JENDL-3.3 Tc- 99 0 0 0 0 4.309900+4 9.805660+1 1 0 0 34331 1451 1 0.000000+0 0.000000+0 0 0 0 64331 1451 2 1.000000+0 2.000000+7 3 0 10 34331 1451 3 0.000000+0 0.000000+0 0 0 235 654331 1451 4 43-Tc- 99 JNDC EVAL-Mar90 JNDC FP ND W.G., T.Nakagawa 4331 1451 5 DIST-MAR02 Rev3-Feb02 20020214 4331 1451 6 ----JENDL-3.3 MATERIAL 4331 4331 1451 7 -----INCIDENT NEUTRON DATA 4331 1451 8 ------ENDF-6 FORMAT 4331 1451 9 4331 1451 10 HISTORY 4331 1451 11 84-10 Evaluation for JENDL-2 was made by JNDC FPND W.G.[1]. 4331 1451 12 90-03 Modification for JENDL-3 was made[2]. 4331 1451 13 93-11 JENDL-3.2 was made by JNDC FPND W.G.[3]. 4331 1451 14 ***** Modified parts for JENDL-3.2 ******************** 4331 1451 15 (2,151) Resolved resonance parameters 4331 1451 16 *********************************************************** 4331 1451 17 4331 1451 18 02-02 Modification was made by T.Nakagawa 4331 1451 19 4331 1451 20 ***** Modified parts ************************************** 4331 1451 21 (2,151) RRP and URP 4331 1451 22 (3,1),(3,2),(3,4),(3,22),(3,51-91),(3,102) 4331 1451 23 All of MF04 and MF05 4331 1451 24 *********************************************************** 4331 1451 25 4331 1451 26 4331 1451 27 MF = 1 General information 4331 1451 28 MT=451 Comments and dictionary 4331 1451 29 4331 1451 30 MF = 2 Resonance parameters 4331 1451 31 MT=151 Resolved and unresolved resonance parameters 4331 1451 32 Resolved resonance region (MLBW formula) : below 6.0 keV 4331 1451 33 Resonance parameters obtained by Gunsing et al.[4] were 4331 1451 34 adopted. They analyzed transmission data with REFIT code, 4331 1451 35 and obtaind the parameters up to 10 keV. However the upper 4331 1451 36 boundary was set to 6 keV in this file, because the capture 4331 1451 37 cross section calculated from their parameters were smaller 4331 1451 38 than experimental data above 6 keV. The scattering radius 4331 1451 39 of 6.7 fm was adopted. 4331 1451 40 4331 1451 41 Unresolved resonance region : 6.0 keV - 100 keV 4331 1451 42 Unresolved resonance parameters were adjusted with ASREP [5] 4331 1451 43 to reproduce the capture and total cross sections calculated 4331 1451 44 with CASTHY. The CASTHY calculation reproduces well the 4331 1451 45 measured capture cross sections [6,7,8]. 4331 1451 46 4331 1451 47 Calculated 2200-m/s cross sections and res. integrals (barns) 4331 1451 48 2200 m/s res. integ. 4331 1451 49 total 27.33 - 4331 1451 50 elastic 4.56 - 4331 1451 51 capture 22.76 324 4331 1451 52 4331 1451 53 4331 1451 54 MF = 3 Neutron cross sections 4331 1451 55 Below 100 keV, resonance parameters were given. 