48-Cd-111 JAEA EVAL-FEB22 S.Kunieda, A.Ichihara, K.Shibata+ DIST-DEC21 20100316 ----JENDL-5 MATERIAL 4840 -----INCIDENT NEUTRON DATA ------ENDF-6 FORMAT History 09-11 Re-evaluation was performed for JENDL-4.0 10-03 Compiled by S.Kunieda 21-11 revised by O.Iwamoto (MF8/MT4,16,17,22,24,28,32,41,102-104,107) JENDL/AD-2017 adopted (MF8/MT105,106) added (MF10/MT4,22,28,32,103,104) JENDL/AD-2017 based 21-11 above 20 MeV, JENDL/ImPACT-2018 merged by O.Iwamoto 21-11 (MF6/MT5) recoil spectrum added by O.Iwamoto MF= 1 General information MT=451 Descriptive data and directory MF= 2 Resonance parameters MT=151 Resolved and unresolved resonance parameters - Resolved resonance region (MLBW formula): below 1.8 keV For JENDL-2, evaluation was made on the basis of experime- ntal data of Liou et al./1/ and Wasson and Allen/2/. The average radiation width was assumed to be 0.102 eV /1/. Scattering radius of 6.5 fm was assumed on the basis of systematics of measured values. For JENDL-3, the lowest two p-wave resonances were added according to the data by Alfimenkov et al./3/ Total spin J of some resonances was tentatively estimated with a random number method. Parameters of a negative resonance were modified so as to reproduce the thermal capture and elastic scattering cross sections given by Mughabghab et al. /4/ For JENDL-3.2, the capture data measured at ORELA of ORNL were renormalized (factor=1.208)/5/. The neutron and/or radiation width were revised to reproduce the normalized capture area for each resonance above 2.76 eV. For JENDL-3.3, R was changed from 6.5fm to 6.2fm so as to reproduce measured elemental total cross sections. For JENDL-4, the parameters for a negative resonance was adjusted so as to be consistent with the thermal capture cross section recommended by Mughabghab /6/. - Unresolved resonance region: 1.8 keV - 200 keV The parameters were obtained by fitting to the total and capture cross sections calculated by the POD code /7/. The ASREP code /8/ was employed in this evaluation. The unresolved parameters should be used only for self-shielding calculation. Thermal cross sections & resonance integrals at 300 K ---------------------------------------------------------- 0.0253 eV res. integ. (*) (barns) (barns) ---------------------------------------------------------- Total 1.16946E+01 Elastic 4.56190E+00 n,gamma 7.13273E+00 4.51825E+01 ---------------------------------------------------------- (*) Integrated from 0.5 eV to 10 MeV. MF= 3 Neutron cross sections MT= 1 Total cross section Sum of partial cross sections. MT= 2 Elastic scattering cross section The OPTMAN /9/ & POD /7/ calculations. MT= 3 Non-elastic cross section Sum of partial non-elastic cross sections. MT= 4,51-91 (n,n') cross section The OPTMAN /9/ & POD /7/ calculations. MT= 16 (n,2n) cross section MT= 17 (n,3n) cross section MT= 22 (n,na) cross section MT= 28 (n,np) cross section MT= 32 (n,nd) cross section Calculated by the POD code /7/. MT=102 Capture cross section Calculated by the POD code /7/. The value of gamma-ray strength function was determined to reproduce experimental capture cross sections measured by Wisshak et al /10/. MT=103 (n,p) cross section MT=104 (n,d) cross section MT=105 (n,t) cross section MT=106 (n,He3) cross section MT=107 (n,a) cross