48-Cd-112 JAEA EVAL-FEB22 S.Kunieda, A.Ichihara, K.Shibata+ DIST-DEC21 20100316 ----JENDL-5 MATERIAL 4843 -----INCIDENT NEUTRON DATA ------ENDF-6 FORMAT History 09-11 Re-evaluation was performed for JENDL-4.0 The resolved resonance parameters were not changed from JENDL-3.3 10-03 Compiled by S.Kunieda 21-08 QI of MT89 was slightly shifted to avoid duplication with MT88 by S. Nakayama. 21-11 revised by O.Iwamoto (MF8/MT4,16,17,22,28,102-104,107) JENDL/AD-2017 adopted (MF8/MT32,105,106) added (MF9/MT102,107) JENDL/AD-2017 adopted (MF10/MT16,28,104) JENDL/AD-2017 based MF= 1 General information MT=451 Descriptive data and directory MF= 2 Resonance parameters MT=151 Resolved and unresolved resonance parameters - Resolved resonance region (MLBW formula): below 7 keV Parameters were taken from JENDL-2. For JENDL-2, evaluation was made on the basis of experimental data of Liou et al./1/ and Musgrove et al./2/ The average radiation width of s-wave resonances was assumed to be 0.1 eV/1/ below 2.0 keV, and to be 0.077 eV above 2.0 keV. For p-wave ones, the average width of 0.096 eV/2/ was assumed. A negative resonance was added so as to reproduce the thermal capture and scattering cross sections given by Mughabghab et al./3/ ***** For JENDL-3.3 ************************************** R was changed from 6.5fm to 6.2fm so as to reproduce measured elemental total cross sections. ************************************************************ No update was made for JENDL-4.0. - Unresolved resonance region: 7 keV - 250 keV The parameters were obtained by fitting to the total and capture cross sections calculated by the POD code /4/. The ASREP code /5/ was employed in this evaluation. The unresolved parameters should be used only for self-shielding calculation. Thermal cross sections & resonance integrals at 300 K ---------------------------------------------------------- 0.0253 eV res. integ. (*) (barns) (barns) ---------------------------------------------------------- Total 8.68971E+00 Elastic 6.49643E+00 n,gamma 2.19328E+00 1.31761E+01 ---------------------------------------------------------- (*) Integrated from 0.5 eV to 10 MeV. MF= 3 Neutron cross sections MT= 1 Total cross section Sum of partial cross sections. MT= 2 Elastic scattering cross section The OPTMAN /6/ & POD /4/ calculations. MT= 3 Non-elastic cross section Sum of partial non-elastic cross sections. MT= 4,51-91 (n,n') cross section The OPTMAN /6/ & POD /4/ calculations. MT= 16 (n,2n) cross section MT= 17 (n,3n) cross section MT= 22 (n,na) cross section MT= 28 (n,np) cross section MT= 32 (n,nd) cross section Calculated by the POD code /4/. MT=102 Capture cross section Calculated by the POD code /4/. The value of gamma-ray strength function was determined to reproduce experimental capture cross sections measured by Wisshak et al /7/. MT=103 (n,p) cross section MT=104 (n,d) cross section MT=105 (n,t) cross section MT=106 (n,He3) cross section MT=107 (n,a) cross section Calculated by the POD code /4/. MT=203 (n,xp) cross section Sum of (n,np) and (n,p) MT=204 (n,xd) cross section Sum of (n,nd) and (n,d) MT=205 (n,xt) cross