4331 1451 56 Above 100 keV, the spherical optical and statistical model 4331 1451 57 calculation was performed with CASTHY[9], by taking account of 4331 1451 58 competing reactions, of which cross sections were calculated 4331 1451 59 with PEGASUS[10] standing on a preequilibrium and multi-step 4331 1451 60 evaporation model. The OMP's for neutron given in Table 1 were 4331 1451 61 determined to reproduce the total cross section measured by 4331 1451 62 Foster and Glasgow[11] in the MeV region, and total cross 4331 1451 63 section of about 8 - 9 b in the 10-100 keV region. The OMP's 4331 1451 64 for charged particles are as follows: 4331 1451 65 Proton = Perey[12] 4331 1451 66 Alpha = Huizenga and Igo[13] 4331 1451 67 Deuteron = Lohr and Haeberli[14] 4331 1451 68 Helium-3 and triton = Becchetti and Greenlees[15] 4331 1451 69 4331 1451 70 Parameters for the composite level density formula of Gilbert 4331 1451 71 and Cameron[16] were evaluated by Iijima et al.[17] More 4331 1451 72 extensive determination and modification were made in the 4331 1451 73 previous work[2]. Table 2 shows the level density parameters 4331 1451 74 used in the calculation. Energy dependence of spin cut-off 4331 1451 75 parameter in the energy range below E-joint is due to Gruppelaar4331 1451 76 [18]. 4331 1451 77 4331 1451 78 MT = 1 Total 4331 1451 79 Spherical optical model calculation was adopted. 4331 1451 80 4331 1451 81 MT = 2 Elastic scattering 4331 1451 82 Calculated as (total - sum of partial cross sections). 4331 1451 83 4331 1451 84 MT = 4, 51 - 91 Inelastic scattering 4331 1451 85 4331 1451 86 The level scheme was taken from Ref.[19] 4331 1451 87 4331 1451 88 No. Energy(MeV) Spin-parity 4331 1451 89 GR. 0.0 9/2 + 4331 1451 90 1 0.1405 7/2 + * 4331 1451 91 2 0.1427 1/2 - 4331 1451 92 3 0.1811 5/2 + * 4331 1451 93 4 0.5091 3/2 - 4331 1451 94 5 0.5344 3/2 - 4331 1451 95 6 0.5369 5/2 + 4331 1451 96 7 0.6125 5/2 - * 4331 1451 97 8 0.6254 9/2 + * 4331 1451 98 9 0.6715 3/2 - 4331 1451 99 10 0.7198 7/2 + * 4331 1451 100 11 0.7267 11/2 + * 4331 1451 101 12 0.7617 5/2 + * 4331 1451 102 13 0.7619 13/2 + * 4331 1451 103 14 0.9206 1/2 + 4331 1451 104 15 0.9861 7/2 - * 4331 1451 105 16 1.0041 3/2 - 4331 1451 106 4331 1451 107 Levels above 1.0175 MeV were assumed to be overlapping. 4331 1451 108 The compound inelastic scattering was calculated with CASTHY. 4331 1451 109 For the levels with "*", direct inelastic scattering was 4331 1451 110 calculated with DWUCK [20,21]. Deformation parameters were 4331 1451 111 based on the recommendation by Raman et al.[22] 4331 1451 112 4331 1451 113 MT = 102 Capture 4331 1451 114 Spherical optical and statistical model calculation with 4331 1451 115 CASTHY was adopted. Direct and semi-direct capture cross 4331 1451 116 sections were estimated according to the procedure of Benzi 4331 1451 117 and Reffo[23] and normalized to 9 mb at 14.7 MeV [24]. 4331 1451 118 4331 1451 119 The gamma-ray strength function (8.01E-03) was adjusted to 4331 1451 120 reproduce the capture cross section of 630 mb at 50 keV. 4331 1451 121 4331 1451 122 MT = 16 (n,2n) Cross Section 4331 1451 123 MT = 17 (n,3n) Cross Section 4331 1451 124 MT = 22 (n,n'a) Cross Section 4331 1451 125 MT = 28 (n,n'p) Cross Section 4331 1451 126 MT = 32 (n,n'd) Cross Section 4331 1451 127 MT = 33 (n,n't) Cross Section 4331 1451 128 MT =103 (n,p) Cross Section 4331 1451 129 MT =104 (n,d) Cross Section 4331 1451 130 MT =105 (n,t) Cross Section 4331 1451 131 MT =106 (n,He3) Cross Section 4331 1451 132 MT =107 (n,alpha) Cross Section 4331 1451 133 These reaction cross sections were calculated with the 4331 1451 134 preequilibrium and multi-step evaporation model code PEGASUS. 