98-Cf-252 JAEA+ EVAL-FEB10 O.Iwamoto,T.Nakagawa,+
DIST-MAY10 20100318
----JENDL-4.0 MATERIAL 9861
-----INCIDENT NEUTRON DATA
------ENDF-6 FORMAT
History
05-12 Fission cross section above 1 keV was revised.
07-09 Theoretical calculation was done with CCONE code.
Data were compiled as JENDL/AC-2008/1/.
10-02 Data of prompt gamma rays due to fission were given.
10-03 Covariance data were given.
MF= 1 General information
MT=452 Number of Neutrons per fission
Sum of MT's = 455 and 456.
MT=455 Delayed neutron data
Semi-empirical formula by Tuttle/2/.
Decay constants were evaluated by Brady and England/3/.
MT=456 Number of prompt neutrons per fission
Semi-empirical formula by Howerton/4/.
MF= 2 Resonance parameters
MT=151
Resolved resonance parameters (MLBW: 1.0e-5 - 1.0 keV)
(same as JENDL-3.3)
Resonance parameters were taken from Moore et al./5/ by
assuming an average radiative capture width of 0.035 eV and
fission width of 0.035 eV. Two hypothetical resonances at
1.4 and -3.5 EV were adopted to reproduce the 2200-m/s
cross sections and resonance integrals/6,7/. Scattering
radius of 9.23 fm was estimated from the shape elastic
scattering cross section calculated with CASTHY/8/.
Unresolved resonance parameters (1 - 150 keV)
Parameters (URP) were determined with ASREP code/9/ so as to
reproduce the cross sections in this energy region. URP are
used only for self-shielding calculations.
Thermal cross sections and resonance integrals (at 300K)
-------------------------------------------------------
0.0253 eV reson. integ.(*)
(barns) (barns)
-------------------------------------------------------
total 64.81
elastic 11.06
fission 33.03 109
capture 20.71 47.3
-------------------------------------------------------
(*) In the energy range from 0.5 eV to 10 MeV.
MF= 3 Neutron cross sections
Cross sections above the resolved resonance region except for
the elastic scattering (MT=2) and fission cross sections (MT=18,
19, 20, 21, 38) were calculated with CCONE code/10/.
MT= 1 Total cross section
The cross section was calculated with CC OMP of Soukhovitskii
et al./11/
MT= 2 Elastic scattering cross section
Calculated as total - non-elastic scattering cross sections.
MT=18 Fission cross section (Above 1 keV)
The experimental data of Moore et al./5/ were analyzed
with the GMA code /12/. The results of GMA were used to
determine the parameters in the CCONE calculation.
In the energy region from 4 to 20 MeV, the data of JENDL-3.3
were adopted.
MT=19, 20, 21, 38 Multi-chance fission cross sections
Calculated with CCONE code, and renormalized to the total
fission cross section (MT=18).
MF= 4 Angular distributions of secondary neutrons
MT=2 Elastic scattering
Calculated with CCONE code.
MT=18 Fission
Isotropic distributions in the laboratory system were assumed.
MF= 5 Energy distributions of secondary neutrons
MT=18 Prompt netrons
Calculated with CCONE code/10/.
MT=455 Delayed neutrons
Calculated by Brady and England/3/.
MF= 6 Energy-angle distributions
Calculated with CCONE code.
Distributions from fission (MT=18) are not included.
MF=12 Photon production multiplicities
MT=18 Fission
Calculated from the total energy released by the prompt
gamma-rays due to fission which was estimated from its
systematics, and the average energy of gamma-rays.
MF=14 Photon angular distributions
MT=18 Fission
Isotoropic distributions were assumed.
MF=15 Continuous photon energy spectra
MT=18 Fission
Experimental data measured by Verbinski et al./13/ for
Pu-239 thermal fission were adopted.
MF=31 Covariances of average number of neutrons per fission
MT=452 Number of neutrons per fission
Sum of covariances for MT=455 and MT=456.
MT=455
Error of 15% was assumed.
MT=456
Covariance was obtained by fitting a linear function to the
data at 0.0 and 5.0 MeV with an uncertainty of 10%.
MF=32 Covariances of resonance parameters
MT=151 Resolved resonance parameterss
Format of LCOMP=0 was adopted.
Uncertainties of parameters were taken from Mughabghab /14/.
For the parameters without any information on uncertainty,
the following uncertainties were assumed:
Resonance energy 0.1 %
Neutron width 10 %
Capture width 20 %
Fission width 20 %
They were further modified by considering experimental data
of the fission and capture cross sections at the thermal
neutron energy.
MF=33 Covariances of neutron cross sections
Covariances were given to all the cross sections by using
KALMAN code/15/ and the covariances of model parameters
used in the cross-section calculations.
For the fission cross section, covariances obtained with the
GMA analysis were adopted. Standard deviations above 8 MeV
were assumed to be 20%.
In the resolved resonance region, the following standard
deviations were added to the contributions from resonance
parameters:
Elastic scattering 20 %
MF=34 Covariances for Angular Distributions
MT=2 Elastic scattering
Covariances were given only to P1 components.
MF=35 Covariances for Energy Distributions
MT=18 Fission spectra
Estimated with CCONE and KALMAN codes.
*****************************************************************
Calculation with CCONE code
*****************************************************************
Models and parameters used in the CCONE/10/ calculation
1) Coupled channel optical model
Levels in the rotational band were included. Optical model
potential and coupled levels are shown in Table 1.
2) Two-component exciton model/16/
* Global parametrization of Koning-Duijvestijn/17/
was used.
* Gamma emission channel/18/ was added to simulate direct
and semi-direct capture reaction.
3) Hauser-Feshbach statistical model
* Moldauer width fluctuation correction/19/ was included.