section Calculated by the POD code /7/. MT=203 (n,xp) cross section Sum of (n,np) and (n,p) MT=204 (n,xd) cross section Sum of (n,nd) and (n,d) MT=205 (n,xt) cross section MT=206 (n,xHe3) cross section Calculated by the POD code /7/. MT=207 (n,xa) cross section Sum of (n,na) and (n,a) MF= 4 Angular distributions of emitted neutrons MT= 2 Elastic scattering The OPTMAN /9/ & POD /7/ calculations. MF= 6 Energy-angle distributions of emitted particles MT= 16 (n,2n) reaction MT= 17 (n,3n) reaction MT= 22 (n,na) reaction MT= 28 (n,np) reaction MT= 32 (n,nd) reaction Neutron spectra calculated by the POD code /7/. MT= 51-90 (n,n') reaction Neutron angular distributions calculated by OPTMAN /9/ & POD /7/. MT= 91 (n,n') reaction Neutron spectra calculated by the POD code /7/. MT= 203 (n,xp) reaction MT= 204 (n,xd) reaction MT= 205 (n,xt) reaction MT= 206 (n,xHe3) reaction MT= 207 (n,xa) reaction Light-ion spectra calculated by the POD code /6/. MF=12 Gamma-ray multiplicities MT= 3 Non-elastic gamma emission Calculated by the POD code /7/. MF=14 Gamma-ray angular distributions MT= 3 Non-elastic gamma emission Assumed to be isotropic. MF=15 Gamma-ray spectra MT= 3 Non-elastic gamma emission Calculated by the POD code /7/. *************************************************************** * Nuclear Model Calculations with POD Code /7/ * *************************************************************** 1. Theoretical models The POD code is based on the spherical optical model, the distorted-wave Born approximaiton (DWBA), one-component exciton preequilibrium model, and the Hauser-Feshbach-Moldauer statis- tical model. With the preequilibrium model, semi-empirical pickup and knockout process can be taken into account for composite-particle emission. The gamma-ray emission from the compound nucleus can be calculated within the framework of the exciton model. The code is capable of reading in particle transmission coefficients calculated by separate spherical or coupled-channel optical model code. In this evaluation, the OPTMAN code /9/ was employed for neutrons, while the ECIS code /11/ was adopted for charged particles. 2. Optical model & parameters Neutrons: Model: The coupled-channel method based on the rigid-rotor model was adopted. OMP : Coupled-channel optical potential /12/ was applied. The original parameters were slightly modified to give precise reaction cross sections. The optical potential parameters used in evaluation are listed as follows. ------------------------------------------------------------ - Real-volume term VR0= -3.80E+1 MeV VR1= 2.70E-2 MeV VR2= 1.20E-4 MeV VR3= 3.50E-7 MeV VRLA= 9.49E+1 MeV ALAVR= 4.33E-3 r= 1.21E+0 a= 6.70E-1 - Imaginary-surface term WDBW= 1.30E+1 MeV WDWID= 1.30E+1 MeV ALAWD= 1.40E-2 r= 1.21E+0 a= 6.50E-1 - Imaginary-volume term WCBW= 1.70E+1 MeV WCWID= 1.01E+2 MeV r= 1.21E+0 a= 6.50E-1 - Spin-orbit term VS= 6.25E+0 MeV ALASO= 5.00E-3 WSBW= -3.10E+0 MeV WSWID= 1.60E+2 MeV r= 1.04E+0 a= 5.90E-1 - Isospin coefficients CISO= 2.43E+1 WCISO= 1.80E+1 CCOUL= 9.00E-1 - Deformation parameter Beta2= -1.50E-1 ------------------------------------------------------------ Protons: Model: Spherical OMP : Koning and Delaroche /13/ Deuterons: Model: Spherical OMP : Bojowald et al. /14/ Tritons: Mode: Spherical OMP : Becchetti and Greenlees /15/ He-3: Model: Spherical OMP : Becchetti and Greenlees /15/ Alphas: Model: Spherical OMP : A simplified folding model potential /16/ (The nucleon OMP was taken from Ref./12/.) 