4331 1451 135 4331 1451 136 The Kalbach's constant K (= 101.5) was estimated by the 4331 1451 137 formula derived from Kikuchi-Kawai's formalism[25] and level 4331 1451 138 density parameters. 4331 1451 139 4331 1451 140 Finally, the (n,2n) and (n,p) cross sections were normalized 4331 1451 141 to the following values at 14.5 MeV: 4331 1451 142 (n,2n) 1230.00 mb (recommended by Bychkov et al.[26]) 4331 1451 143 (n,p) 14.00 mb (recommended by Forrest[27]) 4331 1451 144 The (n,alpha) and (n,n'alpha) cross section was normalized to 4331 1451 145 the data of Ikdeda et al. [28] 4331 1451 146 4331 1451 147 MF = 4 Angular Distributions of Secondary Neutrons 4331 1451 148 Legendre polynomial coefficients for angular distributions are 4331 1451 149 given in the center-of-mass system for MT=2 and discrete inelas-4331 1451 150 tic levels, and in the laboratory system for MT=91. They were 4331 1451 151 calculated with CASTHY. Those of direct inelastic scttering 4331 1451 152 were calculated with DWUCK, and added to the rusults of CASTHY 4331 1451 153 calculation. 4331 1451 154 4331 1451 155 For other reactions, isotropic distributions in the laboratory 4331 1451 156 system were assumed. 4331 1451 157 4331 1451 158 MF = 5 Energy Distributions of Secondary Neutrons 4331 1451 159 Energy distributions of secondary neutrons were calculated with 4331 1451 160 PEGASUS for inelastic scattering to overlapping levels and for 4331 1451 161 other neutron emitting reactions. 4331 1451 162 4331 1451 163 Interpolation of 22 (unit base interpolation) was adopted. 4331 1451 164 4331 1451 165 4331 1451 166 Table 1 Neutron Optical Potential Parameters 4331 1451 167 4331 1451 168 Depth (MeV) Radius(fm) Diffuseness(fm) 4331 1451 169 ---------------------- ------------ --------------- 4331 1451 170 V = 45.5-0.48*En r0 = 1.350 a0 = 0.60 4331 1451 171 Ws = 6.79+0.83*En rs = 1.330 as = 0.40 4331 1451 172 Vso= 7.0 rso= 1.350 aso= 0.60 4331 1451 173 The form of surface absorption part is der. Woods-Saxon type. 4331 1451 174 4331 1451 175 Table 2 Level Density Parameters 4331 1451 176 4331 1451 177 Nuclide a(1/MeV) T(MeV) C(1/MeV) EX(MeV) Pairing 4331 1451 178 --------------------------------------------------------------- 4331 1451 179 41-Nb- 95 1.277E+01 7.500E-01 2.121E+00 5.782E+00 1.120E+00 4331 1451 180 41-Nb- 96 1.331E+01 5.880E-01 3.406E+00 2.530E+00 0.0 4331 1451 181 41-Nb- 97 1.337E+01 6.710E-01 9.771E-01 5.026E+00 1.290E+00 4331 1451 182 41-Nb- 98 1.380E+01 5.110E-01 2.350E+00 1.731E+00 0.0 4331 1451 183 4331 1451 184 42-Mo- 96 1.403E+01 7.410E-01 6.991E-01 7.645E+00 2.400E+00 4331 1451 185 42-Mo- 97 1.517E+01 6.800E-01 2.769E+00 6.036E+00 1.280E+00 4331 1451 186 42-Mo- 98 1.594E+01 6.900E-01 7.358E-01 7.888E+00 2.570E+00 4331 1451 187 42-Mo- 