JENDL-4.0 Ru-100 0 0 0 0 4.410000+4 9.904600+1 1 0 6 14437 1451 1 0.000000+0 0.000000+0 0 0 0 64437 1451 2 1.000000+0 2.000000+7 0 0 10 44437 1451 3 0.000000+0 0.000000+0 0 0 265 614437 1451 4 44-Ru-100 JNDC EVAL-MAR90 JNDC FP NUCLEAR DATA W.G. 4437 1451 5 DIST-MAY10 20091208 4437 1451 6 ----JENDL-4.0 MATERIAL 4437 4437 1451 7 -----INCIDENT NEUTRON DATA 4437 1451 8 ------ENDF-6 FORMAT 4437 1451 9 4437 1451 10 =========================================================== 4437 1451 11 JENDL-3.2 data were automatically transformed to JENDL-3.3. 4437 1451 12 Interpolation of spectra: 22 (unit base interpolation) 4437 1451 13 (3,251) deleted, T-matrix of (4,2) deleted, and others. 4437 1451 14 =========================================================== 4437 1451 15 4437 1451 16 History 4437 1451 17 84-10 Evaluation for JENDL-2 was made by JNDC FPND W.G./1/ 4437 1451 18 90-03 Modification for JENDL-3 was made/2/. 4437 1451 19 09-12 JENDL-4.0. 4437 1451 20 Compiled by A.Ichihara (jaea/ndc). 4437 1451 21 ***** modified parts for JENDL-4.0 ******************* 4437 1451 22 (2,151) Resolved resonance parameters were revised 4437 1451 23 by T.Nakagawa. 4437 1451 24 ********************************************************** 4437 1451 25 4437 1451 26 mf = 1 General information 4437 1451 27 mt=451 Comments and dictionary 4437 1451 28 4437 1451 29 mf = 2 Resonance parameters 4437 1451 30 mt=151 Resolved and unresolved resonance parameters 4437 1451 31 Resolved resonance region (MLBW; below 11.89 keV) 4437 1451 32 4437 1451 33 The data of JENDL-3.3 was adopted, and capture width of a 4437 1451 34 negative resonance was adjusted to repruduce the measured 4437 1451 35 thermal cross section of 5.8 +- 0.4/3/ 4437 1451 36 4437 1451 37 ** comments to JENDL-3.3 ** 4437 1451 38 Resonance parameters were taken from JENDL-2 except for those 4437 1451 39 of negative and hypothetical resonances, angular momentum for 4437 1451 40 some levels and scattering radius. 4437 1451 41 For JENDL-2, the 228.5-eV resonance was adopted from 4437 1451 42 Priesmeyer and Jung/4/. Resonances above 2679.7 eV were 4437 1451 43 mainly based on the experimental data of Macklin and Halperin 4437 1451 44 /5/. Resonances at 120 eV and between 336 and 2497 eV were 4437 1451 45 hypothetical levels generated by assuming S0=0.43e-4, D0=340 4437 1451 46 eV, S1=4.1e-4, D1=110 eV. The average radiation width of 4437 1451 47 0.124+-0.017 eV was deduced and adopted to the levels whose 4437 1451 48 radiation width was unknown. Two negative resonances were 4437 1451 49 added, and parameters of the 120-eV level were adjusted so as 4437 1451 50 to reproduce the capture cross section of 5.0+-0.6 barns at 4437 1451 51 0.0253 eV and the capture resonance integral of 11.2+-1.1 4437 1451 52 barns/6/. 4437 1451 53 For JENDL-3, the reduced neutron width was decreased from 4437 1451 54 43 meV to 23 meV. Scattering radius was changed to 6.1 fm 4437 1451 55 according to the systematics of measured values. Number of 4437 1451 56 negative resonances was reduced to one and its parameters were4437 1451 57 reevaluated. Neutron orbital angular momentum l of some 4437 1451 58 resonances was estimated with a method of Bollinger and Thomas4437 1451 59 /7/. 