44-Ru-103 JNDC EVAL-MAR90 JNDC FP NUCLEAR DATA W.G. DIST-MAY10 20091210 ----JENDL-4.0 MATERIAL 4446 -----INCIDENT NEUTRON DATA ------ENDF-6 FORMAT =========================================================== JENDL-3.2 data were automatically transformed to JENDL-3.3. Interpolation of spectra: 22 (unit base interpolation) (3,251) deleted, T-matrix of (4,2) deleted, and others. =========================================================== History 84-10 Evaluation for JENDL-2 was made by JNDC FPND W.G./1/ 90-03 Modification for JENDL-3 was made/2/. 09-12 JENDL-4.0. Compiled by A.Ichihara (jaea/ndc). ***** modified parts for JENDL-4.0 ******************* (2,151) Resolved resonance parameters were revised by T.Nakagawa. ********************************************************** mf = 1 General information mt=451 Comments and dictionary mf = 2 Resonance parameters mt=151 Resolved and unresolved resonance parameters Resolved Resonance Parameters (MLBW; below 50 eV) The resonance parameters of 8 levels up to 330 eV were obtained by Anufriev et al./3/ Their parameters were adopted. In addition, a negative resonance was assumed at -3.0 eV and its parameters were determined so that the capture cross section at 0.0253 eV was about 10 b. No experimental data are available for any cross sections. An upper bounday of the resolved resonance region was set at 50 eV, because level missing was obvious above this energy. Unresolved resonance region : 50 eV - 100 keV The neutron strength functions, S0, S1 and S2 were calculated with optical model code CASTHY/4/. The observed level spacing was determined to reproduce the capture cross section calculated with CASTHY. The effective scattering radius was obtained from fitting to the calculated total cross section at 100 keV. Typical values of the parameters at 70 keV: S0 = 0.450e-4, S1 = 6.000e-4, S2 = 0.530e-4, Sg = 76.7e-4, Gg = 0.170 eV, R = 5.590 fm. The unresolved resonance parameters were calculated using the ASREP code/5/. The parameters should be used only for self-shielding calculation. Thermal cross sections and resonance integrals at 300K (b) ------------------------------------------------------- 0.0253 eV reson. integ.(*) ------------------------------------------------------- total 14.637 elastic 5.083 capture 9.554 62.0 ------------------------------------------------------- (*) In the energy range from 0.5 eV to 10 MeV. mf = 3 Neutron cross sections In thermal region, the capture and elastic scattering cross sections were assumed to be in 1/v form and constant, respectively. Thermal capture cross section was determined by the systematics from the neighboring Ru isotopes. The scattering cross section was calculated from r = 6.3 fm. Unresolved resonance parameters were given in the energy range from 50 eV to 100 keV. Above 100 keV, the spherical optical and statistical model calculation was performed with CASTHY, by taking account of competing reactions, of which cross sections were calculated with PEGASUS/6/ standing on a preequilibrium and multi-step evaporation model. The OMP's for neutron given in Table 1 were determined to reproduce a systematic trend of the total cross section by changing rso of Iijima-Kawai potential/7/. The OMP's for charged particles are as follows: proton = Perey/8/ alpha = Huizenga and Igo/9/ deuteron = Lohr and Haeberli/10/ helium-3 and triton = Becchetti and Greenlees/11/ Parameters for the composite level density formula of Gilbert and Cameron/12/ were evaluated by Iijima et al./13/ More extensive determination and modification were made in the present work. Table 2 shows the level density parameters used in the present calculation. Energy dependence of spin cut-off parameter in the energy range below E-joint is due to Gruppelaar /14/. mt = 1 Total Spherical optical model calculation was adopted. mt = 2 Elastic scattering Calculated as (total - sum of partial cross sections). mt = 4, 51 - 91 Inelastic scattering Spherical optical and statistical model calculation was adopted. The level scheme was taken from Ref./15/. no. energy(MeV) spin-parity gr. 0.0 3/2 + 1 0.0027 5/2 + 2 0.1360 5/2 + 3 0.1742 1/2 + 4 0.2134 7/2 + 5 0.2380 11/2 - 6 0.2877 1/2 + 7 0.2974 7/2 - 8 0.3465 5/2 + 9 0.4056 3/2 + 10 0.4319 1/2 + 11 0.4990 5/2 + Levels above 0.511 MeV were assumed to be overlapping. mt = 102 Capture Spherical optical and statistical model