99 1.774E+01 6.200E-01 4.294E+00 6.058E+00 1.280E+00 4331 1451 188 4331 1451 189 43-Tc- 97 1.600E+01 6.700E-01 4.756E+00 6.089E+00 1.120E+00 4331 1451 190 43-Tc- 98 1.659E+01 6.120E-01 1.776E+01 4.176E+00 0.0 4331 1451 191 43-Tc- 99 1.600E+01 6.550E-01 2.973E+00 5.984E+00 1.290E+00 4331 1451 192 43-Tc-100 1.637E+01 5.850E-01 1.189E+01 3.635E+00 0.0 4331 1451 193 --------------------------------------------------------------- 4331 1451 194 4331 1451 195 Spin cutoff parameters were calculated as 0.146*SQRT(a)*A**(2/3).4331 1451 196 In the CASTHY calculation, spin cutoff factors at 0 MeV were 4331 1451 197 assumed to be 7.899 for Tc- 99 and 5.0 for Tc-100. 4331 1451 198 4331 1451 199 References 4331 1451 200 1) Aoki T. et al.: Proc. Int. Conf. on Nuclear Data for Basic 4331 1451 201 and Applied Science, Santa Fe., Vol. 2, p.1627 (1985). 4331 1451 202 2) Kawai M. et al.: J. Nucl. Sci. Technol., 29, 195 (1992). 4331 1451 203 3) Kawai M., et al.: J. Nucl. Sci. Technol., 38, 261 (2001). 4331 1451 204 4) Gunsing F., et al.: Phys. Rev., C61, 054608 (2000). 4331 1451 205 5) Kikuchi Y., et al.: JAERI-Data]Code 99-025 (1999). 4331 1451 206 [in Japanese] 4331 1451 207 6) Macklin R.L.: Nucl. Sci. Eng., 81, 520 (1982). 4331 1451 208 7) Kobayashi K., et al.: "Proc. Int. Conf. Nucl. Data for Sci. 4331 1451 209 Technol.," Tsukuba, Japan, 7-12 Oct. 2001, #151 (2002). 4331 1451 210 8) Chou J-C., Werle H.: J. Nucl. Energy, 27, 811 (1973). 4331 1451 211 9) Igarasi S. and Fukahori, T.: JAERI 1321 (1991). 4331 1451 212 10) Nakagawa T., et al.: JAERI-Data/Code 99-031 (1999). 4331 1451 213 11) Foster D.G. Jr., Glasgow D.W.: Phys. Rev., C3, 576 (1971). 4331 1451 214 12) Perey F.G: Phys. Rev. 131, 745 (1963). 4331 1451 215 13) Huizenga J.R. and Igo G.: Nucl. Phys. 29, 462 (1962). 4331 1451 216 14) Lohr, J.M. and Haeberli W.: Nucl. Phys. A232, 381 (1974). 4331 1451 217 15) Becchetti F.D., Jr. and Greenlees G.W.: Polarization 4331 1451 218 Phenomena in Nuclear Reactions ((eds) H.H. Barshall and 4331 1451 219 W. Haeberli), p. 682, The university of Wisconsin Press. 4331 1451 220 (1971). 4331 1451 221 16) Gilbert A. and Cameron A.G.W.: Can. J. Phys., 43, 1446 4331 1451 222 (1965). 4331 1451 223 17) Iijima S., et al.: J. Nucl. Sci. Technol. 21, 10 (1984). 4331 1451 224 18) Gruppelaar H.: ECN-13 (1977). 4331 1451 225 19) Firestone R.B.: "Table of Isotopes, 8th Ed.", Wiley- 4331 1451 226 Interscience Publication (1998). 4331 1451 227 20) Kunz P.D.: private communication. 4331 1451 228 21) Yamamuro N.: JAERI-M 88-140 (1988) [in Japanese] 4331 1451 229 22) Raman S., et al.: Atom. Data and Nucl. Data Tables 36, 1 4331 1451 230 (1987) 4331 1451 231 23) Benzi V. and Reffo, G.: CCDN-NW/10 (1969). 4331 1451 232 24) Qaim S.: J. Inorg. Nucl. Chem., 35, 3669 (1973). 4331 1451 233 25) Kikuchi K. and Kawai, M.: "Nuclear Matter and Nuclear 4331 1451 234 Reactions", North Holland (1968). 4331 1451 235 26) Bychkov V.M. et al.: INDC(CCP)-146/LJ (1980). 4331 1451 236 27) Forrest R.A.: AERE-R 12419 (1986). 