4437 1451 60 4437 1451 61 Unresolved resonance region : 11.89 keV - 100 keV 4437 1451 62 Unresolved resonance parameters were adopted from JENDL-2. 4437 1451 63 The neutron strength functions, S0, S1 and S2 were calculated 4437 1451 64 with optical model code CASTHY/8/. The observed level spacing4437 1451 65 was determined to reproduce the capture cross section 4437 1451 66 calculated with CASTHY. The effective scattering radius was 4437 1451 67 obtained from fitting to the calculated total cross section at4437 1451 68 100 keV. 4437 1451 69 4437 1451 70 Typical values of the parameters at 70 keV: 4437 1451 71 S0 = 0.450e-4, S1 = 6.500e-4, S2 = 0.530e-4, Sg = 3.91e-4, 4437 1451 72 Gg = 0.125 eV, R = 4.971 fm. 4437 1451 73 4437 1451 74 The unresolved resonance parameters were calculated using 4437 1451 75 the ASREP code/9/. 4437 1451 76 The parameters should be used only for self-shielding 4437 1451 77 calculation. 4437 1451 78 4437 1451 79 Thermal cross sections and resonance integrals at 300K (b) 4437 1451 80 ------------------------------------------------------- 4437 1451 81 0.0253 eV reson. integ.(*) 4437 1451 82 ------------------------------------------------------- 4437 1451 83 total 12.341 4437 1451 84 elastic 6.498 4437 1451 85 capture 5.842 11.5 4437 1451 86 ------------------------------------------------------- 4437 1451 87 (*) In the energy range from 0.5 eV to 10 MeV. 4437 1451 88 4437 1451 89 mf = 3 Neutron cross sections 4437 1451 90 Below 100 keV, resonance parameters were given. 4437 1451 91 Above 100 keV, the spherical optical and statistical model 4437 1451 92 calculation was performed with CASTHY, by taking account of 4437 1451 93 competing reactions, of which cross sections were calculated 4437 1451 94 with PEGASUS/10/ standing on a preequilibrium and multi-step 4437 1451 95 evaporation model. The OMP's for neutron given in Table 1 were 4437 1451 96 determined to reproduce a systematic trend of the total cross 4437 1451 97 section by changing rso of Iijima-Kawai potential/11/. The 4437 1451 98 OMP's for charged particles are as follows: 4437 1451 99 proton = Perey/12/ 4437 1451 100 alpha = Huizenga and Igo/13/ 4437 1451 101 deuteron = Lohr and Haeberli/14/ 4437 1451 102 helium-3 and triton = Becchetti and Greenlees/15/ 4437 1451 103 Parameters for the composite level density formula of Gilbert 4437 1451 104 and Cameron/16/ were evaluated by Iijima et al./17/ More 4437 1451 105 extensive determination and modification were made in the 4437 1451 106 present work. Table 2 shows the level density parameters used 4437 1451 107 in the present calculation. Energy dependence of spin cut-off 4437 1451 108 parameter in the energy range below E-joint is due to Gruppelaar4437 1451 109 /18/. 4437 1451 110 4437 1451 111 mt = 1 Total 4437 1451 112 Spherical optical model calculation was adopted. 4437 1451 113 4437 1451 114 mt = 2 Elastic scattering 4437 1451 115 Calculated as (total - sum of partial cross sections). 4437 1451 116 4437 1451 117 mt = 4, 51 - 91 Inelastic scattering 4437 1451 118 Spherical optical and statistical model calculation was 4437 1451 119 adopted. The level scheme was taken from Ref./19/. 