* Neutron, gamma and fission decay channel were included.
* Transmission coefficients of neutrons were taken from
coupled channel calculation in Table 1.
* The level scheme of the target is shown in Table 2.
* Level density formula of constant temperature and Fermi-gas
model were used with shell energy correction and collective
enhancement factor. Parameters are shown in Table 3.
* Fission channel:
Double humped fission barriers were assumed.
Fission barrier penetrabilities were calculated with
Hill-Wheler formula/20/. Fission barrier parameters were
shown in Table 4. Transition state model was used and
continuum levels are assumed above the saddles. The level
density parameters for inner and outer saddles are shown in
Tables 5 and 6, respectively.
* Gamma-ray strength function of Kopecky et al/21/,/22/
was used. The prameters are shown in Table 7.
------------------------------------------------------------------
Tables
------------------------------------------------------------------
Table 1. Coupled channel calculation
--------------------------------------------------
* rigid rotor model was applied
* coupled levels = 0,1,2,3,4 (see Table 2)
* optical potential parameters /11/
Volume:
V_0 = 49.97 MeV
lambda_HF = 0.01004 1/MeV
C_viso = 15.9 MeV
A_v = 12.04 MeV
B_v = 81.36 MeV
E_a = 385 MeV
r_v = 1.2568 fm
a_v = 0.633 fm
Surface:
W_0 = 17.2 MeV
B_s = 11.19 MeV
C_s = 0.01361 1/MeV
C_wiso = 23.5 MeV
r_s = 1.1803 fm
a_s = 0.601 fm
Spin-orbit:
V_so = 5.75 MeV
lambda_so = 0.005 1/MeV
W_so = -3.1 MeV
B_so = 160 MeV
r_so = 1.1214 fm
a_so = 0.59 fm
Coulomb:
C_coul = 1.3
r_c = 1.2452 fm
a_c = 0.545 fm
Deformation:
beta_2 = 0.213
beta_4 = 0.066
beta_6 = 0.0015
* Calculated strength function
S0= 1.42e-4 S1= 3.00e-4 R'= 9.17 fm (En=1 keV)
--------------------------------------------------
Table 2. Level Scheme of Cf-252
-------------------
No. Ex(MeV) J PI
-------------------
0 0.00000 0 + *
1 0.04572 2 + *
2 0.15173 4 + *
3 0.31920 6 + *
4 0.54720 8 + *
5 0.80482 2 +
6 0.83081 2 -
7 0.84572 3 +
8 0.86751 3 -
9 0.90030 4 +
10 0.91703 4 -
-------------------
*) Coupled levels in CC calculation
Table 3. Level density parameters
--------------------------------------------------------
Nuclide a* Pair Eshell T E0 Ematch
1/MeV MeV MeV MeV MeV MeV
--------------------------------------------------------
Cf-253 19.3604 0.7544 2.0655 0.3368 -0.4669 2.4564
Cf-252 19.2945 1.5119 1.7395 0.3655 0.0444 3.5280
Cf-251 19.2285 0.7574 1.2773 0.3926 -0.9361 3.0632
Cf-250 19.1626 1.5179 1.0208 0.3974 -0.1838 3.8400
Cf-249 19.0966 0.7605 0.7689 0.3773 -0.6847 2.7641
--------------------------------------------------------
Table 4. Fission barrier parameters
----------------------------------------
Nuclide V_A hw_A V_B hw_B
MeV MeV MeV MeV
----------------------------------------
Cf-253 5.600 1.000 4.600 0.800
Cf-252 6.000 1.040 5.000 0.800
Cf-251 6.200 0.800 5.000 0.600
Cf-250 6.200 1.040 5.400 0.600
Cf-249 6.700 1.200 5.900 0.800
----------------------------------------
Table 5. Level density above inner saddle
--------------------------------------------------------
Nuclide a* Pair Eshell T E0 Ematch
1/MeV MeV MeV MeV MeV MeV
--------------------------------------------------------
Cf-253 21.6837 0.8802 2.5000 0.3407 -1.8541 3.1802
Cf-252 21.6098 1.7638 2.5000 0.3202 -0.6492 3.7638
Cf-251 21.5360 0.8837 2.5000 0.3208 -1.5294 2.8837
Cf-250 21.4621 1.7709 2.5000 0.2827 -0.1068 3.2709
Cf-249 20.0514 0.8872 2.5000 0.3486 -1.7837 3.0872
--------------------------------------------------------
Table 6. Level density above outer saddle
--------------------------------------------------------
Nuclide a* Pair Eshell T E0 Ematch
1/MeV MeV MeV MeV MeV MeV
--------------------------------------------------------
Cf-253 21.6837 0.8802 1.0800 0.3466 -0.8314 2.8802
Cf-252 21.6098 1.7638 1.0400 0.3477 0.0528 3.7638
Cf-251 21.5360 0.8837 1.0000 0.3488 -0.8268 2.8837
Cf-250 21.4621 1.7709 0.9600 0.3499 0.0610 3.7709
Cf-249 20.0514 0.8872 0.9200 0.3794 -1.0059 3.0872
--------------------------------------------------------
Table 7. Gamma-ray strength function for Cf-253
--------------------------------------------------------
K0 = 1.500 E0 = 4.500 (MeV)
* E1: ER = 11.40 (MeV) EG = 2.72 (MeV) SIG = 258.47 (mb)
ER = 14.19 (MeV) EG = 4.12 (MeV) SIG = 516.94 (mb)
* M1: ER = 6.48 (MeV) EG = 4.00 (MeV) SIG = 1.84 (mb)
* E2: ER = 9.96 (MeV) EG = 3.07 (MeV) SIG = 7.35 (mb)
--------------------------------------------------------
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