000-1 2.34037-109852 5 18 1950 2.200000-1 2.58739-10 2.500000-1 2.75819-10 2.900000-1 2.97068-109852 5 18 1951 3.400000-1 3.21661-10 4.000000-1 3.48893-10 4.600000-1 3.74149-109852 5 18 1952 5.400000-1 4.05384-10 6.300000-1 4.37869-10 7.400000-1 4.74564-109852 5 18 1953 8.600000-1 5.11603-10 1.000000+0 5.51682-10 1.200000+0 6.04347-109852 5 18 1954 1.400000+0 6.52779-10 1.600000+0 6.97860-10 1.800000+0 7.40202-109852 5 18 1955 2.200000+0 8.18344-10 2.500000+0 8.72372-10 2.900000+0 9.39593-109852 5 18 1956 3.400000+0 1.017400-9 4.000000+0 1.103550-9 4.600000+0 1.183460-99852 5 18 1957 5.400000+0 1.282280-9 6.300000+0 1.385070-9 7.400000+0 1.501180-99852 5 18 1958 8.600000+0 1.618390-9 1.000000+1 1.745230-9 1.200000+1 1.911910-99852 5 18 1959 1.400000+1 2.065200-9 1.600000+1 2.207890-9 1.800000+1 2.341930-99852 5 18 1960 2.200000+1 2.589310-9 2.500000+1 2.760380-9 2.900000+1 2.973230-99852 5 18 1961 3.400000+1 3.219630-9 4.000000+1 3.492510-9 4.600000+1 3.745630-99852 5 18 1962 5.400000+1 4.058730-9 6.300000+1 4.384440-9 7.400000+1 4.752440-99852 5 18 1963 8.600000+1 5.123980-9 1.000000+2 5.526140-9 1.200000+2 6.054750-99852 5 18 1964 1.400000+2 6.541040-9 1.600000+2 6.993840-9 1.800000+2 7.419270-99852 5 18 1965 2.200000+2 8.204730-9 2.500000+2 8.748070-9 2.900000+2 9.424380-99852 5 18 1966 3.400000+2 1.020760-8 4.000000+2 1.107540-8 4.600000+2 1.188070-89852 5 18 1967 5.400000+2 1.287740-8 6.300000+2 1.391480-8 7.400000+2 1.508770-89852 5 18 1968 8.600000+2 1.627260-8 1.000000+3 1.755600-8 1.200000+3 1.924440-89852 5 18 1969 1.400000+3 2.079890-8 1.600000+3 2.224750-8 1.800000+3 2.360950-89852 5 18 1970 2.200000+3 2.612670-8 2.500000+3 2.786970-8 2.900000+3 3.004130-89852 5 18 1971 3.400000+3 3.255880-8 4.000000+3 3.535140-8 4.600000+3 3.794580-89852 5 18 1972 5.400000+3 4.116020-8 6.300000+3 4.450980-8 7.400000+3 4.830110-89852 5 18 1973 8.600000+3 5.213560-8 1.000000+4 5.629300-8 1.200000+4 6.176770-89852 5 18 1974 1.400000+4 6.681300-8 1.600000+4 7.151720-8 1.800000+4 7.594200-89852 5 18 1975 2.200000+4 8.412100-8 2.500000+4 8.978410-8 2.900000+4 9.683630-89852 5 18 1976 3.400000+4 1.050040-7 4.000000+4 1.140490-7 4.600000+4 1.224350-79852 5 18 1977 5.400000+4 1.327930-7 6.300000+4 1.435430-7 7.400000+4 1.556460-79852 5 18 1978 8.600000+4 1.678070-7 1.000000+5 1.808880-7 2.000000+5 2.457210-79852 5 18 1979 3.000000+5 2.827110-7 4.000000+5 3.025790-7 5.000000+5 3.136440-79852 5 18 1980 6.000000+5 3.202440-7 7.000000+5 3.196140-7 8.000000+5 3.167530-79852 5 18 1981 9.000000+5 3.101540-7 1.000000+6 3.015330-7 1.100000+6 2.934570-79852 5 18 1982 1.200000+6 2.857200-7 1.300000+6 2.780250-7 1.400000+6 2.702100-79852 5 18 1983 1.500000+6 2.621980-7 1.600000+6 2.539980-7 1.700000+6 2.456470-79852 5 18 1984 1.800000+6 2.372000-7 1.900000+6 2.287120-7 2.000000+6 2.202380-79852 5 18 1985 2.100000+6 2.118230-7 2.200000+6 2.035070-7 2.300000+6 1.953230-79852 5 18 1986 2.400000+6 1.872990-7 2.500000+6 1.794560-7 2.600000+6 1.718100-79852 5 18 1987 2.700000+6 1.643760-7 2.800000+6 1.571630-7 2.900000+6 1.501760-79852 5 18 1988 3.000000+6 1.434210-7 3.100000+6 1.368990-7 3.200000+6 1.306120-79852 5 18 1989 3.300000+6 1.245570-7 3.400000+6 1.187340-7 3.500000+6 1.131380-79852 5 18 1990 3.600000+6 1.077660-7 3.700000+6 1.026140-7 3.800000+6 9.767540-89852 5 18 1991 3.900000+6 9.294580-8 4.000000+6 8.841920-8 4.100000+6 8.408950-89852 5 18 1992 4.200000+6 