calculation with CASTHY was adopted. Direct and semi-direct capture cross sections were estimated according to the procedure of Benzi and Reffo/16/ and normalized to 1 milli-barn at 14 MeV. The gamma-ray strength function (7.69e-03) was determined from the systematics of radiation width (0.170 eV) and average s-wave resonance level spacing (22.1 eV). mt = 16 (n,2n) cross section mt = 17 (n,3n) cross section mt = 22 (n,n'a) cross section mt = 28 (n,n'p) cross section mt = 32 (n,n'd) cross section mt =103 (n,p) cross section mt =104 (n,d) cross section mt =105 (n,t) cross section mt =107 (n,alpha) cross section These reaction cross sections were calculated with the preequilibrium and multi-step evaporation model code PEGASUS. The Kalbach's constant k (= 111.5) was estimated by the formula derived from Kikuchi-Kawai's formalism/17/ and level density parameters. Finally, the (n,p) and (n,alpha) cross sections were normalized to the following values at 14.5 MeV: (n,p) 11.60 mb (systematics of Forrest/18/) (n,alpha) 2.86 mb (systematics of Forrest) mt = 251 mu-bar Calculated with CASTHY. mf = 4 Angular distributions of secondary neutrons Legendre polynomial coefficients for angular distributions are given in the center-of-mass system for mt=2 and discrete inelas- tic levels, and in the laboratory system for mt=91. They were calculated with CASTHY. For other reactions, isotropic distri- butions in the laboratory system were assumed. mf = 5 Energy distributions of secondary neutrons Energy distributions of secondary neutrons were calculated with PEGASUS for inelastic scattering from overlapping levels and for other neutron emitting reactions. TABLE 1 NEUTRON OPTICAL POTENTIAL PARAMETERS DEPTH (MEV) RADIUS(FM) DIFFUSENESS(FM) ---------------------- ------------ --------------- V = 47.5 R0 = 5.972 A0 = 0.62 WS = 9.74 RS = 6.594 AS = 0.35 VSO= 7.0 RSO= 5.97 ASO= 0.62 THE FORM OF SURFACE ABSORPTION PART IS DER. WOODS-SAXON TYPE. TABLE 2 LEVEL DENSITY PARAMETERS NUCLIDE SYST A(1/MEV) T(MEV) C(1/MEV) EX(MEV) PAIRING --------------------------------------------------------------- 42-MO- 99 1.774E+01 6.200E-01 4.294E+00 6.058E+00 1.280E+00 42-MO-100 1.780E+01 6.000E-01 6.702E-01 6.645E+00 2.220E+00 42-MO-101 2.085E+01 5.650E-01 7.153E+00 6.092E+00 1.280E+00 42-MO-102 * 1.856E+01 6.452E-01 1.419E+00 8.145E+00 2.520E+00 43-TC-100 1.637E+01 5.850E-01 1.189E+01 3.635E+00 0.0 43-TC-101 1.675E+01 6.440E-01 6.361E+00 5.761E+00 9.400E-01 43-TC-102 1.761E+01 5.400E-01 1.217E+01 3.317E+00 0.0 43-TC-103 1.810E+01 6.310E-01 6.436E+00 6.379E+00 1.240E+00 44-RU-101 1.726E+01 6.700E-01 7.228E+00 6.836E+00 1.280E+00 44-RU-102 1.643E+01 6.550E-01 8.872E-01 7.106E+00 2.220E+00 44-RU-103 1.890E+01 6.480E-01 1.210E+01 7.110E+00 1.280E+00 44-RU-104 1.650E+01 6.780E-01 8.593E-01 7.878E+00 2.520E+00 --------------------------------------------------------------- syst: * = ldp's were determined from systematics. Spin cutoff parameters were calculated as 0.146*sqrt(a)*a**(2/3). In the CASTHY calculation, spin cutoff factors at 0 MeV were assumed to be 5.045 for Ru-103 and 4.524 for Ru-104. References 1) Aoki, T. et al.: Proc. Int. Conf. on Nuclear Data for Basic and Applied Science, Santa Fe., Vol. 2, p.1627 (1985). 2) Kawai, M. et al.: Proc. Int. Conf. on Nuclear Data for Science and Technology, Mito, p. 569 (1988). 3) V.A.Anufriev et al.: 1980 Kiev, Vol.2, p.156 (1980). 4) Igarasi, S.: J. Nucl. Sci. Technol., 12, 67 (1975). 5) Y.Kikuchi et al., JAERI-Data/Code 99-025 (1999) [in Japanese]. 6) Iijima, S. et al.: JAERI-M 87-025, p. 337 (1987). 7) Iijima, S. and Kawai, M.: J. Nucl. Sci. Technol., 20, 77 (1983). 8) Perey, F.G: Phys. Rev. 131, 745 (1963). 9) Huizenga, J.R. and Igo, G.: Nucl. Phys. 29, 462 (1962). 10) Lohr, J.M. and Haeberli, W.: Nucl. Phys. A232, 381 (1974). 11) Becchetti, F.D., Jr. and Greenlees, G.W.: Polarization Phenomena in Nuclear Reactions ((Eds) H.H. Barshall and W. Haeberli), p. 682, the University of Wisconsin Press. (1971). 12) Gilbert, A. and Cameron, A.G.W.: Can. J. Phys., 43, 1446 (1965). 13) Iijima, S., et al.: J. Nucl. Sci. Technol. 21, 10 (1984). 14) Gruppelaar, H.: ECN-13 (1977). 15) Matsumoto, J.: private communication (1981). 16) Benzi, V. and Reffo, G.: CCDN-NW/10 (1969). 17) Kikuchi, K. and Kawai, M.: "Nuclear Matter and Nuclear Reactions", North Holland (1968). 18) Forrest, R.A.: AERE-R 12419 (1986).