3. Level scheme of Cd-111 ------------------------------------ No. Ex(MeV) J PI CC ------------------------------------ 0 0.00000 1/2 + * 1 0.24539 5/2 + 2 0.34214 3/2 + * 3 0.39621 11/2 - 4 0.41672 7/2 + 5 0.62018 5/2 + 6 0.68048 9/2 - 7 0.70000 9/2 + 8 0.70493 7/2 + 9 0.73600 3/2 + 10 0.75281 5/2 + 11 0.75490 3/2 + 12 0.83126 7/2 - 13 0.85394 7/2 + 14 0.85560 3/2 + 15 0.86480 3/2 + 16 0.86660 3/2 + 17 0.96790 15/2 - 18 0.98653 9/2 + 19 1.01676 3/2 + 20 1.02000 1/2 + 21 1.04676 7/2 + 22 1.05749 5/2 + 23 1.07825 3/2 + 24 1.11556 3/2 + 25 1.11841 7/2 + 26 1.13000 1/2 - 27 1.15100 5/2 + 28 1.18573 1/2 + 29 1.18996 3/2 + 30 1.25659 11/2 + 31 1.27468 5/2 + 32 1.28889 7/2 + 33 1.29858 7/2 + 34 1.32161 5/2 + 35 1.32594 1/2 + 36 1.32662 5/2 - 37 1.33000 3/2 - 38 1.33972 13/2 - 39 1.34067 1/2 + ------------------------------------ Levels above 1.35067 MeV are assumed to be continuous. 4. Level density parameters Energy-dependent parameters of Mengoni-Nakajima /17/ were used ---------------------------------------------------------- Nuclei a* Pair Esh T E0 Ematch Elv_max 1/MeV MeV MeV MeV MeV MeV MeV ---------------------------------------------------------- Cd-112 14.435 2.268 2.419 0.735 -0.781 9.301 2.649 Cd-111 14.779 1.139 2.384 0.681 -1.366 7.239 1.341 Cd-110 13.913 2.288 1.724 0.691 0.276 7.842 2.332 Cd-109 15.088 1.149 1.603 0.656 -0.917 6.585 1.173 Ag-111 13.420 1.139 3.581 0.725 -1.706 7.873 1.277 Ag-110 14.571 0.000 3.382 0.622 -2.061 5.263 0.337 Ag-109 13.214 1.149 2.966 0.745 -1.615 7.875 0.870 Pd-109 14.484 1.149 3.832 0.727 -2.390 8.692 0.327 Pd-108 13.699 2.309 3.184 0.668 0.130 7.935 2.404 Pd-107 14.272 1.160 3.199 0.648 -1.040 6.701 0.688 ---------------------------------------------------------- 5. Gamma-ray strength functions M1, E2: Standard Lorentzian (SLO) E1 : Generalized Lorentzian (GLO) /18/ 6. Preequilibrium process Preequilibrium is on for n, p, d, t, He-3, and alpha. Preequilibrium capture is on. References 1) Liou, H.I., et al.: Phys. Rev., C10, 709 (1974). 2) Wasson, O.A., Allen, B.J.: Phys. Rev., C7, 780 (1973). 3) Alfimenkov et al.: Nucl. Phys. A397, 93(1983). 4) Mughabghab, S.F. et al.: "Neutron Cross Sections, Vol. I, Part A", Academic Press (1981). 5) Allen, B.J. et al.: Nucl. Sci. Eng., 82, 230 (1982). 6) S.F.Mughabghab, "Atlas of Neutron Resonances", Elsevier (2006). 7) A.Ichihara et al., JAEA-Data/Code 2007-012 (2007). 8) Y.Kikuchi et al., JAERI-Data/Code 99-025 (1999) [in Japanese]. 9) E.Soukhovitski et al., JAERI-Data/Code 2005-002 (2005). 10) Wisshak et al., Phys. Rev. C66, 025801 (2002). 11) J.Raynal, CEA Saclay report, CEA-N-2772 (1994). 12) S.Kunieda et al., J. Nucl. Sci. Technol. 44, 838 (2007). 13) A.J.Koning, J.P.Delaroche, Nucl. Phys. A713, 231 (2003). 14) Bojowald et al., Phys. Rev. C 38, 1153 (1988). 15) F.D.Becchetti,Jr., G.W.Greenlees, "Polarization Phenomena in Nuclear Reactions," p.682, The University of Wisconsin Press (1971). 16) D.G.Madland, NEANDC-245 (1988), p. 103. 17) A.Mengoni, Y.Nakajima, J. Nucl. Sci. Technol. 31, 151 (1994). 18) M.Brink, Ph.D thesis, Oxford University, 1955.