4437 1451 120 4437 1451 121 no. energy(MeV) spin-parity dwba cal. 4437 1451 122 gr. 0.0 0 + 4437 1451 123 1 0.5396 2 + * 4437 1451 124 2 1.1304 0 + 4437 1451 125 3 1.2265 4 + 4437 1451 126 4 1.3621 2 + 4437 1451 127 5 1.7407 0 + 4437 1451 128 6 1.8653 1 + 4437 1451 129 7 1.8812 3 + 4437 1451 130 8 2.0517 0 + 4437 1451 131 9 2.0639 3 - * 4437 1451 132 10 2.0777 6 + 4437 1451 133 11 2.0993 2 - 4437 1451 134 12 2.1673 2 - 4437 1451 135 13 2.2406 1 + 4437 1451 136 14 2.3872 0 + 4437 1451 137 15 2.4694 2 - 4437 1451 138 16 2.5168 2 + 4437 1451 139 Levels above 2.613 MeV were assumed to be overlapping. 4437 1451 140 4437 1451 141 For the levels with an asterisk, the contribution of direct 4437 1451 142 inelastic scattering cross sections was calculated by the 4437 1451 143 DWUCK-4 code/20/. Deformation parameters (beta2 = 0.2172 and 4437 1451 144 beta3 = 0.116) were based on the data compiled by Raman et 4437 1451 145 al./21/ and Spear/22/, respectively. 4437 1451 146 4437 1451 147 mt = 102 Capture 4437 1451 148 Spherical optical and statistical model calculation with 4437 1451 149 CASTHY was adopted. Direct and semi-direct capture cross 4437 1451 150 sections were estimated according to the procedure of Benzi 4437 1451 151 and Reffo/23/ and normalized to 1 milli-barn at 14 MeV. 4437 1451 152 4437 1451 153 The gamma-ray strength function (3.79e-04) was adjusted to 4437 1451 154 reproduce the capture cross section of 120 milli-barns at 70 4437 1451 155 keV measured by Macklin et al./24,25/ 4437 1451 156 4437 1451 157 mt = 16 (n,2n) cross section 4437 1451 158 mt = 17 (n,3n) cross section 4437 1451 159 mt = 22 (n,n'a) cross section 4437 1451 160 mt = 28 (n,n'p) cross section 4437 1451 161 mt = 32 (n,n'd) cross section 4437 1451 162 mt =103 (n,p) cross section 4437 1451 163 mt =104 (n,d) cross section 4437 1451 164 mt =105 (n,t) cross section 4437 1451 165 mt =107 (n,alpha) cross section 4437 1451 166 These reaction cross sections were calculated with the 4437 1451 167 preequilibrium and multi-step evaporation model code PEGASUS. 4437 1451 168 4437 1451 169 The Kalbach's constant k (= 89.2) was estimated by the 4437 1451 170 formula derived from Kikuchi-Kawai's formalism/26/ and level 4437 1451 171 density parameters. 4437 1451 172 4437 1451 173 Finally, the (n,p) and (n,alpha) cross sections were 4437 1451 174 normalized to the following values at 14.5 MeV: 4437 1451 175 (n,p) 15.00 mb (recommended by Forrest/27/) 4437 1451 176 (n,alpha) 8.70 mb (systematics of Forrest/27/) 4437 1451 177 4437 1451 178 mt = 251 mu-bar 4437 1451 179 Calculated with CASTHY. 4437 1451 180 4437 1451 181 mf = 4 Angular distributions of secondary neutrons 4437 1451 182 Legendre polynomial coefficients for angular distributions are 4437 1451 183 given in the center-of-mass system for mt=2 and discrete inelas-4437 1451 184 tic levels, and in the laboratory system for mt=91. They were 4437 1451 185 calculated with CASTHY. Contribution of direct inelastic 4437 1451 186 scattering was calculated with DWUCK-4. For other reactions, 4437 1451 187 isotropic distributions in the laboratory system were assumed. 