7.995060-8 4.300000+6 7.599620-8 4.400000+6 7.222000-89852 5 18 1993 4.500000+6 6.861560-8 4.600000+6 6.517680-8 4.700000+6 6.189740-89852 5 18 1994 4.800000+6 5.877110-8 4.900000+6 5.579200-8 5.000000+6 5.295400-89852 5 18 1995 5.100000+6 5.025150-8 5.200000+6 4.767880-8 5.300000+6 4.523030-89852 5 18 1996 5.400000+6 4.290070-8 5.500000+6 4.068490-8 5.600000+6 3.857780-89852 5 18 1997 5.700000+6 3.657470-8 5.800000+6 3.467070-8 5.900000+6 3.286150-89852 5 18 1998 6.000000+6 3.114270-8 6.100000+6 2.951000-8 6.200000+6 2.795960-89852 5 18 1999 6.300000+6 2.648750-8 6.400000+6 2.509000-8 6.500000+6 2.376360-89852 5 18 2000 6.600000+6 2.250490-8 6.700000+6 2.131060-8 6.800000+6 2.017760-89852 5 18 2001 6.900000+6 1.910300-8 7.000000+6 1.808380-8 7.100000+6 1.711740-89852 5 18 2002 7.200000+6 1.620110-8 7.300000+6 1.533250-8 7.400000+6 1.450920-89852 5 18 2003 7.500000+6 1.372890-8 7.600000+6 1.298950-8 7.700000+6 1.228890-89852 5 18 2004 7.800000+6 1.162520-8 7.900000+6 1.099640-8 8.000000+6 1.040080-89852 5 18 2005 8.100000+6 9.836790-9 8.200000+6 9.302640-9 8.300000+6 8.796870-99852 5 18 2006 8.400000+6 8.318000-9 8.500000+6 7.864650-9 8.600000+6 7.435510-99852 5 18 2007 8.700000+6 7.029310-9 8.800000+6 6.644860-9 8.900000+6 6.281040-99852 5 18 2008 9.000000+6 5.936750-9 9.100000+6 5.611000-9 9.200000+6 5.302790-99852 5 18 2009 9.300000+6 5.011210-9 9.400000+6 4.735380-9 9.500000+6 4.474480-99852 5 18 2010 9.600000+6 4.227700-9 9.700000+6 3.994320-9 9.800000+6 3.773610-99852 5 18 2011 9.900000+6 3.564900-9 1.000000+7 3.367550-9 1.010000+7 3.180960-99852 5 18 2012 1.020000+7 3.004550-9 1.030000+7 2.837780-9 1.040000+7 2.680130-99852 5 18 2013 1.050000+7 2.531110-9 1.060000+7 2.390260-9 1.070000+7 2.257140-99852 5 18 2014 1.080000+7 2.131330-9 1.090000+7 2.012440-9 1.100000+7 1.900100-99852 5 18 2015 1.110000+7 1.793940-9 1.120000+7 1.693640-9 1.130000+7 1.598870-99852 5 18 2016 1.140000+7 1.509340-9 1.150000+7 1.424760-9 1.160000+7 1.344860-99852 5 18 2017 1.170000+7 1.269390-9 1.180000+7 1.198110-9 1.190000+7 1.130780-99852 5 18 2018 1.200000+7 1.067190-9 1.210000+7 1.007140-9 1.220000+7 9.50424-109852 5 18 2019 1.230000+7 8.96870-10 1.240000+7 8.46300-10 1.250000+7 7.98551-109852 5 18 2020 1.260000+7 7.53467-10 1.270000+7 7.10902-10 1.280000+7 6.70716-109852 5 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1.939139-3 4.153000+4 6.954615-5 0.000000+0 0.000000+09852 6 16 1964 2.750000+4 3.814917-7 1.100000+5 5.205986-7 2.200000+5 5.261396-79852 6 16 1965 3.300000+5 2.888638-7 4.400000+5 2.947418-7 5.500000+5 5.195236-79852 6 16 1966 6.600000+5 4.504837-7 7.700000+5 5.857336-7 8.800000+5 5.131016-79852 6 16 1967 9.900000+5 4.083197-7 1.100000+6 3.719397-7 1.210000+6 3.361398-79852 6 16 1968 1.320000+6 3.015598-7 1.430000+6 2.686438-7 1.540000+6 2.377228-79852 6 16 1969 1.650000+6 2.090259-7 1.760000+6 1.826889-7 1.870000+6 1.587609-79852 6 16 1970 1.980000+6 1.372219-7 2.090000+6 1.179909-7 2.200000+6 1.009499-79852 6 16 1971 2.310000+6 8.594944-8 2.420000+6 7.282585-8 2.530000+6 6.140886-89852 6 16 1972 2.640000+6 5.152856-8 2.750000+6 4.302047-8 2.860000+6 3.572978-89852 6 16 1973 2.970000+6 2.951128-8 3.080000+6 2.423618-8 3.190000+6 1.977639-89852 6 16 1974 3.300000+6 1.603729-8 3.410000+6 1.292299-8 3.520000+6 1.033479-89852 6 16 1975 3.630000+6 8.199894-9 3.740000+6 6.430186-9 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