4331 1451 237 28) Ikeda Y., et al.: Nucl. Sci. Eng., 116, 28 (1994). 4331 1451 238 4331 1451 239 1 451 304 34331 1451 240 2 151 815 34331 1451 241 3 1 78 34331 1451 242 3 2 78 34331 1451 243 3 4 19 34331 1451 244 3 16 9 24331 1451 245 3 17 5 24331 1451 246 3 22 13 34331 1451 247 3 28 11 24331 1451 248 3 32 7 24331 1451 249 3 33 7 24331 1451 250 3 51 19 34331 1451 251 3 52 18 34331 1451 252 3 53 18 34331 1451 253 3 54 15 34331 1451 254 3 55 15 34331 1451 255 3 56 15 34331 1451 256 3 57 14 34331 1451 257 3 58 14 34331 1451 258 3 59 14 34331 1451 259 3 60 13 34331 1451 260 3 61 13 34331 1451 261 3 62 12 34331 1451 262 3 63 12 34331 1451 263 3 64 11 34331 1451 264 3 65 11 34331 1451 265 3 66 10 34331 1451 266 3 91 10 34331 1451 267 3 102 23 34331 1451 268 3 103 14 24331 1451 269 3 104 12 24331 1451 270 3 105 11 24331 1451 271 3 106 10 24331 1451 272 3 107 15 24331 1451 273 4 2 187 34331 1451 274 4 16 2 34331 1451 275 4 17 2 34331 1451 276 4 22 2 34331 1451 277 4 28 2 34331 1451 278 4 32 2 34331 1451 279 4 33 2 34331 1451 280 4 51 96 34331 1451 281 4 52 26 34331 1451 282 4 53 91 34331 1451 283 4 54 26 34331 1451 284 4 55 27 34331 1451 285 4 56 27 34331 1451 286 4 57 81 34331 1451 287 4 58 81 34331 1451 288 4 59 26 34331 1451 289 4 60 81 34331 1451 290 4 61 81 34331 1451 291 4 62 81 34331 1451 292 4 63 76 34331 1451 293 4 64 27 34331 1451 294 4 65 71 34331 1451 295 4 66 24 34331 1451 296 4 91 24 34331 1451 297 5 16 55 34331 1451 298 5 17 27 34331 1451 299 5 22 189 34331 1451 300 5 28 112 34331 1451 301 5 32 56 34331 1451 302 5 33 49 34331 1451 303 5 91 137 34331 1451 304 4331 1 099999 4331 0 0 0 4.309900+4 9.805660+1 0 0 1 04331 2151 1 4.309900+4 1.000000+0 0 0 2 04331 2151 2 1.000000-5 6.000000+3 1 2 0 04331 2151 3 4.500000+0 6.700000-1 0 0 2 04331 2151 4 9.805660+1 0.000000+0 0 0 3108 5184331 2151 5 -1.500000+1 5.000000+0 1.630000-1 1.300000-2 1.500000-1 0.000000+04331 2151 6 5.580000+0 5.000000+0 1.504500-1 3.450000-3 1.470000-1 0.000000+04331 2151 7 2.027000+1 4.000000+0 1.633700-1 8.370000-3 1.550000-1 0.000000+04331 2151 8 3.984000+1 5.000000+0 1.240800-1 1.080000-3 1.230000-1 0.000000+04331 2151 9 5.668000+1 4.000000+0 1.449000-1 3.900000-3 1.410000-1 0.000000+04331 2151 10 1.112200+2 5.000000+0 1.439400-1 9.940000-3 1.340000-1 0.000000+04331 2151 11 1.237700+2 4.000000+0 1.491100-1 4.110000-3 1.450000-1 0.000000+04331 2151 12 1.630100+2 5.000000+0 2.018000-1 5.780000-2 1.440000-1 0.000000+04331 2151 13 1.820900+2 4.000000+0 2.273000-1 6.730000-2 1.600000-1 0.000000+04331 2151 14 1.917100+2 5.000000+0 1.854000-1 3.640000-2 1.490000-1 0.000000+04331 2151 15 2.064100+2 4.000000+0 1.476900-1 6.900000-4 1.470000-1 0.000000+04331 2151 16 2.148300+2 4.000000+0 1.481900-1 1.190000-3 1.470000-1 0.000000+04331 2151 17 2.206200+2 5.000000+0 1.474890-1 4.890000-4 1.470000-1 0.000000+04331 2151 18 2.412100+2 4.000000+0 1.849000-1 3.790000-2 1.470000-1 0.000000+04331 2151 19 2.731700+2 4.000000+0 1.477910-1 7.910000-4 1.470000-1 0.000000+04331 2151 20 2.799800+2 4.000000+0 1.620000-1 1.500000-2 