4437 1451 188 4437 1451 189 mf = 5 Energy distributions of secondary neutrons 4437 1451 190 Energy distributions of secondary neutrons were calculated with 4437 1451 191 PEGASUS for inelastic scattering to overlapping levels and for 4437 1451 192 other neutron emitting reactions. 4437 1451 193 4437 1451 194 TABLE 1 NEUTRON OPTICAL POTENTIAL PARAMETERS 4437 1451 195 4437 1451 196 DEPTH (MEV) RADIUS(FM) DIFFUSENESS(FM) 4437 1451 197 ---------------------- ------------ --------------- 4437 1451 198 V = 47.5 R0 = 5.972 A0 = 0.62 4437 1451 199 WS = 9.74 RS = 6.594 AS = 0.35 4437 1451 200 VSO= 7.0 RSO= 5.97 ASO= 0.62 4437 1451 201 THE FORM OF SURFACE ABSORPTION PART IS DER. WOODS-SAXON TYPE. 4437 1451 202 4437 1451 203 TABLE 2 LEVEL DENSITY PARAMETERS 4437 1451 204 4437 1451 205 NUCLIDE A(1/MEV) T(MEV) C(1/MEV) EX(MEV) PAIRING 4437 1451 206 --------------------------------------------------------------- 4437 1451 207 42-MO- 96 1.403E+01 7.410E-01 6.991E-01 7.645E+00 2.400E+00 4437 1451 208 42-MO- 97 1.517E+01 6.800E-01 2.769E+00 6.036E+00 1.280E+00 4437 1451 209 42-MO- 98 1.594E+01 6.900E-01 7.358E-01 7.888E+00 2.570E+00 4437 1451 210 42-MO- 99 1.774E+01 6.200E-01 4.294E+00 6.058E+00 1.280E+00 4437 1451 211 4437 1451 212 43-TC- 97 1.600E+01 6.700E-01 4.756E+00 6.089E+00 1.120E+00 4437 1451 213 43-TC- 98 1.659E+01 6.120E-01 1.776E+01 4.176E+00 0.0 4437 1451 214 43-TC- 99 1.600E+01 6.550E-01 2.973E+00 5.984E+00 1.290E+00 4437 1451 215 43-TC-100 1.637E+01 5.850E-01 1.189E+01 3.635E+00 0.0 4437 1451 216 4437 1451 217 44-RU- 98 1.382E+01 7.400E-01 6.070E-01 7.507E+00 2.400E+00 4437 1451 218 44-RU- 99 1.650E+01 6.570E-01 4.016E+00 6.235E+00 1.280E+00 4437 1451 219 44-RU-100 1.520E+01 7.200E-01 7.835E-01 8.078E+00 2.570E+00 4437 1451 220 44-RU-101 1.726E+01 6.700E-01 7.228E+00 6.836E+00 1.280E+00 4437 1451 221 --------------------------------------------------------------- 4437 1451 222 4437 1451 223 Spin cutoff parameters were calculated as 0.146*sqrt(a)*a**(2/3).4437 1451 224 In the CASTHY calculation, spin cutoff factors at 0 MeV were 4437 1451 225 assumed to be 4.062 for Ru-100 and 14.30 for Ru-101. 4437 1451 226 4437 1451 227 References 4437 1451 228 1) Aoki, T. et al.: Proc. Int. Conf. on Nuclear Data for Basic 4437 1451 229 and Applied Science, Santa Fe., Vol. 2, p.1627 (1985). 4437 1451 230 2) Kawai, M. et al.: Proc. Int. Conf. on Nuclear Data for Science4437 1451 231 and Technology, Mito, p. 569 (1988). 4437 1451 232 3) J.Halperin et al.: ORNL 3832, p.4 (1965). 4437 1451 233 4) H.G.Priesmeyer, H.H.Jung: Atomkernenergie, 19, 111 (1972). 4437 1451 234 5) R.L.Macklin, J.Halperin: Nucl. Sci. Eng., 73, 174 (1980). 4437 1451 235 6) S.F.Mughabghab et al.: "Neutron Cross Sections, Vol. I, 4437 1451 236 Part A", Academic Press (1981). 4437 1451 237 7) L.M.Bollinger, G.E.Thomas: Phys. Rev., 171,1293 (1968). 4437 1451 238 8) Igarasi, S.: J. Nucl. Sci. Technol., 12, 67 (1975). 4437 1451 239 9) Y.Kikuchi et al., JAERI-Data/Code 99-025 (1999) 4437 1451 240 [in Japanese]. 4437 1451 241 10) Iijima, S. et al.: JAERI-M 87-025, p. 337 (1987). 4437 1451 242 11) Iijima, S. and Kawai, M.: J. Nucl. Sci. Technol., 20, 77 4437 1451 243 (1983). 