section MT=206 (n,xHe3) cross section Calculated by the POD code /4/. MT=207 (n,xa) cross section Sum of (n,na) and (n,a) MF= 4 Angular distributions of emitted neutrons MT= 2 Elastic scattering The OPTMAN /6/ & POD /4/ calculations. MF= 6 Energy-angle distributions of emitted particles MT= 16 (n,2n) reaction MT= 17 (n,3n) reaction MT= 22 (n,na) reaction MT= 28 (n,np) reaction MT= 32 (n,nd) reaction Neutron spectra calculated by the POD code /4/. MT= 51-90 (n,n') reaction Neutron angular distributions calculated by OPTMAN /6/ & POD /4/. MT= 91 (n,n') reaction Neutron spectra calculated by the POD code /4/. MT= 203 (n,xp) reaction MT= 204 (n,xd) reaction MT= 205 (n,xt) reaction MT= 206 (n,xHe3) reaction MT= 207 (n,xa) reaction Light-ion spectra calculated by the POD code /6/. MF=12 Gamma-ray multiplicities MT= 3 Non-elastic gamma emission Calculated by the POD code /4/. MF=14 Gamma-ray angular distributions MT= 3 Non-elastic gamma emission Assumed to be isotropic. MF=15 Gamma-ray spectra MT= 3 Non-elastic gamma emission Calculated by the POD code /4/. *************************************************************** * Nuclear Model Calculations with POD Code /4/ * *************************************************************** 1. Theoretical models The POD code is based on the spherical optical model, the distorted-wave Born approximaiton (DWBA), one-component exciton preequilibrium model, and the Hauser-Feshbach-Moldauer statis- tical model. With the preequilibrium model, semi-empirical pickup and knockout process can be taken into account for composite-particle emission. The gamma-ray emission from the compound nucleus can be calculated within the framework of the exciton model. The code is capable of reading in particle transmission coefficients calculated by separate spherical or coupled-channel optical model code. In this evaluation, the OPTMAN code /6/ was employed for neutrons, while the ECIS code /8/ was adopted for charged particles. 2. Optical model & parameters Neutrons: Model: The coupled-channel method based on the soft-rotor model was adopted. The Hamiltonian parameters were identical to those reported in ref /9/. OMP : Coupled-channel optical potential /10/ was applied. The original parameters were slightly modified to give precise reaction cross sections. The optical potential parameters used in evaluation are listed as follows. ------------------------------------------------------------ - Real-volume term VR0= -3.90E+1 MeV VR1= 2.70E-2 MeV VR2= 1.20E-4 MeV VR3= 3.50E-7 MeV VRLA= 9.49E+1 MeV ALAVR= 4.32E-3 r= 1.21E+0 a= 6.70E-1 - Imaginary-surface term WDBW= 1.30E+1 MeV WDWID= 1.80E+1 MeV ALAWD= 1.40E-2 r= 1.21E+0 a= 6.50E-1 - Imaginary-volume term WCBW= 1.70E+1 MeV WCWID= 1.01E+2 MeV r= 1.21E+0 a= 6.50E-1 - Spin-orbit term VS= 6.26E+0 MeV ALASO= 5.00E-3 WSBW= -3.10E+0 MeV WSWID= 1.60E+2 MeV r= 1.05E+0 a= 5.90E-1 - Isospin coefficients CISO= 2.43E+1 WCISO= 1.80E+1 CCOUL= 9.00E-1 ------------------------------------------------------------ Protons: Model: Spherical OMP : Koning and Delaroche /11/ Deuterons: Model: Spherical OMP : Bojowald et al. /12/ Tritons: Mode: Spherical OMP : Becchetti and Greenlees /13/ He-3: Model: Spherical OMP : Becchetti and Greenlees /13/ Alphas: Model: Spherical OMP : A simplified folding model potential /14/ (The nucleon OMP was taken from Ref./10/.) 