1.470000-1 0.000000+04331 2151 21 2.999800+2 4.000000+0 1.839000-1 3.690000-2 1.470000-1 0.000000+04331 2151 22 3.068100+2 5.000000+0 1.613000-1 1.430000-2 1.470000-1 0.000000+04331 2151 23 3.432100+2 5.000000+0 1.486200-1 1.620000-3 1.470000-1 0.000000+04331 2151 24 3.586500+2 4.000000+0 1.666000-1 1.960000-2 1.470000-1 0.000000+04331 2151 25 3.614500+2 5.000000+0 1.480300-1 1.030000-3 1.470000-1 0.000000+04331 2151 26 3.626900+2 4.000000+0 1.489700-1 1.970000-3 1.470000-1 0.000000+04331 2151 27 3.649300+2 5.000000+0 2.890000-1 1.420000-1 1.470000-1 0.000000+04331 2151 28 3.798400+2 5.000000+0 1.679000-1 2.090000-2 1.470000-1 0.000000+04331 2151 29 4.168200+2 4.000000+0 2.114000-1 6.440000-2 1.470000-1 0.000000+04331 2151 30 4.265400+2 5.000000+0 2.079000-1 6.090000-2 1.470000-1 0.000000+04331 2151 31 4.477000+2 5.000000+0 1.492200-1 2.220000-3 1.470000-1 0.000000+04331 2151 32 4.599200+2 4.000000+0 1.888000-1 4.180000-2 1.470000-1 0.000000+04331 2151 33 4.787700+2 4.000000+0 1.597000-1 1.270000-2 1.470000-1 0.000000+04331 2151 34 4.865800+2 5.000000+0 1.523500-1 5.350000-3 1.470000-1 0.000000+04331 2151 35 5.164500+2 4.000000+0 1.602000-1 1.320000-2 1.470000-1 0.000000+04331 2151 36 5.205600+2 5.000000+0 1.765000-1 2.950000-2 1.470000-1 0.000000+04331 2151 37 5.366100+2 4.000000+0 1.775000-1 3.050000-2 1.470000-1 0.000000+04331 2151 38 5.632300+2 5.000000+0 1.549700-1 7.970000-3 1.470000-1 0.000000+04331 2151 39 5.937500+2 4.000000+0 1.532000-1 6.200000-3 1.470000-1 0.000000+04331 2151 40 5.981700+2 5.000000+0 1.731000-1 2.610000-2 1.470000-1 0.000000+04331 2151 41 5.995400+2 5.000000+0 1.502600-1 3.260000-3 1.470000-1 0.000000+04331 2151 42 6.067600+2 4.000000+0 1.846000-1 3.760000-2 1.470000-1 0.000000+04331 2151 43 6.234900+2 4.000000+0 1.524900-1 5.490000-3 1.470000-1 0.000000+04331 2151 44 6.325600+2 5.000000+0 1.493900-1 2.390000-3 1.470000-1 0.000000+04331 2151 45 6.547100+2 4.000000+0 1.935000-1 4.650000-2 1.470000-1 0.000000+04331 2151 46 6.722400+2 5.000000+0 1.685000-1 2.150000-2 1.470000-1 0.000000+04331 2151 47 6.862300+2 5.000000+0 1.522100-1 5.210000-3 1.470000-1 0.000000+04331 2151 48 7.240900+2 5.000000+0 1.552700-1 8.270000-3 1.470000-1 0.000000+04331 2151 49 7.453700+2 4.000000+0 2.620000-1 1.150000-1 1.470000-1 0.000000+04331 2151 50 7.536000+2 4.000000+0 2.100000-1 6.300000-2 1.470000-1 0.000000+04331 2151 51 7.660900+2 4.000000+0 1.579000-1 1.090000-2 1.470000-1 0.000000+04331 2151 52 7.745100+2 5.000000+0 1.498900-1 2.890000-3 1.470000-1 0.000000+04331 2151 53 7.986400+2 4.000000+0 1.518200-1 4.820000-3 1.470000-1 0.000000+04331 2151 54 8.055900+2 5.000000+0 1.744000-1 2.740000-2 1.470000-1 0.000000+04331 2151 55 8.159100+2 5.000000+0 1.716000-1 2.460000-2 1.470000-1 0.000000+04331 2151 56 8.280400+2 4.000000+0 1.509600-1 3.960000-3 1.470000-1 0.000000+04331 2151 57 8.387100+2 4.000000+0 2.660000-1 1.190000-1 1.470000-1 0.000000+04331 2151 58 8.472900+2 4.000000+0 2.077000-1 6.070000-2 1.470000-1 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