4437 1451 244 12) Perey, F.G: Phys. Rev. 131, 745 (1963). 4437 1451 245 13) Huizenga, J.R. and Igo, G.: Nucl. Phys. 29, 462 (1962). 4437 1451 246 14) Lohr, J.M. and Haeberli, W.: Nucl. Phys. A232, 381 (1974). 4437 1451 247 15) Becchetti, F.D., Jr. and Greenlees, G.W.: Polarization 4437 1451 248 Phenomena in Nuclear Reactions ((Eds) H.H. Barshall and 4437 1451 249 W. Haeberli), p. 682, the University of Wisconsin Press. 4437 1451 250 (1971). 4437 1451 251 16) Gilbert, A. and Cameron, A.G.W.: Can. J. Phys., 43, 1446 4437 1451 252 (1965). 4437 1451 253 17) Iijima, S., et al.: J. Nucl. Sci. Technol. 21, 10 (1984). 4437 1451 254 18) Gruppelaar, H.: ECN-13 (1977). 4437 1451 255 19) Matsumoto, J.: private communication (1981). 4437 1451 256 20) Kunz, P.D.: private communication. 4437 1451 257 21) Raman, S., et al.: Atom. Data and Nucl. Data Tables 36, 1 4437 1451 258 (1987) 4437 1451 259 22) Spear, R.H.: Atom. Data and Nucl. Data Table, 42, 55 (1989). 4437 1451 260 23) Benzi, V. and Reffo, G.: CCDN-NW/10 (1969). 4437 1451 261 24) Macklin, R.L., et al.: Proc. Specialists' Meeting on Neutron 4437 1451 262 Cross Sections of Fission Products, Bologna 1979, NEANDC(E) 4437 1451 263 209L, 103. 4437 1451 264 25) Macklin, R.L., Winters, R.R.: Nucl. Sci. Eng., 78, 110(1981). 4437 1451 265 26) Kikuchi, K. and Kawai, M.: "Nuclear Matter and Nuclear 4437 1451 266 Reactions", North Holland (1968). 4437 1451 267 27) Forrest, R.A.: AERE-R 12419 (1986). 4437 1451 268 4437 1451 269 1 451 330 14437 1451 270 2 151 182 14437 1451 271 3 1 31 14437 1451 272 3 2 31 14437 1451 273 3 4 16 04437 1451 274 3 16 9 04437 1451 275 3 17 5 04437 1451 276 3 22 13 04437 1451 277 3 28 10 04437 1451 278 3 32 6 04437 1451 279 3 51 16 04437 1451 280 3 52 15 04437 1451 281 3 53 14 04437 1451 282 3 54 14 04437 1451 283 3 55 13 04437 1451 284 3 56 12 04437 1451 285 3 57 12 04437 1451 286 3 58 11 04437 1451 287 3 59 11 04437 1451 288 3 60 11 04437 1451 289 3 61 10 04437 1451 290 3 62 10 04437 1451 291 3 63 10 04437 1451 292 3 64 9 04437 1451 293 3 65 9 04437 1451 294 3 66 9 04437 1451 295 3 91 8 04437 1451 296 3 102 26 14437 1451 297 3 103 13 04437 1451 298 3 104 11 04437 1451 299 3 105 9 04437 1451 300 3 107 15 04437 1451 301 4 2 190 04437 1451 302 4 16 10 04437 1451 303 4 17 10 04437 1451 304 4 22 10 04437 1451 305 4 28 10 04437 1451 306 4 32 10 04437 1451 307 4 51 100 04437 1451 308 4 52 22 04437 1451 309 4 53 22 04437 1451 310 4 54 22 04437 1451 311 4 55 22 04437 1451 312 4 56 22 04437 1451 313 4 57 22 04437 1451 314 4 58 22 04437 1451 315 4 59 65 04437 1451 316 4 60 22 04437 1451 317 4 61 22 04437 1451 318 4 62 22 04437 1451 319 4 63 22 04437 1451 320 4 64 22 04437 1451 321 4 65 22 04437 1451 322 4 66 22 04437 1451 323 4 91 22 04437 1451 324 5 16 51 04437 1451 325 5 17 23 04437 1451 326 5 22 195 04437 1451 327 5 28 88 04437 1451 328 5 32 32 04437 1451 329 5 91 114 04437 1451 330 4437 1 099999 4437 0 0 0 4.410000+4 9.904600+1 0 0 1 04437 2151 1 4.410000+4 1.000000+0 0 0 2 04437 2151 2 1.000000-5 1.189000+4 1 2 0 04437 2151 3 0.000000+0 6.100000-1 0 0 2 04437 2151 4 9.904600+1 0.000000+0 0 0 120 204437 2151 5 -1.800000+2 5.000000-1 1.934000+0 1.550000+0 3.840000-1 0.000000+04437 2151 6 1.200000+2 5.000000-1 1.315000-1 7.500000-3 1.240000-1 0.000000+04437 2151 7 2.285000+2 5.000000-1 2.020000-1 2.700000-2 1.750000-1 0.000000+04437 2151 8 4.450000+2 5.000000-1 4.298780-1 3.058780-1 1.240000-1 0.000000+04437 2151 9 6.610000+2 5.000000-1 4.967940-1 3.727940-1 1.240000-1 0.000000+04437 2151 10 1.200000+3 5.000000-1 6.262950-1 5.022950-1 1.240000-1 0.000000+04437 2151 11 1.417000+3 5.000000-1 6.698240-1 5.458240-1 1.240000-1 0.000000+04437 2151 12 1.633000+3 5.000000-1 7.099510-1 5.859510-1 1.240000-1 0.000000+04437 2151 13 1.957000+3 5.000000-1 7.654510-1 6.414510-1 1.240000-1 0.000000+04437 2151 14 2.173000+3 5.000000-1 7.999240-1 6.759240-1 1.240000-1 0.000000+04437 2151 15 3.712700+3 5.000000-1 3.273300+0 3.160000+0 1.133000-1 0.000000+04437 2151 16 5.112400+3 5.000000-1 1.800100+0 1.700000+0 1.001000-1 0.000000+04437 2151 17 6.790900+3 5.000000-1 2.259700+0 2.200000+0 5.970000-2 0.000000+04437 2151 18 6.944100+3 5.000000-1 5.007000+0 4.890000+0 1.170000-1 0.000000+04437 2151 19 7.514800+3 5.000000-1 5.174600+0 5.070000+0 1.046000-1 0.000000+04437 2151 20 8.408100+3 5.000000-1 3.592900+0 3.480000+0 1.129000-1 0.000000+04437 2151 21 9.109600+3 5.000000-1 2.113000+0 1.960000+0 1.530000-1 0.000000+04437 2151 22 9.236000+3 5.000000-1 3.749000+0 3.630000+0 1.190000-1 0.000000+04437 2151 23 1.165100+4 5.000000-1 7.822000+0 7.700000+0 1.220000-1 0.000000+04437 2151 24 1.173100+4 5.000000-1 7.826000+0 7.700000+0 1.260000-1 0.000000+04437 2151 25 9.904600+1 0.000000+0 1 0 546 914437 2151 26 3.360000+2 5.000000-1 1.242492-1 2.492150-4 1.240000-1 0.000000+04437 2151 27 5.530000+2 5.000000-1 1.245260-1 5.260020-4 1.240000-1 0.000000+04437 2151 28 7.690000+2 5.000000-1 1.248622-1 8.622330-4 1.240000-1 0.000000+04437 2151 29 8.770000+2 5.000000-1 1.250499-1 1.049910-3 1.240000-1 0.000000+04437 2151 30 9.850000+2 5.000000-1 1.252495-1 1.249470-3 1.240000-1 0.000000+04437 2151 31 1.093000+3 5.000000-1 1.254602-1 1.460220-3 1.240000-1 0.000000+04437 2151 32 1.308000+3 5.000000-1 1.259109-1 1.910890-3 1.240000-1 0.000000+04437 2151 33 1.525000+3 5.000000-1 1.264047-1 2.404710-3 1.240000-1 0.000000+04437 2151 34 1.741000+3 5.000000-1 1.269322-1 2.932190-3 1.240000-1 0.000000+04437 2151 35 1.849000+3 5.000000-1 1.272086-1 3.208610-3 1.240000-1 0.000000+04437 2151 36 2.065000+3 5.000000-1 1.277855-1 3.785530-3 1.240000-1 0.000000+04437 2151 37 2.281000+3 5.000000-1 1.283931-1 4.393090-3 1.240000-1 0.000000+04437 2151 38 2.389000+3 5.000000-1 1.287079-1 4.707870-3 1.240000-1 0.000000+04437 2151 39 2.497000+3 5.000000-1 1.290297-1 5.029740-3 1.240000-1 0.000000+04437 2151 40 2.679700+3 5.000000-1 1.889999-1 6.499990-2 1.240000-1 0.000000+04437 2151 41 2.733700+3 1.500000+0 1.860000-1 6.200000-2 1.240000-1 0.000000+04437 2151 42 2.745500+3 5.000000-1 1.570000-1 3.300000-2 1.240000-1 0.000000+04437 2151 43 3.076000+3 1.500000+0 2.410000-1 1.170000-1 1.240000-1 0.000000+04437 2151 44 3.294300+3 1.500000+0 2.040000-1 8.000000-2 1.240000-1 0.000000+04437 2151 45 3.494700+3 5.000000-1 1.480000-1 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