3. Level scheme of Cd-112 ------------------------------------ No. Ex(MeV) J PI CC ------------------------------------ 0 0.00000 0 + * 1 0.61752 2 + * 2 1.22446 0 + 3 1.31239 2 + 4 1.41558 4 + 5 1.43319 0 + 6 1.46886 2 + 7 1.87075 4 + 8 1.87100 0 + 9 2.00533 3 - * 10 2.06458 3 + 11 2.08175 4 + 12 2.12171 2 + 13 2.15619 2 + 14 2.16700 3 - 15 2.16803 6 + 16 2.23110 2 + 17 2.30060 0 + 18 2.30500 1 + 19 2.33500 6 + 20 2.37332 5 - 21 2.40315 3 + 22 2.41618 3 - 23 2.42400 1 - 24 2.45443 4 + 25 2.49338 4 + 26 2.50100 0 + 27 2.50665 2 + 28 2.50688 3 + 29 2.51700 5 + 30 2.53300 3 + 31 2.57020 5 - 32 2.57164 6 + 33 2.58400 1 - 34 2.58900 6 + 35 2.59110 4 - 36 2.63200 5 - 37 2.63500 2 + 38 2.64900 0 + 39 2.64900 3 - ------------------------------------ Levels above 2.65900 MeV are assumed to be continuous. 4. Level density parameters Energy-dependent parameters of Mengoni-Nakajima /15/ were used ---------------------------------------------------------- Nuclei a* Pair Esh T E0 Ematch Elv_max 1/MeV MeV MeV MeV MeV MeV MeV ---------------------------------------------------------- Cd-113 14.918 1.129 2.940 0.622 -0.905 6.375 1.352 Cd-112 14.435 2.268 2.419 0.735 -0.781 9.301 2.649 Cd-111 14.779 1.139 2.384 0.681 -1.366 7.239 1.341 Cd-110 13.913 2.288 1.724 0.691 0.276 7.842 2.332 Ag-112 14.064 0.000 3.764 0.653 -2.318 5.738 0.018 Ag-111 13.420 1.139 3.581 0.725 -1.706 7.873 1.277 Ag-110 14.571 0.000 3.382 0.622 -2.061 5.263 0.337 Pd-110 13.913 2.288 3.640 0.645 0.154 7.754 2.140 Pd-109 14.484 1.149 3.832 0.727 -2.390 8.692 0.327 Pd-108 13.699 2.309 3.184 0.668 0.130 7.935 2.404 ---------------------------------------------------------- 5. Gamma-ray strength functions M1, E2: Standard Lorentzian (SLO) E1 : Generalized Lorentzian (GLO) /16/ 6. Preequilibrium process Preequilibrium is on for n, p, d, t, He-3, and alpha. Preequilibrium capture is on. References 1) Liou, H.I., et al.: Phys. Rev., C10, 709 (1974). 2) Musgrove, A.R. de L., et al.: J. Phsics pt G, 4, 771 (1978). 3) Mughabghab, S.F. et al.: "Neutron Cross Sections, Vol. I, Part A", Academic Press (1981). 4) A.Ichihara et al., JAEA-Data/Code 2007-012 (2007). 5) Y.Kikuchi et al., JAERI-Data/Code 99-025 (1999) [in Japanese]. 6) E.Soukhovitski et al., JAERI-Data/Code 2005-002 (2005). 7) Wisshak et al., Phys. Rev. C66, 025801 (2002). 8) J.Raynal, CEA Saclay report, CEA-N-2772 (1994). 9) S.Kunieda et al., J. Nucl. Sci. Technol. 46, 914 (2009). 10) S.Kunieda et al., J. Nucl. Sci. Technol. 44, 838 (2007). 11) A.J.Koning, J.P.Delaroche, Nucl. Phys. A713, 231 (2003). 12) Bojowald et al., Phys. Rev. C 38, 1153 (1988). 13) F.D.Becchetti,Jr., G.W.Greenlees, "Polarization Phenomena in Nuclear Reactions," p.682, The University of Wisconsin Press (1971). 14) D.G.Madland, NEANDC-245 (1988), p. 103. 15) A.Mengoni, Y.Nakajima, J. Nucl. Sci. Technol. 31, 151 (1994). 16) M.Brink, Ph.D thesis, Oxford University, 1955.